| 11. |
- Roth, Florian, et al.
(författare)
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High spatiotemporal variability of methane concentrations challenges estimates of emissions across vegetated coastal ecosystems.
- 2022
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Ingår i: Global change biology. - : Wiley. - 1365-2486 .- 1354-1013. ; 28:14, s. 4308-4322
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Tidskriftsartikel (refereegranskat)abstract
- Coastal methane (CH4 ) emissions dominate the global ocean CH4 budget and can offset the "blue carbon" storage capacity of vegetated coastal ecosystems. However, current estimates lack systematic, high-resolution, and long-term data from these intrinsically heterogeneous environments, making coastal budgets sensitive to statistical assumptions and uncertainties. Using continuous CH4 concentrations, δ13 C-CH4 values, and CH4 sea-air fluxes across four seasons in three globally pervasive coastal habitats, we show that the CH4 distribution is spatially patchy over meter-scales and highly variable in time. Areas with mixed vegetation, macroalgae, and their surrounding sediments exhibited a spatiotemporal variability of surface water CH4 concentrations ranging two orders of magnitude (i.e., 6-460nM CH4 ) with habitat-specific seasonal and diurnal patterns. We observed (1) δ13 C-CH4 signatures that revealed habitat-specific CH4 production and consumption pathways, (2) daily peak concentration events that could change >100% within hours across all habitats, and (3) a high thermal sensitivity of the CH4 distribution signified by apparent activation energies of ~1eV that drove seasonal changes. Bootstrapping simulations show that scaling the CH4 distribution from few samples involves large errors, and that ~50 concentration samples per day are needed to resolve the scale and drivers of the natural variability and improve the certainty of flux calculations by up to 70%. Finally, we identify northern temperate coastal habitats with mixed vegetation and macroalgae as understudied but seasonally relevant atmospheric CH4 sources (i.e., releasing≥100μmol CH4 m-2 day-1 in summer). Due to the large spatial and temporal heterogeneity of coastal environments, high-resolution measurements will improve the reliability of CH4 estimates and confine the habitat-specific contribution to regional and global CH4 budgets.
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| 12. |
- Roth, Florian, et al.
(författare)
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Methane emissions offset atmospheric carbon dioxide uptake in coastal macroalgae, mixed vegetation and sediment ecosystems
- 2023
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Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723. ; 14
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Tidskriftsartikel (refereegranskat)abstract
- Coastal ecosystems can efficiently remove carbon dioxide (CO2) from the atmosphere and are thus promoted for nature-based climate change mitigation. Natural methane (CH4) emissions from these ecosystems may counterbalance atmospheric CO2 uptake. Still, knowledge of mechanisms sustaining suchCH4 emissions and their contribution to net radiative forcing remains scarce for globally prevalent macroalgae, mixed vegetation, and surrounding depositional sediment habitats. Here we show that these habitats emit CH4 in the range of 0.1 – 2.9 mg CH4 m−2 d−1 to the atmosphere, revealing in situ CH4 emissions from macroalgae that weresustained by divergent methanogenic archaea in anoxic microsites. Over an annual cycle, CO2-equivalent CH4 emissions offset 28 and 35% of the carbon sink capacity attributed to atmospheric CO2 uptake in the macroalgae and mixed vegetation habitats, respectively, and augment net CO2 release of unvegetated sediments by 57%. Accounting for CH4 alongside CO2 sea-air fluxes and identifying the mechanisms controlling these emissions is crucial to constrain the potential of coastal ecosystems as net atmospheric carbon sinks and develop informed climate mitigation strategies.
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| 13. |
- Sotiropoulou, Georgia, et al.
(författare)
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Atmospheric conditions during the Arctic Clouds in Summer Experiment (ACSE) : Contrasting open-water and sea-ice surfaces during melt and freeze-up seasons
- 2016
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Ingår i: Journal of Climate. - 0894-8755 .- 1520-0442. ; 29:24, s. 8721-8744
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Tidskriftsartikel (refereegranskat)abstract
- The Arctic Clouds in Summer Experiment (ACSE) was conducted during summer and early autumn 2014, providing a detailed view of the seasonal transition from ice melt into freeze-up. Measurements were taken over both ice-free and ice-covered surfaces, near the ice edge, offering insight to the role of the surface state in shaping the atmospheric conditions. The initiation of the autumn freeze-up was related to a change in air mass, rather than to changes in solar radiation alone; the lower atmosphere cooled abruptly leading to a surface heat loss. During melt season, strong surface inversions persisted over the ice, while elevated inversions were more frequent over open water. These differences disappeared during autumn freeze-up, when elevated inversions persisted over both ice-free and ice-covered conditions. These results are in contrast to previous studies that found a well-mixed boundary layer persisting in summer and an increased frequency of surface-based inversions in autumn, suggesting that our knowledge derived from measurements taken within the pan-Arctic area and on the central ice-pack does not necessarily apply closer to the ice-edge. This study offers an insight to the atmospheric processes that occur during a crucial period of the year; understanding and accurately modeling these processes is essential for the improvement of ice-extent predictions and future Arctic climate projections.
