| 1. |
- Baró Pérez, Alejandro, 1991-
(författare)
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Aerosol impacts on subtropical low-level clouds: a satellite and modelling perspective
- 2023
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Complex interactions between aerosols, clouds, and radiation impact Earth's climate. However, several aspects of these interactions remain uncertain, which has led to extensive research over the last decades. This thesis explores some unresolved aspects by focusing on subtropical low-level stratocumulus (Sc) clouds, which have a significant cooling effect on climate. The clouds are also sensitive to varying aerosol conditions, which can influence their formation, properties, and lifetime. Clouds over the South East Atlantic have been studied in detail, using both numerical modeling and satellite observations, to shed light on the interactions between aerosols, clouds, and radiation. This geographical region displays a large and semi-permanent Sc cloud deck and is also subjected to meteorological conditions that bring large amounts of light-absorbing aerosols from biomass fires over the African continent. The biomass-burning plumes also bring enhanced levels of moisture, and the individual influence of the aerosols and the moisture on the low-level cloud properties have been investigated.The analysis of satellite retrievals showed a radiative impact (sensitive to aerosol composition and aerosol optical depth) of moist aerosol layers in the free troposphere over the South East Atlantic; however, it was not possible to observe a clear influence of these humid aerosol layers on the underlying low-level clouds. Aerosol-radiation interactions were implemented in a large eddy simulation (LES) code that was used to model stratocumulus to cumulus transitions (SCT) in weather situations where moist absorbing aerosol layers were in contact with low-level clouds and mixed into the marine boundary layer (MBL). In these simulations, the heating by the absorbing aerosol within the MBL affected the persistence of the Sc clouds by accelerating the SCT, especially during daylight and broken cloud conditions. However, the humidity accompanying the absorbing aerosol was also found to be important -- it reduced the deepening of the MBL when located above the Sc deck and delayed the SCT when in contact with clouds. Furthermore, the additional moisture resulted in a radiative cooling effect that was comparable to the radiative cooling effect caused by the aerosol itself. The simulated SCTs were found to be mostly driven by increased sea surface temperatures, regardless of aerosol conditions. This result was different compared to two other LES models where the SCT was driven by drizzle under the same low aerosol conditions. On a larger scale, it was found that an explicit description of aerosol-cloud interactions in a climate model led to smaller differences between the simulated and mean observed values of the shortwave cloud radiative effect compared to when a non-interactive parameterization was used.
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| 2. |
- Baró Pérez, Alejandro, et al.
(författare)
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Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
- 2024
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Ingår i: Atmospheric Chemistry And Physics. - 1680-7316 .- 1680-7324. ; 24:8, s. 4591-4610
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Tidskriftsartikel (refereegranskat)abstract
- Biomass burning plumes are frequently transported over the southeast Atlantic (SEA) stratocumulus deck during the southern African fire season (June-October). The plumes bring large amounts of absorbing aerosols and enhanced moisture, which can trigger a rich set of aerosol-cloud-radiation interactions with climatic consequences that are still poorly understood. We use large-eddy simulation (LES) to explore and disentangle the individual impacts of aerosols and moisture on the underlying stratocumulus clouds, the marine boundary layer (MBL) evolution, and the stratocumulus-to-cumulus transition (SCT) for three different meteorological situations over the southeast Atlantic during August 2017. For all three cases, our LES shows that the SCT is driven by increased sea surface temperatures and cloud-top entrainment as the air is advected towards the Equator. In the LES model, aerosol indirect effects, including impacts on drizzle production, have a small influence on the modeled cloud evolution and SCT, even when aerosol concentrations are lowered to background concentrations. In contrast, local semi-direct effects, i.e., aerosol absorption of solar radiation in the MBL, cause a reduction in cloud cover that can lead to a speed-up of the SCT, in particular during the daytime and during broken cloud conditions, especially in highly polluted situations. The largest impact on the radiative budget comes from aerosol impacts on cloud albedo: the plume with absorbing aerosols produces a total average 3 d of simulations. We find that the moisture accompanying the aerosol plume produces an additional cooling effect that is about as large as the total aerosol radiative effect. Overall, there is still a large uncertainty associated with the radiative and cloud evolution effects of biomass burning aerosols. A comparison between different models in a common framework, combined with constraints from in situ observations, could help to reduce the uncertainty.
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| 3. |
- Baró Pérez, Alejandro, et al.
