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- Hu, W., et al.
(författare)
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Electron transport in self-assembled polymer molecular junctions
- 2006
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Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 96:2, s. 027801-
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Tidskriftsartikel (refereegranskat)abstract
- A molecular junction of a poly(p-phenyleneethynylene)s derivative with thioacetate end groups (TA-PPE) was fabricated by self-assembling. Nanogap electrodes made by electroplating technique was used to couple thiol end groups of TA-PPE molecules. Room temperature current-voltage characteristics of the molecular junction exhibited highly periodic, repeatable, and identical stepwise features. First-principles calculations suggest that one possibility for the equidistant step is due to the opening of different conducting channels that corresponds to the unoccupied molecular orbitals of the polymer in the junction. It is interesting to see that an 18 nm long polymer is of quantized electronic structures and behaves like a quantum transport device.
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- Mancusi, Davide, 1980, et al.
(författare)
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Calculation of Energy-Deposition Distributions and Microdosimetric Estimation of the Biological Effect of a 9C Beam
- 2009
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Ingår i: Radiation and Environmental Biophysics. - 1432-2099 .- 0301-634X. ; 48:2, s. 135-143
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Tidskriftsartikel (refereegranskat)abstract
- Among the alternative beams being recently considered for external cancer radiotherapy, C-9 has received some attention because it is expected that its biological effectiveness could be boosted by the beta-delayed emission of two alpha particles and a proton that takes place at the ion-stopping site. Experiments have been performed to characterise this exotic beam physically and models have been developed to estimate quantitatively its biological effect. Here, the particle and heavy-ion transport code system (PHITS ) is used to calculate energy-deposition and linear energy transfer distributions for a C-9 beam in water and the results are compared with published data. Although PHITS fails to reproduce some of the features of the distributions, it suggests that the decay of C-9 contributes negligibly to the energy-deposition distributions, thus contradicting the previous interpretation of the measured data. We have also performed a microdosimetric calculation to estimate the biological effect of the decay, which was found to be negligible; previous microdosimetric Monte-Carlo calculations were found to be incorrect. An analytical argument, of geometrical nature, confirms this conclusion and gives a theoretical upper bound on the additional biological effectiveness of the decay. However, no explanation can be offered at present for the observed difference in the biological effectiveness between C-9 and C-12; the reproducibility of this surprising result will be verified in coming experiments.
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- Sihver, Lembit, 1962, et al.
(författare)
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Recent developments and benchmarking of the PHITS code
- 2007
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Ingår i: Advances in Space Research. - : Elsevier BV. - 1879-1948 .- 0273-1177. ; 40:9, s. 1320-1331
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Tidskriftsartikel (refereegranskat)abstract
- Many new options have recently been included in PHITS, e.g., to calculate LET distributions of particles in matter or energy-deposition distributions event by event and correlations between energy depositions in different regions. This makes it possible to calculate the effects of particle radiation on biological and non-biological materials, e.g., risk for single event upsets in electronic devices. As a part of an extensive ongoing benchmarking of PHITS, we have compared calculated partial projectile fragmentation cross sections with accelerator-based measurements from the reactions of 200-1000 MeV/n He-4, C-12, N-14, O-16, Ne-20, Si-28, Ar-40, and Fe-56 on polyethylene, carbon, aluminum, copper, tin and lead, with different thicknesses, using different total reaction cross section models in PHITS. We have compared simulated and measured Bragg and attenuation curves of 200 MeV/n C-12 in water, and neutron energy spectra, at different angles, from 100 to 400 MeV/n C-12 stopped in water. Bragg curves for 110, 140, 170, 190 and 225 MeV/n He-3 in water have been studied, as well as gamma-ray dose decay curves of activated Cu target bombarded by 400 and 800 MeV/n Ar-40. When using the default total reaction cross section model developed by Tripathi et al. (1996,1997 and 1999) [Tripathi, R.K., Cucinotta, F.A., Wilson, J.W. Accurate universal parameterization of absorption cross sections, Nucl. Instr. Methods B117, 347, 1996; Tripathi, R.K., Wilson, J.W., Cucinotta, F.A. Accurate universal parameterization of absorption cross sections II - neutron absorption cross sections. Nucl. Instr. Methods B129, 11, 1997; Tripathi, R.K., Cucinotta, F.A., Wilson, J.W. Accurate universal parameterization of absorption cross sections III - light systems. Nucl. Instr. Methods B155, 349, 1999.] the partial fragmentation cross sections appear to be systematically slightly underestimated by a factor which is independent on the fragment species within the same data set, and so do the simulated neutron energy spectra from selected heavy ion reactions; especially in the forward direction. The simulated attenuation and Bragg curves, however, show good agreement with measured ones. These observations stimulate further benchmarking to confirm the accuracy of the code and gives directions on possible improvements to be applied to the code in the near future. (C) 2007 Published by Elsevier Ltd on behalf of COSPAR.
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- Mancusi, Davide, 1980, et al.
(författare)
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PHITS - benchmark of partial charge-changing cross sections for intermediate-mass systems
- 2007
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Ingår i: Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms. - : Elsevier BV. - 0168-583X. ; 254:1, s. 30-38
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Tidskriftsartikel (refereegranskat)abstract
- The PHITS (Particle and Heavy Ion Transport System) code is a three-dimensional Monte Carlo code that is able to simulate the transport of nuclei and other particles in complicated geometries and calculate fluxes, doses, energy-deposition distributions and many other observables. Among its many possible fields of application, it can be used e.g. to design and optimise radiation shields for space vessels. However, the reliability of the predictions of the code depends directly on the certified accuracy of the code components, i.e. the models the code uses to estimate the quantities necessary for the transport calculation. As a part of a comprehensive benchmarking program, we have investigated the possibility of using PHITS to calculate partial charge-changing cross sections and we have compared the results with measurements performed by some of us (CZ, LH, JM, SG). The results, although limited, suggest that the current reaction-cross-section models might be inadequate for use in space radioprotection; we therefore claim the need for a thorough benchmarking of the models and for new reaction-cross-section measurements and experimental techniques.
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- Tafoya, D., et al.
(författare)
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Detection of HCO+ emission toward the planetary nebula K3-35
- 2007
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Ingår i: Astronomical Journal. - 1538-3881 .- 0004-6256. ; 133:2, s. 364-369
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Tidskriftsartikel (refereegranskat)abstract
- We report the detection, for the first time, of HCO+(J = 1 -> 0) emission, as well as marginal CO(J = 1 -> 0) emission, toward the planetary nebula (PN) K3-35 as a result of a molecular survey carried out toward this source. We also report new observations of the previously detected CO( J 2 ! 1) and water maser emission, as well as upper limits for the emission of the SiO, (HCO+)-C-13, HNC, HCN, HC3OH, HC5N, CS, HC3N, (CO)-C-13, CN, and NH3 molecules. From the ratio of CO(J = 2 -> 1) to CO(J = 1 -> 0) emission we have estimated the kinetic temperature of the molecular gas, obtaining a value of similar or equal to 20 K. Using this result we have estimated a molecular mass for the envelope of similar or equal to 0.017M(circle dot) and an HCO+ abundance relative to H-2 of 6 x 10(-7), similar to the abundances found in other PNe. K3-35 is remarkable because it is one of the two PNe reported to exhibit water maser emission, which is present in the central region, as well as at a distance of similar or equal to 5000 AU from the center. The presence of molecular emission provides some clues that could help in understanding the persistence of water molecules in the envelope of K3-35. The HCO+ emission could be arising in dense molecular clumps, which may provide the shielding mechanism that protects water molecules in this source.
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