| 1. |
- Mende, Max, et al.
(författare)
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Strong Rashba Effect and Different f−d Hybridization Phenomena at the Surface of the Heavy-Fermion Superconductor CeIrIn 5
- 2022
-
Ingår i: Advanced Electronic Materials. - : Wiley. - 2199-160X .- 2199-160X. ; 8:3
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Tidskriftsartikel (refereegranskat)abstract
- New temperature scales and remarkable differences from bulk properties have increasingly placed the surfaces of strongly correlated f materials into the focus of research activities. Applying first-principles calculations and angle-resolved photoelectron spectroscopy measurements, a strong Rashba effect and spin-split surface states at the CeIn surface of the heavy-fermion superconductor CeIrIn5 are revealed. The unveiled 4f-derived electron landscape is remarkably distinct for surface and bulk Ce implying the existence of novel temperature scales near the surface region in this material. These results show that ab initio calculations can reliably predict the unusual electronic and spin structure of surfaces of strongly correlated 4f systems where Rashba spin-orbit-coupling phenomena emerge. It is suggested that the structural blocks of such materials can be combined with magnetically active layers for engineering of novel nanostructural objects with appropriate substrates where the diversity of f-driven properties can be applied for the development of novel functionalities.
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| 2. |
- Mende, Max, et al.
(författare)
-
Strong Rashba Effect and Different f−d Hybridization Phenomena at the Surface of the Heavy-Fermion Superconductor CeIrIn5
- 2022
-
Ingår i: Advanced Electronic Materials. - : Wiley. - 2199-160X. ; 8:3
-
Tidskriftsartikel (refereegranskat)abstract
- New temperature scales and remarkable differences from bulk properties have increasingly placed the surfaces of strongly correlated f materials into the focus of research activities. Applying first-principles calculations and angle-resolved photoelectron spectroscopy measurements, a strong Rashba effect and spin-split surface states at the CeIn surface of the heavy-fermion superconductor CeIrIn5 are revealed. The unveiled 4f-derived electron landscape is remarkably distinct for surface and bulk Ce implying the existence of novel temperature scales near the surface region in this material. These results show that ab initio calculations can reliably predict the unusual electronic and spin structure of surfaces of strongly correlated 4f systems where Rashba spin-orbit-coupling phenomena emerge. It is suggested that the structural blocks of such materials can be combined with magnetically active layers for engineering of novel nanostructural objects with appropriate substrates where the diversity of f-driven properties can be applied for the development of novel functionalities.
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| 3. |
- Tarasov, Artem V., et al.
(författare)
-
Structural instability at the In-terminated surface of the heavy-fermion superconductor CeIrIn5
- 2022
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Ingår i: Surfaces and Interfaces. - : Elsevier BV. - 2468-0230. ; 32
-
Tidskriftsartikel (refereegranskat)abstract
- Driven by reconstruction and relaxation, by the appearance of surface electron states and resonances, the surface properties and related temperature scales of strongly correlated f-materials may differ dramatically from those in the bulk. Applying low energy electron and photoelectron diffraction techniques, momentum-resolved photoelectron spectroscopy and ab initio calculations, we demonstrate that the In-terminated surface of the heavyfermion superconductor CeIrIn5 experiences a reconstruction with a (root 2v x root 2)R45 degrees ordered structure. The latter appears due to the displacement of In atoms with respect to the Ir sublattice. We show that the electronic structure and related properties of the reconstructed In surface differ remarkably from the unreconstructed case. Namely, the predicted surface states with Rashba-type spin splitting do not appear. Our results suggest surface instabilities in similar quasi-two-dimensional strongly correlated f-materials, for which surface reconstructions can be unveiled by means of diffraction techniques.
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