| 1. |
- Lehr, C., et al.
(författare)
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Unveiling the two-proton halo character of 17 Ne: Exclusive measurement of quasi-free proton-knockout reactions
- 2022
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Ingår i: Physics Letters, Section B: Nuclear, Elementary Particle and High-Energy Physics. - : Elsevier BV. - 0370-2693 .- 1873-2445. ; 827
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Tidskriftsartikel (refereegranskat)abstract
- The proton drip-line nucleus 17Ne is investigated experimentally in order to determine its two-proton halo character. A fully exclusive measurement of the 17Ne(p,2p)16F→15⁎O+p quasi-free one-proton knockout reaction has been performed at GSI at around 500 MeV/nucleon beam energy. All particles resulting from the scattering process have been detected. The relevant reconstructed quantities are the angles of the two protons scattered in quasi-elastic kinematics, the decay of 16F into 15O (including γ decays from excited states) and a proton, as well as the 15O+p relative-energy spectrum and the 16F momentum distributions. The latter two quantities allow an independent and consistent determination of the fractions of l=0 and l=2 motion of the valence protons in 17Ne. With a resulting relatively small l=0 component of only around 35(3)%, it is concluded that 17Ne exhibits a rather modest halo character only. The quantitative agreement of the two values deduced from the energy spectrum and the momentum distributions supports the theoretical treatment of the calculation of momentum distributions after quasi-free knockout reactions at high energies by taking into account distortions based on the Glauber theory. Moreover, the experimental data allow the separation of valence-proton knockout and knockout from the 15O core. The latter process contributes with 11.8(3.1) mb around 40% to the total proton-knockout cross section of 30.3(2.3) mb, which explains previously reported contradicting conclusions derived from inclusive cross sections.
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| 2. |
- Wamers, F., et al.
(författare)
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Diverse mechanisms in proton knockout reactions from the Borromean nucleus Ne-17
- 2023
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Ingår i: European Physical Journal A. - : Springer. - 1434-6001 .- 1434-601X. ; 59
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Tidskriftsartikel (refereegranskat)abstract
- Nucleon knockout experiments using beryllium or carbon targets reveal a strong dependence of the quenching factors, i.e., the ratio (Rs) of theoretical to the experimental spectroscopic factors (C2S), on the proton-neutron asymmetry in the nucleus under study. However, this dependence is greatly reduced when a hydrogen target is used. To understand this phenomenon, exclusive H-1(Ne-17, 2p F-16) and inclusive C-12(Ne-17, 2p 1(6)F)X, 1(2)C(Ne-17, F-16)X as well as 1H(Ne-17,(16) F)X(X-denotes undetected reaction products) reactions with F-16 in the ground and excited states were anal- ysed. The longitudinal momentum distribution of F-16 and the correlations between the detached protons were studied. In the case of the carbon target, there is a significant deviation from the predictions of the eikonal model. The eikonal approximation was used to extract spectroscopic factor values (CS)-S-2. The experimental (CS)-S-2 value obtained with C target is markedly lower than that for H target. This is interpreted as rescattering due to simultaneous nucleon knockout from both reaction partners, Ne-17 and C-12.
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| 3. |
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| 4. |
- Al-Adili, Ali, et al.
(författare)
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Isomer yields in nuclear fission
- 2021
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Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 2100-014X. ; 256
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Tidskriftsartikel (refereegranskat)abstract
- The generation of angular momentum in the fission process is still an open question. To shed light on this topic, we started a series of measurements at the IGISOL-JYFLTRAP facility in Finland. Highprecision measurements of isomeric yield ratios (IYR) are performed with a Penning trap, partly with the aim to extract average root-mean-square (rms) quantities of fragment spin distributions. The newly installed Phase-Imaging Ion-Cyclotron Resonance (PI-ICR) technique allows the separation of masses down to tens of keV, which is suffcient to disentangle many isomers. In this paper, we first summarize the previous measurements on the neutron and proton-induced fission of uranium and thorium, e.g. the odd cadmium and indium isotopes (119 ≤ A ≤ 127). The measurements revealed systematic trends as function of mass number, which stimulated further exploration. A recent measurement was performed at IGISIOL and several new IYR data will soon be published, for the first time. Secondly, we employ the TALYS nuclear-reaction code to model one of the newly measured isomer yields. Detailed GEF and TALYS calculations are discussed for the fragment angular momentum distribution in 134I.