(författare)
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Impact of smoke and non-smoke aerosols on radiation and low-level clouds over the southeast Atlantic from co-located satellite observations
- 2021
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 21:8, s. 6053-6077
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Tidskriftsartikel (refereegranskat)abstract
- Data derived from instruments on board the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and CloudSat satellites as well as meteorological parameters from reanalysis are used to explore situations when moist aerosol layers overlie stratocumulus clouds over the southeast Atlantic during the biomass burning season (June to October). To separate and quantify the impacts of aerosol loading, aerosol type, and humidity on the radiative fluxes (including cloud top cooling), the data are split into different levels of aerosol and moisture loadings. The aerosol classification available from the CALIPSO products is used to compare and contrast situations with pristine air, with smoke, and with other (non-smoke) types of aerosols. A substantial number of cases with non-smoke aerosols above clouds are found to occur under similar meteorological conditions to the smoke cases. In contrast, the meteorology is substantially different for the pristine situations, making a direct comparison with the aerosol cases ambiguous. The moisture content is enhanced within the aerosol layers, but the relative humidity does not always increase monotonously with increasing optical depth. Shortwave (SW) heating rates within the moist aerosol plumes increase with increasing aerosol loading and are higher in the smoke cases compared to the non-smoke cases. However, there is no clear correlation between moisture changes and SW absorption. Cloud top cooling rates do not show a clear correlation with moisture within the overlying aerosol layers due to the strong variability of the cooling rates caused by other meteorological factors (most notably cloud top temperature). No clear influence of aerosol type or loading on cloud top cooling rates is detected. Further, there is no correlation between aerosol loading and the thermodynamic structure of the atmosphere nor the cloud top height.
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| 4. |
- Böö, Sebastian, 1979-, et al.
(författare)
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Transport of Mineral Dust Into the Arctic in Two Reanalysis Datasets of Atmospheric Composition
- 2023
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Ingår i: Tellus. Series B, Chemical and physical meteorology. - 0280-6509 .- 1600-0889. ; 75:1, s. 13-32
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Tidskriftsartikel (refereegranskat)abstract
- Two three-dimensional reanalysis datasets of atmospheric composition, the Copernicus Atmosphere Monitoring Service reanalysis (CAMSRA) and the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), are analyzed for the years 2003-2018 with respect to dust transport into the Arctic. The reanalyses agree on that the largest mass transport of dust into the Arctic occurs across western Russia during spring and early summer, but substantial transport events occasionally also occur across other geographical areas during all seasons. In many aspects, however, the reanalyses show considerable differences: the mass transport in MERRA-2 is substantially larger, more spread out, and occurs at higher altitudes than in CAMSRA, while the transport in CAMSRA is to a higher degree focused to well-defined events in space and time; the integrated mass transport of the 10 most intense 36-hour dust events in CAMSRA constitutes 6 % of the total integrated dust transport 2003-2018, whereas the corresponding value for MERRA-2 is only 1 %.Furthermore, we compare the reanalyses with surface measurements of dust in the Arctic and dust extinction retrievals from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite data. This comparison indicates that CAMSRA underestimates the dust transport into the Arctic and that MERRA-2 likely overestimates it. The discrepancy between CAMSRA and MERRA-2 can partially be explained by the assimilation process where too little dust is assimilated in CAMSRA while in MERRA-2, the assimilation process increases the dust concentration in remote areas. Despite the profound differences between the reanalyses regarding dust transport into the Arctic, this study still brings new insights into the spatio-temporal distribution of the transport. We estimate the annual dust transport into the Arctic to be within the range 1.5-31 Tg, where the comparison with observations indicates that the lower end of the interval is less likely.
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| 5. |
- Johansson, Erik, et al.
