| 11. |
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| 12. |
- Boll, Rebecca, et al.
(författare)
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Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules
- 2014
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Ingår i: Faraday Discussions. - : Royal Society of Chemistry (RSC). - 1364-5498. ; 171, s. 57-80
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Tidskriftsartikel (refereegranskat)abstract
- This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.
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| 15. |
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| 16. |
- Brasse, Felix, et al.
(författare)
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Time-resolved inner-shell photoelectron spectroscopy : From a bound molecule to an isolated atom
- 2018
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Ingår i: Physical Review A: covering atomic, molecular, and optical physics and quantum information. - 2469-9926 .- 2469-9934. ; 97:4
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Tidskriftsartikel (refereegranskat)abstract
- Due to its element and site specificity, inner-shell photoelectron spectroscopy is a widely used technique to probe the chemical structure of matter. Here, we show that time-resolved inner-shell photoelectron spectroscopy can be employed to observe ultrafast chemical reactions and the electronic response to the nuclear motion with high sensitivity. The ultraviolet dissociation of iodomethane (CH3I) is investigated by ionization above the iodine 4d edge, using time-resolved inner-shell photoelectron and photoion spectroscopy. The dynamics observed in the photoelectron spectra appear earlier and are faster than those seen in the iodine fragments. The experimental results are interpreted using crystal-field and spin-orbit configuration interaction calculations, and demonstrate that time-resolved inner-shell photoelectron spectroscopy is a powerful tool to directly track ultrafast structural and electronic transformations in gas-phase molecules.
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| 17. |
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| 18. |
- Eckersten, Henrik, et al.
(författare)
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Ecosystem C and N dynamics affected by a modified spring barley trait with increased nitrogen use - a simulation case study
- 2018
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Ingår i: Acta Agriculturae Scandinavica - Section B. - : Taylor & Francis. - 0906-4710 .- 1651-1913. ; 68:3, s. 230-242
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Tidskriftsartikel (refereegranskat)abstract
- To what extent might a crop with increased plant N uptake efficiency and/or N demand increase plant biomass and soil carbon storage, decrease N leaching, and reduce the need for N fertilisation? This was assessed for a fertilised sandy loam site in central Sweden cultivated with spring barley for a four year period using a process based crop and soil simulation model (SOILN) calibrated to fit observations of field experiments with non-modified crops. Crop properties were changed in accordance with previous model applications to other crops with higher N uptake and utilisation efficiencies, to resemble potential effects of breeding. For the modified crops a doubling of daily uptake efficiency of soil mineral N and/or increase of radiation use efficiency by 30%, increased plant biomass by 3%-30%, decreased N leaching by 1%-30% and increased soil organic carbon (SOC) content by 1-12 g C m-2 year-1. The larger changes were mainly due to increased uptake efficiency. Fertilisation of the modified spring barley crop could be reduced while still producing the same plant biomass as the non-modified crop. The plant biomass to N leaching ratio of the modified crops increased. The simulated changes in plant biomass and SOC were sensitive to weather conditions suggesting that in situ experiments would need to cover a large range of weather conditions to evaluate the performance of new crop traits under climatic variability. The study suggests a strong need that field experiments are accompanied with model applications, when exploring the potential of the modified crops under variable conditions.
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| 19. |
- Eckersten, Henrik, et al.
(författare)
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Nitrogen leaching and soil organic carbon sequestration of a Barley crop with improved N use efficiency : A regional case study
- 2017
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Ingår i: Acta Agriculturae Scandinavica - Section B. - : Taylor and Francis Ltd.. - 0906-4710 .- 1651-1913. ; 67:7, s. 615-627
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Tidskriftsartikel (refereegranskat)abstract
- The potential of modified spring barley crops with improved nitrogen (N) use efficiency to reduce nitrogen (N) leaching and to increase soil organic carbon (SOC) storage was assessed at the regional scale. This was done using simulation model applications designed for reporting according to the Helcom (Helsinki Commission) and Kyoto protocols. Using model simulations based on modified crops N dynamics and SOC were assessed for three agro-ecological regions (latitudes ranging 55°20′–60°40′ N) in Sweden over a 20-year period. The modified N use properties of spring barley were implemented in the SOILNDB model (simulating soil C, N, water and heat, and plant N dynamics) by changing the parameters for root N uptake efficiency and plant N demand within a range given by previous model applications to different crops. A doubling of the daily N uptake efficiency and increased N demand (by ca 30%) reduced N leaching by 24%–31%, increased plant N content by 9%–12%, depending on region. The effects of the modified crop on SOC was simulated with the ICBM model, resulting in an increased SOC content (0–25 cm depth) by 57–79 kg C ha−1 y−1. The results suggest that a modified crop might reduce N leaching from spring barley area, in a range similar to the targets of relevant environmental protection directives, a result which held more in the northern than southern regions. The simulated SOC increase on a hectare basis was highest for the central region and least for the most northern region. For the total agricultural area the share of spring barley area was small and more crops would need to be modified to reach the emission reduction targets.
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| 20. |
- Ekström, Thomas, et al.
(författare)
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A framework for case study research - highlighting the reviewers' perspectives
- 2009
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Ingår i: Proceedings of The 21st Annual Nofoma Conference, 11-12 June 2009 Jönköping Sweden. - 9789186345013 ; , s. 159-174
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Konferensbidrag (refereegranskat)abstract
- Purpose of this paper The purpose is twofold: to map the reviewers’ perspective of evaluation of case based logistics and supply chain management research; and to develop a framework with all criteria needed to design, conduct, and present rigorous case study research. This framework can be used by both researchers and reviewers. Design/methodology/approach An interview study is performed to establish how reviews currently are being conducted in logistics and supply chain management journals. A literature review in combination with a both divisive and agglomerate cluster analysis is applied to develop the framework. The framework is compared to the evaluation criteria provided by reviewers. Findings There is an expressed need for a more structured and systematic review process for case based articles. An established framework for evaluation of case based research does not exist. There is a lack of standardized terminology in the field. A comprehensive framework for case based research is developed and presented. Research limitations/implications The research is focused on case studies only. What is original/value of paper? This paper present both the reviewers perspective on case study evaluation and it provides a comprehensive framework for all steps of a rigorous case based research process including what aspects that should be included and recommendations for how and why certain aspects should be included.
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