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| 14. |
- Srivastava, Piyush, et al.
(författare)
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Ship-based estimates of momentum transfer coefficient over sea ice and recommendations for its parameterization
- 2022
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 22:7, s. 4763-4778
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Tidskriftsartikel (refereegranskat)abstract
- A major source of uncertainty in both climate projections and seasonal forecasting of sea ice is inadequate representation of surface–atmosphere exchange processes. The observations needed to improve understanding and reduce uncertainty in surface exchange parameterizations are challenging to make and rare. Here we present a large dataset of ship-based measurements of surface momentum exchange (surface drag) in the vicinity of sea ice from the Arctic Clouds in Summer Experiment (ACSE) in July–October 2014, and the Arctic Ocean 2016 experiment (AO2016) in August–September 2016. The combined dataset provides an extensive record of momentum flux over a wide range of surface conditions spanning the late summer melt and early autumn freeze-up periods, and a wide range of atmospheric stabilities. Surface exchange coefficients are estimated from in situ eddy covariance measurements. The local sea-ice fraction is determined via automated processing of imagery from ship-mounted cameras. The surface drag coefficient, CD10n, peaks at local ice fractions of 0.6–0.8, consistent with both recent aircraft-based observations and theory. Two state-of-the-art parameterizations have been tuned to our observations, with both providing excellent fits to the measurements.
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| 15. |
- Thornton, Brett F., et al.
(författare)
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Shipborne eddy covariance observations of methane fluxes constrain Arctic sea emissions
- 2020
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Ingår i: Science Advances. - : American Association for the Advancement of Science (AAAS). - 2375-2548. ; 6:5
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Tidskriftsartikel (refereegranskat)abstract
- We demonstrate direct eddy covariance (EC) observations of methane (CH4) fluxes between the sea and atmosphere from an icebreaker in the eastern Arctic Ocean. EC-derived CH4 emissions averaged 4.58, 1.74, and 0.14 mg m(-2) day(-1) in the Laptev, East Siberian, and Chukchi seas, respectively, corresponding to annual sea-wide fluxes of 0.83, 0.62, and 0.03 Tg year(-1) . These EC results answer concerns that previous diffusive emission estimates, which excluded bubbling, may underestimate total emissions. We assert that bubbling dominates sea-air CH4 fluxes in only small constrained areas: A similar to 100-m(2) area of the East Siberian Sea showed sea-air CH4 fluxes exceeding 600 mg m(-2) day(-1); in a similarly sized area of the Laptev Sea, peak CH4 fluxes were similar to 170 mg m(-2) day(-1). Calculating additional emissions below the noise level of our EC system suggests total ESAS CH4 emissions of 3.02 Tg year(-1) closely matching an earlier diffusive emission estimate of 2.9 Tg year(-1).
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| 16. |
- Tjernström, Michael, et al.
(författare)
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Arctic Summer Airmass Transformation, Surface Inversions, and the Surface Energy Budget
- 2019
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Ingår i: Journal of Climate. - 0894-8755 .- 1520-0442. ; 32:3, s. 769-789
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Tidskriftsartikel (refereegranskat)abstract
- During the Arctic Clouds in Summer Experiment (ACSE) in summer 2014 a weeklong period of warm-air advection over melting sea ice, with the formation of a strong surface temperature inversion and dense fog, was observed. Based on an analysis of the surface energy budget, we formulated the hypothesis that, because of the airmass transformation, additional surface heating occurs during warm-air intrusions in a zone near the ice edge. To test this hypothesis, we explore all cases with surface inversions occurring during ACSE and then characterize the inversions in detail. We find that they always occur with advection from the south and are associated with subsidence. Analyzing only inversion cases over sea ice, we find two categories: one with increasing moisture in the inversion and one with constant or decreasing moisture with height. During surface inversions with increasing moisture with height, an extra 10-25 W m(-2) of surface heating was observed, compared to cases without surface inversions; the surface turbulent heat flux was the largest single term. Cases with less moisture in the inversion were often cloud free and the extra solar radiation plus the turbulent surface heat flux caused by the inversion was roughly balanced by the loss of net longwave radiation.
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| 17. |
- Tjernström, Michael, et al.
