| 1. |
- Lin, Xiaojing, et al.
(författare)
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Metal-enriched Neutral Gas Reservoir around a Strongly Lensed Low-mass Galaxy at z = 4 Identified by JWST/NIRISS and VLT/MUSE
- 2023
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Ingår i: Astrophysical Journal Letters. - : American Astronomical Society. - 2041-8213 .- 2041-8205. ; 944:2
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Tidskriftsartikel (refereegranskat)abstract
- Direct observations of low-mass, low-metallicity galaxies at z ≳ 4 provide an indispensable opportunity for detailed inspection of the ionization radiation, gas flow, and metal enrichment in sources similar to those that reionized the universe. Combining the James Webb Space Telescope (JWST), Very Large Telescope/MUSE, and Atacama Large Millimeter/submillimeter Array, we present detailed observations of a strongly lensed, low-mass (≈107.6 M ⊙) galaxy at z = 3.98 (also see Vanzella et al.). We identify strong narrow nebular emission, including C iv λ λ1548, 1550, He ii λ1640, O iii] λ λ1661, 1666, [Ne iii] λ3868, [O ii] λ3727, and the Balmer series of hydrogen from this galaxy, indicating a metal-poor H ii region (≲0.12 Z ⊙) powered by massive stars. Further, we detect a metal-enriched damped Lyα system (DLA) associated with the galaxy with the H i column density of N H I ≈ 1021.8 cm−2. The metallicity of the associated DLA may reach the supersolar metallicity (≳Z ⊙). Moreover, thanks to JWST and gravitational lensing, we present the resolved UV slope (β) map at the spatial resolution of ≈100 pc at z = 4, with steep UV slopes reaching β ≈ −2.5 around three star-forming clumps. Combining with low-redshift analogs, our observations suggest that low-mass, low-metallicity galaxies, which dominate reionization, could be surrounded by a high covering fraction of the metal-enriched, neutral-gaseous clouds. This implies that the metal enrichment of low-mass galaxies is highly efficient, and further supports that in low-mass galaxies, only a small fraction of ionizing radiation can escape through the interstellar or circumgalactic channels with low-column-density neutral gas.
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| 2. |
- Zhao, Kunsong, et al.
(författare)
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DeepInfer : Deep Type Inference from Smart Contract Bytecode
- 2023
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Ingår i: Proceedings Of The 31St Acm Joint Meeting European Software Engineering Conference And Symposium On The Foundations Of Software Engineering, Esec/Fse 2023. - : Association for Computing Machinery (ACM). ; , s. 745-757
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Konferensbidrag (refereegranskat)abstract
- Smart contracts play an increasingly important role in Ethereum platform. It provides various functions implementing numerous services, whose bytecode runs on Ethereum Virtual Machine. To use services by invoking corresponding functions, the callers need to know the function signatures. Moreover, such signatures provide crucial information for many downstream applications, e.g., identifying smart contracts, fuzzing, detecting vulnerabilities, etc. However, it is challenging to infer function signatures from the bytecode due to a lack of type information. Existing work solving this problem depended heavily on limited databases or hardcoded heuristic patterns. However, these approaches are hard to be adapted to semantic differences in distinct languages and various compiler versions when developing smart contracts. In this paper, we propose a novel framework DeepInfer that first leverages deep learning techniques to automatically infer function signatures and returns. The novelties of DeepInfer are: 1) DeepInfer lifts the byte-code into the Intermediate Representation (IR) to preserve code semantics; 2) DeepInfer extracts the type-related knowledge (e.g., critical data flows, constant values, and control flow graphs) from the IR to recover function signatures and returns. We conduct experiments on Solidity and Vyper smart contracts and the results show that DeepInfer performs faster and more accurate than existing tools, while being immune to changes in different languages and various compiler versions.
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| 3. |
- Zhou, Yueting, et al.
(författare)
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Self-calibrated NICE-OHMS based on an asymmetric signal : theoretical analysis and experimental validation
- 2023
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Ingår i: Optics Express. - : Optical Society of America. - 1094-4087. ; 31:17, s. 27830-27842
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Tidskriftsartikel (refereegranskat)abstract
- As an ultra-sensitive detection technique, the noise-immune cavity enhanced optical heterodyne molecular spectroscopy (NICE-OHMS) technique has great potential for assessment of the concentration of trace gases. To determine gas concentrations at the ppt or lower level with high accuracy, it is desirable that the technique exhibits self-calibration (or calibration-free) capabilities. Although being sensitive, NICE-OHMS has so far not demonstrated any such ability. To remedy this, this paper provides a self-calibrated realization of NICE-OHMS that is based on a switching of the feedback target of the DeVoe-Brewer (DVB) locking procedure from the modulation frequency of the frequency modulation spectroscopy (FMS) to the cavity length, which creates an asymmetrical signal whose form and size can be used to unambiguously assess the gas concentration. A comprehensive theoretical model for self-calibrated NICE-OHMS is established by analyzing the shift of cavity modes caused by intracavity absorption, demonstrating that gas absorption information can be encoded in both the laser frequency and the NICE-OHMS signal. To experimentally verify the methodology, we measure a series of dispersion signals under different levels of absorbance using a built experimental setup. An instrument factor and the partial pressure are obtained by fitting the measured signal through theoretical expressions. Our results demonstrate that fitted values are more accurate for higher partial pressures than for lower. To improve on the accuracy at low partial pressures, it is shown that the instrument factor obtained by fitting the signal at large partial pressures (in this case, above 7.8 µTorr) can be set to a fixed value for all fits. By this, the partial pressures can be assessed with a relative error below 0.65%. This technique has the potential to enable calibration-free ultra-sensitive gas detection.
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| 4. |
- Chen, Zhang, et al.
