| 1. |
- Fuller, Franklin D, et al.
(författare)
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Drop-on-demand sample delivery for studying biocatalysts in action at X-ray free-electron lasers
- 2017
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Ingår i: Nature Methods. - : Macmillan Publishers Ltd.. - 1548-7091 .- 1548-7105. ; 14, s. 443-449
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Tidskriftsartikel (refereegranskat)abstract
- X-ray crystallography at X-ray free-electron laser sources is a powerful method for studying macromolecules at biologically relevant temperatures. Moreover, when combined with complementary techniques like X-ray emission spectroscopy, both global structures and chemical properties of metalloenzymes can be obtained concurrently, providing insights into the interplay between the protein structure and dynamics and the chemistry at an active site. The implementation of such a multimodal approach can be compromised by conflicting requirements to optimize each individual method. In particular, the method used for sample delivery greatly affects the data quality. We present here a robust way of delivering controlled sample amounts on demand using acoustic droplet ejection coupled with a conveyor belt drive that is optimized for crystallography and spectroscopy measurements of photochemical and chemical reactions over a wide range of time scales. Studies with photosystem II, the phytochrome photoreceptor, and ribonucleotide reductase R2 illustrate the power and versatility of this method.
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| 2. |
- Lee, Justin H., et al.
(författare)
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MMS Measurements and Modeling of Peculiar Electromagnetic Ion Cyclotron Waves
- 2019
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Ingår i: Geophysical Research Letters. - : AMER GEOPHYSICAL UNION. - 0094-8276 .- 1944-8007.
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Tidskriftsartikel (refereegranskat)abstract
- Orbiting Earth's dayside outer magnetosphere on 29 September 2015, the Magnetospheric Multiscale (MMS) satellites measured plasma composition, simultaneous electromagnetic ion cyclotron waves, and intermittent fast plasma flows consistent with ultralow frequency waves or convection. Such flows can accelerate typically unobservable low-energy plasma into a measurable energy range of spacecraft plasma instrumentation. We exploit the flow occurrence to ensure measurement of cold ion species alongside the hot particles-consisting of ionospheric heavy ions and solar wind He++-during a subinterval of wave emissions with spectral properties previously described as peculiar. Through application of the composition and multisatellite wave vector data to linear theory, we demonstrate the emissions are in fact consistent with theory, growing naturally in the He++ band with sufficient free energy.
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| 3. |
- Wang, Rongsheng, et al.
(författare)
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An Electron-Scale Current Sheet Without Bursty Reconnection Signatures Observed in the Near-Earth Tail
- 2018
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Ingår i: Geophysical Research Letters. - : AMER GEOPHYSICAL UNION. - 0094-8276 .- 1944-8007. ; 45:10, s. 4542-4549
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Tidskriftsartikel (refereegranskat)abstract
- Observations of a current sheet as thin as the electron scale are extremely rare in the near-Earth magnetotail. By measurement from the novel Magnetospheric Multiscale mission in the near-Earth magnetotail, we identified such an electron-scale current sheet and determined its detailed properties. The electron current sheet was bifurcated, with a half-thickness of nine electron inertial lengths, and was sandwiched between the Hall field. Because of the strong Hall electric field, the super-Alfvenic electron bulk flows were created mainly by the electric field drift, leading to the generation of the strong electron current. Inevitably, a bifurcated current sheet was formed since the Hall electric field was close to zero at the center of the current sheet. Inside the electron current sheet, the electrons were significantly heated while the ion temperature showed no change. The ions kept moving at a low speed, which was not affected by this electron current sheet. The energy dissipation was negligible inside the current sheet. The observations indicate that a thin current sheet, even as thin as electron scale, is not the sufficient condition for triggering bursty reconnection.
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| 4. |
- Eriksson, Elin, 1989-, et al.
