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1.
  • Gomez L, Ana Maria, 1993-, et al. (författare)
  • Determination of the Plasma Delay Time in PIPS detectors for fission fragments at the LOHENGRIN spectrometer
  • 2023
  • Ingår i: 15<sup>th</sup> International Conference on Nuclear Data for Science and Technology (ND2022). - : EDP Sciences.
  • Konferensbidrag (refereegranskat)abstract
    • The VElocity foR Direct particle Identification spectrometer (VERDI) is a 2E-2v fission spectrometer that allows the measurement of the total mass distribution of secondary fission fragments with a resolving power of 1-2 u. It consists of two time-of-flight (ToF) arms, with one Micro Channel Plate (MCP) detector and up to 32 Silicon PIPS (Passive Implanted Planar Silicon) detectors per arm. The MCPs provide the start timing signals and the PIPS detectors provide both the energy and the stopping ToF signals. In real conditions, the PIPS signals are affected by the formation of plasma from the interaction between the heavy ions and the detector material. The plasma contributes to a reduction in signal amplitude, resulting in a Pulse Height Defect (PHD), and introduces a signal delay, known as Plasma Delay Time (PDT). An experiment to characterize the PDT and PHD was performed at the LOHENGRIN recoil separator of the Institut Laue Langevin (ILL). Characteristic fission fragments from the 239Pu(n,f) reaction were separated based on their A/Q and E/Q ratios, allowing the measurement of a wide range of energies from 21 to 110 MeV and masses between 80 and 149 u. Six PIPS detectors were characterized to study their individual responses to the PDT and PHD effects. The signals were recorded in a digital acquisition system to completely exploit the offline analysis capabilities. Achieved combined timing and energy resolutions for fission fragments varied between 72(2) ps and 100(4) ps and 1.4% - 2% (FWHM), respectively. Preliminary PHD and PDT data are presented from the masses A=85, 95, 130 and 143. The PHD trends are strongly correlated with both the ion energy and mass. The PDT, on the other hand, shows a strong variation as a function of the ion kinetic energy but a smaller dependence on the ion mass.
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3.
  • Al-Adili, Ali, et al. (författare)
  • Analysis of prompt fission neutrons in U-235(nth,f) and fission fragment distributions for the thermal neutron induced fission of U-234
  • 2016
  • Ingår i: CNR*15 - 5th International Workshop On Compound-Nuclear Reactions And Related Topics. - : EDP Sciences.
  • Konferensbidrag (refereegranskat)abstract
    • This paper presents the ongoing analysis of two fission experiments. Both projects are part of the collaboration between the nuclear reactions group at Uppsala and the JRC-IRMM. The first experiment deals with the prompt fission neutron multiplicity in the thermal neutron induced fission of U-235(n,f). The second, on the fission fragment properties in the thermal fission of U-234(n,f). The prompt fission neutron multiplicity has been measured at the JRC-IRMM using two liquid scintillators in coincidence with an ionization chamber. The first experimental campaign focused on U-235(nth,f) whereas a second experimental campaign is foreseen later for the same reaction at 5.5 MeV. The goal is to investigate how the so-called saw-tooth shape changes as a function of fragment mass and excitation energy. Some harsh experimental conditions were experienced due to the large radiation background. The solution to this will be discussed along with preliminary results. In addition, the analysis of thermal neutron induced fission of U-234(n,f) will be discussed. Currently analysis of data is ongoing, originally taken at the ILL reactor. The experiment is of particular interest since no measurement exist of the mass and energy distributions for this system at thermal energies. One main problem encountered during analysis was the huge background of U-235(nth, f). Despite the negligible isotopic traces in the sample, the cross section difference is enormous. Solution to this parasitic background will be highlighted.
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4.
  • Al-Adili, Ali, et al. (författare)
  • Employing TALYS to deduce angular momentum rootmean-square values, J(rms), in fission fragments
  • 2020
  • Ingår i: ND 2019. - : E D P SCIENCES. - 9782759891061
  • Konferensbidrag (refereegranskat)abstract
    • Fission fragments exhibit large angular momenta J, which constitutes a challenge for fission models to fully explain. Systematic measurements of isomeric yield ratios (IYR) are needed for basic nuclear reaction physics and nuclear applications, especially as a function of mass number and excitation energy. One goal is to improve the current understanding of the angular momentum generation and sharing in the fission process. To do so, one needs to improve the modeling of nuclear de-excitation. In this work, we have used the TALYS nuclear-reaction code to relax excited fission fragments and to extract root-mean-square (rms) values of initial spin distributions, after comparison with experimentally determined IYRs. The method was assessed by a comparative study on Cf-252(sf) and (235)(nth,f). The results show a consistent performance of TALYS, both in comparison to reported literature values and to other fission codes. A few discrepant Jrms values were also found. The discrepant literature values could need a second consideration as they could possibly be caused by outdated models. Our TALYS method will be refined to better comply with contemporary sophisticated models and to reexamine older deduced values in literature.
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5.
  • Al-Adili, Ali, et al. (författare)
  • Extraction of angular momenta from isomeric yield ratios : Employing TALYS to de-excite primary fission fragments
  • 2019
  • Ingår i: European Physical Journal A. - : Springer Science and Business Media LLC. - 1434-6001 .- 1434-601X. ; 55:4
  • Tidskriftsartikel (refereegranskat)abstract
    • The generation of angular momentum in fission is difficult to model, in particular at higher excitation energies where data are scarce. Isomeric yield ratios (IYR) play an important role in deducing angular momentum properties of fission fragments (FF), albeit this requires some assumptions and simplifications. To estimate FF angular momentum, fission codes can be used to calculate IYRs and compare them to experimental data. Such measurements have systematically been performed at the IGISOL facility using novel experimental techniques. In conjunction, a new method has been developed to infer the angular momentum of the primary FF using the nuclear reaction code TALYS. In this work, we evaluate this new method by comparing our TALYS calculations with values found in the literature and with results from the GEF fission code, for a few well-studied reactions. The overall results show a consistent performance of TALYS and GEF, as well as of many reported literature values. However, some deviations were found, possibly pinpointing the need to re-examine some of the reported literature values. A sensitivity analysis was also performed, in which the role of excitation energy, neutron emission, discrete level structure and level density models were studied. Finally, the role of multiple chance fission, of relevance for the reactions studied at IGISOL, is discussed. Some literature data for this reaction were also re-analyzed using TALYS, revealing significant differences.
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7.
  • Al-Adili, Ali, et al. (författare)
  • Fission Activities of the Nuclear Reactions Group in Uppsala
  • 2015
  • Ingår i: Scientific Workshop on Nuclear Fission Dynamics and the Emission of Prompt Neutrons and Gamma Rays, THEORY-3. - : Elsevier BV. ; , s. 145-149
  • Konferensbidrag (refereegranskat)abstract
    • This paper highlights some of the main activities related to fission of the nuclear reactions group at Uppsala University. The group is involved for instance in fission yield experiments at the IGISOL facility, cross-section measurements at the NFS facility, as well as fission dynamics studies at the IRMM JRC-EC. Moreover, work is ongoing on the Total Monte Carlo (TMC) methodology and on including the GEF fission code into the TALYS nuclear reaction code. Selected results from these projects are discussed.
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8.
