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What is in the fish...
What is in the fish? Collaborative trial in suspect and non-target screening of organic micropollutants using LC- and GC-HRMS
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- Dürig, Wiebke (författare)
- Swedish University of Agricultural Sciences,Sveriges lantbruksuniversitet,Institutionen för vatten och miljö,Department of Aquatic Sciences and Assessment
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- Lindblad, Sofia (författare)
- Swedish University of Agricultural Sciences,Sveriges lantbruksuniversitet,Institutionen för vatten och miljö,Department of Aquatic Sciences and Assessment
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- Golovko, Oksana (författare)
- Swedish University of Agricultural Sciences,Sveriges lantbruksuniversitet,Institutionen för vatten och miljö,Department of Aquatic Sciences and Assessment
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- Gkotsis, Georgios (författare)
- Department of Chemistry, National and Kapodistrian University of Athens, Athens, Greece
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- Aalizadeh, Reza (författare)
- Department of Chemistry, National and Kapodistrian University of Athens, Athens, Greece
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- Nika, Maria-Christina (författare)
- Department of Chemistry, National and Kapodistrian University of Athens, Athens, Greece
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- Thomaidis, Nikolaos (författare)
- Department of Chemistry, National and Kapodistrian University of Athens, Athens, Greece
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- Alygizakis, Nikiforos A. (författare)
- Department of Chemistry, National and Kapodistrian University of Athens, Athens, Greece; Environmental Institute, Okružná 784/42, Koš, Slovakia
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- Plassmann, Merle, 1981- (författare)
- Stockholms universitet,Institutionen för miljövetenskap
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- Haglund, Peter (författare)
- Umeå universitet,Kemiska institutionen
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- Fu, Qiuguo (författare)
- Eawag: Swiss Federal Institute of Aquatic Science and Technology, Überlandstrasse 133, Dübendorf, Switzerland; Helmholtz Centre for Environmental Research - UFZ, Permoserstraße 15, Leipzig, Germany
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- Hollender, Juliane (författare)
- Eawag: Swiss Federal Institute of Aquatic Science and Technology, Überlandstrasse 133, Dübendorf, Switzerland; Institute of Biogeochemistry and Pollutant Dynamics, ETH Zürich, Universitätstrasse 16, Zürich, Switzerland
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- Chaker, Jade (författare)
- Université de Rennes, Inserm, EHESP, Irset - UMR_S, Rennes, France
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- David, Arthur (författare)
- Université de Rennes, Inserm, EHESP, Irset - UMR_S, Rennes, France
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- Kunkel, Uwe (författare)
- Bavarian Environment Agency, Bürgermeister-Ulrich-Straße 160, Augsburg, Germany
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- Macherius, André (författare)
- Bavarian Environment Agency, Bürgermeister-Ulrich-Straße 160, Augsburg, Germany
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- Belova, Lidia (författare)
- Toxicological Centre, University of Antwerp, Universiteitsplein 1, Wilrijk, Belgium
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- Poma, Giulia (författare)
- Toxicological Centre, University of Antwerp, Universiteitsplein 1, Wilrijk, Belgium
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- Preud'Homme, Hugues (författare)
- IPREM-UMR5254, E2S UPPA, CNRS, 2 avenue Angot, Pau cedex, France
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- Munschy, Catherine (författare)
- Ifremer, CCEM Contamination Chimique des Écosystèmes Marins, Nantes, France
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- Aminot, Yann (författare)
- Ifremer, CCEM Contamination Chimique des Écosystèmes Marins, Nantes, France
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- Jaeger, Carsten (författare)
- Bundesanstalt für Materialforschung und -prüfung (BAM), Analytical Chemistry, Richard-Willstätter-Straße 11, Berlin, Germany
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- Lisec, Jan (författare)
- Bundesanstalt für Materialforschung und -prüfung (BAM), Analytical Chemistry, Richard-Willstätter-Straße 11, Berlin, Germany
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- Hansen, Martin (författare)
- Department of Environmental Science, Aarhus University, Frederiksborgvej 399, Roskilde, Denmark
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- Vorkamp, Katrin (författare)
- Department of Environmental Science, Aarhus University, Frederiksborgvej 399, Roskilde, Denmark
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- Zhu, Linyan (författare)
