| 1. |
- Ahrentorp, Fredrik, et al.
(författare)
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Sensitive magnetic biodetection using magnetic multi-core nanoparticles and RCA coils
- 2017
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Ingår i: Journal of Magnetism and Magnetic Materials. - : Elsevier BV. - 0304-8853 .- 1873-4766. ; 427, s. 14-18
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Tidskriftsartikel (refereegranskat)abstract
- We use functionalized iron oxide magnetic multi-core particles of 100 nm in size (hydrodynamic particle diameter) and AC susceptometry (ACS) methods to measure the binding reactions between the magnetic nanoparticles (MNPs) and bio-analyte products produced from DNA segments using the rolling circle amplification (RCA) method. We use sensitive induction detection techniques in order to measure the ACS response. The DNA is amplified via RCA to generate RCA coils with a specific size that is dependent on the amplification time. After about 75 min of amplification we obtain an average RCA coil diameter of about 1 mu m. We determine a theoretical limit of detection (LOD) in the range of 11 attomole (corresponding to an analyte concentration of 55 fM for a sample volume of 200 mu L) from the ACS dynamic response after the MNPs have bound to the RCA coils and the measured ACS readout noise. We also discuss further possible improvements of the LOD.
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| 2. |
- Andersson, Eric, 1992, et al.
(författare)
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Nondestructive cleaning of the LaAlO3/SrTiO3 surface with ultraviolet light and ozone
- 2016
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Ingår i: Journal of Vacuum Science and Technology B: Nanotechnology and Microelectronics. - : American Vacuum Society. - 2166-2746 .- 2166-2754. ; 34:4
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Tidskriftsartikel (refereegranskat)abstract
- The effect of ultraviolet light produced ozone and irradiation (UV/ozone) cleaning on the surface properties and interface electrical properties of 4 unit cell (uc) LaAlO3/SrTiO3 samples is examined. A standard photolithography process is used to contaminate the samples which are then cleaned in UV/ozone. Atomic force microscopy measurements show that the photoresist contaminated samples can be cleaned efficiently using this method. The surface roughness of the cleaned samples is comparable to that of the as-grown samples. Furthermore, electrical transport measurements show that the mobility decreases and the sheet carrier density increases for the contaminated samples, which also display indications of an onset to the Kondo effect. By removing the contaminants with UV/ozone cleaning, the mobility and sheet carrier density can be partially restored toward the as-grown values. The mobility is increased by about two times from approximate to 1000 cm(2) V-1 s(-1) for the contaminated samples to approximate to 2000 cm(2) V-1 s(-1) for the ozone cleaned ones. (C) 2016 American Vacuum Society.
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| 3. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Untwinned YBa2Cu3O7-delta thin films on MgO substrates: A platform to study strain effects on the local orders in cuprates
- 2019
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Ingår i: Physical Review Materials. - 2475-9953. ; 3:11
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Tidskriftsartikel (refereegranskat)abstract
- We have grown untwinned YBa2Cu3O7-delta (YBCO) films on (110) MgO substrates that were preannealed at high temperature in oxygen atmosphere. The annealing results in surface reconstruction with shallow facets, which induce the suppression of the YBCO twinning domains, and the preferential alignment of the CuO chains along one of the in-plane directions of the substrate. Because of the large mismatch between the in-plane lattice parameters of film and substrate, the strain induced by the MgO into the YBCO layer is strong and very peculiar. The YBCO film is compressed, with respect to the bulk, and presents a unidirectional buckling of the atomic planes, along the chains' direction, due to a deformation of the copper-oxygen octahedra. The YBCO films, which can be grown with thicknesses down to few unit cells and oxygen doping levels spanning most of the superconducting dome, are patterned into nanowires with dimensions down to 50 nm. The anisotropies due to the untwinning state are preserved in these structures; moreover, additional anisotropies appear in ultrathin structures where strain effects become more pronounced. Such untwinned and compressively strained films can therefore be used as a platform to study the interplay between strain and the various local orders in the normal state of YBCO.
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| 4. |
- Aurino, Pier Paolo, 1985, et al.