  • Al-Adili, Ali, et al. (författare)
  • Ion counting efficiencies at the IGISOL facility
  • 2014
  • Rapport (övrigt vetenskapligt/konstnärligt)abstract
    • At the IGISOL-JYFLTRAP facility, fission mass yields can be studied at high precision. Fission fragments from a U target are passing through a Ni foil and entering a gas filled chamber. The collected fragments are guided through a mass separator to a Penning trap where their masses are identified. This simulation work focuses on how different fission fragment properties (mass, charge and energy) affect the stopping efficiency in the gas cell. In addition, different experimental parameters are varied (e. g. U and Ni thickness and He gas pressure) to study their impact on the stopping efficiency. The simulations were performed using the Geant4 package and the SRIM code. The main results suggest a small variation in the stopping efficiency as a function of mass, charge and kinetic energy. It is predicted that heavy fragments are stopped about 9% less efficiently than the light fragments. However it was found that the properties of the U, Ni and the He gas influences this behavior. Hence it could be possible to optimize the efficiency.
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9.
  • Al-Adili, Ali, et al. (författare)
  • Isomer yields in nuclear fission
  • 2021
  • Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 2100-014X. ; 256
  • Tidskriftsartikel (refereegranskat)abstract
    • The generation of angular momentum in the fission process is still an open question. To shed light on this topic, we started a series of measurements at the IGISOL-JYFLTRAP facility in Finland. Highprecision measurements of isomeric yield ratios (IYR) are performed with a Penning trap, partly with the aim to extract average root-mean-square (rms) quantities of fragment spin distributions. The newly installed Phase-Imaging Ion-Cyclotron Resonance (PI-ICR) technique allows the separation of masses down to tens of keV, which is suffcient to disentangle many isomers. In this paper, we first summarize the previous measurements on the neutron and proton-induced fission of uranium and thorium, e.g. the odd cadmium and indium isotopes (119 ≤ A ≤ 127). The measurements revealed systematic trends as function of mass number, which stimulated further exploration. A recent measurement was performed at IGISIOL and several new IYR data will soon be published, for the first time. Secondly, we employ the TALYS nuclear-reaction code to model one of the newly measured isomer yields. Detailed GEF and TALYS calculations are discussed for the fragment angular momentum distribution in 134I.
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10.
  • Al-Adili, Ali, et al. (författare)
  • Neutron-multiplicity experiments for enhanced fission modelling
  • 2017
  • Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 9782759890200
  • Konferensbidrag (refereegranskat)abstract
    • The nuclear de-excitation process of fission fragments (FF) provides fundamental information for the understanding of nuclear fission and nuclear structure in neutron-rich isotopes. The variation of the prompt-neutron multiplicity, ν(A), as a function of the incident neutron energy (En) is one of many open questions. It leads to significantly different treatments in various fission models and implies that experimental data are analyzed based on contradicting assumptions. One critical question is whether the additional excitation energy (Eexc) is manifested through an increase of ν(A) for all fragments or for the heavy ones only. A systematic investigation of ν(A) as a function of En has been initiated. Correlations between prompt-fission neutrons and fission fragments are obtained by using liquid scintillators in conjunction with a Frisch-grid ionization chamber. The proof-of-principle has been achieved on the reaction 235U(nth,f) at the Van De Graff (VdG) accelerator of the JRC-Geel using a fully digital data acquisition system. Neutrons from 252Cf(sf) were measured separately to quantify the neutron-scattering component due to surrounding shielding material and to determine the intrinsic detector efficiency. Prelimenary results on ν(A) and spectrum in correlation with FF properties are presented.
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11.
  • Al-Adili, Ali, et al. (författare)
  • Prompt fission neutron yields in thermal fission of U-235 and spontaneous fission of Cf-252
  • 2020
  • Ingår i: Physical Review C. - : American Physical Society (APS). - 2469-9985 .- 2469-9993. ; 102:6
  • Tidskriftsartikel (refereegranskat)abstract
    • Background: The sharing of excitation energy between the fission fragments is one of the key issues in studying nuclear fission. One way to address this is by studying prompt-fission neutron multiplicities as a function of other fission observables such as the mass, (nu) over bar (A). These are vital benchmark data for both fission and nuclear deexcitation models, putting constrains on the fragment excitation energy and hence on the competing prompt neutron/gamma-ray emission. Despite numerous detailed studies, recent measurements done at JRC-Geel with the SCINTIA array in the epithermal region show surprisingly strong discrepancies to earlier thermal fission data and the Wahl systematics. Purpose: The purpose was to perform measurements of the prompt-fission neutron multiplicity, as a function of fragment mass and total kinetic energy (TKE), in U-235(n(th), f) and Cf-252(sf), to verify and extend the SCINTIA results. Another goal was to validate the analysis methods, and prepare for planned investigations at excitation energies up to 5.5 MeV. Methods: The experiments were conducted at the former 7 MV Van de Graaff facility in JRC-Geel, using a Twin Frisch-Grid Ionization Chamber and two liquid scintillation detectors. A neutron beam with an average energy of 0.5 MeV was produced via the Li-7(p,n) reaction. The neutrons were thermalized by a 12 cm thick block of paraffin. Digital data acquisition systems were utilized. Comprehensive simulations were performed to verify the methodology and to investigate the role of the mass and energy resolution on measured (nu) over bar (A) and (nu) over bar (TKE) values. The simulation results also revealed that the partial derivative(nu) over bar/partial derivative A and partial derivative(TKE) over bar/partial derivative(nu) over bar are affected by the mass and energy resolution. However, the effect is small for the estimated resolutions of this work. Detailed Fluka simulations were performed to calculate the fraction of thermal neutron-induced fission, which was estimated to be about 98%. Results: The experimental results on (nu) over bar (A) are in good agreement with earlier data for Cf-252(sf). For U-235(n(th), f), the (nu) over bar (A) data is very similar to the data obtained with SCINTIA, and therefore we verify these disclosed discrepancies to earlier thermal data and to the Wahl evaluation. The experimental results on (nu) over bar (TKE) are also in agreement with the data at epithermal energies. For Cf-252(sf) a slope value of partial derivative(TKE) over bar/partial derivative(nu) over bar = (-12.9 f 0.2) MeV/n was obtained. For U-235(n(th), f) the value is (-12.0 +/- 0.1) MeV/n. Finally, the neutron spectrum in the center-of-mass system was derived and plotted as a function of fragment mass. Conclusions: This work clearly proves the lack of accurate correlation between fission fragment and neutron data even in the best-studied reactions. The new results highlight the need of a new evaluation of the prompt-fission multiplicity for U-225(n(th), f).
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12.
  • Al-Adili, Ali, et al. (författare)
  • Simulations of the fission-product stopping efficiency in IGISOL
  • 2015
  • Ingår i: European Physical Journal A. - : Springer Science and Business Media LLC. - 1434-6001 .- 1434-601X. ; 51:59, s. 1-7
  • Tidskriftsartikel (refereegranskat)abstract
    • At the Jyväskylä Ion Guide Isotope Separator On-Line (IGISOL) facility, independent fission yields are measured employing the Penning-trap technique. Fission products are produced, e.g. by impinging protons on a uranium target, and are stopped in a gas-filled chamber. The products are collected by a flow of He gas and guided through a mass separator to a Penning trap, where their masses are identified. This work investigates how fission-product properties, such as mass and energy, affect the ion stopping efficiency in the gas cell. The study was performed using the Geant4 toolkit and the SRIM code. The main results show a nearly mass-independent ion stopping with regard to the wide spread of ion masses and energies, with a proper choice of uranium target thickness. Although small variations were observed, in the order of 5%, the results are within the systematic uncertainties of the simulations. To optimize the stopping efficiency while reducing the systematic errors, different experimental parameters were varied; for instance material thicknesses and He gas pressure. Different parameters influence the mass dependence and could alter the mass dependencies in the ion stopping efficiency.
