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1.	Le Breton, Michael, 1986, et al. (författare) Chlorine oxidation of VOCs at a semi-rural site in Beijing: significant chlorine liberation from ClNO2 and subsequent gas- and particle-phase Cl-VOC production 2018 Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 18:17, s. 13013-13030:18, s. 13013-13030 Tidskriftsartikel (refereegranskat)abstract Nitryl chloride (ClNO2) accumulation at night acts as a significant reservoir for active chlorine and impacts the following day's photochemistry when the chlorine atom is liberated at sunrise. Here, we report simultaneous measurements of N2O5 and a suite of inorganic halogens including ClNO2 and reactions of chloride with volatile organic compounds (Cl-VOCs) in the gas and particle phases utilising the Filter Inlet for Gas and AEROsols time-of-flight chemical ionisation mass spectrometer (FIGAERO-ToF-CIMS) during an intensive measurement campaign 40 km northwest of Beijing in May and June 2016. A maximum mixing ratio of 2900 ppt of ClNO2 was observed with a mean campaign nighttime mixing ratio of 487 ppt, appearing to have an anthropogenic source supported by correlation with SO2, CO and benzene, which often persisted at high levels after sunrise until midday. This was attributed to such high mixing ratios persisting after numerous e-folding times of the photolytic lifetime enabling the chlorine atom production to reach 2.3 x 10(5) molecules cm(-3) from ClNO2 alone, peaking at 09:30 LT and up to 8.4 x 10(5) molecules cm(-3) when including the supporting inorganic halogen measurements. Cl-VOCs were observed in the particle and gas phases for the first time at high time resolution and illustrate how the iodide ToF-CIMS can detect unique markers of chlorine atom chemistry in ambient air from both biogenic and anthropogenic sources. Their presence and abundance can be explained via time series of their measured and steady-state calculated precursors, enabling the assessment of competing OH and chlorine atom oxidation via measurements of products from both of these mechanisms and their relative contribution to secondary organic aerosol (SOA) formation.
2.	Buckland, Philip I., 1973-, et al. (författare) The Strategic Environmental Archaeology Database : a resource for international, multiproxy and transdisciplinary studies of environmental and climatic change 2015 Konferensbidrag (refereegranskat)abstract Climate and environmental change are global challenges which require global data and infrastructure to investigate. These challenges also require a multi-proxy approach, integrating evidence from Quaternary science and archaeology with information from studies on modern ecology and physical processes among other disciplines. The Strategic Environmental Archaeology Database (SEAD http://www.sead.se) is a Swedish based international research e-infrastructure for storing, managing, analysing and disseminating palaeoenvironmental data from an almost unlimited number of analysis methods. The system currently makes available raw data from over 1500 sites (>5300 datasets) and the analysis of Quaternary fossil insects, plant macrofossils, pollen, geochemistry and sediment physical properties, dendrochronology and wood anatomy, ceramic geochemistry and bones, along with numerous dating methods. This capacity will be expanded in the near future to include isotopes, multi-spectral and archaeo-metalurgical data. SEAD also includes expandable climate and environment calibration datasets, a complete bibliography and extensive metadata and services for linking these data to other resources. All data is available as Open Access through http://qsead.sead.se and downloadable software. SEAD is maintained and managed at the Environmental Archaeology Lab and HUMlab at Umea University, Sweden. Development and data ingestion is progressing in cooperation with The Laboratory for Ceramic Research and the National Laboratory for Wood Anatomy and Dendrochronology at Lund University, Sweden, the Archaeological Research Laboratory, Stockholm University, the Geoarchaeological Laboratory, Swedish National Historical Museums Agency and several international partners and research projects. Current plans include expanding its capacity to serve as a data source for any system and integration with the Swedish National Heritage Board's information systems. SEAD is partnered with the Neotoma palaeoecology database (http://www.neotomadb.org) and a new initiative for building cyberinfrastructure for transdisciplinary research and visualization of the long-term human ecodynamics of the North Atlantic funded by the National Science Foundation (NSF).
3.	Hahlin, Maria, et al. (författare) Electronic and molecular structures of organic dye/TiO2 interfaces for solar cell applications : a core level photoelectron spectroscopy study 2010 Ingår i: Physical Chemistry, Chemical Physics - PCCP. - : Royal Society of Chemistry (RSC). - 1463-9076 .- 1463-9084. ; 12:7, s. 1507-1517 Tidskriftsartikel (refereegranskat)abstract The electronic and molecular properties of three organic dye molecules with the general structure donor-linker-anchor have been investigated using core level photoelectron spectroscopy (PES). The molecules contain a diphenylaniline donor unit, a thiophene linker unit, and cyanoacrylic acid or rhodanine-3-acetic acid anchor units. They have been investigated both in the form of a multilayer and adsorbed onto nanoporous TiO2 and the experimental results were also compared with DFT calculations. The changes at the dye-sensitized TiO2 surface due to the modification of either the donor unit or the anchor unit was investigated and the results showed important differences in coverage as well as in electronic and molecular surface properties. By measuring the core level binding energies, the sub-molecular properties were characterized and the result showed that the adsorption to the TiO2 influences the energy levels of the sub-molecular units differently.
4.	Magnusson, Joel, 1991, et al. (författare) Multiple colliding laser pulses as a basis for studying high-field high-energy physics 2019 Ingår i: Physical Review A - Atomic, Molecular, and Optical Physics. - 2469-9926 .- 2469-9934. ; 100:6 Tidskriftsartikel (refereegranskat)abstract Apart from maximizing the strength of optical electromagnetic fields achievable at high-intensity laser facilities, the collision of several phase-matched laser pulses has been identified theoretically as a trigger of and way to study various phenomena. These range from the basic processes of strong-field quantum electrodynamics to the extraordinary dynamics of the generated electron-positron plasmas. This has paved the way for several experimental proposals aimed at both fundamental studies of matter at extreme conditions and the creation of particle and radiation sources. Because of the unprecedented capabilities of such sources, they have the potential to open up new opportunities for experimental studies in nuclear and quark-gluon physics. We perform here a systematic analysis of different regimes and opportunities achievable with the concept of multiple colliding laser pulses, for both current and upcoming laser facilities. We reveal that several distinct regimes could be within reach of multi-petawatt laser facilities.
5.	Midtvedt, Daniel, et al. (författare) Deep learning in light-matter interactions 2022 Ingår i: Nanophotonics. - : Walter de Gruyter GmbH. - 2192-8606 .- 2192-8614. ; 11:14, s. 3189-3214 Tidskriftsartikel (refereegranskat)abstract The deep-learning revolution is providing enticing new opportunities to manipulate and harness light at all scales. By building models of light-matter interactions from large experimental or simulated datasets, deep learning has already improved the design of nanophotonic devices and the acquisition and analysis of experimental data, even in situations where the underlying theory is not sufficiently established or too complex to be of practical use. Beyond these early success stories, deep learning also poses several challenges. Most importantly, deep learning works as a black box, making it difficult to understand and interpret its results and reliability, especially when training on incomplete datasets or dealing with data generated by adversarial approaches. Here, after an overview of how deep learning is currently employed in photonics, we discuss the emerging opportunities and challenges, shining light on how deep learning advances photonics.
