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Träfflista för sökning "WFRF:(Rosén Tomas 1985 ) srt2:(2023)"

Sökning: WFRF:(Rosén Tomas 1985 ) > (2023)

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1.
  • Motezakker, Ahmad Reza, et al. (författare)
  • Effect of Stiffness on the Dynamics of Entangled Nanofiber Networks at Low Concentrations
  • 2023
  • Ingår i: Macromolecules. - : American Chemical Society (ACS). - 0024-9297 .- 1520-5835. ; 56:23, s. 9595-9603
  • Tidskriftsartikel (refereegranskat)abstract
    • Biopolymer network dynamics play a significant role in both biological and materials science. This study focuses on the dynamics of cellulose nanofibers as a model system given their relevance to biology and nanotechnology applications. Using large-scale coarse-grained simulations with a lattice Boltzmann fluid coupling, we investigated the reptation behavior of individual nanofibers within entangled networks. Our analysis yields essential insights, proposing a scaling law for rotational diffusion, quantifying effective tube diameter, and revealing release mechanisms during reptation, spanning from rigid to semiflexible nanofibers. Additionally, we examine the onset of entanglement in relation to the nanofiber flexibility within the network. Microrheology analysis is conducted to assess macroscopic viscoelastic behavior. Importantly, our results align closely with previous experiments, validating the proposed scaling laws, effective tube diameters, and onset of entanglement. The findings provide an improved fundamental understanding of biopolymer network dynamics and guide the design of processes for advanced biobased materials. 
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2.
  • Rosén, Tomas, 1985-, et al. (författare)
  • Exploring nanofibrous networks with x-ray photon correlation spectroscopy through a digital twin
  • 2023
  • Ingår i: Physical review. E. - 2470-0045 .- 2470-0053. ; 108:1
  • Tidskriftsartikel (refereegranskat)abstract
    • We demonstrate a framework of interpreting data from x-ray photon correlation spectroscopy experiments with the aid of numerical simulations to describe nanoscale dynamics in soft matter. This is exemplified with the transport of passive tracer gold nanoparticles in networks of charge-stabilized cellulose nanofibers. The main structure of dynamic modes in reciprocal space could be replicated with a simulated system of confined Brownian motion, a digital twin, allowing for a direct measurement of important effective material properties describing the local environment of the tracers. 
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