| 1. |
- Kuang, Chaoyang, et al.
(författare)
-
Switchable Broadband Terahertz Absorbers Based on Conducting Polymer-Cellulose Aerogels
- 2023
-
Ingår i: Advanced Science. - : WILEY. - 2198-3844.
-
Tidskriftsartikel (refereegranskat)abstract
- Terahertz (THz) technologies provide opportunities ranging from calibration targets for satellites and telescopes to communication devices and biomedical imaging systems. A main component will be broadband THz absorbers with switchability. However, optically switchable materials in THz are scarce and their modulation is mostly available at narrow bandwidths. Realizing materials with large and broadband modulation in absorption or transmission forms a critical challenge. This study demonstrates that conducting polymer-cellulose aerogels can provide modulation of broadband THz light with large modulation range from ≈ 13% to 91% absolute transmission, while maintaining specular reflection loss < −30 dB. The exceptional THz modulation is associated with the anomalous optical conductivity peak of conducting polymers, which enhances the absorption in its oxidized state. The study also demonstrates the possibility to reduce the surface hydrophilicity by simple chemical modifications, and shows that broadband absorption of the aerogels at optical frequencies enables de-frosting by solar-induced heating. These low-cost, aqueous solution-processable, sustainable, and bio-friendly aerogels may find use in next-generation intelligent THz devices.
|
|
| 2. |
- Wang, Lanjing, et al.
(författare)
-
Non-linear effects of the built environment and social environment on bus use among older adults in china : An application of the xgboost model
- 2021
-
Ingår i: International Journal of Environmental Research and Public Health. - : MDPI AG. - 1661-7827 .- 1660-4601. ; 18:18
-
Tidskriftsartikel (refereegranskat)abstract
- Global aging has raised increasing concerns on the health and well-being of older adults. Public transport is a viable option to improve the mobility and quality of life among older adults. However, policies that promote the public transport use among older adults are rare. This study utilizes the eXtreme Gradient Boosting (XGBoost) decision tree to explore the non-linear associations of the built and social environment with bus use among older adults in China. The bus use of older adults was obtained from the Zhongshan Household Travel Survey (ZHTS) in 2012. Results show that non-linear relationships exist among all built environment and social environment characteristics. Within certain thresholds, the percentage of green space land use, land use mixture, bus-stop density, and dwelling unit density are positively related to bus use among older adults. Like-wise, one social environment variable, the proportion of older adults in a neighborhood, is the key social environment variable. Furthermore, the dwelling unit density and proportion of older adults appear to have an inverse U-shaped relationship. Additionally, age, ownership of motorcycles, and distance from home to the nearest bus stop also show non-linearity. The findings presented in this paper facilitate effective planning interventions to promote bus use among older adults.
|
|
| 3. |
- Wang, Wenxiao, et al.
(författare)
-
Nonlinear associations of the built environment with cycling frequency among older adults in Zhongshan, China
- 2021
-
Ingår i: International Journal of Environmental Research and Public Health. - : MDPI AG. - 1661-7827 .- 1660-4601. ; 18:20
-
Tidskriftsartikel (refereegranskat)abstract
- The health and welfare of older adults have raised increasing attention due to global aging. Cycling is a physical activity and mode of transportation to enhance the mobility and quality of life among older adults. Nevertheless, the planning strategies to promote cycling among older adults are underutilized. Therefore, this paper describes the nonlinear associations of the built environment with cycling frequency among older adults. The data were collected from the Zhongshan Household Travel Survey (ZHTS) in 2012. The modeling approach was the eXtreme Gradient Boosting (XGBoost) model. The findings demonstrated that nonlinear relationships exist among all the selected built environment attributes. Within specific intervals, the population density, the land-use mixture, the distance from home to the nearest bus stop, and the distance from home to CBD are positively correlated to the cycling among older adults. Additionally, an inverse “U”-shaped relationship appears in the percentage of green space land use among all land uses. Moreover, the intersection density is inversely related to the cycling frequency among older adults. These findings provide nuanced and appropriate guidance for establishing age-friendly neighborhoods.
|
|
| 4. |
- Wu, Jiani, et al.
(författare)
-
Non-linear Relationships Between the Built Environment and Walking Frequency Among Older Adults in Zhongshan, China
- 2021
-
Ingår i: Frontiers in Public Health. - : Frontiers Media SA. - 2296-2565. ; 9
-
Tidskriftsartikel (refereegranskat)abstract
- Aim: Promoting walking activity is an effective way to improve the health of older adults. Walking frequency is a critical component of walking behavior and an essential determinant of daily walking levels. To decipher the association between the built environment and walking frequency among older adults, this study's aims are as follows: (1) to empirically test whether non-linear relationships between the two exist, and (2) to identify the thresholds of the built environment characteristics that promote walking. Methods: The walking frequency of old adults was derived from the Zhongshan Household Travel Survey (ZHTS) in 2012. The sample size of old adults aged 60 or over was 4784 from 274 urban and rural neighborhoods. A semi-parametric generalized additive model (GAMM) is used to analyze the non-linear or non-monotonic relationships between the built environment and the walking frequency among older adults. Results: We found that non-linear relationships exist among five out of the six built environment characteristics. Within certain thresholds, the population density, sidewalk density, bus stop density, land use mixture, and the percentage of green space are positively related to older adults' walking trips. Furthermore, the land use mixture and the percentage of green space show an inverse “V”-shaped relationship. Conclusions: Built environment features can either support or hinder the walking frequency among older adults. The findings in the current study contribute to effective land use and transport policies for promoting active travel among older adults.
|
|
| 5. |
- Zhao, Chaoyang, et al.
