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Sökning: WFRF:(Sala Leonardo) > (2022)

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1.
  • Martinelli, Leonardo, et al. (författare)
  • Fractional Spin Excitations in the Infinite-Layer Cuprate CaCuO2
  • 2022
  • Ingår i: Physical Review X. - 2160-3308. ; 12:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We use resonant inelastic x-ray scattering (RIXS) to investigate the magnetic dynamics of the infinite-layer cuprate CaCuO2. We find that close to the (1/2,0) point, the single magnon decays into a broad continuum of excitations accounting for about 80% of the total magnetic spectral weight. Polarization-resolved RIXS spectra reveal the overwhelming dominance of the spin-flip (Delta S = 1) character of this continuum with respect to the Delta S = 0 multimagnon contributions. Moreover, its incident-energy dependence is identical to that of the magnon, supporting a common physical origin. We propose that the continuum originates from the decay of the magnon into spinon pairs, and we relate it to the exceptionally high ring exchange J(c) similar to J(1) of CaCuO2. In the infinite-layer cuprates, long-range and multisite hopping integrals are very important, and they amplify the 2D quantum magnetism effects in spite of the 3D antiferromagnetic Neel order.
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2.
  • Peng, Y. Y., et al. (författare)
  • Doping dependence of the electron-phonon coupling in two families of bilayer superconducting cuprates
  • 2022
  • Ingår i: Physical Review B. - 2469-9969 .- 2469-9950. ; 105:11
  • Tidskriftsartikel (refereegranskat)abstract
    • While electron-phonon coupling (EPC) is crucial for Cooper pairing in conventional superconductors, its role in high-Tc superconducting cuprates is debated. Using resonant inelastic x-ray scattering at the oxygen K edge, we study the EPC in Bi2Sr2CaCu2O8+δ (Bi2212) and Nd1+xBa2-xCu3O7-δ (NBCO) at different doping levels ranging from heavily underdoped (p=0.07) to overdoped (p=0.21). We analyze the data with a localized Lang-Firsov model that allows for the coherent excitations of two phonon modes. While electronic band dispersion effects are non-negligible, we are able to perform a study of the relative values of EPC matrix elements in these cuprate families. In the case of NBCO, the choice of the excitation energy allows us to disentangle modes related to the CuO chains and the CuO2 planes. Combining the results from the two families, we find the EPC strength decreases with doping at q∥=(-0.25,0) r.l.u., but has a nonmonotonic trend as a function of doping at smaller momenta. This behavior is attributed to the screening effect of charge carriers. We also find that the phonon intensity is enhanced in the vicinity of the charge-density-wave excitations while the extracted EPC strength appears to be less sensitive to their proximity. By performing a comparative study of two cuprate families, we are able to identify general trends in the EPC for the cuprates and provide experimental input to theories invoking a synergistic role for this interaction in d-wave pairing.
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