| 1. |
- Fredricsson, Malin, et al.
(författare)
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Nationell luftövervakning Sakrapport med data från övervakning inom Programområde Luft t.o.m 2019
- 2021
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Rapport (övrigt vetenskapligt/konstnärligt)abstract
- Naturvårdsverket ansvarar för den nationella luftövervakningen i bakgrundsmiljö i Sverige. I rapporten redovisas resultat från verksamheten inom Programområde Luft avseende mätningar (genomförda av IVL, SU, SLU och SMHI) till och med 2019 och regionala modellberäkningar (utförda av SMHI) till och med 2018.För flertalet av de luftföroreningskomponenter som övervakas inom den nationella miljöövervakningen har det, sedan mätningarna startade för mellan 20 och 40 år sedan, generellt sett skett en avsevärd förbättring avseende såväl halter i luft som deposition i bakgrundsmiljö. Utvecklingen har dock varierat i något olika utsträckning beroende på komponenter och lokalisering i landet. Föroreningsbelastningen är oftast lägre ju längre norrut i landet man kommer.För de flesta ämnen som det finns miljökvalitetsnormer (MKN) respektive miljömål för ligger halterna i regional bakgrund avsevärt lägre än angivna gräns- och målvärden. Halterna av ozon överskrider dock i dagsläget (2019) MKN för hälsa.
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| 2. |
- Klemetz, Viktor, et al.
(författare)
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Nationell luftövervakning : Sakrapport med data från övervakning inom Programområde Luft t. o. m. 2021
- 2023
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Rapport (övrigt vetenskapligt/konstnärligt)abstract
- Naturvårdsverket ansvarar för den nationella luftövervakningen i bakgrundsmiljö. I rapporten redovisas resultat från verksamheten inom Programområde Luft avseende mätningar (genomförda av IVL Svenska Miljöinstitutet (IVL),Institutionen för Miljövetenskap vid Stockholms universitet (SU), Institutionen för Mark och Miljö vid Sveriges lantbruksuniversitet (SLU), Chalmers tekniska högskola och Sveriges meteorologiska och hydrologiska institut (SMHI) till och med 2021 samt regionala modellberäkningar (utförda av SMHI) till och med 2020. För flertalet av de luftföroreningskomponenter som övervakas inom den nationella miljöövervakningen har det, sedan mätningarna startade för mellan 20 och 45 år sedan, generellt skett en avsevärd förbättring avseende såväl halter i luft som deposition i bakgrundsmiljö.Utvecklingen har dock varierat i något olika utsträckning beroende på komponenter och lokalisering i landet. Föroreningsbelastningen är oftast lägre ju längre norrut i landet man kommer.För de flesta ämnen som det finns miljökvalitetsnormer (MKN) respektive miljömål för ligger halterna avsevärt lägre än angivna gräns- och målvärden. Halterna av marknära ozon överskrider i dagsläget MKN för hälsa vid ett flertal mätstationer i södra Sverige.För såväl partiklar (i form av PM2,5) och bensen (i urban bakgrund) är risken låg att haltnivåer överstiger miljömålens preciseringar.
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| 3. |
- Andersson, Camilla, et al.
(författare)
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Achievements and experiences from science–policy interaction in the field of air pollution : Synthesising 20 years of research and outreach,thinking about future needs
- 2021
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Rapport (övrigt vetenskapligt/konstnärligt)abstract
- For 20 years, the Swedish Environmental Protection Agency together with the MISTRA research foundation have funded five air pollution research programmes with focus on producing knowledge that supports policy and emission control in national and international arenas. The research has been multidisciplinary and has included research on emissions, atmospheric transport and transformation processes, human health effects, ecosystem effects, and emission control strategies. Research has also been conducted on the interaction between air pollution and climate change.Over these years, the link between the research programmes and the development of emission control strategies and policies in Sweden, the EU, and the UNECE Air Convention has been of high importance. This report presents how the research programmes have created societal benefits through support for the development of air pollution policies and emission control measures. The report also identifies future research needs to ensure continued progress towards even better air quality for future generations.
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| 4. |
- Artaxo, Paulo, et al.