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| 5. |
- Gao, Zhihao, et al.
(författare)
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Applying machine learning methods for the analysis of two-dimensional mass spectra
- 2023
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Ingår i: European Physical Journal A. - : Springer Nature. - 1434-6001 .- 1434-601X. ; 59:169
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Tidskriftsartikel (refereegranskat)abstract
- In a measurement of isomeric yield-ratios in fission, the Phase-Imaging Ion-Cyclotron-Resonance technique, which projects the radial motions of ions in the Penning trap (JYFLTRAP) onto a position-sensitive micro-channel plate detector, has been applied. To obtain the yield ratio, that is the relative population of two states of an isomer pair, a novel analysis procedure has been developed to determine the number of detected ions in each state, as well as corrections for the detector efficiency and decay losses. In order to determine the population of the states in cases where their mass difference is too small to reach full separation, a Bayesian Gaussian Mixture model was implemented. The position-dependent efficiency of the micro-channel plate detector was calibrated by mapping it with 133Cs+ ions, and a Gaussian Process was trained with the position data to construct an efficiency function that could be used to correct the recorded distributions. The obtained numbers of counts of excited and ground-state ions were used to derive the isomeric yield ratio, taking into account decay losses as well as feeding from precursors.
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| 6. |
- Gao, Zhihao, et al.
(författare)
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Benchmark of a multi-physics Monte Carlo simulation of an ionguide for neutron-induced fission products
- 2022
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Ingår i: European Physical Journal. - : Springer Nature. - 1286-0042 .- 1286-0050. ; 58:2
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Tidskriftsartikel (refereegranskat)abstract
- To enhance the production of medium-heavy,neutron-rich nuclei, and to facilitate measurements of independentyields of neutron-induced fission, a proton-toneutronconverter and a dedicated ion guide for neutroninducedfission have been developed for the IGISOL facilityat the University of Jyväskylä. The ion guide holds thefissionable targets, and the fission products emerging fromthe targets are collected in helium gas and transported to thedownstream experimental stations.Acomputer model, basedon a combination of MCNPX for modeling the neutron production,the fission code GEF, and GEANT4 for the transportof the fission products, was developed. The model willbe used to improve the setup with respect to the productionand collection of fission products. In this paper we benchmarkthe model by comparing simulations to a measurementin which fission products were implanted in foils located atdifferent positions in the ion guide. In addition, the productsfrom neutron activation in the titanium foil and the uraniumtargets are studied. The result suggests that the neutron fluxat the high-energy part of the neutron spectrum is overestimatedby approximately 40%.However, the transportation offission products in the uranium targets agrees with the experimentwithin 10%. Furthermore, the simulated transportationof fission products in the helium gas achieves almost perfectagreement with the measurement. Hence, we conclude thatthe model, after correction for the neutron flux, is well suitedfor optimization studies of future ion guide designs.
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| 7. |
- Gao, Zhihao, et al.