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13.
  • Al-Adili, Ali, et al. (författare)
  • Studying fission neutrons with 2E-2v and 2E
  • 2018
  • Ingår i: SCIENTIFIC WORKSHOP ON NUCLEAR FISSION DYNAMICS AND THE EMISSION OF PROMPT NEUTRONS AND GAMMA RAYS (THEORY-4). - : EDP Sciences. - 9782759890316
  • Konferensbidrag (refereegranskat)abstract
    • This work aims at measuring prompt-fission neutrons at different excitation energies of the nucleus. Two independent techniques, the 2E-2v and the 2E techniques, are used to map the characteristics of the mass-dependent prompt fission neutron multiplicity, 7(A), when the excitation energy is increased. The VERDI 2E-2v spectrometer is being developed at JRC-GEEL. The Fission Fragment (FF) energies are measured using two arrays of 16 silicon (Si) detectors each. The FFs velocities are obtained by time-of-flight, measured between micro-channel plates (MCP) and Si detectors. With MCPs placed on both sides of the fission source, VERDI allows for independent timing measurements for both fragments. Cf-252(sf) was measured and the present results revealed particular features of the 2E-2v technique. Dedicated simulations were also performed using the GEF code to study important aspects of the 2E-2v technique. Our simulations show that prompt neutron emission has a non-negligible impact on the deduced fragment data and affects also the shape of 17(A). Geometrical constraints lead to a total-kinetic energy-dependent detection efficiency. The 2E technique utilizes an ionization chamber together with two liquid scintillator detectors. Two measurements have been performed, one of Cf-252(sf) and another one of thermal-neutron induced fission in U-235(n,f). Results from Cf-252(sf) are reported here.
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14.
  • Cannarozzo, Simone, et al. (författare)
  • Global comparison between experimentally measured isomeric yield ratios and nuclear model calculations
  • 2023
  • Ingår i: European Physical Journal A. - : Springer. - 1434-6001 .- 1434-601X. ; 59:12
  • Tidskriftsartikel (refereegranskat)abstract
    • The level density steers transition probabilities between different states in the decay and de-excitation of excited nuclei. Reliable level density modelling is, therefore, key in describing, e.g., de-excitation of fission fragments, with implications on neutron and gamma-rays multiplicities, and also manifested in the population of isomeric states. We test six currently used level density models and the spin distribution in the level density by comparing calculations with measured isomeric yield ratios. The model calculations are performed with the TALYS code and experimental data for nuclear reactions populating spin isomers are retrieved from the EXFOR database. On average, calculations are in agreement with measured data. However, we find that the population of the high-spin state in an isomeric pair is clearly favoured in all of the six studied level density models. Further studies are then performed on the three used phenomenological level density models, to investigate the significance of their effect. We find that a significant reduction of the spin width distribution improves the agreement between calculated and experimentally observed isomeric yield ratios. This result is independent of the incident particle in the nuclear reaction. The needed reduction of the spin width distribution to comply with empirical data has, e.g., implications for studies in angular momentum generation in fission using isomeric yield rations, calculations of anti-neutrino spectra from nuclear reactors, as well as neutron and gamma-ray multiplicities in nuclear reactor calculations.
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15.
  • Cannarozzo, Simone (författare)
  • Isomeric yield ratio studies in nuclear reactions and alpha-particle induced fission of Thorium
  • 2024
  • Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • Despite decades of research since the initial discovery of nuclear fission, numerous unresolved questions still persist. It is known empirically that fission fragments emerge with high angular momentum. The mechanism responsible for the generation of the large angular momenta observed is one of these open questions. Since the characteristics of fission fragments are not directly measurable, experimentally accessible observables are used to derive the angular momenta using nuclear model codes. One of these observables is the yield ratio between fission products produced in different isomeric states, i.e., metastable energy levels of the same nucleus.In this thesis, a study of the level density models implemented in the nuclear model code TALYS is presented. Simulated and experimental isomeric yield ratios of a large number of nuclear reactions is compared. The results show a bias in the models that favours the population of the high-spin states and that this can be produced by the overestimation of the spin width distribution. The reason for this study is to improve the models then used in the angular momentum calculation. Moreover, the isomeric yield ratio measurement of twenty-one FFs is presented. The measurement was performed using the JYFLTRAP system at the University of Jyväskylä. The fission fragments were produced by the 32 MeV alpha-particle induced fission of 232Th. The analysis process, involving different identification and correction methods, and preliminary results are presented.
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16.
  • Chiodaroli, Marco, et al. (författare)
  • “Every morning I take two steps to my desk…” : students’ perspectives on distance learning during the COVID-19 pandemic
  • 2024
  • Ingår i: Higher Education. - : Springer Science+Business Media B.V.. - 0018-1560 .- 1573-174X.
  • Tidskriftsartikel (refereegranskat)abstract
    • During the COVID-19 pandemic, distance learning became the predominant teaching method at most universities, exposing students and teachers alike to novel and unexpected challenges and learning opportunities. Our study is situated in the context of higher physics education at a large Swedish university and adopts a mixed-methods approach to explore how students perceive shifts to distance learning. Quantitative student survey responses comparing distance learning during the pandemic with previous in-person learning are analyzed with k-means cluster analysis and with a random-intercept multilevel linear model. Combined analyses produce a consistent picture of students who report having experienced the greatest challenges. They are on average younger, report being less autonomous in their learning, and find it harder than peers to ask questions to the instructor. They are also less likely to have access to a place where they can study without interruptions. Variation across courses is small with students being largely subjected to the same set of challenges. Qualitative data from semi-structured focus group interviews and open-ended questions supports these findings, provides a deeper understanding of the struggles, and reveals possibilities for future interventions. Students report an overall collapse of structure in their learning that takes place along multiple dimensions. Our findings highlight a fundamental role played by informal peer-to-peer and student-instructor interactions, and by the exchange of what we refer to as “structural information.” We discuss implications for teachers and institutions regarding the possibility of providing support structures, such as study spaces, as well as fostering student autonomy.
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17.
  • Fritioff, Tomas, et al. (författare)
  • Precise measurements of ionic masses for QED tests
  • 2006
  • Ingår i: International Journal of Mass Spectrometry. - : Elsevier BV. - 1387-3806 .- 1873-2798. ; 251:2-3, s. 281-285
  • Tidskriftsartikel (refereegranskat)abstract
    • The Penning trap mass spectrometer SMILETRAP is designed for precision mass measurements using the merits of highly charged ions. In this paper we describe the feature of SMILETRAP and give examples of mass measurements involving , , and ions. These emphasize the importance of accurate masses of hydrogen-like and lithium-like ions that are required in the evaluation of g-factor measurements of electrons bound to even–even nuclei and test of QED effects. Highly precise mass measurements can also be used for testing atomic structure calculations and determining atomic binding energies. Relevance of such measurements throughout the periodic system is discussed.
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18.
