| 1. |
- Cuni-Sanchez, Aida, et al.
(författare)
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High aboveground carbon stock of African tropical montane forests
- 2021
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Ingår i: Nature. - : Springer Science and Business Media LLC. - 0028-0836 .- 1476-4687. ; 596:7873, s. 536-542
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Tidskriftsartikel (refereegranskat)abstract
- Tropical forests store 40–50per cent of terrestrial vegetation carbon. However, spatial variations in aboveground live tree biomass carbon (AGC) stocks remain poorly understood, in particular in tropical montane forests. Owing to climatic and soil changes with increasing elevation, AGC stocks are lower in tropical montane forests compared with lowland forests. Here we assemble and analyse a dataset of structurally intact old-growth forests (AfriMont) spanning 44 montane sites in 12 African countries. We find that montane sites in the AfriMont plot network have a mean AGC stock of 149.4megagrams of carbon per hectare (95% confidence interval 137.1–164.2), which is comparable to lowland forests in the African Tropical Rainforest Observation Network4 and about 70per cent and 32per cent higher than averages from plot networks in montane and lowland forests in the Neotropics, respectively. Notably, our results are two-thirds higher than the Intergovernmental Panel on Climate Change default values for these forests in Africa8. We find that the low stem density and high abundance of large trees of African lowland forests is mirrored in the montane forests sampled. This carbon store is endangered: we estimate that 0.8 million hectares of old-growth African montane forest have been lost since 2000. We provide country-specific montane forest AGC stock estimates modelled from our plot network to helpto guide forest conservation and reforestation interventions. Our findings highlight the need for conserving these biodiverse and carbon-rich ecosystems.
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| 2. |
- Jones, Geraint H., et al.
(författare)
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The Comet Interceptor Mission
- 2024
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Ingår i: Space Science Reviews. - : Springer Nature. - 0038-6308 .- 1572-9672. ; 220:1
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Tidskriftsartikel (refereegranskat)abstract
- Here we describe the novel, multi-point Comet Interceptor mission. It is dedicated to the exploration of a little-processed long-period comet, possibly entering the inner Solar System for the first time, or to encounter an interstellar object originating at another star. The objectives of the mission are to address the following questions: What are the surface composition, shape, morphology, and structure of the target object? What is the composition of the gas and dust in the coma, its connection to the nucleus, and the nature of its interaction with the solar wind? The mission was proposed to the European Space Agency in 2018, and formally adopted by the agency in June 2022, for launch in 2029 together with the Ariel mission. Comet Interceptor will take advantage of the opportunity presented by ESA’s F-Class call for fast, flexible, low-cost missions to which it was proposed. The call required a launch to a halo orbit around the Sun-Earth L2 point. The mission can take advantage of this placement to wait for the discovery of a suitable comet reachable with its minimum Δ V capability of 600 ms − 1 . Comet Interceptor will be unique in encountering and studying, at a nominal closest approach distance of 1000 km, a comet that represents a near-pristine sample of material from the formation of the Solar System. It will also add a capability that no previous cometary mission has had, which is to deploy two sub-probes – B1, provided by the Japanese space agency, JAXA, and B2 – that will follow different trajectories through the coma. While the main probe passes at a nominal 1000 km distance, probes B1 and B2 will follow different chords through the coma at distances of 850 km and 400 km, respectively. The result will be unique, simultaneous, spatially resolved information of the 3-dimensional properties of the target comet and its interaction with the space environment. We present the mission’s science background leading to these objectives, as well as an overview of the scientific instruments, mission design, and schedule.
