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Sökning: WFRF:(Nommiste E)

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1.
  • Itala, E, et al. (författare)
  • Molecular fragmentation of pyrimidine derivatives following site-selective carbon core ionization
  • 2011
  • Ingår i: Journal of Electron Spectroscopy and Related Phenomena. - : Elsevier BV. - 0368-2048 .- 1873-2526. ; 184:3-6, s. 119-124
  • Tidskriftsartikel (refereegranskat)abstract
    • Ionization-site-dependent fragmentation of three cyclic biomolecules - uracil, 5-bromouracil and thymine - has been studied using electron-energy-resolved photoelectronphotoion-photoion coincidence spectroscopy. Previous studies concerning ionization site dependent fragmentation have mainly been carried out with linear molecules. The results reported here show that all studied molecules have dicationic fragmentation channels whose intensity depends on the initial core-ionization site, although these channels cover only a relatively small fraction of the total fragment yield. The present study shows on one hand, that it is often the surrounding bond(s) of the ionized atom that will break following the initial core ionization, and on the other hand, that some specific fragmentation channels can display strong site-dependency where there is no direct correlation between the ionization site and the bond breakage locations.
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2.
  • AKSELA, H, et al. (författare)
  • PARTIAL AUGER DECAY-RATES OF CORE-IONIZED MOLECULAR-STATES IN HCL AND DCL
  • 1995
  • Ingår i: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS. - : IOP PUBLISHING LTD. - 0953-4075. ; 28:19, s. 4259-4268
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • The Cl 2p ionization and the subsequent 2p(-1) --> 2 pi(-2) Auger decay in HCl and DCl molecules have been studied using synchrotron radiation. The Anger spectra have been decomposed and assigned to the transitions from the (2) Pi(1/2), (2) Sigma(1/2) and
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3.
  • Kikas, A., et al. (författare)
  • Resonant inelastic x-ray scattering and UV-VUV luminescence at the Be 1s edge in BeO
  • 2010
  • Ingår i: Journal of Physics: Condensed Matter. - : IOP Publishing. - 1361-648X .- 0953-8984. ; 22:37
  • Tidskriftsartikel (refereegranskat)abstract
    • We carried out a combined study of UV-VUV luminescence and resonant x-ray emission from BeO single crystals with incident photon energies in the vicinity of the Be 1s absorption edge. The x-ray emission spectra show that at the Be 1s photoabsorption edge the lattice relaxation processes in the excitation site take place already on the timescale of the radiative decay of the core excitation. Comparison of the x-ray emission and the luminescence spectra indicates that the maximum energy loss of the process of lattice relaxation during the decay of inner-shell holes is similar to the loss that occurs in the self-trapping process of valence excitons. The possible decay channels of core excitations have been discussed and the mechanism for the creation of 5.2 eV luminescence at the photoabsorption resonances has been suggested.
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4.
  • Kukk, E, et al. (författare)
  • Auger decay of the dissociating core-excited states in the HCl and DCl molecules
  • 1996
  • Ingår i: JOURNAL OF CHEMICAL PHYSICS. - : AMER INST PHYSICS. ; 104:12, s. 4475-4480
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • High-resolution Auger electron spectra from the decay of the Cl 2p-->sigma* excitation in HCl and DCl have been measured. The spectra are analyzed, separating molecular and atomic features, which are assigned to transitions to the HCl (5 sigma 2 pi)(4) si
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5.
  • Kukk, E, et al. (författare)
  • Core-to-Rydberg excitations and their Auger decay in the HCl and DCl molecules
  • 1996
  • Ingår i: PHYSICAL REVIEW A. - : AMER INST PHYSICS. - 1050-2947. ; 54:3, s. 2121-2126
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • The resonant Anger electron spectra of the HCl and DCl molecules have been measured at the first core-to-Rydberg resonances. The low binding energy region of the spectra has been decomposed into transitions to different bound states and their vibrational
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6.