  • Gao, Zhihao, et al. (författare)
  • Applying machine learning methods for the analysis of two-dimensional mass spectra
  • 2023
  • Ingår i: European Physical Journal A. - : Springer Nature. - 1434-6001 .- 1434-601X. ; 59:169
  • Tidskriftsartikel (refereegranskat)abstract
    • In a measurement of isomeric yield-ratios in fission, the Phase-Imaging Ion-Cyclotron-Resonance technique, which projects the radial motions of ions in the Penning trap (JYFLTRAP) onto a position-sensitive micro-channel plate detector, has been applied. To obtain the yield ratio, that is the relative population of two states of an isomer pair, a novel analysis procedure has been developed to determine the number of detected ions in each state, as well as corrections for the detector efficiency and decay losses. In order to determine the population of the states in cases where their mass difference is too small to reach full separation, a Bayesian Gaussian Mixture model was implemented. The position-dependent efficiency of the micro-channel plate detector was calibrated by mapping it with 133Cs+ ions, and a Gaussian Process was trained with the position data to construct an efficiency function that could be used to correct the recorded distributions. The obtained numbers of counts of excited and ground-state ions were used to derive the isomeric yield ratio, taking into account decay losses as well as feeding from precursors.
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19.
  • Gao, Zhihao, et al. (författare)
  • Benchmark of a multi-physics Monte Carlo simulation of an ionguide for neutron-induced fission products
  • 2022
  • Ingår i: European Physical Journal. - : Springer Nature. - 1286-0042 .- 1286-0050. ; 58:2
  • Tidskriftsartikel (refereegranskat)abstract
    • To enhance the production of medium-heavy,neutron-rich nuclei, and to facilitate measurements of independentyields of neutron-induced fission, a proton-toneutronconverter and a dedicated ion guide for neutroninducedfission have been developed for the IGISOL facilityat the University of Jyväskylä. The ion guide holds thefissionable targets, and the fission products emerging fromthe targets are collected in helium gas and transported to thedownstream experimental stations.Acomputer model, basedon a combination of MCNPX for modeling the neutron production,the fission code GEF, and GEANT4 for the transportof the fission products, was developed. The model willbe used to improve the setup with respect to the productionand collection of fission products. In this paper we benchmarkthe model by comparing simulations to a measurementin which fission products were implanted in foils located atdifferent positions in the ion guide. In addition, the productsfrom neutron activation in the titanium foil and the uraniumtargets are studied. The result suggests that the neutron fluxat the high-energy part of the neutron spectrum is overestimatedby approximately 40%.However, the transportation offission products in the uranium targets agrees with the experimentwithin 10%. Furthermore, the simulated transportationof fission products in the helium gas achieves almost perfectagreement with the measurement. Hence, we conclude thatthe model, after correction for the neutron flux, is well suitedfor optimization studies of future ion guide designs.
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20.
  • Gao, Zhihao (författare)
  • Benchmark of simulation of an ion guide for neutron-induced fission products
  • 2022
  • Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • Independent yield distributions of high-energy neutron-induced fission are of importance to achieve a good understanding of fission. Even though the mass and charge yield distributions of thermal neutron-induced fission are well known, there are few experimental data for high-energy neutron-induced fission. In addition to basic research on the fission process, independent yield distributions of high-energy neutron-induced fission play a key role in the development of Generation IV fast nuclear reactors.To facilitate measurements of independent fission yields of high-energy neutron-induced fission, a dedicated ion guide and a proton-neutron converter were developed and put to use in experiments at the isotope separator facility IGISOL in Jyväskylä. In parallel, a simulation model of the system was developed in order to optimize the collecting efficiency of fission products in the ion guide. The model uses the Monte Carlo code MCNPX to simulate the neutron production, the fission model code GEF to simulate the fission process, and GEANT4 for ion transportation. In order to benchmark the simulation model, metal foils were inserted in the ion guide with the purpose of collecting fission products. At the same time, nickel, cobalt and indium foils were located between the pn-converter and the ion guide to record the neutron flux from the pn-converter. After the beam was turned off, and after several days of cooling, g-ray spectroscopy measurements of the foils were conducted using a well shielded HPGe detector. Based on the identified g-ray transitions in the spectroscopy data, the productions of corresponding fission products and neutron activation products were calculated, and then used to benchmark the transportation and collection of fission products, as well as neutron production, in the simulations.The conclusion from the benchmark is that the transportation of fission products in the helium gas, as simulated by GEANT4, agrees very well with the measurement, while the transportation of fission products in the uranium targets agrees with the measurement within 10%. The neutron flux at the high-energy part of the neutron spectrum is overestimated by about 40%.Thanks to the benchmark it has been shown that the predictive power of the model is satisfactory and sufficient for the purpose of modeling the ion guide. Furthermore, the parameters involved in the simulations, such as neutron production, distance between the neutron source and the ion guide, volume of the ion guide and so on, play an important role in the optimization of the setup. However, the lower than expected fission rate suggests that the optimization on these parameters may not be enough to achieve a sufficiently high intensity of fission products, especially for nuclei far from the stability line. To achieve a sufficiently high intensity, an electric field guidance, similar to the RF structure of the CARIBU gas catcher presented in G.Savard et al. Nucl. Inst. Meth. B, 376: 246, 2016, to collect fission products is considered.
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21.
  • Gao, Zhihao, et al. (författare)
  • Estimating angular momenta of fission fragments from isomeric yield ratios using TALYS
  • 2024
  • Ingår i: Physical Review C. - : American Physical Society. - 2469-9985 .- 2469-9993. ; 109:6
  • Tidskriftsartikel (refereegranskat)abstract
    • Background: Angular momenta of fission fragments considerably higher than that of the fissioning nucleus have been observed in many experiments, raising the question of how these high angular momenta are generated. Wilson et al. have proposed a model for the angular momentum as a function of the mass of fission products based on the assumption that the angular momentum is generated from the collective motion of nucleons in the ruptured neck of the fissioning system. This assumption has caused a lot of debate in the community.Purpose: To estimate the angular momenta of fission fragments based on the observed isomeric yield ratios in 25 -MeV proton -induced fission of 238 U.Method: A surrogate model of the fission code general description of fission observables (GEF) has been developed to generate properties of primary fission fragments. Based on the excitation energy and angular momentum of fission fragments from GEF, an energy -versus -angular -momentum matrix is reconstructed using a set of parameters. With such matrices as input, the reaction code TALYS is used to calculate the deexcitation of the fission fragments, including the population of the isomers, from which the isomeric yield ratios are obtained. By varying one of the parameters, the root -mean -square angular momentum ( J rms ), which determines the angular momentum distribution of the matrix, J rms -dependent isomeric yield ratios are obtained. Considering all primary fission fragments contributing to the isomeric yield ratio for a given fission product, the average angular momentum of those fragments is estimated.Results: Data of 31 isomeric yield ratios in 25 -MeV proton -induced fission of 238 U were analyzed. From the analysis, the average J rms , equivalent to average angular momentum J av , with uncertainties are obtained for 24 fission products, while in seven cases no conclusive result for the angular momentum could be obtained. Furthermore, considering the neutron emissions of the primary fission fragments, the average angular momentum as a function of the average mass number of the primary fission fragment was estimated.Conclusion: A mass dependency of the average angular momentum is observed in the proton -induced fission of 238 U. Moreover, the average angular momenta for mass numbers larger than 131 could be fairly well described by the parametrization proposed by Wilson et al. However, the average angular momenta of 130 Sn and 131 Te cannot be described by Wilson's model, which suggests a different lower limit for the validation of the parametrization in the model. In general, higher average angular momenta for A 132 are observed in the present work compared to those from Wilson et al. This is likely due to the higher excitation energy of the fissioning nuclei in this work. Furthermore, the first systematic observation of the average angular momenta of fission products in the symmetric mass region is presented. In this region, a decreasing trend with mass number is observed, which cannot be explained by the proposal in Wilson's paper. Thus, a different mechanism is needed to explain this observation.
  •  
22.