6.	Andersson, Egil, et al. (författare) Single-photon core-valence double ionization of molecular oxygen 2008 Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 78, s. 023409- Tidskriftsartikel (refereegranskat)abstract Single-photon core-valence double ionization of molecular oxygen has been studied using a magnetic bottle time-of-flight electron coincidence spectrometer. The K-1V-1 double ionization electron spectrum of O-2 is reported and is assigned with the aid of ab initio calculations. A direct comparison of the core-valence double ionization electron spectra with the conventional valence band photoelectron spectrum is made. The lowest core-valence double ionization energy is found to be 571.6 eV and is associated with a (3)Pi dicationic state.
7.	Windelius, Olle, 1972, et al. (författare) Photoelectron angular distributions in photodetachment from P 2021 Ingår i: Physical Review A. - 2469-9926 .- 2469-9934. ; 103:3 Tidskriftsartikel (refereegranskat)abstract The angular distributions of electrons ejected in laser photodetachment of the P- ion have been studied in the photon energy range of 0.95-3.28 eV using a photoelectron spectrometer designed to accommodate a source consisting of collinearly overlapping photon and negative ion beams. We observe the value of the asymmetry parameter beta starting at zero near the threshold, falling to almost -1 about 0.5 eV above the threshold and eventually rising to a positive value. The experimental data has been fitted to a simplified model of the Cooper-Zare formula which yields a qualitative understanding of the quantum interference between the outgoing s and d waves representing the free electron. The present results are also compared with previous results for other elements involving p-electron photodetachment.
8.	Klacar, Simon, 1984 (författare) Chemical Properties of Oxidized Silver - A Density Functional Theory Study 2011 Licentiatavhandling (övrigt vetenskapligt/konstnärligt)
9.	Volpe, Giovanni, 1979, et al. (författare) Roadmap for optical tweezers 2023 Ingår i: Journal of Physics-Photonics. - : IOP Publishing. - 2515-7647. ; 5:2 Tidskriftsartikel (refereegranskat)abstract Optical tweezers are tools made of light that enable contactless pushing, trapping, and manipulation of objects, ranging from atoms to space light sails. Since the pioneering work by Arthur Ashkin in the 1970s, optical tweezers have evolved into sophisticated instruments and have been employed in a broad range of applications in the life sciences, physics, and engineering. These include accurate force and torque measurement at the femtonewton level, microrheology of complex fluids, single micro- and nano-particle spectroscopy, single-cell analysis, and statistical-physics experiments. This roadmap provides insights into current investigations involving optical forces and optical tweezers from their theoretical foundations to designs and setups. It also offers perspectives for applications to a wide range of research fields, from biophysics to space exploration.
10.	Hartman, Henrik, et al. (författare) First storage of ion beams in the Double Electrostatic Ion-Ring Experiment : DESIREE 2013 Ingår i: Review of Scientific Instruments. - : American Institute of Physics (AIP). - 0034-6748 .- 1089-7623. ; 84:5 Tidskriftsartikel (refereegranskat)abstract We report on the first storage of ion beams in the Double ElectroStatic Ion Ring ExpEriment, DESIREE, at Stockholm University. We have produced beams of atomic carbon anions and small carbon anion molecules (Cn-, n = 1, 2, 3, 4) in a sputter ion source. The ion beams were accelerated to 10 keV kinetic energy and stored in an electrostatic ion storage ring enclosed in a vacuum chamber at 13 K. For 10 keV C2- molecular anions we measure the residual-gas limited beam storage lifetime to be 448 s +/- 18 s with two independent detector systems. Using the measured storage lifetimes we estimate that the residual gas pressure is in the 10-14 mbar range. When high current ion beams are injected, the number of stored particles does not follow a single exponential decay law as would be expected for stored particles lost solely due to electron detachment in collision with the residual-gas. Instead, we observe a faster initial decay rate, which we ascribe to the effect of the space charge of the ion beam on the storage capacity.
11.	Hartman, Henrik, et al. (författare) The FERRUM project : experimental and theoretical transition rates of forbidden [Sc II] lines and radiative lifetimes of metastable ScII levels 2008 Ingår i: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 480:2, s. 575-580 Tidskriftsartikel (refereegranskat)abstract Context. In many plasmas, long-lived metastable atomic levels are depopulated by collisions (quenched) before they decay radiatively. In low-density regions, however, the low collision rate may allow depopulation by electric dipole (E1) forbidden radiative transitions, so-called forbidden lines (mainly M1 and E2 transitions). If the atomic transition data are known, these lines are indicators of physical plasma conditions and used for abundance determination. Aims. Transition rates can be derived by combining relative intensities between the decay channels, so-called branching fractions (BFs), and the radiative lifetime of the common upper level. We use this approach for forbidden [Sc II] lines, along with new calculations. Methods. Neither BFs for forbidden lines, nor lifetimes of metastable levels, are easily measured in a laboratory. Therefore, astrophysical BFs measured in Space Telescope Imaging Spectrograph (STIS) spectra of the strontium filament of Eta Carinae are combined with lifetime measurements using a laser probing technique on a stored ion-beam (CRYRING facility, MSL, Stockholm). These quantities are used to derive the absolute transition rates (A-values). New theoretical transition rates and lifetimes are calulated using the CIV3 code. Results. We report experimental lifetimes of the Sc II levels 3d(2) a(3)P(0,1,2) with lifetimes 1.28, 1.42, and 1.24 s, respectively, and transition rates for lines from these levels down to 3d4s a(3)D in the region 8270-8390 angstrom. These are the most important forbidden [Sc II] transitions. New calculations for lines and metastable lifetimes are also presented, and are in good agreement with the experimental data.
12.	Manzetti, Sergio, et al. (författare) A Korteweg-DeVries type model for helical soliton solutions for quantum and continuum phenomena 2021 Ingår i: International Journal of Modern Physics C. - : World Scientific. - 0129-1831. ; 32:03 Tidskriftsartikel (refereegranskat)abstract Quantum mechanical states are normally described by the Schrödinger equation, which generates real eigenvalues and quantizable solutions which form a basis for the estimation of quantum mechanical observables, such as momentum and kinetic energy. Studying transition in the realm of quantum physics and continuum physics is however more difficult and requires different models. We present here a new equation which bears similarities to the Korteweg–DeVries (KdV) equation and we generate a description of transitions in physics. We describe here the two- and three-dimensional form of the KdV like model dependent on the Plank constant ℏ and generate soliton solutions. The results suggest that transitions are represented by soliton solutions which arrange in a spiral-fashion. By helicity, we propose a conserved pattern of transition at all levels of physics, from quantum physics to macroscopic continuum physics.
13.	Waltersson, Erik, 1979-, et al. (författare) Controlled operations in a strongly correlated two-electron quantum ring 2009 Ingår i: Physical Review B. Condensed Matter and Materials Physics. - : American Physical Society. - 1098-0121 .- 1550-235X. ; 79:11, s. 115318- Tidskriftsartikel (refereegranskat)abstract We have analyzed the electronic spectrum and wave-function characteristics of a strongly correlated two-electron quantum ring with model parameters close to those observed in experiments. The analysis is based on an exact diagonalization of the Hamiltonian in a large B-spline basis. We propose a qubit pair for storing quantum information, where one component is stored in the total electron spin and one multivalued “quMbit” is represented by the total angular momentum. In this scheme the controlled-NOT quantum gate is demonstrated with near 100% fidelity for a realistic far-infrared electromagnetic pulse.
