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PEDOT:PSS-based Mul...
PEDOT:PSS-based Multilayer Bacterial-Composite Films for Bioelectronics
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- Zajdel, Tom J. (författare)
- Univ Calif Berkeley, CA 94720 USA; Lawrence Berkeley Natl Lab, CA 94720 USA
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- Baruch, Moshe (författare)
- Lawrence Berkeley Natl Lab, CA 94720 USA
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- Méhes, Gábor (författare)
- Linköpings universitet,Fysik och elektroteknik,Tekniska fakulteten,Lawrence Berkeley Natl Lab, CA 94720 USA
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- Stavrinidou, Eleni (författare)
- Linköpings universitet,Fysik och elektroteknik,Tekniska fakulteten
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- Berggren, Magnus (författare)
- Linköpings universitet,Fysik och elektroteknik,Tekniska fakulteten
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- Maharbiz, Michel M. (författare)
- Univ Calif Berkeley, CA 94720 USA; Univ Calif Berkeley, CA 94720 USA; Chan Zuckerberg Biohub, CA USA
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- Simon, Daniel (författare)
- Linköpings universitet,Fysik och elektroteknik,Tekniska fakulteten
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- Ajo-Franklin, Caroline M. (författare)
- Lawrence Berkeley Natl Lab, CA 94720 USA
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(creator_code:org_t)
- 2018-10-16
- 2018
- Engelska.
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Ingår i: Scientific Reports. - : NATURE PUBLISHING GROUP. - 2045-2322. ; 8
- Relaterad länk:
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https://liu.diva-por... (primary) (Raw object)
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https://www.nature.c...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Microbial electrochemical systems provide an environmentally-friendly means of energy conversion between chemical and electrical forms, with applications in wastewater treatment, bioelectronics, and biosensing. However, a major challenge to further development, miniaturization, and deployment of bioelectronics and biosensors is the limited thickness of biofilms, necessitating large anodes to achieve sufficient signal-to-noise ratios. Here we demonstrate a method for embedding an electroactive bacterium, Shewanella oneidensis MR-1, inside a conductive three-dimensional poly(3,4-ethylenedioxy thiophene): poly(styrenesulfonate) (PEDOT:PSS) matrix electropolymerized on a carbon felt substrate, which we call a multilayer conductive bacterial-composite film (MCBF). By mixing the bacteria with the PEDOT:PSS precursor in a flow-through method, we maintain over 90% viability of S. oneidensis during encapsulation. Microscopic analysis of the MCBFs reveal a tightly interleaved structure of bacteria and conductive PEDOT:PSS up to 80 mu m thick. Electrochemical experiments indicate S. oneidensis in MCBFs can perform both direct and riboflavin-mediated electron transfer to PEDOT:PSS. When used in bioelectrochemical reactors, the MCBFs produce 20 times more steady-state current than native biofilms grown on unmodified carbon felt. This versatile approach to control the thickness of bacterial composite films and increase their current output has immediate applications in microbial electrochemical systems, including field-deployable environmental sensing and direct integration of microorganisms into miniaturized organic electronics.
Ämnesord
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
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