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  • Dunås, Petter, 1990, et al. (author)
  • Palladium-catalyzed stereoselective domino arylation-acylation: an entry to chiral tetrahydrofluorenone scaffolds
  • 2021
  • In: Chemical Communications. - : Royal Society of Chemistry (RSC). - 1364-548X .- 1359-7345. ; 57:53, s. 6518-6521
  • Journal article (peer-reviewed)abstract
    • A palladium-catalyzed domino arylation-cyclization of biocatalytically derived cyclic 1,3-dienes is demonstrated. The reaction introduces a high degree of structural complexity in a single step, giving access to tricyclic tetrahydrofluorenones with full regio- and stereoselectivity. The transformation proceeds through a novel acylation-terminated Heck-type sequence, and quantum chemical calculations indicate that C-H activation is involved in the terminating acylation step.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Lewis, Simon E. (1)
Rahm, Martin, 1982 (1)
Kann, Nina, 1964 (1)
Dunås, Petter, 1990 (1)
Paterson, Andrew, 19 ... (1)
Kociok-Kohn, Gabriel ... (1)
University
Chalmers University of Technology (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year
2021 (1)

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