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| 3. |
- Müller, Alexandra
(författare)
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An evaluation of sources contributing to urban runoff pollution
- 2022
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Urban runoff is a significant pathway for the transport of diverse substances from the urban environment to receiving water bodies. Many of these substances are pollutants of environmental concern with potentially harmful effects on aquatic life. Detailed knowledge of the sources of pollutants entering stormwater runoff is needed to mitigate these effects.The overall aim of this doctoral thesis is therefore to provide new knowledge on the sources contributing to urban runoff pollution and to evaluate the specific contributions of micropollutants from two known major sources: building and structure surface materials, and vehicular activities. The work presented herein also (i) identifies pollutants that are expected to occur in runoff from buildings and other structure surfaces in the urban environment as well as in runoff from the road environment, (ii) estimates the concentrations of these pollutants released into runoff, and (iii) evaluates methods for identifying sources contributing to the pollution of urban stormwater runoff.The novel work presented in the thesis includes a critical review of the literature on sources contributing to urban runoff pollution, laboratory leaching tests and open-air sampling of pilot panels of building and structure surface materials, and field sampling of urban roadside snow. The literature review was not restricted in terms of type of pollution, while the experiments focused on selected metals and organic micropollutants including phthalates, alkylphenols, bisphenol A, and polycyclic aromatic hydrocarbons (PAHs).According to the literature review, atmospheric deposition, vehicular activities, and metallic building envelopes are the major pollution sources in the urban environment and have been studied far more extensively than other sources. Moreover, their dominance is likely to continue given their central roles in urban environments. The experimental results confirmed that vehicular activities were sources of octylphenols, bisphenol A, and phthalates as well as the metal(loid)s Sb and W, both of which were rarely determined in previous studies on urban runoff. Building and structure surface materials such as copper sheets, zinc sheets, and polyvinyl chloride (PVC) roofing membranes were found to release Cu, Zn, nonylphenols, and phthalates. Among alkylphenols, nonylphenols were predominantly found in building surface runoff while octylphenols occurred predominantly in roadside snow. Metals occurred more commonly in dissolved (<0.45 μm) form in building surface runoff than in roadside snow, where metals were mainly attached to particles.A comparison of methods for identifying building surface materials contributing to runoff pollution showed that laboratory leaching tests were generally effective for source identification but not for estimating concentrations in actual runoff, whereas open-air pilot studies were resource-intensive but give results that agree well with analyses of real runoff. In addition, the release of pollutants from building surface materials subjected to in-situ ageing was investigated and the water quality of rainwater-induced runoff was compared to that of snowmelt-induced runoff; neither of these issues were adequately addressed in the previous literature. These studies showed that pollutant concentrations were generally higher in rain runoff than in snowmelt runoff and that pollutant releases from most materials and substances exhibited no decreasing or increasing trend over time. However, the release of nonylphenols from one of the PVCs did decrease over time, possibly because of washing out and material ageing.
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| 4. |
- Müller, Alexandra, et al.
(författare)
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Comparison of three explorative methods for identifying building surface materials contributing pollutants to stormwater
- 2021
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Ingår i: Journal of Environmental Management. - : Elsevier. - 0301-4797 .- 1095-8630. ; 299
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Tidskriftsartikel (refereegranskat)abstract
- Runoff from building and structure surfaces may contribute to the pollution of urban stormwater and, thereby, to the degradation of the receiving water quality. Various micropollutants have been found in surface runoff from buildings in the urban environment, including metals and organic micropollutants. Effective methods for identification of such pollutants and their sources are the prerequisites for the development of control measures. In this paper, three different methods for the identification of building surface materials acting as sources of metals (Cd, Cr, Cu, Ni, Pb and Zn), nonylphenols and phthalates are presented: (i) screening of the material composition, (ii) laboratory leaching experiments with synthetic rainwater, and (iii) open-air pilot testing of material panels exposed to actual rainfall and runoff. These three methods cover a wide span of experimental aspects, including, e.g., size of material samples, resource demands, and control of influential factors. Nine materials commonly used on building and structure surfaces in the urban environment were tested: metal sheets of zinc, copper, galvanised steel, coated corrugated steel and stainless steel; and, four different roofing membranes of bitumen as well as polyvinyl chloride (PVC). The experimental results indicated that all three methods were meritorious in providing some information contributing to the identification of pollutant sources. The screening of material composition for targeted pollutants is relatively quick and inexpensive, but may fail to identify minor sources of pollutants, or may identify the substances present in the material, but not released in contact with water. Laboratory leaching was generally effective in identifying sources of substances present in surface runoff, but was unsuitable for estimating the magnitude of actual concentrations in building runoff. Open-air pilot studies of material samples (exposed area = 2 m2) were thought to provide the results corresponding well to concentrations in runoff from actual building surfaces, but required relatively large financial and labour resources. Thus, the choice of the method for pollutant identification should be based on study objectives, and some benefits may be achieved using more than one method in an integrated manner; e.g., composition screening and lab or open-air leaching of targeted materials.
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| 5. |
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| 6. |
- Müller, Alexandra, et al.
(författare)
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Exploiting urban roadside snowbanks as passive samplers of organic micropollutants and metals generated by traffic
- 2022
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Ingår i: Environmental Pollution. - : Elsevier. - 0269-7491 .- 1873-6424. ; 308
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Tidskriftsartikel (refereegranskat)abstract
- Stormwater and snowmelt runoff is known to contribute to the deterioration of quality of urban surface waters. Vehicular traffic is recognised as a major source of a wide range of pollutants to urban runoff, including conventional pollutants, such as suspended solids and metals, and those referred to as ‘contaminants of emerging concern’. The aim of this study was to investigate the contribution of selected metal(loid)s (Cd, Cr, Cu, Ni, Pb, Pd, Sb, W, Zn), polycyclic aromatic hydrocarbons (PAHs), nonylphenols, octylphenols and –ethoxylates, phthalates and bisphenol A (BPA) from vehicular traffic by sampling urban roadside snow at eight sites, with varying traffic intensities, and one control site without direct impacts of traffic. Our results confirmed that vehicles and traffic-related activities were the sources of octylphenols, BPA and phthalates as well as the metal(loid)s Sb and W, infrequently reported in previous studies. Among metal(loid)s, Cu, Zn and W occurred in the highest concentrations (up to 1.2 mg/L Cu, 2.4 mg/L Zn and 1.9 mg/L W), while PAHs and phthalates occurred in the highest concentrations among the trace organic pollutants (up to 540 μg/L phthalate diisononyl phthalate). Among the phthalates, di-(2-ethylhexyl)phthalate had the highest frequency of detection (43% of the roadside samples). While BPA and octylphenols had relatively high frequencies of detection (50% for BPA and 81% for octylphenols), they were present in comparatively low concentrations (up to 0.2 μg/L BPA and 1.1 μg/L octylphenols). The control site displayed generally low concentrations of the pollutants studied, indicating that atmospheric deposition was not a significant source of the pollutants found in the roadside snow. Several of the pollutants in the roadside snow exceeded the applicable surface water and stormwater effluent guideline values. Thus, the transport of these pollutants with runoff posed risk of causing adverse effects in the receiving surface waters.