(författare)
-
A massive expansion of effector genes underlies gall-formation in the wheat pest Mayetiola destructor
- 2015
-
Ingår i: Current Biology. - : Elsevier BV. - 1879-0445 .- 0960-9822. ; 25:5, s. 613-620
-
Tidskriftsartikel (refereegranskat)abstract
- Gall-forming arthropods are highly specialized herbivores that, in combination with their hosts, produce extended phenotypes with unique morphologies [1]. Many are economically important, and others have improved our understanding of ecology and adaptive radiation [2]. However, the mechanisms that these arthropods use to induce plant galls are poorly understood. We sequenced the genome of the Hessian fly (Mayetiola destructor; Diptera: Cecidomyiidae), a plant parasitic gall midge and a pest of wheat (Triticum spp.), with the aim of identifying genic modifications that contribute to its plant-parasitic lifestyle. Among several adaptive modifications, we discovered an expansive reservoir of potential effector proteins. Nearly 5% of the 20,163 predicted gene models matched putative effector gene transcripts present in the M. destructor larval salivary gland. Another 466 putative effectors were discovered among the genes that have no sequence similarities in other organisms. The largest known arthropod gene family (family SSGP-71) was also discovered within the effector reservoir. SSGP-71 proteins lack sequence homologies to other proteins, but their structures resemble both ubiquitin E3 ligases in plants and E3-ligase-mimicking effectors in plant pathogenic bacteria. SSGP-71 proteins and wheat Skp proteins interact in vivo. Mutations in different SSGP-71 genes avoid the effector-triggered immunity that is directed by the wheat resistance genes H6 and H9. Results point to effectors as the agents responsible for arthropod-induced plant gall formation.
|
|
| 6. |
- Zhao, Haifeng, et al.
(författare)
-
Efficient and High-Luminance Perovskite Light-Emitting Diodes Based on CsPbBr3 Nanocrystals Synthesized from a Dual-Purpose Organic Lead Source
- 2020
-
Ingår i: Small. - : WILEY-V C H VERLAG GMBH. - 1613-6810 .- 1613-6829.
-
Tidskriftsartikel (refereegranskat)abstract
- Rational engineering of the surface properties of perovskite nanocrystals (PeNCs) is critical to obtain light emitters with simultaneous high photoluminescence efficiency and excellent charge transport properties for light-emitting diodes (LEDs). However, the commonly used lead halide sources make it hard to rationally optimize the surface compositions of the PeNCs. In addition, previously developed ligand engineering strategies for conventional inorganic nanocrystals easily deteriorate surface properties of the PeNCs, bringing additional difficulties in optimizing their optoelectronic properties. In this work, a novel strategy of employing a dual-purpose organic lead source for the synthesis of highly luminescent PeNCs with enhanced charge transport property is developed. Lead naphthenate (Pb(NA)(2)), of which the metal ions work as lead sources while the naphthenate can function as the surface ligands afterward, is explored and the obtained products under different synthesis conditions are comprehensively investigated. Monodispersed cesium lead bromide (CsPbBr3) with controllable size and excellent optical properties, showing superior photoluminescence quantum yields up to 80%, is obtained. Based on the simultaneously enhanced electrical properties of the Pb(NA)(2)-derived PeNCs, the resultant LEDs demonstrate a high peak external quantum efficiency of 8.44% and a superior maximum luminance of 31 759 cd cm(-2).
|
|
| 7. |
- Zhao, Haifeng, et al.
(författare)
-
High-Brightness Perovskite Light-Emitting Diodes Based on FAPbBr(3) Nanocrystals with Rationally Designed Aromatic Ligands
- 2021
-
Ingår i: ACS Energy Letters. - : AMER CHEMICAL SOC. - 2380-8195. ; 6:7, s. 2395-2403
-
Tidskriftsartikel (refereegranskat)abstract
- Despite rapid developments of light-emitting diodes (LEDs) based on emerging perovskite nanocrystals (PeNCs), it remains challenging to achieve devices with integrated high efficiencies and high brightness because of the insulating long-chain ligands used for the PeNCs. Herein, we develop highly luminescent and stable formamidinium lead bromide PeNCs capped with rationally designed short aromatic ligands of 2-naphthalenesulfonic acid (NSA) for LEDs. Compared with commonly used oleic acid ligands, the NSA molecules not only preserve the surface properties of the PeNCs during the purification but also notably improve the electrical properties of the assembled emissive layers, ensuring efficient charge injection/transport in the devices. The resulting champion LED with electroluminescence approaching the Rec. 2020 green primary color demonstrates a high brightness of 67 115 cd cm(-2) and a peak external quantum efficiency of 19.2%. More impressively, the device shows negligibly decreased efficiency at an elevated brightness of 20 000 cd cm(-2) and a well-retained efficiency of over 10% at around 65 000 cd cm(-2), presenting a breakthrough in LEDs based on PeNCs.
|
|