14.	Larson, Jonas, et al. (författare) Spin-orbit-coupled Bose-Einstein condensate in a tilted optical lattice 2010 Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - : APS. - 1050-2947 .- 1094-1622. ; 82:4, s. 043620- Tidskriftsartikel (refereegranskat)abstract Bloch oscillations appear for a particle in a weakly tilted periodic potential. The intrinsic spin Hall effect is an outcome of a spin-orbit coupling. We demonstrate that both of these phenomena can be realized simultaneously in a gas of weakly interacting ultracold atoms exposed to a tilted optical lattice and to a set of spatially dependent light fields inducing an effective spin-orbit coupling. It is found that both the spin Hall and the Bloch oscillation effects may coexist, showing, however, a strong correlation between the two. These correlations are manifested as a transverse spin current oscillating in-phase with the Bloch oscillations. On top of the oscillations originating from the periodicity of the model, a trembling motion is found which is believed to be atomic Zitterbewegung. It is argued that the damping of these Zitterbewegung oscillations may to a large extent be prevented in the present setup considering a periodic optical lattice potential.
15.	Liu, Yanfeng, et al. (författare) In Situ Optical Spectroscopy Demonstrates the Effect of Solvent Additive in the Formation of All-Polymer Solar Cells 2022 Ingår i: The Journal of Physical Chemistry Letters. - : American Chemical Society (ACS). - 1948-7185. ; 13:50, s. 11696-11702 Tidskriftsartikel (refereegranskat)abstract 1-Chloronaphthalene (CN) has been a common solvent additive in both fullerene- A nd nonfullerene-based organic solar cells. In spite of this, its working mechanism is seldom investigated, in particular, during the drying process of bulk heterojunctions composed of a donor:acceptor mixture. In this work, the role of CN in all-polymer solar cells is investigated by in situ spectroscopies and ex situ characterization of blade-coated PBDB-T:PF5-Y5 blends. Our results suggest that the added CN promotes self-aggregation of polymer donor PBDB-T during the drying process of the blend film, resulting in enhanced crystallinity and hole mobility, which contribute to the increased fill factor and improved performance of PBDB-T:PF5-Y5 solar cells. Besides, the nonradiative energy loss of the corresponding device is also reduced by the addition of CN, corresponding to a slightly increased open-circuit voltage. Overall, our observations deepen our understanding of the drying dynamics, which may guide further development of all-polymer solar cells.
16.	Lee, Kyuho, et al. (författare) Benchmarking van der Waals density functionals with experimental data: potential-energy curves for H2 molecules on Cu(111), (100) and (110) surfaces 2012 Ingår i: Journal of Physics: Condensed Matter. - : IOP Publishing. - 0953-8984 .- 1361-648X. ; 24:42 Tidskriftsartikel (refereegranskat)abstract Detailed physisorption data from experiment for the H2 molecule on low-index Cu surfaces challenge theory. Recently, density functional theory (DFT) has been developed to account for nonlocal correlation effects, including van der Waals (dispersion) forces. We show that the functional vdW-DF2 gives a potential-energy curve, potential-well energy levels and difference in lateral corrugation promisingly close to the results obtained by resonant elastic backscattering–diffraction experiments. The backscattering barrier is sensitive to the choice of exchange functional approximation. Further, the DFT-D3 and TS-vdW corrections to traditional DFT formulations are also benchmarked, and deviations are analyzed.
17.	Bertilson, Michael, 1979- (författare) Laboratory soft x-ray microscopy and tomography 2011 Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract Soft x-ray microscopy in the water-window (λ = 2.28 nm – 4.36 nm) is based on zone-plate optics and allows high-resolution imaging of, e.g., cells and soils in their natural or near-natural environment. Three-dimensional imaging is provided via tomographic techniques, soft x-ray cryo tomography. However, soft x-ray microscopes with such capabilities have been based on large-scale synchrotron x‑ray facilities, thereby limiting their accessibility for a wider scientific community. This Thesis describes the development of the Stockholm laboratory soft x-ray microscope to three-dimensional cryo tomography and to new optics-based contrast mechanisms. The microscope relies on a methanol or nitrogen liquid-jet laser-plasma source, normal-incidence multilayer or zone-plate condenser optics, in-house fabricated zone-plate objectives, and allows operation at two wavelengths in the water-window, λ = 2.48 nm and λ = 2.48 nm. With the implementation of a new state-of-the-art normal-incidence multilayer condenser for operation at λ = 2.48 nm and a tiltable cryogenic sample stage the microscope now allows imaging of dry, wet or cryo-fixed samples. This arrangement was used for the first demonstration of laboratory soft x-ray cryo microscopy and tomography. The performance of the microscope has been demonstrated in a number of experiments described in this Thesis, including, tomographic imaging with a resolution of 140 nm, cryo microscopy and tomography of various cells and parasites, and for studies of aqueous soils and clays. The Thesis also describes the development and implementation of single-element differential-interference and Zernike phase-contrast zone-plate objectives. The enhanced contrast provided by these optics reduce exposure times or lowers the dose in samples and are of major importance for harder x-ray microscopy. The implementation of a high-resolution 50 nm compound zone-plate objective for sub-25-nm resolution imaging is also described. All experiments are supported by extensive numerical modelling for improved understanding of partially coherent image formation and stray light in soft x-ray microscopes. The models are useful tools for studying effects of zone plate optics or optical design of the microscope on image formation and quantitative accuracy in soft x-ray tomography.
18.	Magnuson, Martin, et al. (författare) Competition between decay and dissociation of core-excited carbonyl sulfide studied by x-ray scattering 1999 Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 59:6, s. 4281-4287 Tidskriftsartikel (refereegranskat)abstract We show evidence of dissociation during resonant inelastic soft x-ray scattering Carbon and oxygen K-shell and sulfur L-shell resonant and nonresonant x-ray emission spectra were measured using monochromatic synchrotron radiation for excitation and ionization. After sulfur L-2,L-3-->pi, sigma excitation, atomic lines are observed in the emission spectra as a consequence of competition between de-excitation and dissociation. In contrast thr carbon and oxygen spectra show weaker line-shape variations and no atomic Lines. The spectra are compared to results from ab initio calculations. The discussion of the dissociation paths is based on calculated potential energy surfaces and atomic transition energies.