  • Levola, H., et al. (författare)
  • Fragmentation of thymidine induced by ultraviolet photoionization and thermal degradation
  • 2013
  • Ingår i: International Journal of Mass Spectrometry. - : Elsevier BV. - 1387-3806 .- 1873-2798. ; 353, s. 7-11
  • Tidskriftsartikel (refereegranskat)abstract
    • Fragmentation of gas phase thymidine at different temperatures was studied with vacuum ultraviolet radiation and time-of-flight spectroscopy. Partial ion yield measurements were carried out in order to study the appearance energies of thymidine and its main fragments. The appearance energies of thymidine and its deoxyribose- and thymine-based fragments were determined to be 8.39, 8.77 and 8.81 eV, independently of temperature. The thermal decomposition of the sample was observed to start around 138-139 C and it was explained by the breakage of the glycosidic bond, accompanied by hydrogen transfer from the deoxyribose ring to the thymine base.
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7.
  • Patanen, M., et al. (författare)
  • High-resolution study of K 3p photoabsorption and resonant Auger decay in KF
  • 2009
  • Ingår i: Physical Review A (Atomic, Molecular and Optical Physics). - 1050-2947. ; 80:1
  • Tidskriftsartikel (refereegranskat)abstract
    • High-resolution (K3p sigma and pi)->sigma absorption spectrum of KF in the photon energy range of 18.2-19.4 eV was measured at the new FINEST beamline branch on the I3 beamline on MAX III. The experimental spectrum is presented and interpreted using nonrelativistic ab initio molecular calculations corrected with perturbation theory treatment to account for spin-orbit interaction. Resonant Auger decay recorded at the strongest resonances is also presented and reproduced by theoretical calculations. Also a brief introduction to the FINEST beamline branch is presented.
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8.
  • Pärna, R., et al. (författare)
  • FinEstBeaMS – A wide-range Finnish-Estonian Beamline for Materials Science at the 1.5 GeV storage ring at the MAX IV Laboratory
  • 2017
  • Ingår i: Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment. - : Elsevier BV. - 0168-9002. ; 859, s. 83-89
  • Tidskriftsartikel (refereegranskat)abstract
    • The FinEstBeaMS beamline is under construction at the 1.5 GeV storage ring of the MAX IV Laboratory at Lund, Sweden. It has been designed to cover an unusually wide energy range from ultraviolet (4.3 eV) to soft X-rays (1000 eV) but experiments will also be possible at the Mg and Al Kα energies. Instead of having two different insertion devices and optical schemes for low and high photon energy regions, we have based our design on a single long-period, elliptically polarizing undulator and a plane grating monochromator. This solution will provide very good conditions for planned experiments in the whole photon energy region. The beamline will have two branches: one will mainly be used to investigate free atoms, molecules and clusters with photoelectron/photoion coincidence spectroscopy as well as solids with photoluminescence spectroscopy whereas the other one will be dedicated to ultra-high vacuum studies of surfaces and interfaces, utilizing X-ray photoelectron spectroscopy and X-ray absorption spectroscopy. This paper focuses on the optical design of the beamline and general design concepts of the gas phase and solid state end stations.
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9.
  • Urpelainen, S., et al. (författare)
  • FINEST:A high performance branch-line for VUV photon energy range gas phase studies at MAX-lab
  • 2010
  • Ingår i: AIP Conference Proceedings. - : AIP. - 0094-243X. - 9780735407824 ; 1234, s. 411-414
  • Konferensbidrag (refereegranskat)abstract
    • We present a dedicated beamline branch for high flux and ultra-high resolution (R>100000) gas and vapor phase studies in the vacuum-ultra-violet (VUV) region of light on the undulator beamline I3, located on the 700 MeV MAX-III storage ring. The mechanical and optical design of the branch-line, the differential pumping setup as well as performance characteristics are presented.
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10.
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11.
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12.
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13.
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14.
  • AUSMEES, A, et al. (författare)
  • OBSERVATION OF ANOMALOUS BEHAVIOR OF THE XE 4D PHOTOELECTRON SATELLITES
  • 1995
  • Ingår i: PHYSICAL REVIEW A. - : AMER INST PHYSICS. - 1050-2947. ; 52:4, s. 2943-2947
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • The Xe 4d photoelectron satellites have been studied in the photon energy region 90-200 eV. The substantially improved energy resolution has enabled us to determine a wealth of satellites. A comparison of the satellite spectra at the intermediate excitati
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15.
