| 1. |
- Kirkevag, A., et al.
(författare)
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Aerosol-climate interactions in the Norwegian Earth System Model-NorESM1-M
- 2013
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Ingår i: Geoscientific Model Development. - : Copernicus GmbH. - 1991-959X .- 1991-9603. ; 6:1, s. 207-244
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Tidskriftsartikel (refereegranskat)abstract
- The objective of this study is to document and evaluate recent changes and updates to the module for aerosols and aerosol-cloud-radiation interactions in the atmospheric module CAM4-Oslo of the core version of the Norwegian Earth System Model (NorESM), NorESM1-M. Particular attention is paid to the role of natural organics, sea salt, and mineral dust in determining the gross aerosol properties as well as the anthropogenic contribution to these properties and the associated direct and indirect radiative forcing. The aerosol module is extended from earlier versions that have been published, and includes life-cycling of sea salt, mineral dust, particulate sulphate, black carbon, and primary and secondary organics. The impacts of most of the numerous changes since previous versions are thoroughly explored by sensitivity experiments. The most important changes are: modified prognostic sea salt emissions; updated treatment of precipitation scavenging and gravitational settling; inclusion of biogenic primary organics and methane sulphonic acid (MSA) from oceans; almost doubled production of land-based biogenic secondary organic aerosols (SOA); and increased ratio of organic matter to organic carbon (OM/OC) for biomass burning aerosols from 1.4 to 2.6. Compared with in situ measurements and remotely sensed data, the new treatments of sea salt and dust aerosols give smaller biases in near-surface mass concentrations and aerosol optical depth than in the earlier model version. The model biases for mass concentrations are approximately unchanged for sulphate and BC. The enhanced levels of modeled OM yield improved overall statistics, even though OM is still underestimated in Europe and overestimated in North America. The global anthropogenic aerosol direct radiative forcing (DRF) at the top of the atmosphere has changed from a small positive value to -0.08 W m(-2) in CAM4-Oslo. The sensitivity tests suggest that this change can be attributed to the new treatment of biomass burning aerosols and gravitational settling. Although it has not been a goal in this study, the new DRF estimate is closer both to the median model estimate from the AeroCom intercomparison and the best estimate in IPCC AR4. Estimated DRF at the ground surface has increased by ca. 60 %, to -1.89 W m(-2). We show that this can be explained by new emission data and omitted mixing of constituents between updrafts and downdrafts in convective clouds. The increased abundance of natural OM and the introduction of a cloud droplet spectral dispersion formulation are the most important contributions to a considerably decreased estimate of the indirect radiative forcing (IndRF). The IndRF is also found to be sensitive to assumptions about the coating of insoluble aerosols by sulphate and OM. The IndRF of -1.2 W m(-2), which is closer to the IPCC AR4 estimates than the previous estimate of -1.9 W m(-2), has thus been obtained without imposing unrealistic artificial lower bounds on cloud droplet number concentrations.
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| 2. |
- Lewinschal, Anna, 1983-
(författare)
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Interactions between aerosols and large-scale circulation systems in the atmosphere
- 2013
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Anthropogenic aerosol emissions have increased during the last century. The higher atmospheric aerosol burden is believed to partly have masked the enhanced greenhouse gas warming during the same period. However, the many different types of aerosols, and the uncertainties regarding their effect on clouds, makes it difficult to estimate their total climate impact. With their strong effect on atmospheric radiation and their varying spatial and temporal distribution, aerosols may also affect the atmospheric circulation. This thesis focuses on aspects of aerosol-induced circulation changes as represented in general circulations models.Anthropogenic aerosol forcing is believed to generally cool the earth system, but model simulations show that the strongest cooling is not necessarily co-located with the strongest aerosol radiative forcing. It is shown that aerosol forcing can cause anomalies in the stationary wave pattern, which affects surface temperatures far from the region of aerosol forcing. In absence of a substantial global mean aerosol-induced cooling, the anomalous stationary wave pattern has a large influence on the simulated temperature-response pattern. The waves are primarily generated by aerosol-induced precipitation changes in the tropics, showing an important connection between aerosol emissions at low latitudes and surface temperate changes in the extra-tropics.It is also demonstrated that the aerosol climate response differs depending on how the ocean surface is represented in a model, i.e. if a sea surface temperature response is permitted or not. The anthropogenic aerosol forcing generates a stronger cooling of the northern hemisphere when the sea surface temperatures can change compared to when they are fixed. The stronger inter-hemispheric temperature gradient affects both the tropical and extra-tropical zonal mean circulation. Thus, aerosol-induced circulation changes are dependent on the simulated surface temperature response.
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| 3. |
- Lewinschal, Anna, 1983-, et al.
(författare)
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The role of precipitation in aerosol-induced changes in northern hemisphere wintertime stationary waves
- 2013
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Ingår i: Climate Dynamics. - : Springer Science and Business Media LLC. - 0930-7575 .- 1432-0894. ; 41:3-4, s. 647-661
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Tidskriftsartikel (refereegranskat)abstract
- The coupled climate model EC-Earth2 is used to investigate the impact of direct radiative effects of aerosols on stationary waves in the northern hemisphere wintertime circulation. The direct effect of aerosols is simulated by introducing prescribed mixing ratios of different aerosol compounds representing pre-industrial and present-day conditions, no indirect effects are included. In the EC-Earth2 results, the surface temperature response is uncorrelated with the highly asymmetric aerosol radiative forcing pattern. Instead, the anomalous extratropical temperature field bears a strong resemblance to the aerosol-induced changes in the stationary-wave pattern. It is demonstrated that the main features of the wave pattern of EC-Earth2 can be replicated by a linear, baroclinic model forced with latent heat changes corresponding to the anomalous convective precipitation generated by EC-Earth2. The tropical latent heat release is an effective means of generating stationary wave trains that propagate into the extratropics. Hence, the results of the present study indicate that aerosol-induced convective precipitation anomalies govern the extratropical wave-field changes, and that the far-field temperature response dominates over local effects of aerosol radiative forcing.