19.	Yu, Shun, et al. (författare) Adsorption geometry, molecular interaction, and charge transfer of triphenylamine-based dye on rutile TiO2(110) 2010 Ingår i: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 133:22, s. 224704- Tidskriftsartikel (refereegranskat)abstract The fast development of new organic sensitizers leads to the need for a better understanding of the complexity and significance of their adsorption processes on TiO2 surfaces. We have investigated a prototype of the triphenylamine-cyanoacrylic acid (donor-acceptor) on rutile TiO2 (110) surface with special attention on the monolayer region. This molecule belongs to the type of dye, some of which so far has delivered the record efficiency of 10%-10.3% for pure organic sensitizers [W. Zeng, Y. Cao, Y. Bai, Y. Wang, Y. Shi, M. Zhang, F. Wang, C. Pan, and P. Wang, Chem. Mater. 22, 1915 (2010)]. The molecular configuration of this dye on the TiO2 surface was found to vary with coverage and adopt gradually an upright geometry, as determined from near edge x-ray absorption fine structure spectroscopy. Due to the molecular interaction within the increasingly dense packed layer, the molecular electronic structure changes systematically: all energy levels shift to higher binding energies, as shown by photoelectron spectroscopy. Furthermore, the investigation of charge delocalization within the molecule was carried out by means of resonant photoelectron spectroscopy. A fast delocalization (similar to 1.8 fs) occurs at the donor part while a competing process between delocalization and localization takes place at the acceptor part. This depicts the "push-pull" concept in donor-acceptor molecular system in time scale. (C) 2010 American Institute of Physics. [doi:10.1063/1.3509389]
20.	Warbinek, Jessica, et al. (författare) A graphene-based neutral particle detector 2019 Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 114:6 Tidskriftsartikel (refereegranskat)abstract A neutral particle detector is presented, in which the traditionally used target material, indium tin oxide (ITO), is replaced by graphene. The graphene-based detector enables collinear photodetachment measurements at a significantly shorter wavelength of light down to 230nm compared to ITO-based detectors, which are limited at 335 nm. Moreover, the background signal from the photoelectric effect is drastically reduced when using graphene. The graphene based detector, reaching 1.7 eV further into the UV energy range, allows increased possibilities for photodetachment studies of negatively charged atoms, molecules, and clusters. Published under license by AIP Publishing.
21.	Baggioli, Matteo, et al. (författare) Holographic plasmon relaxation with and without broken translations 2019 Ingår i: Journal of High Energy Physics (JHEP). - : SPRINGER. - 1126-6708 .- 1029-8479. ; :9 Tidskriftsartikel (refereegranskat)abstract We study the dynamics and the relaxation of bulk plasmons in strongly coupled and quantum critical systems using the holographic framework. We analyze the dispersion relation of the plasmonic modes in detail for an illustrative class of holographic bottom-up models. Comparing to a simple hydrodynamic formula, we entangle the complicated interplay between the three least damped modes and shed light on the underlying physical processes. Such as the dependence of the plasma frequency and the effective relaxation time in terms of the electromagnetic coupling, the charge and the temperature of the system. Introducing momentum dissipation, we then identify its additional contribution to the damping. Finally, we consider the spontaneous symmetry breaking (SSB) of translational invariance. Upon dialing the strength of the SSB, we observe an increase of the longitudinal sound speed controlled by the elastic moduli and a decrease in the plasma frequency of the gapped plasmon. We comment on the condensed matter interpretation of this mechanism.
22.	Ferri, Julien, et al. (författare) Generation of attosecond electron bunches and x-ray pulses from few-cycle femtosecond laser pulses 2021 Ingår i: Plasma Physics and Controlled Fusion. - : IOP Publishing. - 0741-3335 .- 1361-6587. ; 63:4 Tidskriftsartikel (refereegranskat)abstract Laser-plasma electron accelerators can be used to produce high-intensity x-rays, as electrons accelerated in wakefields emit radiation due to betatron oscillations. Such x-ray sources inherit the features of the electron beam; sub-femtosecond electron bunches produce betatron sources of the same duration, which in turn allow probing matter on ultrashort time scales. In this paper we show, via Particle-in-Cell simulations, that attosecond electron bunches can be obtained using low-energy, ultra-short laser beams both in the self-injection and the controlled injection regimes at low plasma densities. However, only in the controlled regime does the electron injection lead to a stable, isolated attosecond electron bunch. Such ultrashort electron bunches are shown to emit attosecond x-ray bursts with high brilliance.
23.	Grigoriev, Anton, et al. (författare) Electron transport in stretched monoatomic gold wires 2006 Ingår i: Physical Review Letters. - : American Physical Society. - 0031-9007 .- 1079-7114. ; 97, s. 236807- Tidskriftsartikel (refereegranskat)abstract The conductance of monoatomic gold wires containing 3-7 gold atoms has been obtained from ab initio calculations. The transmission is found to vary significantly depending on the wire stretching and the number of incorporated atoms. Such oscillations are determined by the electronic structure of the one-dimensional (1D) part of the wire between the contacts. Our results indicate that the conductivity of 1D wires can be suppressed without breaking the contact.
24.	Isaksson, Oscar, et al. (författare) An optical levitation system for a physics teaching laboratory 2018 Ingår i: American Journal of Physics. - : American Association of Physics Teachers (AAPT). - 0002-9505 .- 1943-2909. ; 86:2, s. 135-142 Tidskriftsartikel (refereegranskat)abstract We describe an experimental system based on optical levitation of an oil droplet. When combined with an applied electric field and a source of ionizing radiation, the setup permits the investigation of physical phenomena such as radiation pressure, light diffraction, the motion of a charged particle in an oscillating electric field, and the interaction of ionizing radiation with matter. The trapping occurs by creating an equilibrium between a radiation pressure force and the force of gravity. We have found that an oil droplet can be trapped for at least nine hours. The system can be used to measure the size and total electric charge on the trapped droplet. The intensity of the light from the trapping laser that is scattered by the droplet is sufficient to allow the droplet to be easily seen with the naked eye, covered by laser alignment goggles. When oscillating under the influence of an ac electric field, the motion of the droplet can be described as that of a driven, damped harmonic oscillator. The magnitude and polarity of the charge can be altered by exposing the droplet to ionizing radiation from a low-activity radioactive source. Our goal was to design a hands-on setup that allows undergraduate and graduate students to observe and better understand fundamental physical processes. (C) 2018 American Association of Physics Teachers.
25.	Monsel, Juliette, 1994, et al. (författare) Optomechanical cooling with coherent and squeezed light: The thermodynamic cost of opening the heat valve 2021 Ingår i: Physical Review A. - 2469-9926 .- 2469-9934. ; 103:6 Tidskriftsartikel (refereegranskat)abstract Ground-state cooling of mechanical motion by coupling to a driven optical cavity has been demonstrated in various optomechanical systems. In our paper, we provide a thermodynamic performance analysis of optomechanical sideband cooling in terms of a heat valve. As performance quantifiers, we examine not only the lowest reachable effective temperature (phonon number) but also the evacuated-heat flow as an equivalent to the cooling power of a standard refrigerator, as well as appropriate thermodynamic efficiencies, which all can be experimentally inferred from measurements of the cavity output light field. Importantly, in addition to the standard optomechanical setup fed by coherent light, we investigate two recent alternative setups for achieving ground-state cooling: replacing the coherent laser drive by squeezed light or using a cavity with a frequency-dependent (Fano) mirror. We study the dynamics of these setups within and beyond the weak-coupling limit and give concrete examples based on parameters of existing experimental systems. By applying our thermodynamic framework, we gain detailed insights into these three different optomechanical cooling setups, allowing a comprehensive understanding of the thermodynamic mechanisms at play.