(författare)
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Making monolayer graphene photoluminescent by electron-beam-activated fluorination approach
- 2023
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Ingår i: Applied Surface Science. - : Elsevier. - 0169-4332 .- 1873-5584. ; 608
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Tidskriftsartikel (refereegranskat)abstract
- The past one and half decades have witnessed a tremendous development of graphene electronics, and the key to the success of graphene is its exceptional properties. The lacking of an inherent bandgap endows graphene with excellent electrical properties but considerably limits its applications in light-emitting and high-performance graphene-based devices. Herein, an approach for the direct writing of semiconducting and photoluminescent fluorinated graphene (C4F) patterns on monolayer graphene by an optimized electron-beam-activated fluorination technique is reported. A series of characterization approaches, such as atomic force microscopy, X-ray photoelectron spectroscopy and Raman spectroscopy were used to demonstrate the successful preparation of C4F for maskless lithography. Specially, a sharp and strong photoluminescence located at the purple light range of ∼380 nm was observed in C4F, demonstrating a desirable semiconducting nature, and the bandgap was further confirmed by follow-up electrical measurements, where the C4F filed-effect transistor exhibited a p-type semiconductor behavior and significantly enhanced on/off ratio. Therefore, this work provides a novel technique for the fabrication of graphene devices for promising electronic and optoelectronic applications, but also opens a route towards the tailoring and engineering of electronic properties of graphene.
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| 5. |
- Ge, Quanbo, et al.
(författare)
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A Novel Adaptive Kalman Filter Based on Credibility Measure
- 2023
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Ingår i: IEEE-CAA JOURNAL OF AUTOMATICA SINICA. - : Institute of Electrical and Electronics Engineers (IEEE). - 2329-9266. ; 10:1, s. 103-120
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Tidskriftsartikel (refereegranskat)abstract
- It is quite often that the theoretic model used in the Kalman filtering may not be sufficiently accurate for practical applications, due to the fact that the covariances of noises are not exactly known. Our previous work reveals that in such scenario the filter calculated mean square errors (FMSE) and the true mean square errors (TMSE) become inconsistent, while FMSE and TMSE are consistent in the Kalman filter with accurate models. This can lead to low credibility of state estimation regardless of using Kalman filters or adaptive Kalman filters. Obviously, it is important to study the inconsistency issue since it is vital to understand the quantitative influence induced by the inaccurate models. Aiming at this, the concept of credibility is adopted to discuss the inconsistency problem in this paper. In order to formulate the degree of the credibility, a trust factor is constructed based on the FMSE and the TMSE. However, the trust factor can not be directly computed since the TMSE cannot be found for practical applications. Based on the definition of trust factor, the estimation of the trust factor is successfully modifled to online estimation of the TMSE. More importantly, a necessary and sufficient condition is found, which turns out to be the basis for better design of Kalman filters with high performance. Accordingly, beyond trust factor estimation with Sage-Husa technique (TFE-SHT), three novel trust factor estimation methods, which are directly numerical solving method (TFE-DNS), the particle swarm optimization method (PSO) and expectation max-imization-particle swarm optimization method (EM-PSO) are proposed. The analysis and simulation results both show that the proposed TFE-DNS is better than the TFE-SHT for the case of single unknown noise covariance. Meanwhile, the proposed EM-PSO performs completely better than the EM and PSO on the estimation of the credibility degree and state when both noise covariances should be estimated online.
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| 6. |
- Li, Jian, et al.
(författare)
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A 3D extra-large-pore zeolite enabled by 1D-to-3D topotactic condensation of a chain silicate
- 2023
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Ingår i: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 379:6629, s. 283-287
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Tidskriftsartikel (refereegranskat)abstract
- Zeolites are microporous silicates with a large variety of applications as catalysts, adsorbents, and cation exchangers. Stable silica-based zeolites with increased porosity are in demand to allow adsorption and processing of large molecules but challenge our synthetic ability. We report a new, highly stable pure silica zeolite called ZEO-3, which has a multidimensional, interconnected system of extra-large pores open through windows made by 16 and 14 silicate tetrahedra, the least dense polymorph of silica known so far. This zeolite was formed by an unprecedented one-dimensional to three-dimensional (1D-to-3D) topotactic condensation of a chain silicate. With a specific surface area of more than 1000 square meters per gram, ZEO-3 showed a high performance for volatile organic compound abatement and recovery compared with other zeolites and metal-organic frameworks.
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| 7. |
- Wang, Hao, et al.
(författare)
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In-situ growth of low-dimensional perovskite-based insular nanocrystals for highly efficient light emitting diodes
- 2023
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Ingår i: Light. - : SPRINGERNATURE. - 2095-5545 .- 2047-7538. ; 12:1
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Tidskriftsartikel (refereegranskat)abstract
- Regulation of perovskite growth plays a critical role in the development of high-performance optoelectronic devices. However, judicious control of the grain growth for perovskite light emitting diodes is elusive due to its multiple requirements in terms of morphology, composition, and defect. Herein, we demonstrate a supramolecular dynamic coordination strategy to regulate perovskite crystallization. The combined use of crown ether and sodium trifluoroacetate can coordinate with A site and B site cations in ABX(3) perovskite, respectively. The formation of supramolecular structure retard perovskite nucleation, while the transformation of supramolecular intermediate structure enables the release of components for slow perovskite growth. This judicious control enables a segmented growth, inducing the growth of insular nanocrystal consist of low-dimensional structure. Light emitting diode based on this perovskite film eventually brings a peak external quantum efficiency up to 23.9%, ranking among the highest efficiency achieved. The homogeneous nano-island structure also enables high-efficiency large area (1 cm(2)) device up to 21.6%, and a record high value of 13.6% for highly semi-transparent ones.
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