(författare)
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Retention of Electronic Conductivity in LaAlO3/SrTiO3 Nanostructures Using a SrCuO2 Capping Layer
- 2016
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Ingår i: Physical Review Applied. - : American Physical Society. - 2331-7019. ; 6:2
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Tidskriftsartikel (refereegranskat)abstract
- The interface between two wide band-gap insulators, LaAlO3 and SrTiO3 (LAO/STO) offers a unique playground to study the interplay and competitions between different ordering phenomena in a strongly correlated two- dimensional electron gas. Recent studies of the LAO/STO interface reveal the inhomogeneous nature of the 2DEG that strongly influences electrical-transport properties. Nanowires needed in future applications may be adversely affected, and our aim is, thus, to produce a more homogeneous electron gas. In this work, we demonstrate that nanostructures fabricated in the quasi-2DEG at the LaAlO3/SrTiO3 interface, capped with a SrCuO2 layer, retain their electrical resistivity and mobility independent of the structure size, ranging from 100 nm to 30 mu m. This is in contrast to noncapped LAO/STO structures, where the room-temperature electrical resistivity significantly increases when the structure size becomes smaller than 1 mu m. High-resolution intermodulation electrostatic force microscopy reveals an inhomogeneous surface potential with "puddles" of a characteristic size of 130 nm in the noncapped samples and a more uniform surface potential with a larger characteristic size of the puddles in the capped samples. In addition, capped structures show superconductivity below 200 mK and nonlinear currentvoltage characteristics with a clear critical current observed up to 700 mK. Our findings shed light on the complicated nature of the 2DEG at the LAO/STO interface and may also be used for the design of electronic devices.
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| 5. |
- Aurino, Pier Paolo, 1985, et al.
(författare)
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Reversible metal-insulator transition of Ar-irradiated LaAlO3/SrTiO3 interfaces
- 2015
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Ingår i: Physical Review B - Condensed Matter and Materials Physics. - 2469-9950 .- 2469-9969. ; 92:15
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Tidskriftsartikel (refereegranskat)abstract
- The conducting state of a quasi-two-dimensional electron gas (q2DEG), formed at the heterointerface between the two wide-bandgap insulators LaAlO3 (LAO) and SrTiO3, can be made completely insulating by low-energy, 150-eV, Ar+ irradiation. The metallic behavior of the interface can be recovered by high-temperature oxygen annealing. The electrical transport properties of the recovered q2DEG are exactly the same as before the irradiation. Microstructural investigations confirm that the transition is not due to physical etching or crystal lattice distortion of the LAO film below its critical thickness. They also reveal a correlation between electrical state, LAO film surface amorphization, and argon ion implantation. The experimental results are in agreement with density functional theory calculations of Ar implantation and migration in the LAO film. This suggests that the metal-insulator transition may be caused by charge trapping in the defect amorphous layer created during the ion irradiation.
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| 6. |
- Blomgren, Jakob, et al.
(författare)
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Development of a sensitive induction-based magnetic nanoparticle biodetection method
- 2018
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Ingår i: Nanomaterials. - : MDPI AG. - 2079-4991. ; 8:11
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Tidskriftsartikel (refereegranskat)abstract
- We developed a novel biodetection method for influenza virus based on AC magnetic susceptibility measurement techniques (the DynoMag induction technique) together with functionalized multi-core magnetic nanoparticles. The sample consisting of an incubated mixture of magnetic nanoparticles and rolling circle amplified DNA coils is injected into a tube by a peristaltic pump. The sample is moved as a plug to the two well-balanced detection coils and the dynamic magnetic moment in each position is read over a range of excitation frequencies. The time for making a complete frequency sweep over the relaxation peak is about 5 minutes (10 Hz–10 kHz with 20 data points). The obtained standard deviation of the magnetic signal at the relaxation frequency (around 100 Hz) is equal to about 10−5 (volume susceptibility SI units), which is in the same range obtained with the DynoMag system. The limit of detection with this method is found to be in the range of 1 pM.
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| 7. |
- Calvani, P., et al.
(författare)
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Infrared spectroscopy of two-dimensional electron systems
- 2019
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Ingår i: European Physical Journal: Special Topics. - : Springer Science and Business Media LLC. - 1951-6401 .- 1951-6355. ; 228:3, s. 669-673
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Tidskriftsartikel (refereegranskat)abstract
- © 2019, EDP Sciences, Springer-Verlag GmbH Germany, part of Springer Nature. We have used grazing-angle infrared spectroscopy with polarized radiation to detect the Berreman effect (BE) in the two-dimensional electron systems (2DES) which form spontaneously at two interfaces: one between an amorphous film LaAlO3 and its SrTiO3 substrate (LAO/STO), and another at the interface between the topological insulator (TI) Bi2Se3 and its sapphire substrate. In both systems we have thus extracted the 2DES parameters at different temperatures. In the quasi-2DES under amorphous LAO, the surface density ns is higher than under crystalline LAO, while the mobility is nearly the same and the thickness d is 7 nm. In ultrapure Bi2Se3 on sapphire, preliminary data provided d
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| 8. |
- Charpentier, Sophie, 1983, et al.