  • Gao, Zhihao, et al. (författare)
  • Fission studies at IGISOL/JYFLTRAP : Simulations of the ion guide for neutron-induced fission and comparison with experimental data
  • 2020
  • Ingår i: ND 2019. - : EDP Sciences. - 9782759891061
  • Konferensbidrag (refereegranskat)abstract
    • For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation.In order to allow fission yield measurements in the low yield regions, towards the tails and in the symmetric part of the mass distribution, the stopping and extraction efficiency of the ion guide has to be significantly improved. This objective can be achieved by increasing the size while introducing electric field guidance using a combination of static electrodes and an RF-carpet. To this end, the GEANT4 model is used to optimise the design of such an ion guide.
  •  
23.
  • Gao, Zhihao (författare)
  • Isomeric yield ratios in nuclear fission
  • 2023
  • Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • Isomeric yield ratios (IYR), referring to the relative yield of the high spin states of a nucleus to the total yield of all observed states, is an observable of nuclear fission that has the potential to improve our understanding of the fission dynamics. Apart from that, systematic observations of IYRs can also contribute to other areas, such as the validation of fission models, modelling of the r-process in stellar nucleosynthesis, studies of the antineutrino mixing angle, the safety of present-day nuclear reactors, and the design of advanced reactor systems.With these motivations in mind, an IYR measurement in proton-induced fission was performed at the IGISOL facility in Jyväskylä, Finland. In the measurement, the Penning trap JYFLTRAP was used to separate the excited state from the ground state and to project those onto a position-sensitive MCP detector. The obtained phase images were used to train a Bayesian Gaussian Mixture model to identify the states. After considering corrections for the detector efficiency and radioactive decay, 19 IYRs were obtained.In this thesis, the measurement of IYRs with the IGISOL technique is described, and a systematic study of IYRs in proton-induced fission is presented. Furthermore, the measured ratios are compared with calculations using three different models: the Madland-England (ME) model, the fission model GEF, and the combination of GEF + TALYS. The experimental results show that, in general, the IYR decreases with the spins of measured states. While this, to some degree, confirms the ME model, variations in the IYR between nuclides with the same spin assignments reveal that the model is too simple to predict individual ratios. Furthermore,discrepancies in the IYRs between the measurement and GEF are observed in most cases, indicating a need to optimize the performance of GEF against nuclear data from proton-induced fission. The combination of GEF + TALYS results in an overall under estimation of the observedIYRs, which could be explained by the different assumptions used in GEF and TALYS.To investigate how the angular momenta of the primary fission fragments relate to the IYRs, a surrogate model of GEF has been developed. By reproducing the measured IYR with the calculated ratios from the model, the average angular momentum Jav, is deduced. The Jav for fission products with a mass number greater than 131 show a mass dependency which fits the parameterisation proposed by J. Wilson et al,. For IYRs in the mass region 119 ≤ A < 132, in which no measurements are presented by Wilson, a decrease in the Jav with increasing mass number is observed for the first time.Besides the study of IYRs, a benchmark of a multi-physics simulation model of the ion guide for neutron-induced fission products has been performed using γ-ray spectroscopy data. The results of the benchmark show that the high-energy part of the neutron flux from the simulation with MCNPX is overestimated by about 40 %, while the ion transportation simulated with GEANT4 agrees well with the experimental data. Based on the benchmark, the ion guide can be optimized to achieve high enough intensities of the collected ions to reach reasonable measurement times. In the next step, the addition of electric fields is considered to direct the ions in and to reduce the ion drifting time. However, this task lies outside the scope of this PhD thesis.
  •  
24.
  • Gao, Zhihao, et al. (författare)
  • Isomeric yield ratios in proton-induced fission of 238U
  • 2023
  • Ingår i: Physical Review C. - : American Physical Society. - 2469-9985 .- 2469-9993. ; 108:5
  • Tidskriftsartikel (refereegranskat)abstract
    • Background: Isomeric yield ratios are an important observable in nuclear fission as they can guide model development by providing insight into the angular momentum generation. Furthermore, isomeric yield ratios are important in applications for nuclear energy, as well as in the study of the r-process in stellar nucleosynthesis, and in the antineutrino mixing angle from reactor spectra. In nuclear data evaluations, the Madland-England model is commonly used to estimate isomeric yield ratios that have not been measured.Purpose: To measure isomeric yield ratios in 25-MeV proton-induced fission of 238U, and to compare the result with the values obtained from the Madland-England model and the fission model code GEF. Furthermore, to evaluate whether the predictions of GEF can be improved by coupling it to the nuclear reaction code TALYS.Methods: Isomeric yield ratios in 25-MeV proton-induced fission of 238U have been measured at the Ion GuideIsotope Separate On-Line facility. The excited state and the ground state were separated by mass using the Phase-Imaging Ion-Cyclotron-Resonance technique in the double Penning trap JYFLTRAP. The number of counts of each state was extracted from the phase-images using a Bayesian Gaussian Mixture model and, after corrections fordetector efficiency and decay, the isomeric yield ratios were derived. The experimental values have been compared with the calculated results from the Madland-England model and the GEF code. Furthermore, GEF has been combined with the nuclear reaction code TALYS, in order to take advantage of the latter codes’ implementation of the Hauser-Feshbach formalism, and the results have been compared with the experimental values.Results: From the measurements, 19 new isomeric yield ratios in 25-MeV proton-induced fission of 238U are reported and are, together with another 12 isomeric yield ratios (IYRs) from a previous campaign, compared with the model calculations. It is shown that, though the models manage to capture some of the features observed, there is room for improvement.Conclusions: As predicted by the Madland-England model, a strong correlation between the measured IYRs and the spins of the long-lived states of the fission products is confirmed. However, the IYRs also vary between nuclides with the same spin-parity of the two states, and systematic trends in the IYRs of close-lying isotopes and isotones with similar nuclear configurations are observed.From the comparison of the experimental data with the prediction of GEF it is concluded that more data from proton-induced fission are needed to optimize the internal parameters of GEF. Furthermore, using a combination of GEF and TALYS in most cases results in an underestimation of the yield ratios. This might be explained by an underestimation of the angular momentum on the initial fission fragments by GEF. Altogether, these results highlight the possibility to use measurements of IYRs to improve model predictions and to study the angular momentum generation in nuclear fission.
  •  
25.
  • Gao, Zhihao, et al. (författare)
  • New design and simulation of the ion guide for neutron-induced fission products at the IGISOL facility
  • 2023
  • Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 2100-014X. ; 284
  • Tidskriftsartikel (refereegranskat)abstract
    • Measurements of independent fission yield distributions in neutron-induced fission at high neutron energies are important for our fundamental understanding of the fission process, and are also relevant for reactor physics applications. So far, measurements of independent fission yields in proton-induced fission have been performed at the IGISOL facility at the University of Jyväskylä, using the Penning trap as a high resolving-power mass-filter. In order to also facilitate measurements of neutron-induced fission, a dedicated ion guide and a proton-to-neutron converter was developed. However, the first measurement indicates that fewer fission products than expected reach the Penning trap. To explore potential reasons and possible improvements, a simulation model was also developed and benchmarked. The benchmark showed that the model is able to reproduce the performance of the ion guide remarkably well and that the main reason for the low yield of fission products is the low collection efficiency of the ion guide.Based on the benchmark, a new ion guide is being designed. In the new design, the positions of the uranium targets and volume of the ion guide have been changed to increase the collection of fission products. This results in a five-fold increase of the yield. However, the collection efficiency of the new ion guide still needs to be improved in order to achieve intensities of the extracted fission products that are large enough to allow for reasonable measurement times.Because the volume of the ion guide is increased significantly, the extraction time of the ions is expected to be longer than that from the previous ion guide. Therefore, an electric field guidance system that consists of a combination of a stationary electric field and an RF-carpet is considered to be deployed. The stationary field, produced from a set of DC-ring electrodes, accelerates the ions towards the RF-carpet at end plate of the ion guide. The RF-carpet consists of a time-dependent field, produced from a radio-frequent structure of concentric rings, with a DC-component that guides the ions towards the exit hole in the center of the end plate. In this paper we present the current status of the simulations and design of the new ion guide.