(författare)
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Estimating angular momenta of fission fragments from isomeric yield ratios using TALYS
- 2024
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Ingår i: Physical Review C. - : American Physical Society. - 2469-9985 .- 2469-9993. ; 109:6
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Tidskriftsartikel (refereegranskat)abstract
- Background: Angular momenta of fission fragments considerably higher than that of the fissioning nucleus have been observed in many experiments, raising the question of how these high angular momenta are generated. Wilson et al. have proposed a model for the angular momentum as a function of the mass of fission products based on the assumption that the angular momentum is generated from the collective motion of nucleons in the ruptured neck of the fissioning system. This assumption has caused a lot of debate in the community.Purpose: To estimate the angular momenta of fission fragments based on the observed isomeric yield ratios in 25 -MeV proton -induced fission of 238 U.Method: A surrogate model of the fission code general description of fission observables (GEF) has been developed to generate properties of primary fission fragments. Based on the excitation energy and angular momentum of fission fragments from GEF, an energy -versus -angular -momentum matrix is reconstructed using a set of parameters. With such matrices as input, the reaction code TALYS is used to calculate the deexcitation of the fission fragments, including the population of the isomers, from which the isomeric yield ratios are obtained. By varying one of the parameters, the root -mean -square angular momentum ( J rms ), which determines the angular momentum distribution of the matrix, J rms -dependent isomeric yield ratios are obtained. Considering all primary fission fragments contributing to the isomeric yield ratio for a given fission product, the average angular momentum of those fragments is estimated.Results: Data of 31 isomeric yield ratios in 25 -MeV proton -induced fission of 238 U were analyzed. From the analysis, the average J rms , equivalent to average angular momentum J av , with uncertainties are obtained for 24 fission products, while in seven cases no conclusive result for the angular momentum could be obtained. Furthermore, considering the neutron emissions of the primary fission fragments, the average angular momentum as a function of the average mass number of the primary fission fragment was estimated.Conclusion: A mass dependency of the average angular momentum is observed in the proton -induced fission of 238 U. Moreover, the average angular momenta for mass numbers larger than 131 could be fairly well described by the parametrization proposed by Wilson et al. However, the average angular momenta of 130 Sn and 131 Te cannot be described by Wilson's model, which suggests a different lower limit for the validation of the parametrization in the model. In general, higher average angular momenta for A 132 are observed in the present work compared to those from Wilson et al. This is likely due to the higher excitation energy of the fissioning nuclei in this work. Furthermore, the first systematic observation of the average angular momenta of fission products in the symmetric mass region is presented. In this region, a decreasing trend with mass number is observed, which cannot be explained by the proposal in Wilson's paper. Thus, a different mechanism is needed to explain this observation.
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| 8. |
- Gao, Zhihao, et al.
(författare)
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Fission studies at IGISOL/JYFLTRAP : Simulations of the ion guide for neutron-induced fission and comparison with experimental data
- 2020
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Ingår i: ND 2019. - : EDP Sciences. - 9782759891061
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Konferensbidrag (refereegranskat)abstract
- For the production of exotic nuclei at the IGISOL facility, an ion guide for neutron-induced fission has been developed and tested in experiments. Fission fragments are produced inside the ion guide and collected using a helium buffer gas. Meanwhile, a GEANT4 model has been developed to simulate the transportation and stopping of the charged fission products. In a recent measurement of neutron-induced fission yields, implantation foils were located at different positions in the ion guide. The gamma spectra from these foils and the fission targets are compared to the results from the GEANT4 simulation.In order to allow fission yield measurements in the low yield regions, towards the tails and in the symmetric part of the mass distribution, the stopping and extraction efficiency of the ion guide has to be significantly improved. This objective can be achieved by increasing the size while introducing electric field guidance using a combination of static electrodes and an RF-carpet. To this end, the GEANT4 model is used to optimise the design of such an ion guide.
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| 9. |
- Gao, Zhihao
(författare)
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Isomeric yield ratios in nuclear fission
- 2023