  • Ausmees, A., et al. (författare)
  • Secondary photoelectron spectra of ionic solids as a function of the incident photon energy
  • 1991
  • Ingår i: Nuclear Instruments & Methods in Physics Research. Section A: Accelerators, Spectrometers, Detectors, and Associated Equipment. - 0168-9002. ; 308:1-2, s. 219-222
  • Tidskriftsartikel (refereegranskat)abstract
    • Energy distributions of slow electrons (0-10 eV) emitted by thin layers of NaCl, KBr, CsBr, and CsI irradiated by monochromatic XUV photons with various energies in the interval of 50-300 eV are measured. The contributions of slow secondaries, hot secondaries and primary photoelectrons are obtained. It is shown that the higher the absorption coefficient for incident photons, the stronger the contribution of hot secondaries. The relationship between their contribution and the electron-phonon scattering process is discussed.
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16.
  • Ausmees, A., et al. (författare)
  • Secondary photoelectron spectra of NaCl and KBr excited by XUV radiation : Experiments and computer simulations
  • 1990
  • Ingår i: Solid State Communications. - 0038-1098. ; 76:12, s. 1383-1386
  • Tidskriftsartikel (refereegranskat)abstract
    • Energy distributions of slow electrons (0 to 10eV) emitted by thin layers of NaCl and KBr irradiated by monochromatic XUV photons with various energies in the interval of 50 to 300 eV are measured. For all cases the photoelectron spectrum starts with an intense peak of slow secondaries and has a hot-secondary structure at the energies 1 to 5 eV. The smaller the photon absorption depth, the stronger is this structure. An attempt is made to reproduce such a behaviour of spectra by a Monte Carlo simulation of electron-electron and electron-phonon scattering sequences induced in solids by XUV photon absorption. It appears that for high-energy ( > 2 to 3 eV) conduction electrons the electron-phonon scattering is mainly due to acoustic phonons.
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17.
  • deBrito, AN, et al. (författare)
  • Auger decay of the molecular field split S 2p core excited states in HS radical
  • 1997
  • Ingår i: JOURNAL OF CHEMICAL PHYSICS. - : AMER INST PHYSICS. - 0021-9606. ; 106:1, s. 18-23
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • Using synchrotron radiation, very high resolution electron spectra at the 2p --> 6a(1) and 2p --> 3b(2) resonances of H2S have been recorded. Auger transitions from molecular field split S 2p hole states of HS* fragment, created by fast dissociation of th
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18.
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19.
  • Elango, M., et al. (författare)
  • Autoionization phenomena involving the 2p53d configuration of argonlike ions in ionic solids
  • 1993
  • Ingår i: Physical Review B (Condensed Matter). - 0163-1829. ; 47:18, s. 11736-11748
  • Tidskriftsartikel (refereegranskat)abstract
    • The photon-induced Auger and photoelectron spectra of the argonlike ions Cl- (in NaCl), K+ (in KCl), Ca2+ (in CaCl2 and CaF2), and Sc3+ (in Sc2O3) have been measured in the vicinity of the L23 absorption edges of these ions. It is shown that at the 2p6→2p53d(4s) resonance a spectator structure appears in the L23M23M23 Auger spectra, which shifts to higher kinetic energies with increasing photon energy. This structure originates from the 3p-23d(4s) final configuration arising as a product of the Auger resonant-inelastic-scattering process of the incident photons. We demonstrate that the peculiarities of this process and the role of the collapsing 3d electron in it can be largely understood in terms of an atomic treatment. The solid-state effects, caused by the crystal field and the lattice polarization, may play an additional role.
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20.