(författare)
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Tropical and Boreal Forest – Atmosphere Interactions : A Review
- 2022
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Ingår i: Tellus. Series B, Chemical and physical meteorology. - : Stockholm University Press. - 0280-6509 .- 1600-0889. ; 74:1, s. 24-163
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Forskningsöversikt (refereegranskat)abstract
- This review presents how the boreal and the tropical forests affect the atmosphere, its chemical composition, its function, and further how that affects the climate and, in return, the ecosystems through feedback processes. Observations from key tower sites standing out due to their long-term comprehensive observations: The Amazon Tall Tower Observatory in Central Amazonia, the Zotino Tall Tower Observatory in Siberia, and the Station to Measure Ecosystem-Atmosphere Relations at Hyytiäla in Finland. The review is complemented by short-term observations from networks and large experiments.The review discusses atmospheric chemistry observations, aerosol formation and processing, physiochemical aerosol, and cloud condensation nuclei properties and finds surprising similarities and important differences in the two ecosystems. The aerosol concentrations and chemistry are similar, particularly concerning the main chemical components, both dominated by an organic fraction, while the boreal ecosystem has generally higher concentrations of inorganics, due to higher influence of long-range transported air pollution. The emissions of biogenic volatile organic compounds are dominated by isoprene and monoterpene in the tropical and boreal regions, respectively, being the main precursors of the organic aerosol fraction.Observations and modeling studies show that climate change and deforestation affect the ecosystems such that the carbon and hydrological cycles in Amazonia are changing to carbon neutrality and affect precipitation downwind. In Africa, the tropical forests are so far maintaining their carbon sink.It is urgent to better understand the interaction between these major ecosystems, the atmosphere, and climate, which calls for more observation sites, providing long-term data on water, carbon, and other biogeochemical cycles. This is essential in finding a sustainable balance between forest preservation and reforestation versus a potential increase in food production and biofuels, which are critical in maintaining ecosystem services and global climate stability. Reducing global warming and deforestation is vital for tropical forests.
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| 5. |
- Boyer, Matthew, et al.
(författare)
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A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation : insights from the Multidisciplinarydrifting Observatory for the Study of Arctic Climate (MOSAiC) expedition
- 2023
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 23:1, s. 389-415
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Tidskriftsartikel (refereegranskat)abstract
- The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an important role in the radiative balance and hence the climate response in the region, yet direct observations of aerosols over the Arctic Ocean are limited. In this study, we investigate the annual cycle in the aerosol particle number size distribution (PNSD), particle number concentration (PNC), and black carbon (BC) mass concentration in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. This is the first continuous, year-long data set of aerosol PNSD ever collected over the sea ice in the central Arctic Ocean. We use a k-means cluster analysis, FLEXPART simulations, and inverse modeling to evaluate seasonal patterns and the influence of different source regions on the Arctic aerosol population. Furthermore, we compare the aerosol observations to land-based sites across the Arctic, using both long-term measurements and observations during the year of the MOSAiC expedition (2019–2020), to investigate interannual variability and to give context to the aerosol characteristics from within the central Arctic. Our analysis identifies that, overall, the central Arctic exhibits typical seasonal patterns of aerosols, including anthropogenic influence from Arctic haze in winter and secondary aerosol processes in summer. The seasonal pattern corresponds to the global radiation, surface air temperature, and timing of sea ice melting/freezing, which drive changes in transport patterns and secondary aerosol processes. In winter, the Norilsk region in Russia/Siberia was the dominant source of Arctic haze signals in the PNSD and BC observations, which contributed to higher accumulation-mode PNC and BC mass concentrations in the central Arctic than at land-based observatories. We also show that the wintertime Arctic Oscillation (AO) phenomenon, which was reported to achieve a record-breaking positive phase during January–March 2020, explains the unusual timing and magnitude of Arctic haze across the Arctic region compared to longer-term observations. In summer, the aerosol PNCs of the nucleation and Aitken modes are enhanced; however, concentrations were notably lower in the central Arctic over the ice pack than at land-based sites further south. The analysis presented herein provides a current snapshot of Arctic aerosol processes in an environment that is characterized by rapid changes, which will be crucial for improving climate model predictions, understanding linkages between different environmental processes, and investigating the impacts of climate change in future Arctic aerosol studies.