  •  
26.
  • Gomez L, Ana Maria, 1993- (författare)
  • Simulations And Experiments Of Plasma-Induced Effects In Silicon Detectors
  • 2023
  • Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • When an atomic nucleus undergoes fission, two fragments with different mass and kinetic energy are emitted. The highly unstable fission fragments (FFs) evaporate prompt neutrons soon after the nucleus splits. A precise measurement of both, the mass yield distribution of the FFs and the average prompt neutron emission, $\bar{\nu}$, is important not only for current nuclear technologies but also for the development of future technologies such as Generation IV nuclear power plants. Moreover, the experimental determination of the mass yield distributions, both pre- and post-neutron emission, is valuable for testing fission models. Additionally, a precise measurement of the average neutron multiplicity as a function of the FFs mass, , is crucial in the understanding of how the excitation energy is shared between nascent FFs. The VElocity foR DIrect particle identification spectrometer (VERDI) is designed to achieve pre- and post-fission mass distributions with resolutions between 1-2 u. VERDI is a double-energy double-velocity instrument that consists of two arms. On each arm is operated one Microchannel Plate detector (MCP) for the collection of the FFs start time and up to 32 Passive Implanted Planar Silicon (PIPS) detectors for the stop time and energy detection of the FFs. However, challenges in the experimental measurements with VERDI arise due to the high degree of ionization (plasma) in the detector material from the interaction with the FFs. The plasma causes a delay in the charge carriers' migration for the signal start, known as the plasma delay time effect (PDT). Furthermore, the recombination of charge carriers in the plasma causes a shrinking in the signal's height, known as pulse height defect (PHD). This phenomenon leads to inaccuracies in the measurement of FFs mass distributions and increased systematic uncertainties. Previous studies on PDT and PHD have shown varying behaviors across different detector types, which motivated dedicated studies in the type of PIPS detectors used in VERDI. An experimental campaign to characterize the PDT and PHD in PIPS detectors was conducted in the LOHENGRIN recoil separator, which is part of the ILL nuclear facility in Grenoble, France. Measurements of FFs in a range of masses between 80 u and 149 u, with energies between 20 MeV to 110 MeV, were taken to fully characterize six PIPS detectors. The resulting PDT and PHD values were 1 ns to 4 ns and 2 MeV to 10 MeV respectively. The PDT and PHD exhibited consistent energy and mass dependencies across the detectors, which enables the possibility of an event-by-event correction of VERDI data. In this thesis, the basis for discussing the results of the studies of the PDT and PHD effects will be presented.
  •  
27.
  •  
28.
  • Gorelov, D., et al. (författare)
  • Developments for neutron-induced fission at IGISOL-4
  • 2016
  • Ingår i: Nuclear Instruments and Methods in Physics Research Section B. - : Elsevier BV. - 0168-583X .- 1872-9584.
  • Tidskriftsartikel (refereegranskat)abstract
    • Abstract At the IGISOL-4 facility, neutron-rich, medium mass nuclei have usually been produced via charged particle-induced fission of natural uranium and thorium. Neutron-induced fission is expected to have a higher production cross section of the most neutron-rich species. Development of a neutron source along with a new ion guide continues to be one of the major goals since the commissioning of IGISOL-4. Neutron intensities at different angles from a beryllium neutron source have been measured in an on-line experiment with a 30 MeV proton beam. Recently, the new ion guide coupled to the neutron source has been tested as well. Details of the neutron source and ion guide design together with preliminary results from the first neutron-induced fission experiment at IGISOL-4 are presented in this report.
  •  
29.
  • Gorelov, D., et al. (författare)
  • Isomeric Yield Ratios of Fission Products Measured with the Jyfltrap
  • 2014
  • Ingår i: Acta Physica Polonica B. - 0587-4254 .- 1509-5770. ; 45:2, s. 211-216
  • Tidskriftsartikel (refereegranskat)abstract
    • Experimental methods to determine isomeric yield ratios usually apply gamma-spectroscopic techniques. In such methods, ground and isomeric states are distinguished by their decays. In the present work, several isomeric yield ratios of fission products have been measured by utilizing capabilities of the double Penning-trap mass spectrometer JYFLTRAP, where isomeric and ground state were separated by their masses. To verify the new experimental technique, the results were compared to those from gamma-spectroscopy measurements.
  •  
30.
  • Gorelov, D., et al. (författare)
  • Measuring independent yields of fission products using a penning trap
  • 2015
  • Ingår i: Bulletin of the Russian Academy of Sciences: Physics. - 1062-8738. ; 79:7, s. 869-871
  • Tidskriftsartikel (refereegranskat)abstract
    • A new method for determining independent fission products is used in an experiment at the Accelerator Laboratory of the University of Jyväskylä. The method combines the chemical universality of the ion guide technique and the unique properties of the Penning trap. A beam of charged particles is formed by stopping fission products in gaseous helium. The Penning trap is employed as a highly accurate filter to identify particles by their mass. The yields of fission products are determined by the ion count downstream of the trap. The setup’s mass resolving power is on the order of 105 with a radio frequency excitation time of 400 ms. Such high mass resolution occasionally allows us not only to separate nuclides but to separate the isomeric and ground states of nuclei as well. Independent yields of fission products are measured in the fission reaction of the 232Th isotope by protons with an energy of 25 MeV. A short description of the method ae nd soexperimental data are supplememnted by the results fro theoretical calculations.
  •  
31.
  • Hambsch, Franz-Josef, et al. (författare)
  • Prompt fission neutron emission from 235U(n,f): thermal and resonance region
  • 2015
  • Ingår i: Conference: 14th International Conference on Nuclear Reaction Mechanisms - CERN-Proceedings-2015-001, At Villa Monastero, Varenna, Italy. - 9789290834182
  • Konferensbidrag (refereegranskat)abstract
    • For nuclear modelling and improved evaluation of nuclear data, knowledge of fluctuations of the prompt neutron multiplicity as a function of incident neutron energy is requested for the major actinides 235U and 239Pu. Experimental investigations of the prompt fission neutron emission in resonance-neutron induced fission on 235U are taking place at the GELINA facility of the IRMM. The experiment employs an array of scintillation detectors (SCINTIA) in conjunction with a newly designed 3D position-sensitive twin Frisch-grid ionization chamber. In addition, the mass-dependent prompt neutron multiplicity, (A), has attracted particular attention. Recent, sophisticated nuclear fission models predict that the additional excitation energy, brought into the fission system at higher incident neutron energies, leads to an increased neutron multiplicity only for heavy fragments, as observed in the 237Np(n,f) reaction. A first feasibility study has been performed at the JRC-IRMM VdG accelerator to measure nu(A) for 235U(n,f).
  •  
32.