- Department of Environmental Science, Aarhus University, Frederiksborgvej 399, Roskilde, Denmark
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- Cappelli, Francesca (författare)
- Water Research Institute, National Research Council of Italy, Via del Mulino 19, MB, Brugherio, Italy
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- Roscioli, Claudio (författare)
- Water Research Institute, National Research Council of Italy, Via del Mulino 19, MB, Brugherio, Italy
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- Valsecchi, Sara (författare)
- Water Research Institute, National Research Council of Italy, Via del Mulino 19, MB, Brugherio, Italy
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- Bagnati, Renzo (författare)
- Department of Environmental Health Sciences, Istituto di Ricerche Farmacologiche Mario Negri IRCCS, Via Mario Negri 2, Milan, Italy
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- González, Belén (författare)
- Department of Analytical Chemistry, Faculty of Science and Technology, University of the Basque Country (UPV/EHU), Barrio Sarriena s/n, Leioa, Spain; Research Centre for Experimental Marine Biology and Biotechnology (PIE), University of the Basque Country (UPV/EHU), Areatza Pasealekua 47, Plentzia, Spain
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- Prieto, Ailette (författare)
- Department of Analytical Chemistry, Faculty of Science and Technology, University of the Basque Country (UPV/EHU), Barrio Sarriena s/n, Leioa, Spain; Research Centre for Experimental Marine Biology and Biotechnology (PIE), University of the Basque Country (UPV/EHU), Areatza Pasealekua 47, Plentzia, Spain
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- Zuloaga, Olatz (författare)
- Department of Analytical Chemistry, Faculty of Science and Technology, University of the Basque Country (UPV/EHU), Barrio Sarriena s/n, Leioa, Spain; Research Centre for Experimental Marine Biology and Biotechnology (PIE), University of the Basque Country (UPV/EHU), Areatza Pasealekua 47, Plentzia, Spain
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- Gil-Solsona, Ruben (författare)
- Catalan Institute for Water Research (ICRA), Carrer Emili Grahit 101, Girona, Spain; Universitat de Girona, Girona, Spain; Institute of Environmental Assessment and Water Research – Severo Ochoa Excellence Center (IDAEA), Spanish Council of Scientific Research (CSIC), Barcelona 08034, Spain
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- Gago-Ferrero, Pablo (författare)
- Catalan Institute for Water Research (ICRA), Carrer Emili Grahit 101, Girona, Spain; Institute of Environmental Assessment and Water Research – Severo Ochoa Excellence Center (IDAEA), Spanish Council of Scientific Research (CSIC), Barcelona 08034, Spain
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- Rodriguez-Mozaz, Sara (författare)
- Catalan Institute for Water Research (ICRA), Carrer Emili Grahit 101, Girona, Spain; Universitat de Girona, Girona, Spain
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- Budzinski, Hélène (författare)
- University Bordeaux, CNRS, Bordeaux INP, EPOC, UMR 5805, Pessac, France
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- Devier, Marie-Helene (författare)
- University Bordeaux, CNRS, Bordeaux INP, EPOC, UMR 5805, Pessac, France
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- Dierkes, Georg (författare)
- Federal Institute of Hydrology, Am Mainzer Tor 1, Koblenz, Germany
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- Boulard, Lise (författare)
- Federal Institute of Hydrology, Am Mainzer Tor 1, Koblenz, Germany; Metabolomics Core Facility, Centre de Ressources et Recherches Technologiques (C2RT), Institut Pasteur, 25-28 Rue du Dr Roux, Paris, France
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- Jacobs, Griet (författare)
- Flemish Institute for Technological Research (VITO), Unit Separation and Conversion Technology, Boeretang 200, Mol, Belgium
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- Voorspoels, Stefan (författare)
- Flemish Institute for Technological Research (VITO), Unit Separation and Conversion Technology, Boeretang 200, Mol, Belgium
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- Rüdel, Heinz (författare)
- Fraunhofer Institute for Molecular Biology and Applied Ecology (Fraunhofer IME), Auf dem Aberg 1, Schmallenberg, Germany
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- Ahrens, Lutz (författare)
- Swedish University of Agricultural Sciences,Sveriges lantbruksuniversitet,Institutionen för vatten och miljö,Department of Aquatic Sciences and Assessment
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(creator_code:org_t)
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- Elsevier, 2023
- 2023
- Engelska.
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Ingår i: Environment International. - : Elsevier. - 0160-4120 .- 1873-6750. ; 181
- Relaterad länk:
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https://doi.org/10.1...
