| 1. |
- Blomquist, Emil, et al.
(författare)
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Unbiased description of magnetic polarons in a Mott insulator
- 2020
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Ingår i: Communications Physics. - : Springer Nature. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- Polarons are elementary quasi-particles characterizing several interacting many-body quantum systems. The authors present an unbiased Quantum Monte Carlo simulation of a magnetic polaron in a t-J model at low-temperature, and find excellent agreement with a recent experimental realization in the framework of cold-atoms systems. Polarons are among the most elementary quasiparticles of interacting quantum matter, consisting of a charge carrier dressed by an excited background. In Mott insulators, they take the form of a dopant surrounded by a distorted spin-background. Despite the fundamental importance of polarons for the electronic structure of strongly correlated systems, access to their internal structure was only recently realized in experiments, while controllable theoretical results are still lacking due to the sign problem. Here we report unbiased high-precision data obtained from worm-algorithm Monte Carlo that reveal the real-space structure of a polaron in thet-Jmodel deep inside the region where the sign problem becomes significant. These results are directly comparable to recent quantum gas microscopy experiments, but give access to significantly lower temperatures.
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| 2. |
- Kuttruff, Joel, et al.
(författare)
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Ultrafast all-optical switching enabled by epsilon-near-zero-tailored absorption in metal-insulator nanocavities
- 2020
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Ingår i: Communications Physics. - : Nature Publishing Group. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- Ultrafast control of light−matter interactions is fundamental in view of new technological frontiers of information processing. However, conventional optical elements are either static or feature switching speeds that are extremely low with respect to the time scales at which it is possible to control light. Here, we exploit the artificial epsilon-near-zero (ENZ) modes of a metal-insulator-metal nanocavity to tailor the linear photon absorption of our system and realize a nondegenerate all-optical ultrafast modulation of the reflectance at a specific wavelength. Optical pumping of the system at its high energy ENZ mode leads to a strong redshift of the low energy mode because of the transient increase of the local dielectric function, which leads to a sub-3-ps control of the reflectance at a specific wavelength with a relative modulation depth approaching 120%.
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| 3. |
- Mewes, L., et al.
(författare)
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Energy relaxation pathways between light-matter states revealed by coherent two-dimensional spectroscopy
- 2020
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Ingår i: Communications Physics. - : Springer Science and Business Media LLC. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- Coupling matter excitations to electromagnetic modes inside nano-scale optical resonators leads to the formation of hybrid light-matter states, so-called polaritons, allowing the controlled manipulation of material properties. Here, we investigate the photo-induced dynamics of a prototypical strongly-coupled molecular exciton-microcavity system using broadband two-dimensional Fourier transform spectroscopy and unravel the mechanistic details of its ultrafast photo-induced dynamics. We find evidence for a direct energy relaxation pathway from the upper to the lower polariton state that initially bypasses the excitonic manifold of states, which is often assumed to act as an intermediate energy reservoir, under certain experimental conditions. This observation provides new insight into polariton photophysics and could potentially aid the development of applications that rely on controlling the energy relaxation mechanism, such as in solar energy harvesting, manipulating chemical reactivity, the creation of Bose-Einstein condensates and quantum computing. Recent spectroscopic studies have elucidated light-matter interactions in exciton-polaritons at room temperature, yet their precise excited-state dynamics remain unclear. Here, broadband 2D Fourier transform spectroscopy reveals the relaxation between polaritonic states and the role of dark states.
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| 4. |
- Sobolev, Egor, et al.
(författare)
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Megahertz single-particle imaging at the European XFEL
- 2020
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Ingår i: Communications Physics. - : Springer Science and Business Media LLC. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- The emergence of high repetition-rate X-ray free-electron lasers (XFELs) powered by superconducting accelerator technology enables the measurement of significantly more experimental data per day than was previously possible. The European XFEL is expected to provide 27,000 pulses per second, over two orders of magnitude more than any other XFEL. The increased pulse rate is a key enabling factor for single-particle X-ray diffractive imaging, which relies on averaging the weak diffraction signal from single biological particles. Taking full advantage of this new capability requires that all experimental steps, from sample preparation and delivery to the acquisition of diffraction patterns, are compatible with the increased pulse repetition rate. Here, we show that single-particle imaging can be performed using X-ray pulses at megahertz repetition rates. The results obtained pave the way towards exploiting high repetition-rate X-ray free-electron lasers for single-particle imaging at their full repetition rate.