  • Hobein, Matthias, et al. (författare)
  • A compact time-resolving pepperpot emittance meter for low-energy highly charged ions
  • 2011
  • Ingår i: Physica Scripta. - 0031-8949 .- 1402-4896. ; T144, s. 014062-
  • Tidskriftsartikel (refereegranskat)abstract
    • An emittance meter for pulsed, low-energy ion beams was developed. Based on the pepperpot method, the device is compact and portable. It has been installed at the S-EBIT Laboratory at AlbaNova, Stockholm University, to measure the emittance of highly charged ions extracted from the electron beam ion trap R-EBIT and the cooling trap of the high-precision Penning trap mass spectrometer SMILETRAP II. Using a fast delay-line anode detector, the emittance and time-of-flight of the extracted ions can be measured simultaneously. In this paper, design and data processing system are described and preliminary results are presented.
  •  
33.
  •  
34.
  • Hobein, Matthias, et al. (författare)
  • Evaporative Cooling and Coherent Axial Oscillations of Highly Charged Ions in a Penning Trap
  • 2011
  • Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 106:1, s. 013002-
  • Tidskriftsartikel (refereegranskat)abstract
    • Externally, in an electron beam ion trap, generated Ar16+ ions were retrapped in a Penning trap and evaporatively cooled in their axial motion. The cooling was observed by a novel extraction technique based on the excitation of a coherent axial oscillation which yields short ion bunches of well-defined energies. The initial temperature of the ion cloud was decreased by a factor of more than 140 within 1 s, while the phase-space density of the coldest extracted ion pulses was increased by a factor of up to about 9.
  •  
35.
  • Hobein, Matthias, 1981-, et al. (författare)
  • Optimization of the Stockholm R-EBIT for the production and extraction of highly charged ions
  • 2010
  • Ingår i: Journal of Instrumentation. - 1748-0221. ; 5:C11003
  • Tidskriftsartikel (refereegranskat)abstract
    • We describe a refrigerated EBIT (R-EBIT) commissioned at the AlbaNova Research Center at Stockholm University. As an innovative solution, the superconducting magnet and the trapping drift tubes of the R-EBIT are cooled to a temperature of 4 K by a set of two cooling heads connected to helium compressors. This dry, i.e. liquid helium and liquid nitrogen free, system is easily operated and creates highly charged ions at a fraction of the cost of traditional liquid-cooled systems. A pulsed and continuous gas injection system was developed to feed neutral particles into the electron beam in the trap region. This improves significantly the highly charged ion production and R-EBIT performance. Fast extraction of ions from the R-EBIT yields very short ( < 100 ns), charge-separated ion bunches which can be either analysed using a straight time-of-flight section or sent to experimental beam lines following selection in a bending magnet. An emittance meter was used to measure the emittance of the ions extracted from the R-EBIT. The extracted ions were also re-trapped in a cylindrical Penning trap and properties of the re-trapped ions have been measured using the emittance meter. Results of these measurements are reported in this publication.
  •  
36.
  • Hobein, Matthias, et al. (författare)
  • Re-trapping and cooling of highly-charged
  • 2009
  • Ingår i: Journal of Physics, Conference Series. - : IOP Publishing. - 1742-6588 .- 1742-6596. ; 163, s. 012109-
  • Tidskriftsartikel (refereegranskat)abstract
    • Presently, a trapping system for cooling highly-charged ions (HCI) is being set up at AlbaNova at Stockholm University. The experiment aims at production of low temperature (emittance) HCI at very low energy. HCI are extracted from the new Stockholm EBIT (S-EBIT) before evaporative cooling is applied in a Penning trap. In the future the cooled ions will be injected into the precision trap of the high-precision mass spectrometer SMILETRAP II. In first tests the emittance of trapped ions was measured and it was shown that highly and low-charged ions could be simultaneously stored
  •  
37.
  • Hobein, Matthias, 1981-, et al. (författare)
  • SMILETRAP II
  • 2011
  • Ingår i: Hyperfine Interactions. - : Springer Netherlands. - 0304-3843 .- 1572-9540. ; 199:1-3, s. 141-150
  • Tidskriftsartikel (refereegranskat)abstract
    • The new Penning trap mass spectrometer SMILETRAP II has been set up at the AlbaNova Research Center, Stockholm. Based on the former spectrometer SMILETRAP I, it uses the merits of highly-charged ions to achieve high precision in the mass measurements. Various improvements over the SMILETRAP I setup will allow to routinely perform mass measurements with relative uncertainties of 10−10 and below. In this paper we will discuss the limitations of SMILETRAP I and present the corresponding improvements of SMILETRAP II. An overview on the SMILETRAP II setup is given.
  •  
38.
  • Jansson, Kaj, 1987-, et al. (författare)
  • Simulated production rates of exotic nuclei from the ion guide for neutron-induced fission at IGISOL
  • 2017
  • Ingår i: European Physical Journal A. - : Springer. - 1434-6001 .- 1434-601X. ; 53:12
  • Tidskriftsartikel (refereegranskat)abstract
    • An investigation of the stopping efficiency of fission products, in the new ion guide designed for ion production through neutron-induced fission at IGISOL in Jyväskylä, Finland, has been conducted. Our simulations take into account the new neutron converter, enabling measurements of neutron-induced fission yields, and thereby provide estimates of the obtained yields as a function of primary proton beam current. Different geometries, targets, and pressures, as well as models for the effective charge of the stopped ions were tested, and optimisations to the setup for higher yields are suggested. The predicted number of ions stopped in the gas lets us estimate the survival probability of the ions reaching the downstream measurements stations.
  •  
39.
  • Lantz, Mattias, et al. (författare)
  • Design of a High Intensity Neutron Source for Neutron-Induced Fission Yield Studies
  • 2012
  • Ingår i: Use of Neutron Beams for High Precision Nuclear Data Measurements. - Vienna.
  • Konferensbidrag (refereegranskat)abstract
    • The upgraded IGISOL facility with JYFLTRAP, at the accelerator laboratory of the University of Jyväskylä, has been supplied with a new cyclotron which will provide protons of the order of 100 μA with up to 30 MeV energy, or deuterons with half the energy and intensity. This makes it an ideal place for measurements of neutron-induced fission products from various actinides, in view of proposed future nuclear fuel cycles. The groups at Uppsala University and University of Jyväskylä are working on the design of a neutron converter that will be used as neutron source in fission yield studies. The design is based on simulations with Monte Carlo codes and a benchmark measurement that was recently performed at The Svedberg Laboratory in Uppsala. Inorder to obtain a competitive count rate the fission targets will be placed very close to the neutron converter. The goal is to have a flexible design that will enable the use of neutron fields with different energy distributions. In the present paper, some considerations for the design of the neutron converter will be discussed, together with different scenarios for which fission targets and neutron energies to focus on.
  •  
40.
  •  
41.
  • Lantz, Mattias, et al. (författare)
  • Fission yield measurements at IGISOL
  • 2016
  • Ingår i: CNR*15 - 5th International Workshop On Compound-Nuclear Reactions And Related Topics. - : EDP Sciences.
  • Konferensbidrag (refereegranskat)abstract
    • The fission product yields are an important characteristic of the fission process. In fundamental physics, knowledge of the yield distributions is needed to better understand the fission process. For nuclear energy applications good knowledge of neutron-induced fission-product yields is important for the safe and efficient operation of nuclear power plants. With the Ion Guide Isotope Separator On-Line (IGISOL) technique, products of nuclear reactions are stopped in a buffer gas and then extracted and separated by mass. Thanks to the high resolving power of the JYFLTRAP Penning trap, at University of Jyvaskyla, fission products can be isobarically separated, making it possible to measure relative independent fission yields. In some cases it is even possible to resolve isomeric states from the ground state, permitting measurements of isomeric yield ratios. So far the reactions U(p,f) and Th(p,f) have been studied using the IGISOL-JYFLTRAP facility. Recently, a neutron converter target has been developed utilizing the Be(p,xn) reaction. We here present the IGISOL-technique for fission yield measurements and some of the results from the measurements on proton induced fission. We also present the development of the neutron converter target, the characterization of the neutron field and the first tests with neutron-induced fission.