  • Kaambre, T., et al. (författare)
  • Resonant inelastic X-ray scattering at the Be 1s edge in BeO
  • 2007
  • Ingår i: Journal of Electron Spectroscopy and Related Phenomena. - : Elsevier BV. - 0368-2048. ; 156, s. 299-302
  • Tidskriftsartikel (refereegranskat)abstract
    • We present the resonant inelastic X-ray scattering (RIXS) spectra of BeO at the Be 1s photoabsorption edge. The RIXS spectra excited in the vicinity of the core exciton resonance show two principal features: the scattering on a valence exciton (which at higher excitation energies verges into the characteristic K alpha emission), and a remarkably strong energy loss side-band to the elastic scattering peak, which has a maximum width of 6 eV and has intensity, at resonance, comparable to the valence scattering. The energy loss side-band appears to result from rapid lattice relaxation at the absorption site on the X-ray scattering time-span. (c) 2006 Elsevier B.V. All rights reserved.
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21.
  • Kikas, A, et al. (författare)
  • NaK photoabsorption and resonant KLL Auger spectra in naf and NaCl
  • 2002
  • Ingår i: Surface Review and Letters. - 0218-625X. ; 9:2, s. 1303-1308
  • Tidskriftsartikel (refereegranskat)abstract
    • The nature of Na Is photoabsorption in NaF and NaCl is investigated using the resonant Auger decay of Na Is core excitations. The appearance of new peaks in Auger spectra, when the energy of excitation coincides with the photoabsorption thresholds, shows that the core excitons are created in the threshold region of the Na 1s photoabsorption spectrum. The core excitons around 1074.2 eV originate from the dipole-forbidden 1s(-1)3s final state, the population of which is made possible by the symmetry disruption at the photoabsorption site. Another core exciton, excited at photon energies of 1076.8 eV in NaF and 1076.3 eV in NaCl, originates from 1s(-1)3p states similar to atoms of Ne and Na. Resonant Auger spectra show also that in NaCl the first sharp photoabsorption maximum at 1076.6 eV has only partially excitonic character.
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22.
  • Kikas, A., et al. (författare)
  • Resonant inelastic x-ray scattering at the F 1s photoabsorption edge in LiF : Interplay of excitonic and conduction states, and Stokes' doubling
  • 2004
  • Ingår i: Physical Review B. Condensed Matter and Materials Physics. - : American Physical Society. - 1098-0121 .- 1550-235X. ; 70:8
  • Tidskriftsartikel (refereegranskat)abstract
    • The excitation-decay processes at the F 1s photoabsorption edge in LiF crystal are studied using resonant inelastic x-ray scattering spectroscopy. The Raman-type linear dispersion and the narrowing of the x-ray fluorescence peak are observed at resonant excitation. A theoretical model based on the Kramers-Heisenberg formula describes well the main features in fluorescence spectra and allows one to separate the contributions of the exciton and the conduction states in the scattering spectra. At the same time, the role of the shape of the spectral distribution within the incident radiation is emphasized as being critically sensitive to the number, kind, and onset of the spectral features which finally appear in the scattering spectra at a particular incident photon energy, particularly in the subthreshold excitation region.
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23.
  • Kikas, A, et al. (författare)
  • Resonant inelastic X-ray scattering at the K edge of oxygen and fluorine in insulators
  • 2005
  • Ingår i: Journal of Electron Spectroscopy and Related Phenomena. - : Elsevier BV. - 0368-2048. ; 144-147, s. 845-848
  • Tidskriftsartikel (refereegranskat)abstract
    • Here we present the results of a study of the electronic structure using the resonant inelastic scattering process at the F 1s photoabsorption edge in LiF and O 1s edge of MgO crystals. In case of excitations in the sub-threshold region, the Raman-type linear dispersion of X-ray fluorescence peak was observed for the studied compounds. In LiF, the narrowing of the X-ray fluorescence peak is observed at pre-threshold excitation, which can be related to the creation of a core exciton, but no core excitons were identified in MgO.
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24.
  • Kikas, A, et al. (författare)
  • Resonant photoemission of CoCl2
  • 1999
  • Ingår i: JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA. - : ELSEVIER SCIENCE BV. - 0368-2048. ; 103, s. 745-749
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • We present the results of a study of the resonant photoemission from polycrystalline in situ evaporated thin him of CoCl2 excited at 2p photoabsorption edges of Co and Cl. At the Co 2p-->3d resonance strong enhancement was observed for the Co 3p, valence
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25.