26.	Zámečníková, Martina, et al. (författare) Formation of CO+ by radiative association II 2020 Ingår i: Monthly notices of the Royal Astronomical Society. - : Oxford University Press. - 0035-8711 .- 1365-2966. ; 492:3, s. 3794-3802 Tidskriftsartikel (refereegranskat)abstract Radiative association of an oxygen atom with a carbon cation is investigated using quantal and semiclassical methods. The total rate coefficient for spontaneous radiative association of O(2s22p4, 3P) with C+(2s22p, 2P) on the doublet manifold is determined from the corresponding cross-sections. The cross-sections for the 12 Σ - → A2 II, 22 Σ - → A2II, and C2 Δ → A2II continuum-bound processes are calculated either semiclassically, in combination with the Breit-Wigner approach, or fully quantum mechanically. In the temperature range 10-10 000 K, our recommended total rate coefficient, obtained from these calculations and the data of Zámecniková et al. (2019), slowly increases from 7.5 × 10-18 cm3s-1 to 2.1 × 10-17 cm3s-1. Corresponding aspects of the CO+ and CO formations in SN 1987A are discussed
27.	Morris, B. M., et al. (författare) CHEOPS precision phase curve of the Super-Earth 55 Cancri e 2021 Ingår i: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 653 Tidskriftsartikel (refereegranskat)abstract Context. 55 Cnc e is a transiting super-Earth (radius 1.88 R-circle plus and mass 8 M-circle plus) orbiting a G8V host star on a 17-h orbit. Spitzer observations of the planet's phase curve at 4.5 mu m revealed a time-varying occultation depth, and MOST optical observations are consistent with a time-varying phase curve amplitude and phase offset of maximum light. Both broadband and high-resolution spectroscopic analyses are consistent with either a high mean molecular weight atmosphere or no atmosphere for planet e. A long-term photometric monitoring campaign on an independent optical telescope is needed to probe the variability in this system. Aims. We seek to measure the phase variations of 55 Cnc e with a broadband optical filter with the 30 cm effective aperture space telescope CHEOPS and explore how the precision photometry narrows down the range of possible scenarios. Methods. We observed 55 Cnc for 1.6 orbital phases in March of 2020. We designed a phase curve detrending toolkit for CHEOPS photometry which allowed us to study the underlying flux variations in the 55 Cnc system. Results. We detected a phase variation with a full-amplitude of 72 +/- 7 ppm, but did not detect a significant secondary eclipse of the planet. The shape of the phase variation resembles that of a piecewise-Lambertian; however, the non-detection of the planetary secondary eclipse, and the large amplitude of the variations exclude reflection from the planetary surface as a possible origin of the observed phase variations. They are also likely incompatible with magnetospheric interactions between the star and planet, but may imply that circumplanetary or circumstellar material modulate the flux of the system. Conclusions. This year, further precision photometry of 55 Cnc from CHEOPS will measure variations in the phase curve amplitude and shape over time.
28.	Londero, Elisa, 1982, et al. (författare) Desorption of n-alkanes from graphene: a van der Waals density functional study 2012 Ingår i: Journal of Physics Condensed Matter. - : IOP Publishing. - 0953-8984 .- 1361-648X. ; 24:42, s. 424212- Tidskriftsartikel (refereegranskat)abstract A recent study of temperature-programmed desorption (TPD) measurements of small linear alkane molecules (n-alkanes, with formula CNH2N+2) from C(0001) deposited on Pt(111) shows a linear relationship of the desorption energy with increasing n-alkane chain length N. We here present a van der Waals density functional study of the desorption barrier energy of the ten smallest n-alkanes (of carbon chain length N = 1–10) from graphene. We find linear scaling with N, including a non-zero intercept with the energy axis, i.e. an offset at the extrapolation to N = 0. This calculated offset is quantitatively similar to the results of the TPD measurements. From further calculations of the polyethylene polymer we offer a suggestion for the origin of the offset.
29.	Kong, Xiangrui, et al. (författare) Dynamics and Kinetics of Methanol-Graphite Interactions at Low Surface Coverage 2019 Ingår i: Chemphyschem. - : Wiley. - 1439-4235 .- 1439-7641. ; 20:17, s. 2171-2178 Tidskriftsartikel (refereegranskat)abstract The processes of molecular clustering, condensation, nucleation, and growth of bulk materials on surfaces, represent a spectrum of vapor-surface interactions that are important to a range of physical phenomena. Here, we describe studies of the initial stages of methanol condensation on graphite, which is a simple model system where gas-surface interactions can be described in detail using combined experimental and theoretical methods. Experimental molecular beam methods and computational molecular dynamics simulations are used to investigate collision dynamics and surface accommodation of methanol molecules and clusters at temperatures from 160 K to 240 K. Both single molecules and methanol clusters efficiently trap on graphite, and even in rarified systems methanol-methanol interactions quickly become important. A kinetic model is developed to simulate the observed behavior, including the residence time of trapped molecules and the quantified Arrhenius kinetics. Trapped molecules are concluded to rapidly diffuse on the surface to find and/or form clusters already at surface coverages below 10(-6) monolayers. Conversely, clusters that undergo surface collisions fragment and subsequently lose more loosely bound molecules. Thus, the surface mediates molecular collisions in a manner that minimizes the importance of initial cluster size, but highlights a strong sensitivity to surface diffusion and intermolecular interactions between the hydrogen bonded molecules.
30.	Lestinsky, M., et al. (författare) Physics book: CRYRING@ESR 2016 Ingår i: European Physical Journal: Special Topics. - : Springer Science and Business Media LLC. - 1951-6401 .- 1951-6355. ; 225:5, s. 797-882 Forskningsöversikt (refereegranskat)abstract The exploration of the unique properties of stored and cooled beams of highly-charged ions as provided by heavy-ion storage rings has opened novel and fascinating research opportunities in the realm of atomic and nuclear physics research. Since the late 1980s, pioneering work has been performed at the CRYRING at Stockholm (Abrahamsson et al. 1993) and at the Test Storage Ring (TSR) at Heidelberg (Baumann et al. 1988). For the heaviest ions in the highest charge-states, a real quantum jump was achieved in the early 1990s by the commissioning of the Experimental Storage Ring (ESR) at GSI Helmholtzzentrum für Schwerionenforschung (GSI) in Darmstadt (Franzke 1987) where challenging experiments on the electron dynamics in the strong field regime as well as nuclear physics studies on exotic nuclei and at the borderline to atomic physics were performed. Meanwhile also at Lanzhou a heavy-ion storage ring has been taken in operation, exploiting the unique research opportunities in particular for medium-heavy ions and exotic nuclei (Xia et al. 2002).
31.	Siminos, Evangelos, 1979, et al. (författare) Laser Wakefield Driven Generation of Isolated Carrier-Envelope-Phase Tunable Intense Subcycle Pulses 2021 Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 126:4 Tidskriftsartikel (refereegranskat)abstract Sources of intense, ultrashort electromagnetic pulses enable applications such as attosecond pulse generation, control of electron motion in solids, and the observation of reaction dynamics at the electronic level. For such applications, both high intensity and carrier-envelope-phase (CEP) tunability are beneficial, yet hard to obtain with current methods. In this Letter, we present a new scheme for generation of isolated CEP tunable intense subcycle pulses with central frequencies that range from the midinfrared to the ultraviolet. It utilizes an intense laser pulse that drives a wake in a plasma, copropagating with a long-wavelength seed pulse. The moving electron density spike of the wake amplifies the seed and forms a subcycle pulse. Controlling the CEP of the seed pulse or the delay between driver and seed leads to CEP tunability, while frequency tunability can be achieved by adjusting the laser and plasma parameters. Our 2D and 3D particle-in-cell simulations predict laser-to-subcycle-pulse conversion efficiencies up to 1%, resulting in relativistically intense subcycle pulses.