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| 6. |
- Hansson, Hans-Christen, et al.
(författare)
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The Atmospheric Aerosol over Western Greece-Six Years of Aerosol Observations at the Navarino Environmental Observatory
- 2021
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Ingår i: Atmosphere. - : MDPI AG. - 2073-4433 .- 2073-4433. ; 12:4
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Tidskriftsartikel (refereegranskat)abstract
- The Eastern Mediterranean is a highly populated area with air quality problems. It is also where climate change is already noticed by higher temperatures and s changing precipitation pattern. The anthropogenic aerosol affects health and changing concentrations and properties of the atmospheric aerosol affect radiation balance and clouds. Continuous long-term observations are essential in assessing the influence of anthropogenic aerosols on climate and health. We present six years of observations from Navarino Environmental Observatory (NEO), a new station located at the south west tip of Peloponnese, Greece. The two sites at NEO, were evaluated to show the influence of the local meteorology and to assess the general background aerosol possible. It was found that the background aerosol was originated from aged European aerosols and was strongly influenced by biomass burning, fossil fuel combustion, and industry. When subsiding into the boundary layer, local sources contributed in the air masses moving south. Mesoscale meteorology determined the diurnal variation of aerosol properties such as mass and number by means of typical sea breeze circulation, giving rise to pronounced morning and evening peaks in pollutant levels. While synoptic scale meteorology, mainly large-scale air mass transport and precipitation, strongly influenced the seasonality of the aerosol properties.
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| 7. |
- Heslin-Rees, Dominic, et al.
(författare)
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From a polar to a marine environment : has the changing Arctic led to a shift in aerosol light scattering properties?
- 2020
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 20:21, s. 13671-13686
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Tidskriftsartikel (refereegranskat)abstract
- The study of long-term trends in aerosol optical properties is an important task to understand the underlying aerosol processes influencing the change of climate. The Arctic, as the place where climate change manifests most, is an especially sensitive region of the world. Within this work, we use a unique long-term data record of key aerosol optical properties from the Zeppelin Observatory, Svalbard, to ask the question of whether the environmental changes of the last 2 decades in the Arctic are reflected in the observations. We perform a trend analysis of the measured particle light scattering and backscattering coefficients and the derived scattering Angstrom exponent and hemispheric backscattering fraction. In contrast to previous studies, the effect of in-cloud scavenging and of potential sampling losses at the site are taken explicitly into account in the trend analysis. The analysis is combined with a back trajectory analysis and satellite-derived sea ice data to support the interpretation of the observed trends. We find that the optical properties of aerosol particles have undergone clear and significant changes in the past 2 decades. The scattering Angstrom exponent exhibits statistically significant decreasing of between -4.9 % yr(-1) and -6.5 % yr(-1) (using wavelengths of lambda = 450 and 550 nm), while the particle light scattering coefficient exhibits statistically significant increasing trends of between 2.6 % yr(-1) and 2.9 % yr(-1) (at a wavelength of lambda = 550 nm). The magnitudes of the trends vary depending on the season. These trends indicate a shift to an aerosol dominated more by coarse-mode particles, most likely the result of increases in the relative amount of sea spray aerosol. We show that changes in air mass circulation patterns, specifically an increase in air masses from the south-west, are responsible for the shift in aerosol optical properties, while the decrease of Arctic sea ice in the last 2 decades only had a marginal influence on the observed trends.
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| 8. |
- Krishnan, Srinath, et al.
(författare)
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The Roles of the Atmosphere and Ocean in Driving Arctic Warming Due to European Aerosol Reductions
- 2020
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Ingår i: Geophysical Research Letters. - 0094-8276 .- 1944-8007. ; 47:7
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Tidskriftsartikel (refereegranskat)abstract
- Clean air policies can have significant impacts on climate in remote regions. Previous modeling studies have shown that the temperature response to European sulfate aerosol reductions is largest in the Arctic. Here we investigate the atmospheric and ocean roles in driving this enhanced Arctic warming using a set of fully coupled and slab‐ocean simulations (specified ocean heat convergence fluxes) with the Norwegian Earth system model (NorESM), under scenarios with high and low European aerosol emissions relative to year 2000. We show that atmospheric processes drive most of the Arctic response. The ocean pathway plays a secondary role inducing small temperature changes mostly in the opposite direction of the atmospheric response. Important modulators of the temperature response patterns are changes in sea ice extent and subsequent turbulent heat flux exchange, suggesting that a proper representation of Arctic sea ice and turbulent changes is key to predicting the Arctic response to midlatitude aerosol forcing.