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| 4. |
- Rastak, Narges, et al.
(författare)
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Modeling Aerosol Water Uptake in The Arctic Based on The kappa-Kohler Theory
- 2013
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Ingår i: Nucleation and Atmospheric Aerosols. - : American Institute of Physics (AIP). - 9780735411524 ; , s. 702-705
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Konferensbidrag (refereegranskat)abstract
- Water uptake or hygroscopicity is one of the most fundamental properties of atmospheric aerosols. Aerosol particles containing soluble materials can grow in size by absorbing water in ambient atmosphere. This property is measured by a parameter known as growth factor (GF), which is defined as the ratio of the wet diameter to the dry diameter. Hygroscopicity controls the size of an aerosol particle and therefore its optical properties in the atmosphere. Hygroscopic growth depends on the dry size of the particle, its chemical composition and the relative humidity in the ambient air (Fitzgerald, 1975; Pilinis et al., 1995). One of the typical problems in aerosol studies is the lack of measurements of aerosol size distributions and optical properties in ambient conditions. The gap between dry measurements and the real humid atmosphere is filled in this study by utilizing a hygroscopic model which calculates the hygroscopic growth of aerosol particles at Mt Zeppelin station, Ny Alesund, Svalbard during 2008.
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| 5. |
- Struthers, Hamish, et al.
(författare)
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Climate-induced changes in sea salt aerosol number emissions : 1870 to 2100
- 2013
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Ingår i: Journal of Geophysical Research-Atmospheres. - : American Geophysical Union (AGU). - 2169-897X. ; 118:2, s. 670-682
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Tidskriftsartikel (refereegranskat)abstract
- Global climate model output is combined with an emission parameterization to estimate the change in the global and regional sea salt aerosol number emission from 1870 to 2100. Global average results suggest a general increase in sea salt aerosol number emission due to increasing surface wind speed. However, the emission changes are not uniform over the aerosol size spectrum due to an increase in sea surface temperature. From 1870 to 2100 the emission of coarse mode particles (dry diameter D-P > 655 nm) increase by approximately 10 % (global average), whereas no significant change in the emission of ultrafine mode aerosols (dry diameter D-p < 76 nm) was found over the same period. Significant regional differences in the number emission trends were also found. Based on CAM-Oslo global climate model output, no straight-forward relationship was found between the change in the number emissions and changes in the sea salt aerosol burden or optical thickness. This is attributed to a change in the simulated residence time of the sea salt aerosol. For the 21st century, a decrease in the residence time leads to a weaker sea salt aerosol-climate feedback that what would be inferred based on changes in number emissions alone. Finally, quantifying any potential impact on marine stratocumulus cloud microphysical and radiative properties due to changes in sea salt aerosol number emissions is likely to be complicated by commensurate changes in anthropogenic aerosol emissions and changes in meteorology.
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| 6. |
- Zabori, Julia, et al.
(författare)
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Comparison between summertime and wintertime Arctic Ocean primary marine aerosol properties
- 2013
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 13:9, s. 4783-4799
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Tidskriftsartikel (refereegranskat)abstract
- Primary marine aerosols (PMAs) are an important source of cloud condensation nuclei, and one of the key elements of the remote marine radiative budget. Changes occurring in the rapidly warming Arctic, most importantly the decreasing sea ice extent, will alter PMA production and hence the Arctic climate through a set of feedback processes. In light of this, laboratory experiments with Arctic Ocean water during both Arctic winter and summer were conducted and focused on PMA emissions as a function of season and water properties. Total particle number concentrations and particle number size distributions were used to characterize the PMA population. A comprehensive data set from the Arctic summer and winter showed a decrease in PMA concentrations for the covered water temperature (T-w) range between - 1 degrees C and 15 degrees C. A sharp decrease in PMA emissions for a T-w increase from -1 degrees C to 4 degrees C was followed by a lower rate of change in PMA emissions for T-w up to about 6 degrees C. Near constant number concentrations for water temperatures between 6 degrees C to 10 degrees C and higher were recorded. Even though the total particle number concentration changes for overlapping T-w ranges were consistent between the summer and winter measurements, the distribution of particle number concentrations among the different sizes varied between the seasons. Median particle number concentrations for a dry diameter (D-p) < 0.125 mu m measured during winter conditions were similar (deviation of up to 3 %), or lower (up to 70 %) than the ones measured during summer conditions (for the same water temperature range). For D-p > 0.125 mu m, the particle number concentrations during winter were mostly higher than in summer (up to 50 %). The normalized particle number size distribution as a function of water temperature was examined for both winter and summer measurements. An increase in T-w from -1 degrees C to 10 degrees C during winter measurements showed a decrease in the peak of relative particle number concentration at about a D-p of 0.180 mu m, while an increase was observed for particles with D-p > 1 mu m. Summer measurements exhibited a relative shift to smaller particle sizes for an increase of T-w in the range 7-11 degrees C. The differences in the shape of the number size distributions between winter and summer may be caused by different production of organic material in water, different local processes modifying the water masses within the fjord (for example sea ice production in winter and increased glacial meltwater inflow during summer) and different origin of the dominant sea water mass. Further research is needed regarding the contribution of these factors to the PMA production.
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