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- Gorgoi, M, et al.
(författare)
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The high kinetic energy photoelectron spectroscopy facility at BESSY progress and first results
- 2009
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Ingår i: Nuclear Instruments and Methods in Physics Research Section A. - : Elsevier BV. - 0168-9002 .- 1872-9576. ; 601:1-2, s. 48-53
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Tidskriftsartikel (refereegranskat)abstract
- Photoelectron spectroscopy at high kinetic energy is a research field that receives an increasing interest due to the possibility of studying bulk properties of materials and deeply buried interfaces. Recently the high kinetic energy electron (HIKE) spectroscopy facility at BESSY in Berlin has become operative at the bending magnet beamline KMC-1. The first results show very good performance. Electron spectra have been recorded using X-ray energies from 2 keV up to 12 keV. Using back-scattering conditions in the crystal monochromator, very high-resolution has been achieved for photon energies around 2, 6 and 8 keV. In the latter case, spectra with a resolving power from the monochromator of >= 80 000 have been achieved and it has been possible to perform electron spectroscopy with resolving power of >= 60 000, yielding a total instrument resolution of about 150 meV as determined directly from spectra. This paper describes the facility and reports some of the first results. (C) 2009 Elsevier B.V. All rights reserved.
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| 3. |
- Karis, O., et al.
(författare)
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High-kinetic-energy photoemission spectroscopy of Ni at 1s: 6-eV satellite at 4 eV
- 2008
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Ingår i: Physical Review B (Condensed Matter and Materials Physics). - 1098-0121 .- 1550-235X. ; 78:23, s. 3-3
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Tidskriftsartikel (refereegranskat)abstract
- Electron correlations are responsible for many profound phenomena in solid-state physics. A classical example is the 6-eV satellite in the photoelectron spectrum of Ni. Until now the satellite structure has only been investigated at the L shell and more shallow levels. Here we report a high-kinetic-energy photoemission spectroscopy (HIKE) investigation of Ni metal. We present 1s and 2p photoelectron spectra, obtained using excitation energies up to 12.6 keV. Our investigation demonstrates that the energy position of the satellite relative to the main line is different for the 1s and the 2p levels. In combination with electronic structure calculations, we show that this energy shift is attributed to unique differences in the core-valence coupling for the K and L-2,L-3 shells in 3d transition metals, resulting in different screening of the core holes.
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