  •  
42.
  • Liu, Yuwen, et al. (författare)
  • Improved temperature regulation of Penning trap mass spectrometers
  • 2010
  • Ingår i: Nuclear Instruments and Methods in Physics Research Section A. - : Elsevier BV. - 0168-9002 .- 1872-9576. ; 294:1, s. 28-32
  • Tidskriftsartikel (refereegranskat)abstract
    • In order to reach relative uncertainties in mass measurements with Penning traps of 10-10 or better, the temperature variation of the trap and surrounding materials must be kept below 10 mK. Temperature variations induce a shift in the measured ion cyclotron frequency because of non-zero, temperature dependent magnetic susceptibilities of the construction materials. In this paper we report of a new temperature regulation system recently installed at SMILETRAP II that manages to keep the temperature fixed at the set point with a standard deviation of only 2.6 mK. −10 or better, the temperature variation of the trap and surrounding.
  •  
43.
  • Malec, Jan, et al. (författare)
  • On teaching experimental reactor physics in times of pandemic
  • 2021
  • Ingår i: ANIMMA 2021 - Advancements in nuclear instrumentation measurement methods and their applications. - : EDP Sciences.
  • Konferensbidrag (refereegranskat)abstract
    • The COVID-19 induced restrictions have prevented reactor physics students from attending in-person reactor physics exercises which are a vital part of their education. Jozef Stefan Institute has organized remote exercises with the help of off-the-shelf technology, including multiple videoconferencing setups, remote desktop software, portable cameras, a dome camera, shared spreadsheets, and a common whiteboard. The students were encouraged to actively participate in the exercises by giving instructions to the reactor operator, asking and answering questions, logging data, operating digital acquisition systems, and performing analysis during the exercise. The first remote exercises were organized as a five-day course of experimental reactor physics for students from Uppsala University. The feedback was collected after the course using an anonymous online form and was generally positive but has revealed some problems with sound quality which were resolved later. The Jozef Stefan Institute can also organize a remote course during a full lockdown when the reactor is not able to operate using the in-house developed Research Reactor Simulator based on a point kinetics approximation and a simple thermohydraulic module.
  •  
44.
  • Malec, Jan, et al. (författare)
  • Remote research reactor exercises during pandemic induced lockdown
  • 2021
  • Ingår i: 30TH INTERNATIONAL CONFERENCE NUCLEAR ENERGY FOR NEW EUROPE (NENE 2021). - : NUCLEAR SOCIETY SLOVENIA. - 9789616207515
  • Konferensbidrag (refereegranskat)abstract
    • The COVID-19 induced restrictions have prevented reactor physics students from attending in-person reactor physics exercises which are a vital part of their education. Jo.zef Stefan Institute has organized remote exercises with the help of off-the-shelf technology, including multiple videoconferencing setups, remote desktop software, portable cameras, a dome camera, shared spreadsheets, and a common whiteboard. The students were encouraged to actively participate in the exercises by giving instructions to the reactor operator, asking and answering questions, logging data, operating digital acquisition systems, and performing analysis during the exercise. The first remote exercises were organized as a five-day course of experimental reactor physics for students from Uppsala University. The feedback was collected after the course using an anonymous online form. The aspects being evaluated included the technical content, quality of material, performance of the individual lecturers and the quality of the remote session. In general, the response was overwhelmingly positive, with most questions with a rating scale answered with "excellent".
  •  
45.
  •  
46.
  • Mattera, Andrea, 1985-, et al. (författare)
  • A methodology for the intercomparison of nuclear fission codes using TALYS
  • 2017
  • Ingår i: ND 2016. - Les Ulis : EDP Sciences. - 9782759890200
  • Konferensbidrag (refereegranskat)abstract
    • Codes for the calculation of fission observables are frequently used to describe experimentally observed phenomena as well as provide predictions in cases where measurements are missing. Assumptions in the models, and tuning of parameters within the codes, often result in a good reproduction of experimental data. In this work we propose a methodology, coded in the newly developed program DELFIN (De-Excitation of FIssion fragmeNts), that can be used to compare some of the assumptions of the various models. Our code makes use of the fission fragments information after scission and processes them in an independent and consistent fashion to obtain measurable fission observables (such as ν(A) distributions and Isomeric Fission Yield ratios). All the available information from the models, such as fragments' excitation energies, spin distributions and yields are provided as input to DELFIN that uses the nuclear reaction code TALYS to handle the de-excitation of the fission fragments. In this way we decouple the fragments relaxation from the actual fission models. We report here the first results of a comparison carried out on the GEF, Point-by-Point and FREYA models for thermal fission of 235U and 239Pu and spontaneous fission of 252Cf.
  •  
47.
  • Mattera, Andrea, 1985-, et al. (författare)
  • A neutron source for IGISOL-JYFLTRAP : Design and characterisation
  • 2017
  • Ingår i: European Physical Journal A. - : Springer Science and Business Media LLC. - 1434-6001 .- 1434-601X. ; 53:173
  • Tidskriftsartikel (refereegranskat)abstract
    • A white neutron source based on the Be(p,nx) reaction for fission studies at the IGISOLJYFLTRAP facility has been designed and tested. 30 MeV protons impinge on a 5mm thick water-cooled beryllium disc. The source was designed to produce at least 1012 fast neutrons/s on a secondary fission target, in order to reach competitive production rates of fission products far from the valley of stability.The Monte Carlo codes MCNPX and FLUKA were used in the design phase to simulate the neutron energy spectra. Two experiments to characterise the neutron field were performed: the first was carried out at The Svedberg Laboratory in Uppsala (SE), using an Extended-Range Bonner Sphere Spectrometer and a liquid scintillator which used the time-of-flight (TOF) method to determine the energy of the neutrons; the second employed Thin-Film Breakdown Counters for the measurement of the TOF, and activation foils, at the IGISOL facility in Jyväskylä (FI). Design considerations and the results of the two characterisation measurements are presented, providing benchmarks for the simulations.
  •  
48.
  •  
49.
  • Mattera, Andrea, 1985-, et al. (författare)
  • Characterization of a Be(p,xn) neutron source for fission yields measurements
  • 2014
  • Ingår i: Nuclear Data Sheets. - : Elsevier BV. - 0090-3752 .- 1095-9904. ; 119, s. 416-418
  • Tidskriftsartikel (refereegranskat)abstract
    • We report on measurements performed at The Svedberg Laboratory (TSL) to characterize a proton-neutron converter for independent fission yield studies at the IGISOL-JYFLTRAP facility (Jyväskylä, Finland). A 30-MeV proton beam impinged on a 5 mm water-cooled Beryllium target. Two independent experimental techniques have been used to measure the neutron spectrum: a Time-of-Flight (TOF) system to estimate the high-energy contribution, and a Bonner Sphere Spectrometer to provide precise results from thermal energies up to 20 MeV. An overlap between the energy regions covered by the two systems will permit a cross-check of the results from the different techniques. In this paper, the measurement and the analysis technique will be presented together with some preliminary results.
  •  
50.
  •  
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