| 1. |
- Li, Yaohui, et al.
(författare)
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Improved efficiency of organic solar cell using MoS2 doped poly (3,4-ethylenedioxythiophene)(PEDOT) as hole transport layer
- 2022
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Ingår i: Applied Surface Science. - : ELSEVIER. - 0169-4332 .- 1873-5584. ; 590
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Tidskriftsartikel (refereegranskat)abstract
- We report an efficient hole transporting layer (HTL) for organic solar cell (OSC) based on solution-processed organic-inorganic hybrid composed of ultrasonic-exfoliated MoS2 nanosheets and dopamine-copolymerized poly(3,4-ethylenedioxythiophene) (PEDOT) derivative (DA-P). The OSCs based on this new hybrid HTL show a marked performance improvement over those with single-component HTLs, and they retain up to 80% of their original power conversion efficiency after 35 days. Our investigations reveal that the boost in performance is due to a synergistic effect that improves both hole transport and extraction ability. This effect is mainly due to the doping of exfoliated-MoS2 nanosheets on DA-P. We employ a comprehensive range of spectroscopies to uncover that the dopant is derived from the oxidation products of MoS2 nanosheets during the ultrasonic exfoliation. Our work demonstrates an efficient hybrid HTL and offers new insights into the interaction of exfoliated-MoS2 nanosheets and the PEDOT derivatives.
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| 2. |
- Li, Yaohui, et al.
(författare)
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An n-n Heterojunction Configuration for Efficient Electron Transport in Organic Photovoltaic Devices
- 2023
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Ingår i: Advanced Functional Materials. - : WILEY-V C H VERLAG GMBH. - 1616-301X .- 1616-3028. ; 33:9
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Tidskriftsartikel (refereegranskat)abstract
- Selective electron transport and extraction are essential to the operation of photovoltaic devices. Electron transport layer (ETL) is therefore critical to organic photovoltaics (OPV). Herein, an ETL configuration is presented comprising a solution-processed n-n organic heterojunction to enhance electron transport and hole blocking, and boost power conversion efficiency (PCE) in OPV. Specifically, the n-n heterojunction is constructed by stacking a narrow-band n-type conjugated polymer layer (PNDIT-F3N) and a wide-band n-type conjugated molecule layer (Phen-NaDPO). Based on the ultraviolet photoelectron spectroscopy measurement and numerical simulation of current density-voltage characteristics, the formation of the built-in potential is investigated. In three OPVs with different active layers, substantial improvements are observed in performance following the introduction of this ETL configuration. The performance enhancement arises from the combination of selective carrier transport properties and reduced recombination. Another contributing factor is the good film-forming quality of the new ETL configuration, where the surface energies of the related materials are well-matched. The n-n organic heterojunction represents a viable and promising ETL construction strategy for efficient OPV devices.
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| 3. |
- Li, Yong, et al.
(författare)
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Effects of horizontal self-rotation on flow and heat transfer of supercritical n-decane in regenerative circular/rectangular cooling channels
- 2024
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Ingår i: International Journal of Heat and Fluid Flow. - 0142-727X. ; 105
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Tidskriftsartikel (refereegranskat)abstract
- Concerning the rotation flight of a hypersonic vehicle centered on its geometric axis, the rotational flow and heat transfer characteristics of supercritical n-decane in horizontal circular and rectangular tubes were comprehensively analyzed based on numerical simulation. The computational domain was established and the corresponding governing equations of mass conservation, momentum conservation, and energy conservation were mathematically formulated as well were the thermophysical properties and boundary conditions. A procedure for setting up the numerical simulation was finally implemented. A mesh independence study in the case of a rotating speed of 300 rpm and a turbulence model study based on a stationary/swinging tube were comprehensively conducted and the RANS model was well validated. For the circular tube, the wall temperature distribution trend along the flow direction is similar but the magnitude is not uniform. Also, the fluid temperature near the upper wall is larger than that in the vicinity of the lower wall, i.e., the relaminarization plays an essential role in this phenomenon. The velocity difference near the wall can be weakened by the centrifugal force. For the rectangular tube, the velocity magnitude and temperature distribution are found to be greatly affected by the rotation (i.e., centrifugal force). The relative temperature magnitude near the upper and lower walls will be reversed at a rotation speed of n = 100–500 rpm. Subsequently, a symmetrical temperature distribution can be observed once the speed increases to a certain value (e.g., n = 700–900 rpm). In summary, the centrifugal force plays a more important role in a rectangular tube than in a circular tube.
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| 4. |
- Li, Yong, et al.
(författare)
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Transient Flow and Heat Transfer in a Horizontal Rectangular Channel Considering Thermal-Fluid-Structure Interaction
- 2022
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Ingår i: Journal of Energy Resources Technology, Transactions of the ASME. - : ASME International. - 0195-0738. ; 144:11
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Tidskriftsartikel (refereegranskat)abstract
- For the supercritical n-decane horizontally flowing in a rectangular channel of an active regenerative cooling system, a transient thermal-fluid-structure coupling method is employed to investigate the unsteady thermal-hydraulic characteristics and the wall deformation at a starting stage. The temperature distributions of the fluid domain and solid domain along the flow direction are investigated at fixed times as well as at a certain cross section. Streamlines in cross sections are employed to explain the temperature distribution. The velocity and pressure at a fixed point versus time are also given. Besides, the solid deformation is presented according to the uneven pressure distribution and temperature distribution. It is found that the response time is less than 30 s when the heat flux is less than 3.0 MW/m2. A larger heat flux contributes to promoting the steady state. The high-temperature part of the solid domain is close to the heated wall, but the situation is reversed for the fluid domain. This is because a bunch of dead-zone vortices appears in the vicinity of the upper wall of the channel. The maximum deformation is 0.132 mm for the condition of heat flux 3.0 MW/m2 and it is exacerbated by the uneven temperature and pressure distributions on the solid domain.
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| 5. |
- Liu, Li, et al.
(författare)
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Involvement of yes-associated protein 1 activation in the matrix degradation of human-induced-pluripotent-stem-cell-derived chondrocytes induced by T-2 toxin and deoxynivalenol alone and in combination
- 2024
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Ingår i: International Journal of Molecular Sciences. - : MDPI. - 1661-6596 .- 1422-0067. ; 25:2
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Tidskriftsartikel (refereegranskat)abstract
- T-2 toxin and deoxynivalenol (DON) are two prevalent mycotoxins that cause cartilage damage in Kashin-Beck disease (KBD). Cartilage extracellular matrix (ECM) degradation in chondrocytes is a significant pathological feature of KBD. It has been shown that the Hippo pathway is involved in cartilage ECM degradation. This study aimed to examine the effect of YAP, a major regulator of the Hippo pathway, on the ECM degradation in the hiPS-derived chondrocytes (hiPS-Ch) model of KBD. The hiPS-Ch injury models were established via treatment with T-2 toxin/DON alone or in combination. We found that T-2 toxin and DON inhibited the proliferation of hiPS-Ch in a dose-dependent manner; significantly increased the levels of YAP, SOX9, and MMP13; and decreased the levels of COL2A1 and ACAN (all p values < 0.05). Immunofluorescence revealed that YAP was primarily located in the nuclei of hiPS-Ch, and its expression level increased with toxin concentrations. The inhibition of YAP resulted in the dysregulated expression of chondrogenic markers (all p values < 0.05). These findings suggest that T-2 toxin and DON may inhibit the proliferation of, and induce the ECM degradation, of hiPS-Ch mediated by YAP, providing further insight into the cellular and molecular mechanisms contributing to cartilage damage caused by toxins.
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