32.	Siminos, Evangelos, 1979, et al. (författare) Parametric study of laser wakefield driven generation of intense sub-cycle pulses 2022 Ingår i: Plasma Physics and Controlled Fusion. - : IOP Publishing. - 0741-3335 .- 1361-6587. ; 64:3 Tidskriftsartikel (refereegranskat)abstract Intense sub-cycle electromagnetic pulses allow one to drive nonlinear processes in matter with unprecedented levels of control. However, it remains challenging to scale such sources in the relativistic regime. Recently, a scheme that utilizes laser-driven wakes in plasmas to amplify and compress seed laser pulses to produce tunable, carrier-envelope-phase stable, relativistic sub-cycle pulses has been proposed. Here, we present parametric studies of this process using particle-in-cell simulations, showing its robustness over a wide range of experimentally accessible laser-plasma interaction parameters, spanning more than two orders of magnitude of background plasma density. The method is shown to work with different gas-jet profiles, including structured density profiles and is robust over a relatively wide range of driver laser intensities. Our study shows that sub-cycle pulses of up to 10mJ of energy can be produced.
33.	Thiele, Illia, 1989, et al. (författare) Electron Beam Driven Generation of Frequency-Tunable Isolated Relativistic Subcycle Pulses 2019 Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 122 Tidskriftsartikel (refereegranskat)abstract © 2019 American Physical Society. We propose a novel scheme for frequency-tunable subcycle electromagnetic pulse generation. To this end a pump electron beam is injected into an electromagnetic seed pulse as the latter is reflected by a mirror. The electron beam is shown to be able to amplify the field of the seed pulse while upshifting its central frequency and reducing its number of cycles. We demonstrate the amplification by means of 1D and 2D particle-in-cell simulations. In order to explain and optimize the process, a model based on fluid theory is proposed. We estimate that using currently available electron beams and terahertz pulse sources, our scheme is able to produce millijoule-strong midinfrared subcycle pulses.
34.	Bahrova, O. M., et al. (författare) Cooling of nanomechanical vibrations by Andreev injection 2022 Ingår i: Low Temperature Physics. - : AIP Publishing. - 1063-777X .- 1090-6517. ; 48:6, s. 476-482 Tidskriftsartikel (refereegranskat)abstract A nanoelectromechanical weak link composed of a carbon nanotube suspended between two normal electrodes in a gap between two superconducting leads is considered. The nanotube is treated as a movable single level quantum dot in which the position-dependent superconducting order parameter is induced due to the Cooper pair tunneling. We show that electron tunneling processes significantly affect the state of the mechanical subsystem. We found that at a given direction of the applied voltage between the electrodes, the stationary state of the mechanical subsystem has a Boltzmann form with an effective temperature dependent on the parameters of the device. As this takes place, the effective temperature can reach significantly small values (cooling effect). We also demonstrate that nanotube fluctuations strongly affect the dc current through the system. The latter can be used to probe the predicted effects in an experiment. Published under an exclusive license by AIP Publishing.
35.	Jiao, Yang, 1985, et al. (författare) Signatures of van der Waals binding: A coupling-constant scaling analysis 2018 Ingår i: Physical Review B. - 2469-9969 .- 2469-9950. ; 97:8 Tidskriftsartikel (refereegranskat)abstract The van der Waals (vdW) density functional (vdW-DF) method [Rep. Prog. Phys. 78, 066501 (2015)RPPHAG0034-488510.1088/0034-4885/78/6/066501] describes dispersion or vdW binding by tracking the effects of an electrodynamic coupling among pairs of electrons and their associated exchange-correlation holes. This is done in a nonlocal-correlation energy term Ecnl, which permits density functional theory calculation in the Kohn-Sham scheme. However, to map the nature of vdW forces in a fully interacting materials system, it is necessary to also account for associated kinetic-correlation energy effects. Here, we present a coupling-constant scaling analysis, which permits us to compute the kinetic-correlation energy Tcnl that is specific to the vdW-DF account of nonlocal correlations. We thus provide a more complete spatially resolved analysis of the electrodynamical-coupling nature of nonlocal-correlation binding, including vdW attraction, in both covalently and noncovalently bonded systems. We find that kinetic-correlation energy effects play a significant role in the account of vdW or dispersion interactions among molecules. Furthermore, our mapping shows that the total nonlocal-correlation binding is concentrated to pockets in the sparse electron distribution located between the material fragments.
36.	Parafilo, A. V., et al. (författare) Pumping and Cooling of Nanomechanical Vibrations Generated by Cooper-Pair Exchange 2022 Ingår i: Journal of Low Temperature Physics. - : Springer Science and Business Media LLC. - 0022-2291 .- 1573-7357. ; 210:1-2, s. 150-65 Tidskriftsartikel (refereegranskat)abstract We consider a nanoelectromechanical system composed of a carbon nanotube suspended between two normal leads and coupled to a superconducting scanning tunneling microscope (STM) tip via vacuum tunnel barrier. Treating the nanotube as a single-level quantum dot, it is shown that an applied voltage between the superconducting STM tip and normal leads gives rise to a pumping or a cooling of the mechanical subsystem depending on the direction of the electronic flow. It is also demonstrated that the transition between these two regimes is controlled by the strength of the tunnel coupling between the nanotube and superconducting STM tip and the relative position of the electronic level. Such phenomena are realized due to a specific electromechanical coupling that is fully governed by the quantum dynamics of the Cooper pairs. The amplitude of the self-sustained oscillations in the pumping regime is analyzed numerically, and the effective temperature of the mechanical subsystem in the cooling regime is obtained.
37.	Sjöqvist, Erik, et al. (författare) Conceptual aspects of geometric quantum computation 2016 Ingår i: Quantum Information Processing. - : Springer Science and Business Media LLC. - 1570-0755 .- 1573-1332. ; 15:10, s. 3995-4011 Tidskriftsartikel (refereegranskat)abstract Geometric quantum computation is the idea that geometric phases can be used to implement quantum gates, i.e., the basic elements of the Boolean network that forms a quantum computer. Although originally thought to be limited to adiabatic evolution, controlled by slowly changing parameters, this form of quantum computation can as well be realized at high speed by using nonadiabatic schemes. Recent advances in quantum gate technology have allowed for experimental demonstrations of different types of geometric gates in adiabatic and nonadiabatic evolution. Here, we address some conceptual issues that arise in the realizations of geometric gates. We examine the appearance of dynamical phases in quantum evolution and point out that not all dynamical phases need to be compensated for in geometric quantum computation. We delineate the relation between Abelian and non-Abelian geometric gates, and find an explicit physical example where the two types of gates coincide. We identify differencies and similarities between adiabatic and nonadiabatic realizations of quantum computation based on non-Abelian geometric phases.