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https://umu.diva-por... (primary) (Raw object)
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https://pub.epsilon.... (primary) (Raw object) (free)
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https://urn.kb.se/re...
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https://doi.org/10.1...
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https://urn.kb.se/re...
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https://res.slu.se/i...
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Abstract
Ämnesord
Stäng
- A collaborative trial involving 16 participants from nine European countries was conducted within the NORMAN network in efforts to harmonise suspect and non-target screening of environmental contaminants in whole fish samples of bream (Abramis brama). Participants were provided with freeze-dried, homogenised fish samples from a contaminated and a reference site, extracts (spiked and non-spiked) and reference sample preparation protocols for liquid chromatography (LC) and gas chromatography (GC) coupled to high resolution mass spectrometry (HRMS). Participants extracted fish samples using their in-house sample preparation method and/or the protocol provided. Participants correctly identified 9–69 % of spiked compounds using LC-HRMS and 20–60 % of spiked compounds using GC-HRMS. From the contaminated site, suspect screening with participants’ own suspect lists led to putative identification of on average ∼145 and ∼20 unique features per participant using LC-HRMS and GC-HRMS, respectively, while non-target screening identified on average ∼42 and ∼56 unique features per participant using LC-HRMS and GC-HRMS, respectively. Within the same sub-group of sample preparation method, only a few features were identified by at least two participants in suspect screening (16 features using LC-HRMS, 0 features using GC-HRMS) and non-target screening (0 features using LC-HRMS, 2 features using GC-HRMS). The compounds identified had log octanol/water partition coefficient (KOW) values from −9.9 to 16 and mass-to-charge ratios (m/z) of 68 to 761 (LC-HRMS and GC-HRMS). A significant linear trend was found between log KOW and m/z for the GC-HRMS data. Overall, these findings indicate that differences in screening results are mainly due to the data analysis workflows used by different participants. Further work is needed to harmonise the results obtained when applying suspect and non-target screening approaches to environmental biota samples.
Ämnesord
- NATURVETENSKAP -- Kemi -- Analytisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Analytical Chemistry (hsv//eng)
- NATURVETENSKAP -- Geovetenskap och miljövetenskap -- Miljövetenskap (hsv//swe)
- NATURAL SCIENCES -- Earth and Related Environmental Sciences -- Environmental Sciences (hsv//eng)
Nyckelord
- Biota
- Collaborative trial
- Exposome
- GC-HRMS
- LC-HRMS
- Suspect and non-target analysis
Publikations- och innehållstyp
- ref (ämneskategori)
- art (ämneskategori)
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Till lärosätets databas
- Av författaren/redakt...
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Dürig, Wiebke
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Lindblad, Sofia
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Golovko, Oksana
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Gkotsis, Georgio ...
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Aalizadeh, Reza
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Nika, Maria-Chri ...
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visa fler...
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Thomaidis, Nikol ...
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Alygizakis, Niki ...
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Plassmann, Merle ...
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Haglund, Peter
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Fu, Qiuguo
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Hollender, Julia ...
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Chaker, Jade
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David, Arthur
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Kunkel, Uwe
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Macherius, André
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Belova, Lidia
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Poma, Giulia
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Preud'Homme, Hug ...
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Munschy, Catheri ...
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Aminot, Yann
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Jaeger, Carsten
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Lisec, Jan
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Hansen, Martin
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Vorkamp, Katrin
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Zhu, Linyan
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Cappelli, France ...
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Roscioli, Claudi ...
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Valsecchi, Sara
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Bagnati, Renzo
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González, Belén
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Prieto, Ailette
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Zuloaga, Olatz
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Gil-Solsona, Rub ...
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Gago-Ferrero, Pa ...
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Rodriguez-Mozaz, ...
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Budzinski, Hélèn ...
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Devier, Marie-He ...
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Dierkes, Georg
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Boulard, Lise
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Jacobs, Griet
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Voorspoels, Stef ...
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Rüdel, Heinz
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Ahrens, Lutz
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- Om ämnet
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- NATURVETENSKAP
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NATURVETENSKAP
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och Kemi
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och Analytisk kemi
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- NATURVETENSKAP
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NATURVETENSKAP
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och Geovetenskap och ...
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och Miljövetenskap
- Artiklar i publikationen
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Environment Inte ...
- Av lärosätet
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Umeå universitet
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Stockholms universitet
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Sveriges Lantbruksuniversitet