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| 7. |
- Müller, Alexandra, et al.
(författare)
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Releases of micropollutants from building surface materials into rainwater and snowmelt induced runoff
- 2023
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Ingår i: Chemosphere. - : Elsevier. - 0045-6535 .- 1879-1298. ; 330
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Tidskriftsartikel (refereegranskat)abstract
- Building surface materials, exposed to wash-off by rainwater or snowmelt, are recognised as one of the significant urban diffuse pollution sources contributing to the impairment of stormwater quality. The pollution conveyed by roof runoff originates from two potential sources, migration of surface material constituents, or wash-off of pollutants deposited on the surface by atmospheric deposition. This study investigated the releases of metals and several groups of contaminants of emerging concern: alkylphenols, alkylphenol ethoxylates, and phthalates, from commercially available materials, which are commonly used on buildings and structure surfaces in the urban environment. The materials tested included the following: metal sheets of stainless steel, copper, zinc, galvanised steel, corten steel, corrugated and coated steel, coated zinc; and bitumen-based roofing felt and shingles, as well as polyvinyl chloride (PVC) from two manufacturers. The stainless steel was considered a control material serving to estimate pollutant contributions deposited on the pilot panels from the surrounding environment. Moreover, this study presents novel data on roof snowmelt induced runoff quality, not reported in the previous literature. The experimental setup consisted of 2-m2 rectangular panels mounted in triplicates of each material and placed in an open-air setting on the campus of Luleå University of Technology, Sweden. Runoff leaving the gently sloping material panels was collected during 11 rain and three snowmelt driven runoff events occurring over a five-year period. The results showed that, in general, the micropollutant concentrations and loads were lower in snowmelt than rain induced runoff, and no decreasing trend was detected in the releases of phthalates or metals during the study period. Moreover, on a yearly basis, copper sheets were estimated to release 0.6 g/m2 Cu to runoff, zinc and galvanised sheets 1.3 and 0.7 g/m2 Zn, respectively, and, PVC sheets were estimated to release up to 78 mg/m2 of diisononyl phthalate (DINP).
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| 8. |
- Müller, Alexandra, et al.
(författare)
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The pollution conveyed by urban runoff : A review of sources
- 2020
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Ingår i: Science of the Total Environment. - : Elsevier. - 0048-9697 .- 1879-1026. ; 709
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Forskningsöversikt (refereegranskat)abstract
- Urban stormwater and snowmelt pollution contributes significantly to the deterioration of surface waters quality in many locations. Consequently, the sources of such pollution have been studied for the past 50 years, with the vehicular transportation sector and the atmospheric deposition identified early as the major pollution sources. In search for mitigation of this pollution, source controls, besides other measures, were recognised as effective pollution mitigation tools, whose successful implementation requires a good knowledge of pollution sources. Even though great research efforts have been exerted to document specific sources of urban runoff pollution, or specific groups of pollutants present in urban runoff, a comprehensive overview of all known contributing sources is still missing. This review contributes to closing this gap by compiling findings of previous research and critically synthesizing the current knowledge of various stormwater pollution sources. As the emphasis is placed on the sources, the related issues of implications for urban surface water quality and possible source controls for individual sources are touched upon just briefly, where required. The review showed that the atmospheric deposition, vehicular transportation-related activities and metallic building envelopes continue to be among the major pollution sources, which have been studied in a far greater detail than other sources. Furthermore, it was noted that because of the rapid advances in clean manufacturing and pollution control technologies, a large part of the body of data on stormwater quality available in the literature should be considered as historical data, which may no longer describe well the current conditions. Progressing historical data obsolescence, combined with continuing releases of new materials and chemicals, and, in some cases of new substances of potential concern, into the environment, suggests that the identification of important stormwater runoff/snowmelt pollution sources, and the associated pollutants, has been and will remain to be a work in progress.
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