38.	Fredenberg, Erik, 1979- (författare) Spectral Mammography with X-Ray Optics and a Photon-Counting Detector 2009 Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract Early detection is vital to successfully treating breast cancer, and mammography screening is the most efficient and wide-spread method to reach this goal. Imaging low-contrast targets, while minimizing the radiation exposure to a large population is, however, a major challenge. Optimizing the image quality per unit radiation dose is therefore essential. In this thesis, two optimization schemes with respect to x-ray photon energy have been investigated: filtering the incident spectrum with refractive x-ray optics (spectral shaping), and utilizing the transmitted spectrum with energy-resolved photon-counting detectors (spectral imaging). Two types of x-ray lenses were experimentally characterized, and modeled using ray tracing, field propagation, and geometrical optics. Spectral shaping reduced dose approximately 20% compared to an absorption-filtered reference system with the same signal-to-noise ratio, scan time, and spatial resolution. In addition, a focusing pre-object collimator based on the same type of optics reduced divergence of the radiation and improved photon economy by about 50%. A photon-counting silicon detector was investigated in terms of energy resolution and its feasibility for spectral imaging. Contrast-enhanced tumor imaging with a system based on the detector was characterized and optimized with a model that took anatomical noise into account. Improvement in an ideal-observer detectability index by a factor of 2 to 8 over that obtained by conventional absorption imaging was found for different levels of anatomical noise and breast density. Increased conspicuity was confirmed by experiment. Further, the model was extended to include imaging of unenhanced lesions. Detectability of microcalcifications increased no more than a few percent, whereas the ability to detect large tumors might improve on the order of 50% despite the low attenuation difference between glandular and cancerous tissue. It is clear that inclusion of anatomical noise and imaging task in spectral optimization may yield completely different results than an analysis based solely on quantum noise.
39.	Scandariato, Gaetano, et al. (författare) Phase curve and geometric albedo of WASP-43b measured with CHEOPS, TESS, and HST WFC3/UVIS 2022 Ingår i: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 668 Tidskriftsartikel (refereegranskat)abstract Context. Observations of the phase curves and secondary eclipses of extrasolar planets provide a window onto the composition and thermal structure of the planetary atmospheres. For example, the photometric observations of secondary eclipses lead to the measurement of the planetary geometric albedo, Ag, which is an indicator of the presence of clouds in the atmosphere. Aims. In this work, we aim to measure the Ag in the optical domain of WASP-43b, a moderately irradiated giant planet with an equilibrium temperature of ~1400 K. Methods. For this purpose, we analyzed the secondary eclipse light curves collected by CHEOPS together with TESS along with observations of the system and the publicly available photometry obtained with HST WFC3/UVIS. We also analyzed the archival infrared observations of the eclipses and retrieve the thermal emission spectrum of the planet. By extrapolating the thermal spectrum to the optical bands, we corrected for the optical eclipses for thermal emission and derived the optical Ag. Results. The fit of the optical data leads to a marginal detection of the phase-curve signal, characterized by an amplitude of 160 ± 60 ppm and 80a-? 50+60 ppm in the CHEOPS and TESS passbands, respectively, with an eastward phase shift of ~50 (1.5Ï ? detection). The analysis of the infrared data suggests a non-inverted thermal profile and solar-like metallicity. The combination of the optical and infrared analyses allows us to derive an upper limit for the optical albedo of Ag< 0.087, with a confidence of 99.9%. Conclusions. Our analysis of the atmosphere of WASP-43b places this planet in the sample of irradiated hot Jupiters, with monotonic temperature-pressure profile and no indication of condensation of reflective clouds on the planetary dayside.
40.	Bylander, Jonas, 1978 (författare) Writing to Learn Quantum Engineering: Improved Understanding and Communication by Revising a Writing Assignment 2016 Ingår i: KUL2016 Konferens om Undervisning och Lärande på Chalmers. ; Extended Abstracts Konferensbidrag (refereegranskat)abstract I present an improved lab-report writing assignment for formative assessment in master’s-level physics. Prompted by poorly written reports in an earlier version of the course, suggesting insufficient subject understanding, I aligned aims, learning objectives, instruction, and assessment, and introduced a component of student peer review. This method enhanced learning of the subject matter, indicated by clearly improved reports.
41.	Posada Borbon, Alvaro, 1990, et al. (författare) Initial oxidation of Cu(100) studied by X-ray photo-electron spectroscopy and density functional theory calculations 2018 Ingår i: Surface Science. - : Elsevier BV. - 0039-6028 .- 1879-2758. ; 675, s. 64-69 Tidskriftsartikel (refereegranskat)abstract Density functional theory calculations and ambient pressure X-ray photoelectron spectroscopy are used to investigate initial oxidation of Cu(100). Surface stability with respect to oxygen coverage is calculated together with O 1s core level shifts. Oxidation of Cu(100) is found to occur via the formation of a p(2  ×  2) overlayer (0.25 ML) followed by a reconstructed  r2×r2 R45° -O missing-row (MR) structure (0.50 ML). A c(4  ×  6) structure with a 0.3 ML coverage is close in stability for intermediate oxygen chemical potentials. The relative stability is found to be weakly dependent on the applied exchange-correlation functional. The calculated shifts in the O 1s binding energy are in good agreement with the measured evolution of the binding energy. The shift to higher O 1s binding energies with increasing oxygen coverage is found to correlate with the charge on neighboring copper atoms. The O 1s core-level shifts here obtained with CO2 as oxidant, are similar to previous measurements of Cu(100) oxidation with O2.
42.	Petersson, Per, 1978-, et al. (författare) Ion beam micro analysis of deposits at tokamak divertor surfaces 2010 Ingår i: Nuclear Instruments and Methods in Physics Research Section B. - Amsterdam : Elsevier BV. - 0168-583X .- 1872-9584. ; 268:11-12, s. 1838-1841 Tidskriftsartikel (refereegranskat)abstract Cross sections of deposited layers in the Joint European Torus (JET) were analysed using the nuclear micro analysis at the Tandem Laboratory, Uppsala University. For deuterium and beryllium the nuclear reactions D-2(He-3,p)He-4 and Be-9(He-3,p(n))B-11 were exploited for analysis. Typically the analyses have been made with 10 mu m spatial resolution and a sensitivity of better than one atomic percent for beryllium or deuterium in carbon matrix. Comparing several different surface treatment techniques shows that polishing the sample surface give very good optical surface information but that some amount of deuterium and beryllium probably is removed. For good quantitative results the measurement can either be done on a rough surface or the top of the polished surface can be cut off. (C) 2010 Elsevier B.V. All rights reserved.
43.	Sznitko, L., et al. (författare) Low-threshold stimulated emission from lysozyme amyloid fibrils doped with a blue laser dye 2015 Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 106:2 Tidskriftsartikel (refereegranskat)abstract © 2015 AIP Publishing LLC. Amyloid fibrils are excellent self-assembling nanotemplates for organic molecules such as dyes. Here, we demonstrate that laser dye-doped lysozyme type fibrils exhibit significantly reduced threshold for stimulated emission compared to that observed in usual matrices. Laser action was studied in slab planar waveguides of the amyloids doped with Stilbene 420 laser dye prepared using a film casting technique. The lowering of the threshold of stimulated emission is analyzed in the context of intrinsic structure of the amyloid nanotemplates, electrostatic interaction of different microstructures with dye molecules, as well as material properties of the cast layers. All these factors are considered to be of importance for introducing gain for random laser operation.