(författare)
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Warm-air advection, air mass transformation and fog causes rapid ice melt
- 2015
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Ingår i: Geophysical Research Letters. - 0094-8276 .- 1944-8007. ; 42:13, s. 5594-5602
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Tidskriftsartikel (refereegranskat)abstract
- Direct observations during intense warm-air advection over the East Siberian Sea reveal a period of rapid sea-ice melt. A semistationary, high-pressure system north of the Bering Strait forced northward advection of warm, moist air from the continent. Air-mass transformation over melting sea ice formed a strong, surface-based temperature inversion in which dense fog formed. This induced a positive net longwave radiation at the surface while reducing net solar radiation only marginally; the inversion also resulted in downward turbulent heat flux. The sum of these processes enhanced the surface energy flux by an average of similar to 15Wm(-2) for a week. Satellite images before and after the episode show sea-ice concentrations decreasing from > 90% to similar to 50% over a large area affected by the air-mass transformation. We argue that this rapid melt was triggered by the increased heat flux from the atmosphere due to the warm-air advection.
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| 18. |
- Vüllers, Jutta, et al.
(författare)
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Meteorological and cloud conditions during the Arctic Ocean 2018 expedition
- 2021
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 21:1, s. 289-314
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Tidskriftsartikel (refereegranskat)abstract
- The Arctic Ocean 2018 (AO2018) took place in the central Arctic Ocean in August and September 2018 on the Swedish icebreaker Oden. An extensive suite of instrumentation provided detailed measurements of surface water chemistry and biology, sea ice and ocean physical and biogeochemical properties, surface exchange processes, aerosols, clouds, and the state of the atmosphere. The measurements provide important information on the coupling of the ocean and ice surface to the atmosphere and in particular to clouds. This paper provides (i) an overview of the synoptic-scale atmospheric conditions and their climatological anomaly to help interpret the process studies and put the detailed observations from AO2018 into a larger context, both spatially and temporally; (ii) a statistical analysis of the thermodynamic and near-surface meteorological conditions, boundary layer, cloud, and fog characteristics; and (iii) a comparison of the results to observations from earlier Arctic Ocean expeditions – in particular AOE1996 (Arctic Ocean Expedition 1996), SHEBA (Surface Heat Budget of the Arctic Ocean), AOE2001 (Arctic Ocean Experiment 2001), ASCOS (Arctic Summer Cloud Ocean Study), ACSE (Arctic Clouds in Summer Experiment), and AO2016 (Arctic Ocean 2016) – to provide an assessment of the representativeness of the measurements. The results show that near-surface conditions were broadly comparable to earlier experiments; however the thermodynamic vertical structure was quite different. An unusually high frequency of well-mixed boundary layers up to about 1 km depth occurred, and only a few cases of the “prototypical” Arctic summer single-layer stratocumulus deck were observed. Instead, an unexpectedly high amount of multiple cloud layers and mid-level clouds were present throughout the campaign. These differences from previous studies are related to the high frequency of cyclonic activity in the central Arctic in 2018.
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| 19. |
- Willis, Megan D., et al.
(författare)
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Polar oceans and sea ice in a changing climate
- 2023
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Ingår i: Elementa. - 2325-1026. ; 11:1
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Forskningsöversikt (refereegranskat)abstract
- Polar oceans and sea ice cover 15% of the Earth's ocean surface, and the environment is changing rapidly at both poles. Improving knowledge on the interactions between the atmospheric and oceanic realms in the polar regions, a Surface Ocean-Lower Atmosphere Study (SOLAS) project key focus, is essential to understanding the Earth system in the context of climate change. However, our ability to monitor the pace and magnitude of changes in the polar regions and evaluate their impacts for the rest of the globe is limited by both remoteness and sea-ice coverage. Sea ice not only supports biological activity and mediates gas and aerosol exchange but can also hinder some in-situ and remote sensing observations. While satellite remote sensing provides the baseline climate record for sea-ice properties and extent, these techniques cannot provide key variables within and below sea ice. Recent robotics, modeling, and in-situ measurement advances have opened new possibilities for understanding the ocean-sea ice-atmosphere system, but critical knowledge gaps remain. Seasonal and long-term observations are clearly lacking across all variables and phases. Observational and modeling efforts across the sea-ice, ocean, and atmospheric domains must be better linked to achieve a system-level understanding of polar ocean and sea-ice environments. As polar oceans are warming and sea ice is becoming thinner and more ephemeral than before, dramatic changes over a suite of physicochemical and biogeochemical processes are expected, if not already underway. These changes in sea-ice and ocean conditions will affect atmospheric processes by modifying the production of aerosols, aerosol precursors, reactive halogens and oxidants, and the exchange of greenhouse gases. Quantifying which processes will be enhanced or reduced by climate change calls for tailored monitoring programs for high-latitude ocean environments. Open questions in this coupled system will be best resolved by leveraging ongoing international and multidisciplinary programs, such as efforts led by SOLAS, to link research across the ocean-sea ice-atmosphere interface.
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