(författare)
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Induced unconventional superconductivity on the surface states of Bi2Te3 topological insulator
- 2017
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Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723 .- 2041-1723. ; 8:1
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Tidskriftsartikel (refereegranskat)abstract
- Topological superconductivity is central to a variety of novel phenomena involving the interplay between topologically ordered phases and broken-symmetry states. The key ingredient is an unconventional order parameter, with an orbital component containing a chiral p(x) + ip(y) wave term. Here we present phase-sensitive measurements, based on the quantum interference in nanoscale Josephson junctions, realized by using Bi2Te3 topological insulator. We demonstrate that the induced superconductivity is unconventional and consistent with a sign-changing order parameter, such as a chiral px + ipy component. The magnetic field pattern of the junctions shows a dip at zero externally applied magnetic field, which is an incontrovertible signature of the simultaneous existence of 0 and pi coupling within the junction, inherent to a non trivial order parameter phase. The nano-textured morphology of the Bi2Te3 flakes, and the dramatic role played by thermal strain are the surprising key factors for the display of an unconventional induced order parameter.
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| 9. |
- Coll, M., et al.
(författare)
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Towards Oxide Electronics: a Roadmap
- 2019
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Ingår i: Applied Surface Science. - : Elsevier BV. - 0169-4332 .- 1873-5584. ; 482, s. 1-93
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Tidskriftsartikel (refereegranskat)abstract
- At the end of a rush lasting over half a century, in which CMOS technology has been experiencing a constant and breathtaking increase of device speed and density, Moore’s law is approaching the insurmountable barrier given by the ultimate atomic nature of matter. A major challenge for 21st century scientists is finding novel strategies, concepts and materials for replacing silicon-based CMOS semiconductor technologies and guaranteeing a continued and steady technological progress in next decades. Among the materials classes candidate to contribute to this momentous challenge, oxide films and heterostructures are a particularly appealing hunting ground. The vastity, intended in pure chemical terms, of this class of compounds, the complexity of their correlated behaviour, and the wealth of functional properties they display, has already made these systems the subject of choice, worldwide, of a strongly networked, dynamic and interdisciplinary research community. Oxide science and technology has been the target of a wide four-year project, named Towards Oxide-Based Electronics (TO-BE), that has been recently running in Europe and has involved as participants several hundred scientists from 29 EU countries. In this review and perspective paper, published as a final deliverable of the TO-BE Action, the opportunities of oxides as future electronic materials for Information and Communication Technologies ICT and Energy are discussed. The paper is organized as a set of contributions, all selected and ordered as individual building blocks of a wider general scheme. After a brief preface by the editors and an introductory contribution, two sections follow. The first is mainly devoted to providing a perspective on the latest theoretical and experimental methods that are employed to investigate oxides and to produce oxide-based films, heterostructures and devices. In the second, all contributions are dedicated to different specific fields of applications of oxide thin films and heterostructures, in sectors as data storage and computing, optics and plasmonics, magnonics, energy conversion and harvesting, and power electronics.
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| 10. |
- Constantinian, K. Y., et al.
(författare)
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Spin-Triplet Superconducting Current in Metal-Oxide Heterostructures With Composite Ferromagnetic Interlayer
- 2016
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Ingår i: IEEE Transactions on Applied Superconductivity. - : Institute of Electrical and Electronics Engineers (IEEE). - 1558-2515 .- 1051-8223. ; 26:3
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Tidskriftsartikel (refereegranskat)abstract
- Superconducting heterostructures fabricated from oxide superconductor YBa2Cu2O7-delta and a composite ferromagnet La0.7Sr0.3MnO3/SrRuO3 interlayer and Au/Nb counter electrode were studied experimentally. Superconducting current was observed at magnetic field H raised up to 2000 Oe, which is greater than saturation magnetic field of manganite La0.7Sr0.3MnO3 (of order 100 Oe) and greater by a few orders than the value of magnetic field corresponding to penetration of one magnetic flux quantum. Microwave measurements of integer and half-integer Shapiro steps in conditions when relatively low external magnetic fieldH < 30 Oe was applied showed that the second harmonic in the current-phase relation of superconducting current becomes as big as the first harmonic. Fourier analysis of I-C(H) dependence allows extracting the components of fractional periods in I-C(H) function that also confirms a deviation from the sinusoidal current-phase relation. The obtained experimental data are explained by theoretical models that predict a huge enhancement of the second harmonic of the spin-triplet component in the superconducting current. The current-phase relation could be controlled by an external magnetic field, changing the directions of magnetization in the composite bilayer ferromagnet, which is inserted between two spin-singlet superconductors.
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