44.	Krog, Jens, et al. (författare) Stochastic unfolding of nanoconfined DNA: Experiments, model and Bayesian analysis 2018 Ingår i: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 149:21 Tidskriftsartikel (refereegranskat)abstract Nanochannels provide a means for detailed experiments on the effect of confinement on biomacro-molecules, such as DNA. Here we introduce a model for the complete unfolding of DNA from the circular to linear configuration. Two main ingredients are the entropic unfolding force and the friction coefficient for the unfolding process, and we describe the associated dynamics by a non-linear Langevin equation. By analyzing experimental data where DNA molecules are photo-cut and unfolded inside a nanochannel, our model allows us to extract values for the unfolding force as well as the friction coefficient for the first time. In order to extract numerical values for these physical quantities, we employ a recently introduced Bayesian inference framework. We find that the determined unfolding force is in agreement with estimates from a simple Flory-type argument. The estimated friction coefficient is in agreement with theoretical estimates for motion of a cylinder in a channel. We further validate the estimated friction constant by extracting this parameter from DNA's center-of -mass motion before and after unfolding, yielding decent agreement. We provide publically available software for performing the required image and Bayesian analysis. Published by AIP Publishing.
45.	von Hofsten, Olof, 1982- (författare) Phase-Contrast and High-Resolution Optics for X-Ray Microscopy 2010 Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract X-ray microscopy is a well-established technique for nanoscale imaging. Zone plates are used as microscope objectives and provide high resolution, approaching 10 nm, currently limited by fabrication issues. This Thesis presents zone plate optics that achieve either high resolution or phase contrast in x-ray microscopy. The high-resolution optics use high orders of the zone plate, which alleviates the demands on fabrication, and the phase-contrast optics are single-element diffractive optical elements that produce contrast by Zernike or differential-interference contrast methods. The advantage of phase contrast in x-ray microscopy is shorter exposure times, and is crucial in the hard x-ray regime. Microscopy in the absorption‑contrast region of the water-window (2.34 - 4.37 nm) also benefits from these optics. The development of the optics for a laboratory soft x-ray microscope spans from theoretical and numerical analysis of coherence and stray light to experimental implementation and testing. The laboratory microscope uses laser-produced plasma-sources in the water-window and is unique in its design and performance. It will be shown that the laboratory microscope in its current form is a user-oriented and stable instrument, and has been used in a number of applications. The implementation of a cryogenic sample stage for tomographic imaging of biological samples in their natural environment has enabled applications in biology, and 3D x-ray microscopy of cells was performed for the first time with a laboratory instrument.
46.	Jones, K., et al. (författare) The stable climate of KELT-9b 2022 Ingår i: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 666 Tidskriftsartikel (refereegranskat)abstract Even among the most irradiated gas giants, so-called ultra-hot Jupiters, KELT-9b stands out as the hottest planet thus far discovered with a dayside temperature of over 4500 K. At these extreme irradiation levels, we expect an increase in heat redistribution efficiency and a low Bond albedo owed to an extended atmosphere with molecular hydrogen dissociation occurring on the planetary dayside. We present new photometric observations of the KELT-9 system throughout 4 full orbits and 9 separate occultations obtained by the 30 cm space telescope CHEOPS. The CHEOPS bandpass, located at optical wavelengths, captures the peak of the thermal emission spectrum of KELT-9b. In this work we simultaneously analyse CHEOPS phase curves along with public phase curves from TESS and Spitzer to infer joint constraints on the phase curve variation, gravity-darkened transits, and occultation depth in three bandpasses, as well as derive 2D temperature maps of the atmosphere at three different depths. We find a day-night heat redistribution efficiency of similar to 0.3 which confirms expectations of enhanced energy transfer to the planetary nightside due to dissociation and recombination of molecular hydrogen. We also calculate a Bond albedo consistent with zero. We find no evidence of variability of the brightness temperature of the planet, excluding variability greater than 1% (1 sigma).
47.	Ulfat, I., et al. (författare) Effects of nonuniform Mn distribution in (Ga,Mn)As 2014 Ingår i: Physical Review B Condensed Matter. - : American Physical Society. - 0163-1829 .- 1095-3795. ; 89:4, s. art no 045312- Tidskriftsartikel (refereegranskat)abstract Resonant in situ photoemission from Mn 3d states in Ga(1−x)MnxAs is reported for Mn concentrations down to the very dilute level of 0.1%. Concentration-dependent spectral features are analyzed on the basis of first-principles calculations for systems with selected impurity positions as well as for random alloys. Effects of direct Mn-Mn interaction are found for concentrations as low as 2.5%, and are ascribed to statistical (nonuniform) distribution of Mn atoms.
48.	Franz, Jan, 1973, et al. (författare) Computational study of vibrational-inelastic positron and electron scattering off CF4 molecules 2009 Ingår i: Atoms and Antimatter. Konferensbidrag (övrigt vetenskapligt/konstnärligt)
49.	Hedin, Lage, et al. (författare) Single site double core level ionisation of OCS 2014 Ingår i: Chemical Physics. - : Elsevier BV. - 0301-0104 .- 1873-4421. ; 439, s. 111-116 Tidskriftsartikel (refereegranskat)abstract Single site O1s, C1s and S2p double ionisation of the OCS molecule has been investigated using a magnetic bottle multi-electron coincidence time-of-flight spectrometer. Photon energies of 1300, 750 and 520 eV, respectively, were used for the ionisation, and spectra were obtained from which the double core ionisation energies could be determined. The energies measured for 1s double ionisation are 1172 eV (O1s(-2)) and 659 eV (C1s(-2)). For the S2p double ionisation three dicationic states are expected, P-3, D-1 and S-1. The ionisation energies obtained for these states are 373 eV (P-3), 380 eV (D-1) and 388 eV (S-1). The ratio between the double and single core ionisation energies are in all cases equal or close to 2.20. Auger spectra of OCS, associated with the O1s(-2), C1s(-2) and S2p(-2) dicationic states, were also recorded incorporating both electrons emitted as a result of the filling of the two core vacancies. As for other small molecules, the spectra show an atomic-like character with Auger bands located in the range 480-560 eV for oxygen, 235-295 eV for carbon and 100-160 eV for sulphur. The interpretation of the spectra is supported by CASSCF and CASCI calculations. The cross section ratio between double and single core hole creation was estimated as 3.7 x 10(-4) for oxygen at 1300 eV, 3.7 x 10(-4) for carbon at 750 eV and as 2.2 x 10(-3) for sulphur at 520 eV. (C) 2014 Elsevier B.V. All rights reserved.
50.	Marcellini, Moreno, et al. (författare) Transient isomers in the photodissociation of bromoiodomethane 2018 Ingår i: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 148:13 Tidskriftsartikel (refereegranskat)abstract The photochemistry of halomethanes is fascinating for the complex cascade reactions toward either the parent or newly synthesized molecules. Here, we address the structural rearrangement of photodissociated CH2IBr in methanol and cyclohexane, probed by time-resolved X-ray scattering in liquid solution. Upon selective laser cleavage of the C-I bond, we follow the reaction cascade of the two geminate geometrical isomers, CH2I-Br and CH2Br-I. Both meta-stable isomers decay on different time scales, mediated by solvent interaction, toward the original parent molecule. We observe the internal rearrangement of CH2Br-I to CH2I-Br in cyclohexane by extending the time window up to 3 mu s. We track the photoproduct kinetics of CH2Br-I in methanol solution where only one isomer is observed. The effect of the polarity of solvent on the geminate recombination pathways is discussed. Published by AIP Publishing.

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