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| 9. |
- Platt, Stephen M., et al.
(författare)
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Atmospheric composition in the European Arctic and 30 years of the Zeppelin Observatory, Ny-Ålesund
- 2022
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 22:5, s. 3321-3369
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Tidskriftsartikel (refereegranskat)abstract
- The Zeppelin Observatory (78.90∘ N, 11.88∘ E) is located on Zeppelin Mountain at 472 m a.s.l. on Spitsbergen, the largest island of the Svalbard archipelago. Established in 1989, the observatory is part of Ny-Ålesund Research Station and an important atmospheric measurement site, one of only a few in the high Arctic, and a part of several European and global monitoring programmes and research infrastructures, notably the European Monitoring and Evaluation Programme (EMEP); the Arctic Monitoring and Assessment Programme (AMAP); the Global Atmosphere Watch (GAW); the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS); the Advanced Global Atmospheric Gases Experiment (AGAGE) network; and the Integrated Carbon Observation System (ICOS). The observatory is jointly operated by the Norwegian Polar Institute (NPI), Stockholm University, and the Norwegian Institute for Air Research (NILU). Here we detail the establishment of the Zeppelin Observatory including historical measurements of atmospheric composition in the European Arctic leading to its construction. We present a history of the measurements at the observatory and review the current state of the European Arctic atmosphere, including results from trends in greenhouse gases, chlorofluorocarbons (CFCs) and hydrochlorofluorocarbons (HCFCs), other traces gases, persistent organic pollutants (POPs) and heavy metals, aerosols and Arctic haze, and atmospheric transport phenomena, and provide an outline of future research directions.
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| 10. |
- Sand, Maria, et al.
(författare)
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Surface temperature response to regional black carbon emissions : do location and magnitude matter?
- 2020
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 20:5, s. 3079-3089
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Tidskriftsartikel (refereegranskat)abstract
- Aerosol radiative forcing can influence climate both locally and far outside the emission region. Here we investigate black carbon (BC) aerosols emitted in four major emission areas and evaluate the importance of emission location and magnitude as well as the concept of the absolute regional temperature-change potentials (ARTP). We perform simulations with a climate model (NorESM) with a fully coupled ocean and with fixed sea surface temperatures. BC emissions for year 2000 are increased by factors of 10 and 20 in South Asia, North America, and Europe, respectively, and by 5 and 10 in East Asia (due to higher emissions there). The perturbed simulations and a reference simulation are run for 100 years with three ensemble members each. We find strikingly similar regional surface temperature responses and geographical patterns per unit BC emission in Europe and North America but somewhat lower temperature sensitivities for East Asian emissions. BC emitted in South Asia shows a different geographical pattern in surface temperatures, by changing the Indian monsoon and cooling the surface. We find that the ARTP approach rather accurately reproduces the fully coupled temperature response of NorESM. Choosing the highest emission rate results in lower surface temperature change per emission unit compared to the lowest rate, but the difference is generally not statistically significant except for the Arctic. An advantage of high-perturbation simulations is the clearer emergence of regional signals. Our results show that the linearity of normalized temperature effects of BC is fairly well preserved despite the relatively large perturbations but that regional temperature coefficients calculated from high perturbations may be a conservative estimate. Regardless of emission region, BC causes a northward shift of the ITCZ, and this shift is apparent both with a fully coupled ocean and with fixed sea surface temperatures. For these regional BC emission perturbations, we find that the effective radiative forcing is not a good measure of the climate response. A limitation of this study is the uncertainties in BC-cloud interactions and the amount of BC absorption, both of which are model dependent.
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