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| 5. |
- Venkateshwarlu, Sarangi, et al.
(författare)
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Large electromechanical strain and unconventional domain switching near phase convergence in a Pb-free ferroelectric
- 2020
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Ingår i: Communications Physics. - : Springer Science and Business Media LLC. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- In many ferroelectrics, large electromechanical strains are observed near regions of composition- or temperature- driven phase coexistence. Phenomenologically, this is attributed to easy re-orientation of the polarization vector and/or phase transition, although their effects are highly convoluted and difficult to distinguish experimentally. Here, we used synchrotron X-ray scattering and digital image correlation to differentiate between the microscopic mechanisms leading to large electrostrains in an exemplary Pb-free piezoceramic Sn-doped barium calcium zirconate titanate. Large electrostrains of ~0.2% measured at room-temperature are attributed to an unconventional effect, wherein polarization switching is aided by a reversible phase transition near the tetragonal-orthorhombic phase boundary. Additionally, electrostrains of ~0.1% or more could be maintained from room temperature to 140 °C due to a succession of different microscopic mechanisms. In situ X-ray diffraction elucidates that while 90° domain reorientation is pertinent below the Curie temperature (TC), isotropic distortion of polar clusters is the dominant mechanism above TC.
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| 6. |
- Xavier, Guilherme B., et al.
(författare)
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Quantum information processing with space-division multiplexing optical fibres
- 2020
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Ingår i: Communications Physics. - : Springer Nature. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- The optical fibre is an essential tool for our communication infrastructure since it is the main transmission channel for optical communications. The latest major advance in optical fibre technology is space-division multiplexing, where new fibre designs and components establish multiple co-existing data channels based on light propagation over distinct transverse optical modes. Simultaneously, there have been many recent developments in the field of quantum information processing, with novel protocols and devices in areas such as computing and communication. Here, we review recent results in quantum information based on space-division multiplexing optical fibres, and discuss new possibilities based on this technology.
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| 7. |
- Xu, Zhangli, et al.
(författare)
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Driving positron beam acceleration with coherent transition radiation
- 2020
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Ingår i: Communications Physics. - : Springer Science and Business Media LLC. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- Positron acceleration in plasma wakefield faces significant challenges, as the positron beam must be pre-generated and precisely coupled into the wakefield and, most critically, suffers from defocusing issues. Here we propose a scheme that utilizes laser-driven electrons to produce, inject, and accelerate positrons in a single setup. The high-charge electron beam from wakefield acceleration creates copious electron–positron pairs via the Bethe–Heitler process, followed by enormous coherent transition radiation due to the electrons’ exiting from the metallic foil. Simulation results show that the coherent transition radiation field reaches up to tens of GV m−1, which captures and accelerates the positrons to cut-off energy of 1.5 GeV with energy peak of 500 MeV (energy spread ~ 24.3%). An external longitudinal magnetic field of 30 T is also applied to guide the electrons and positrons during the acceleration process. This proposed method offers a promising way to obtain GeV fast positron sources.
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| 8. |
- Yordanov, Deyan T., et al.
(författare)
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Structural trends in atomic nuclei from laser spectroscopy of tin
- 2020
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Ingår i: Communications Physics. - : Springer Nature. - 2399-3650. ; 3:1
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Tidskriftsartikel (refereegranskat)abstract
- Tin is the chemical element with the largest number of stable isotopes. Its complete proton shell, comparable with the closed electron shells in the chemically inert noble gases, is not a mere precursor to extended stability; since the protons carry the nuclear charge, their spatial arrangement also drives the nuclear electromagnetism. We report high-precision measurements of the electromagnetic moments and isomeric differences in charge radii between the lowest 1/2(+), 3/2(+), and 11/2(-) states in Sn117-131, obtained by collinear laser spectroscopy. Supported by state-of-the-art atomic-structure calculations, the data accurately show a considerable attenuation of the quadrupole moments in the closed-shell tin isotopes relative to those of cadmium, with two protons less. Linear and quadratic mass-dependent trends are observed. While microscopic density functional theory explains the global behaviour of the measured quantities, interpretation of the local patterns demands higher-fidelity modelling. Measurements of the hyperfine structure of chemical elements isotopes provide unique insight into the atomic nucleus in a nuclear model-independent way. The authors present collinear laser spectroscopy data obtained at the CERN ISOLDE and measure hyperfine splitting along a long chain of odd-mass tin isotopes.
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