(författare)
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Vertical structure of cloud radiative heating in the tropics : confronting the EC-Earth v3.3.1/3P model with satellite observations
- 2021
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Ingår i: Geoscientific Model Development. - : Copernicus GmbH. - 1991-959X .- 1991-9603. ; 14:6, s. 4087-4101
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Tidskriftsartikel (refereegranskat)abstract
- Understanding the coupling of clouds to large-scale circulation is one of the grand challenges for the global climate research community. In this context, realistically modelling the vertical structure of cloud radiative heating (CRH) and/or cooling in Earth system models is a key premise to understand this coupling. Here, we evaluate CRH in two versions of the European Community Earth System Model (EC-Earth) using retrievals derived from the combined radar and lidar data from the CloudSat and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellites. One model version is also used with two different horizontal resolutions. Our study evaluates large-scale intraseasonal variability in the vertical structure of CRH and cloud properties and investigates the changes in CRH during different phases of the El Niño–Southern Oscillation (ENSO), a process that dominates the interannual climate variability in the tropics.EC-Earth generally captures both the intraseasonal and meridional pattern of variability in CRH over the convectively active and stratocumulus regions and the CRH during the positive and negative phases of ENSO. However, two key differences between model simulations and satellite retrievals emerge. First, the magnitude of CRH, in the upper troposphere, over the convectively active zones is up to twice as large in the models compared to the satellite data. Further dissection of net CRH into its shortwave and longwave components reveals noticeable differences in their vertical structure. The shortwave component of the radiative heating is overestimated by all model versions in the lowermost troposphere and underestimated in the middle troposphere. These over- and underestimates of shortwave heating are partly compensated by an overestimate of longwave cooling in the lowermost troposphere and heating in the middle troposphere. The biases in CRH can be traced back to disagreement in cloud amount and cloud water content. There is no noticeable improvement of CRH by increasing the horizontal resolution in the model alone. Our findings highlight the importance of evaluating models with satellite observations that resolve the vertical structure of clouds and cloud properties.
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| 6. |
- Norin, Lars, et al.
(författare)
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Anomalous Propagation and the Sinking of the Russian Warship Moskva
- 2023
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Ingår i: Bulletin of The American Meteorological Society - (BAMS). - : American Meteorological Society. - 0003-0007 .- 1520-0477. ; 104:12, s. E2286-E2304
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Tidskriftsartikel (refereegranskat)abstract
- On 13 April 2022, the Russian warship Moskva was hit by two Ukrainian Neptune anti-ship missiles in the Black Sea, leading to its demise. Before launching an anti-ship missile, a target must first be detected and positioned, for example, by an accompanying radar system. However, when the missiles hit the Moskva she was well beyond the normal radar horizon of any ground-based radar system, making the ship undetectable under normal circumstances. Using meteorological reanalysis data, we show that at the time of the missile launch the prevailing weather conditions allowed a ground-based radar to detect targets far beyond the normal radar horizon through anomalous propagation conditions. During such conditions, the atmospheric index of refraction decreases rapidly with height, making electromagnetic radiation bend downward to, partly or fully, compensate the curvature of the Earth. The results show that atmospheric conditions must be considered carefully, even during warfare, as their impact on radar wave propagation can be considerable.
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| 7. |
- Thomas, Manu Anna, et al.
(författare)
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Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions
- 2022
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Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 22:1, s. 119-137
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Tidskriftsartikel (refereegranskat)abstract
- Given the vast expanse of oceans on our planet, marine aerosols (and sea salt in particular) play an important role in the climate system via multitude of direct and indirect effects. The efficacy of their net impact, however, depends strongly on the local meteorological conditions that influence their physical, optical and chemical properties. Understanding the coupling between aerosol properties and meteorological conditions is therefore important. It has been historically difficult to statistically quantify this coupling over larger oceanic areas due to the lack of suitable observations, leading to large uncertainties in the representation of aerosol processes in climate models. Perhaps no other region shows higher uncertainties in the representation of marine aerosols and their effects than the Southern Ocean. During winter the Southern Ocean boundary layer is dominated by sea salt emissions. Here, using 10 years of austral winter period (June, July and August, 2007-2016) space-based aerosol profiling by CALIOP-CALIPSO in combination with meteorological reanalysis data, we investigated the sensitivity of marine aerosol properties over the Southern Ocean (40-65 degrees S) to various meteorological parameters, such as vertical relative humidity (RH), surface wind speed and sea surface temperature (SST) in terms of joint histograms. The sensitivity study is done for the climatological conditions and for the enhanced cyclonic and anticyclonic conditions in order to understand the impact of large-scale atmospheric circulation on the aerosol