  • Mursu, J, et al. (författare)
  • Decay of the 2p(5)4s, 2p(5)3d and 2p(5)4d states of Ar studied by utilizing the Auger resonant Raman effect
  • 1996
  • Ingår i: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS. - : IOP PUBLISHING LTD. - 0953-4075. ; 29:19, s. 4387-4399
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • The 2p electrons of Ar have been excited selectively to the 4s, 3d and 4d orbitals and high-resolution de-excitation spectra have been recorded by utilizing the Auger resonant Raman effect. Fine structures in the resonant Anger spectra have been clearly r
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26.
  • Reisberg, L., et al. (författare)
  • UPS and DFT investigation of the electronic structure of gas-phase trimesic acid
  • 2016
  • Ingår i: Journal of Electron Spectroscopy and Related Phenomena. - : Elsevier BV. - 0368-2048. ; 213, s. 11-16
  • Tidskriftsartikel (refereegranskat)abstract
    • Benzene-1,3,5-tricarboxylic acid (trimesic acid, TMA) molecules in gas-phase have been investigated by using valence band photoemission. The photoelectron spectrum in the binding energy region from 9 to 22 eV is interpreted by using density functional theory calculations. The electronic structure of TMA is compared with benzene and benzoic acid in order to demonstrate changes in molecular orbital energies induced by addition of carboxyl groups to benzene ring.
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27.
  • Ruus, R., et al. (författare)
  • Cs 3d absorption and resonant photoemission study of caesium halogenides
  • 2005
  • Ingår i: Physica Scripta. - 0031-8949. ; T115, s. 396-398
  • Tidskriftsartikel (refereegranskat)abstract
    • The highly localized 4f electrons play an important role in forming of the electronic structure and properties of compounds. The 3d photoabsorption and resonant decay spectra of Cs halides represent an interesting case showing both the localized and spatially extended f wave function features. We present and discuss the Cs 3d X-ray absorption and resonant photoelectron emission spectra of the Cs halides. The Cs 3d absorption spectra exhibit a strong atom-like shape resonance behavior, solid-state effects play a minor role. The appearance of the spectral features, which are intrinsic to a localized state, in the decay spectra show that the Cs 3d photoelectron, temporally and spatially trapped in the Cs 3d shape resonance due to the potential barrier for epsilon f electrons near threshold, has substantially localized nature.
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28.
  • Ruus, R., et al. (författare)
  • M4,5N4,5N4,5 Auger decay spectra of the resonantly excited 3d94f configuration of xenonlike ions in solids
  • 1994
  • Ingår i: Physical Review B (Condensed Matter). - 0163-1829. ; 49:21, s. 14836-14844
  • Tidskriftsartikel (refereegranskat)abstract
    • The synchrotron-radiation-induced Auger and photoelectron spectra of the xenonlike ions I- (in CsI), Cs+ (in CsI), Ba2+ (in BaF2), and La3+ (in LaF3) have been measured in the vicinity of the M4,5 absorption edges of these ions. It is shown that the spectra of La and Ba measured at 3d10→3d94f resonances exhibit a very intense 4f-spectator structure which changes its energy and intensity with the energy of the exciting photons. Calculation of the Auger decay of the 3d-14f configuration shows that this structure is due to transitions to the 4d-24f+4p-1 final ionic configuration, the high-energy part of which overlaps the 4d-2 continuum. In the case of Ba this structure coexists with the normal Auger structure which appears as a result of the M4M5N6,7 Coster-Kronig transitions. The spectra of I- contain only the normal M4,5N4,5N4,5 Auger structure related to the 3d-1→4d-2 transitions. The spectra of Cs+ are similar to those of I- with a small admixture of the 4f-spectator-like structure.
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29.