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Isomeric yield ratios (IYR), referring to the relative yield of the high spin states of a nucleus to the total yield of all observed states, is an observable of nuclear fission that has the potential to improve our understanding of the fission dynamics. Apart from that, systematic observations of IYRs can also contribute to other areas, such as the validation of fission models, modelling of the r-process in stellar nucleosynthesis, studies of the antineutrino mixing angle, the safety of present-day nuclear reactors, and the design of advanced reactor systems.With these motivations in mind, an IYR measurement in proton-induced fission was performed at the IGISOL facility in Jyväskylä, Finland. In the measurement, the Penning trap JYFLTRAP was used to separate the excited state from the ground state and to project those onto a position-sensitive MCP detector. The obtained phase images were used to train a Bayesian Gaussian Mixture model to identify the states. After considering corrections for the detector efficiency and radioactive decay, 19 IYRs were obtained.In this thesis, the measurement of IYRs with the IGISOL technique is described, and a systematic study of IYRs in proton-induced fission is presented. Furthermore, the measured ratios are compared with calculations using three different models: the Madland-England (ME) model, the fission model GEF, and the combination of GEF + TALYS. The experimental results show that, in general, the IYR decreases with the spins of measured states. While this, to some degree, confirms the ME model, variations in the IYR between nuclides with the same spin assignments reveal that the model is too simple to predict individual ratios. Furthermore,discrepancies in the IYRs between the measurement and GEF are observed in most cases, indicating a need to optimize the performance of GEF against nuclear data from proton-induced fission. The combination of GEF + TALYS results in an overall under estimation of the observedIYRs, which could be explained by the different assumptions used in GEF and TALYS.To investigate how the angular momenta of the primary fission fragments relate to the IYRs, a surrogate model of GEF has been developed. By reproducing the measured IYR with the calculated ratios from the model, the average angular momentum Jav, is deduced. The Jav for fission products with a mass number greater than 131 show a mass dependency which fits the parameterisation proposed by J. Wilson et al,. For IYRs in the mass region 119 ≤ A < 132, in which no measurements are presented by Wilson, a decrease in the Jav with increasing mass number is observed for the first time.Besides the study of IYRs, a benchmark of a multi-physics simulation model of the ion guide for neutron-induced fission products has been performed using γ-ray spectroscopy data. The results of the benchmark show that the high-energy part of the neutron flux from the simulation with MCNPX is overestimated by about 40 %, while the ion transportation simulated with GEANT4 agrees well with the experimental data. Based on the benchmark, the ion guide can be optimized to achieve high enough intensities of the collected ions to reach reasonable measurement times. In the next step, the addition of electric fields is considered to direct the ions in and to reduce the ion drifting time. However, this task lies outside the scope of this PhD thesis.
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| 10. |
- Gao, Zhihao, et al.
(författare)
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Isomeric yield ratios in proton-induced fission of 238U
- 2023
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Ingår i: Physical Review C. - : American Physical Society. - 2469-9985 .- 2469-9993. ; 108:5
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Tidskriftsartikel (refereegranskat)abstract
- Background: Isomeric yield ratios are an important observable in nuclear fission as they can guide model development by providing insight into the angular momentum generation. Furthermore, isomeric yield ratios are important in applications for nuclear energy, as well as in the study of the r-process in stellar nucleosynthesis, and in the antineutrino mixing angle from reactor spectra. In nuclear data evaluations, the Madland-England model is commonly used to estimate isomeric yield ratios that have not been measured.Purpose: To measure isomeric yield ratios in 25-MeV proton-induced fission of 238U, and to compare the result with the values obtained from the Madland-England model and the fission model code GEF. Furthermore, to evaluate whether the predictions of GEF can be improved by coupling it to the nuclear reaction code TALYS.Methods: Isomeric yield ratios in 25-MeV proton-induced fission of 238U have been measured at the Ion GuideIsotope Separate On-Line facility. The excited state and the ground state were separated by mass using the Phase-Imaging Ion-Cyclotron-Resonance technique in the double Penning trap JYFLTRAP. The number of counts of each state was extracted from the phase-images using a Bayesian Gaussian Mixture model and, after corrections fordetector efficiency and decay, the isomeric yield ratios were derived. The experimental values have been compared with the calculated results from the Madland-England model and the GEF code. Furthermore, GEF has been combined with the nuclear reaction code TALYS, in order to take advantage of the latter codes’ implementation of the Hauser-Feshbach formalism, and the results have been compared with the experimental values.Results: From the measurements, 19 new isomeric yield ratios in 25-MeV proton-induced fission of 238U are reported and are, together with another 12 isomeric yield ratios (IYRs) from a previous campaign, compared with the model calculations. It is shown that, though the models manage to capture some of the features observed, there is room for improvement.Conclusions: As predicted by the Madland-England model, a strong correlation between the measured IYRs and the spins of the long-lived states of the fission products is confirmed. However, the IYRs also vary between nuclides with the same spin-parity of the two states, and systematic trends in the IYRs of close-lying isotopes and isotones with similar nuclear configurations are observed.From the comparison of the experimental data with the prediction of GEF it is concluded that more data from proton-induced fission are needed to optimize the internal parameters of GEF. Furthermore, using a combination of GEF and TALYS in most cases results in an underestimation of the yield ratios. This might be explained by an underestimation of the angular momentum on the initial fission fragments by GEF. Altogether, these results highlight the possibility to use measurements of IYRs to improve model predictions and to study the angular momentum generation in nuclear fission.
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