properties. We find a clear demarcation in the 532 nm aerosol backscatter and extinction at RH around 60 %, irrespective of the state of the atmosphere. The backscatter and extinction increase at higher relative humidity as a function of surface wind speed. This is mainly because of the water uptake by the wind-driven sea salt aerosols at high RH near the ocean surface resulting in an increase in size, which is confirmed by the decreased depolarization for the wet aerosols. An increase in aerosol backscatter and extinction is observed during the anticyclonic conditions compared to cyclonic conditions for the higher wind speeds and relative humidity, mainly due to aerosols being confined to the boundary layer, and their proximity to the ocean surface facilitates the growth of the particles. We further find a very weak dependency of aerosol backscatter on SSTs at lower wind speeds. However, when the winds are stronger than about 12 m s(-1), the backscattering coefficient generally increases with SST. When aerosol properties are investigated in terms of aerosol verticality and in relation to meteorological parameters, it is seen that the aerosol backscatter values in the free troposphere (pressure <850 hPa) are much lower than in the boundary layer, irrespective of the RH and the three weather states. This indicates that the local emissions from the ocean surface make the dominant contribution to aerosol loads over the Southern Ocean. A clear separation of particulate depolarization is observed in the free and lower troposphere, more prominent in the climatological mean and the cyclonic states. For RH > 60 %, low depolarization values are noticeable in the lower troposphere, which is an indication of the dominance of water-coated and mostly spherical sea salt particles. For RH < 60 %, there are instances when the aerosol depolarization increases in the boundary layer; this is more prominent in the mean and anticyclonic cases, which can be associated with the presence of drier aerosol particles. Based on the joint histograms investigated here, we provide third-degree polynomials to obtain aerosol extinction and backscatter as a function of wind speed and relative humidity. Additionally, backscattering coefficient is also expressed jointly in terms of wind speed and sea surface temperature. Furthermore, depolarization is expressed as a function of relative humidity. These fitting functions would be useful to test and improve the parameterizations of sea salt aerosols in the climate models. We also note some limitations of our study. For example, interpreting the verticality of aerosol properties (especially depolarization) in relation to the meteorological conditions in the free and upper troposphere (pressure <850 hPa) was challenging. Furthermore, we do not see any direct evidence of sudden crystallization (efflorescence), deliquescence or hysteresis effects of the aerosols. Observing such effects will likely require a targeted investigation of individual cases considering tracer transport, rather than the statistical sensitivity study that entails temporally and geographically averaged large data sets.
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| 8. |
- You, Cheng, 1990-
(författare)
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Arctic Atmospheric Rivers : Eulerian and Lagrangian features, and trends over the last 40 years
- 2021
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Arctic Atmospheric rivers, termed ‘warm-and-moist intrusion’ (WaMAI) in this thesis, transporting heat and moisture into the Arctic from lower latitudes, is a key contributor to the amplified warming in the Arctic under global change (Arctic Amplification). However, the warming effect of WaMAIs and its transformation along the trajectories into high Arctic still remain unclear, as well as their relation with the large-scale atmospheric circulation.A positive trend of poleward moisture and heat transport during 1979-2018 has been identified over the Barents Sea in winter and East Siberian Sea in summer. These positive trends are attributed to an increased blocking occurrence, as quantified by a blocking track algorithm. Given the increase in poleward energy transport and its impacts on the atmospheric energy budgets, it is necessary to focus on the Arctic atmospheric rivers in more detail. Therefore, a method is developed to detect WaMAIs during December~Febrary, June~August from 1979 to 2018, and to identify the Lagrangian transformation of warm-and-moist air mass in temperature, humidity, cloud water path, surface and boundary-layer energy-budget, along the trajectories of WaMAIs. The analysis shows that WaMAIs, driven by blocking high-pressure systems over the respective ocean sectors, induce an air mass transformation in the atmospheric boundary layer, resulting in surface warming and presumably additional sea ice melt, from positive anomalies of surface net longwave irradiance and turbulent flux. In summer, from a Lagrangian perspective, the surface energy-budget anomaly decreases linearly with the downstream distance from the sea-ice edge, while total column cloud liquid water (TCLW) increases linearly. An initially stably stratified boundary layer at the ice edge transforms into a deepening well-mixed boundary layer along the trajectories, from the continuous turbulent mixing. The boundary-layer energy-budget structures are categorized into two categories: one dominated by surface turbulent mixing (TBL) and one dominated by cloud-top radiative cooling (RAD). The magnitude of the large-scale atmospheric vertical motion, the subsidence, is critical in determining if the boundary layer develops into TBL or RAD.In winter, over the completely ice-covered ocean sectors where the sea ice reaches all the way to the coast, the Lagrangian transformation of the boundary-layer energy-budget is similar to summer WaMAIs, while the surface energy-budget is dominated by longwave irradiance. On the other hand, over the Barents Sea, with an open ocean to the south, the net surface energy budget is dominated by the surface turbulent fluxes. The boundary-layer energy-budget over the Barents Sea can also be categorized into RAD and TBL, but are different from their summer counterparts.