(författare)
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Electron Energization at a Reconnecting Magnetosheath Current Sheet
- 2018
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Ingår i: Geophysical Research Letters. - : American Geophysical Union (AGU). - 0094-8276 .- 1944-8007. ; 45:16, s. 8081-8090
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Tidskriftsartikel (refereegranskat)abstract
- We present observations of electron energization within a sub-ion-scale magnetosheath current sheet (CS). A number of signatures indicate ongoing reconnection, including the thickness of the CS (similar to 0.7 ion inertial length), nonzero normal magnetic field, Hall magnetic fields with electrons carrying the Hall currents, and electron heating. We observe localized electron acceleration and heating parallel to the magnetic field at the edges of the CS. Electrostatic waves observed in these regions have low phase velocity and small wave potentials and thus cannot provide the observed acceleration and heating. Instead, we find that the electrons are accelerated by a parallel potential within the separatrix regions. Similar acceleration has been reported based on magnetopause and magnetotail observations. Thus, despite the different plasma conditions in magnetosheath, magnetopause, and magnetotail, the acceleration mechanism and corresponding heating of electrons is similar. Plain Language Summary Magnetic reconnection is an important physical energy conversion process in astrophysical and laboratory plasmas. The easiest place to analyze magnetic reconnection is in near-Earth space. Due to lack of sufficient electron resolution of previous spacecraft missions, there are many unanswered questions regarding electron heating and acceleration processes at small scales. In particular, the regime where thermal pressure dominates over magnetic pressure, the most common state of plasmas in the Universe, is little explored. In this letter we study such a regime using the four-spacecraft Magnetospheric Multiscale mission. We analyze a reconnecting current sheet in the magnetosheath. We show that electrons are energized by a parallel potential, similar to what has been observed in the different plasma regimes the magnetopause and magnetotail. Thus, despite different plasma conditions, a similar acceleration mechanism and corresponding heating of electrons is occurring in all these regions.
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| 5. |
- Li, Jinxing, et al.
(författare)
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Local Excitation of Whistler Mode Waves and Associated Langmuir Waves at Dayside Reconnection Regions
- 2018
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Ingår i: Geophysical Research Letters. - : American Geophysical Union (AGU). - 0094-8276 .- 1944-8007. ; 45:17, s. 8793-8802
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Tidskriftsartikel (refereegranskat)abstract
- In the Earth's dayside reconnection boundary layer, whistler mode waves coincide with magnetic field openings and the formation of the resultant anisotropic electrons. Depending on the energy range of anisotropic electrons, whistlers can grow at frequencies in the upper and/or lower band. Observations show that whistler mode waves modulate Langmuir wave amplitude as they propagate toward the X line. Observations of whistler mode wave phase and Langmuir waves packets, as well as coincident electron measurements, reveal that whistler mode waves can accelerate electrons via Landau resonance at locations where E(parallel to)is antiparallel to the wave propagation direction. The accelerated electrons produce localized beams, which subsequently drive the periodically modulated Langmuir waves. The close association of those two wave modes reveals the microscale electron dynamics in the exhaust region, and the proposed mechanism could potentially be applied to explain the modulation events observed in planetary magnetospheres and in the solar wind. Plain Language Summary The Sun's and Earth's magnetic field can merge and reconnect on dayside magnetopause. Using measurements from NASA's MMS spacecraft, we report that a class of electromagnetic wave, named whistler mode wave, coincides with the reconnected magnetic field lines. Besides, those whistlers are observed to modulate the electric field oscillations, known as Langmuir waves. Using high-resolution wave and particle measurements, we explain that the whistlers are locally excited when electrons from both sides of the magnetopause mix and form an unstable distribution. The modulated Langmuir waves are generated due to localized electron acceleration, which occurs when the velocity of electrons matches that of whistlers in the direction along the magnetic field. The whistler mode waves and associated Langmuir waves can be used as an additional tool to remotely sense the occurrence of magnetic reconnections.
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| 6. |
- Toledo-Redondo, Sergio, et al.
(författare)
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Cold ion demagnetization near the X-line of magnetic reconnection
- 2016
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Ingår i: Geophysical Research Letters. - : Blackwell Publishing. - 0094-8276 .- 1944-8007. ; 43:13, s. 6759-6767
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Tidskriftsartikel (refereegranskat)abstract
- Although the effects of magnetic reconnection in magnetospheres can be observed at planetary scales, reconnection is initiated at electron scales in a plasma. Surrounding the electron diffusion region, there is an Ion-Decoupling Region (IDR) of the size of the ion length scales (inertial length and gyroradius). Reconnection at the Earth's magnetopause often includes cold magnetospheric (few tens of eV), hot magnetospheric (10keV), and magnetosheath (1keV) ions, with different gyroradius length scales. We report observations of a subregion inside the IDR of the size of the cold ion population gyroradius (approximate to 15km) where the cold ions are demagnetized and accelerated parallel to the Hall electric field. Outside the subregion, cold ions follow the E x B motion together with electrons, while hot ions are demagnetized. We observe a sharp cold ion density gradient separating the two regions, which we identify as the cold and hot IDRs.
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