  • Ruus, R, et al. (författare)
  • Potential barrier effects in Cs 3d resonance photoemission of CsF
  • 2004
  • Ingår i: ICESS-9 Proceedings of the 9th International Conference on Electronic Spectroscopy and Structure (Journal of Electron Spectroscopy and Related Phenomena). - : Elsevier BV. - 0368-2048. ; 137-40, s. 377-381
  • Konferensbidrag (refereegranskat)abstract
    • We present and discuss the Cs 3d X-ray absorption spectra and resonant photoelectron emission spectra of CsF. The resonant photoelectron spectra excited at the Cs 3d absorption maxima, exhibit a strong resonance behavior. The different behaviour of participator and spectator channels and interference effects of the 4d partial photoionisation cross-section at the 3d resonances are discussed. The experimental evidence of the phenomenon of spin-orbit activated interchannel coupling in the 3d photoionization of Cs is presented. (C) 2004 Elsevier B.V. All rights reserved.
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30.
  • Ruus, R, et al. (författare)
  • Ti 2p and O 1s X-ray absorption of TiO2 polymorphs
  • 1997
  • Ingår i: SOLID STATE COMMUNICATIONS. - : PERGAMON-ELSEVIER SCIENCE LTD. - 0038-1098. ; 104:4, s. 199-203
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • We present and discuss the Ti 2p and O 1s X-ray absorption spectra (XAS) and resonant photoelectron emission spectra (RPES) of the various polymorphic forms (TiO2-II, rutile and anatase) of TiO2. The largest differences between the Ti 2p XAS of polymorphs
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31.
  • SAIRANEN, OP, et al. (författare)
  • THE RESONANCE AUGER DECAY OF THE XE 4D(3/2,5/2)(-1)NP, N=7,8 STATES STUDIED BY HIGH-RESOLUTION EXPERIMENT
  • 1995
  • Ingår i: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS. - : IOP PUBLISHING LTD. - 0953-4075. ; 28:20, s. 4509-4528
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • The de-excitation of the resonantly excited Xe 4d(3/2,5/27p)(-1) and 4d(3/2,5/2)(-1)8p states is studied with very high photon and electron energy resolution using the new Finnish beamline at MAX-laboratory, Lund, Sweden. The fine structure of the spectra
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32.
  • SVENSSON, S, et al. (författare)
  • FAST DISSOCIATION OF NEUTRAL DOUBLY-EXCITED STATES ABOVE THE S-2P IONIZATION THRESHOLD IN H2S
  • 1995
  • Ingår i: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS. - : IOP PUBLISHING LTD. ; 28:10
  • Annan publikation (övrigt vetenskapligt/konstnärligt)abstract
    • A very rapid dissociation of core doubly excited stares in a molecule has been observed for the first time. The channel is identified in the Anger electron spectra of H2S where the resonating structures, at higher kinetic energy than the normal Auger LVV
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33.
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34.
  • Svensson, S, et al. (författare)
  • New end station for the study of gases, liquids, and solid films at the MAX laboratory
  • 1996
  • Ingår i: REVIEW OF SCIENTIFIC INSTRUMENTS. - : AMER INST PHYSICS. ; 67:6, s. 2149-2156
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • A new end station equipped with a very high-resolution SES-200 electron energy analyzer has been constructed for the study of gases and soft molecular materials. The analyzer is rotatable around the direction of the photon beam, allowing angular-dependent
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35.
  • Thiagarajan, Balasubramanian, et al. (författare)
  • The Normal Incidence Monochromator Beamline I3 on MAX III
  • 2010
  • Ingår i: AIP Conference Proceedings. - : AIP. - 1551-7616 .- 0094-243X. ; 1234, s. 661-664
  • Konferensbidrag (refereegranskat)abstract
    • On the 700 MeV MAX III ring at MAX-lab, a 6.65 m off-axis eagle type monochromator beamline has recently been commissioned. The beamline is sourced by an apple type variable polarization undulator. The energy range of the beamline is 4.6-50 eV and the resolving power achieved is more than 100,000. There are two branch lines, one for angle and spin resolved photoemission studies from solids and the other for gas phase and luminescence experiments. We present the design and performance of the beamline.
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