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| 9. |
- You, Cheng, et al.
(författare)
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Eulerian and Lagrangian views of warm and moist air intrusions into summer Arctic
- 2021
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Ingår i: Atmospheric research. - : Elsevier BV. - 0169-8095 .- 1873-2895. ; 256
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Tidskriftsartikel (refereegranskat)abstract
- In this study, warm and moist air intrusions (WaMAI) over the sea sectors of Kara, Laptev, East Siberian and Beaufort from 1979 to 2018 are identified in ERA5 reanalysis and their air-mass transformation is analysed using interpolation in ERA5 and satellite products along trajectories. The analysis shows that WaMAIs, driven by blocking high-pressure systems over the respective ocean sectors, induce surface warming (11–18 W m−2) and sea ice melt from positive anomalies of net longwave radiation (5–8 W m−2) and turbulent flux (8–13 W m−2) to the surface, although the anomaly of net shortwave radiation (−9 ~ +1 W m−2) is negative. From a Lagrangian perspective, the surface energy-budget anomaly decreases linearly, while total column cloud liquid water (TCLW) increases linearly with the downstream distance from the sea-ice edge. However, the cloud radiative effects of both longwave and shortwave radiation reach an equilibrium as TCLW increases in a much lower rate beyond 7 degrees north of the sea ice edge. The boundary-layer energy-budget pattern can be categorized into two classes: radiation-dominated and turbulence-dominated, comprised of 26% and 62% WaMAIs respectively. Statistically, turbulence-dominated cases occur with 3 times stronger large-scale subsidence, and also feature a larger anomaly in net shortwave radiation. In radiation-dominated WaMAIs, stratocumulus develops more strongly and hence exerts larger longwave and shortwave forcing to the surface. In both categories, a well-mixed boundary layer deepens by 500 m along the trajectories, from the continuous turbulent mixing.
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| 10. |
- You, Cheng, et al.
(författare)
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On Warm and Moist Air Intrusions into Winter Arctic
- 2024
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Annan publikation (övrigt vetenskapligt/konstnärligt)abstract
- In this study, warm and moist air intrusions (WaMAI) over the Arctic Ocean sectors of Barents, Kara, Laptev, East Siberian, Chukchi and Beaufort Seas in recent 40 winters (from 1979 to 2018) are identified from ERA5 reanalysis using both Eulerian and Lagrangian views. The analysis shows that WaMAIs, fuelled by Arctic blockings, causes a relative surface warming and hence a sea ice reduction by exerting positive anomalies of net thermal irradiances and turbulent fluxes to the surface. Over Arctic Ocean sectors with land-locked sea ice in winter, such as Laptev, East Siberian, Chukchi and Beaufort Seas, total surface energy budget is dominated by net thermal irradiance. From a Lagrangian perspective, total water path (TWP) increases linearly with the downstream distance from the sea ice edge over the completely ice-covered sectors, inducing almost linearly increasing net thermal irradiance and total surface energy-budget. However, over the Barents Sea, with an open ocean to the south, total net surface energy-budget is dominated by the surface turbulent flux. With the energy in the warm-and-moist air continuously transported to the surface, net surface turbulent flux gradually decreases with distance, especially within the first 2 degrees north of the ice edge, inducing a decreasing but still positive total surface energy budget. The boundary-layer energy-budget patterns over the Barents Sea can be categorized into three classes: radiation-dominated, turbulence-dominated and turbulence-dominated with cold dome, comprising about 52 %, 40 % and 8 % of all WaMAIs, respectively. Statistically, turbulence-dominated cases with or without cold dome occur along with one order of magnitude larger large-scale subsidence than the radiation-dominated cases. For the turbulence-dominated category, larger turbulent fluxes are exerted to the surface, probably because of stronger wind shear. In radiation-dominated WaMAIs, stratocumulus develops more strongly and triggers intensive cloud-top radiative cooling and related buoyant mixing that extends from cloud top to the surface, inducing a thicker well-mixed layer under the cloud. With the existence of cold dome, fewer liquid water clouds were formed and less or even negative turbulent fluxes could reach the surface.
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