| 1. |
- Liu, H., et al.
(författare)
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Optical and extreme UV studies of spin dynamics in metallic and insulating ferrimagnets
- 2021
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Ingår i: Journal of Applied Physics. - : American Institute of Physics (AIP). - 0021-8979 .- 1089-7550. ; 130:24
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Tidskriftsartikel (refereegranskat)abstract
- We present all-optical studies of spin dynamics in two classes of ferrimagnets. Both sets of experiments use table-top laser-based pump–probe techniques to examine the ultrafast and longer timescale spin excitations. We use the visible/near infra-red time-resolved magneto-optical Kerr effect (tr-MOKE) to follow the spin dynamics of a series of metallic (FeCo)1−xGdx thin films with varying Gd content. Magnetic compensation in the films occurs at a Gd concentration of ≈26%, and the spin dynamics of the films exhibit a non-monotonic variation in effective magnetization. We also examine spin dynamics in an insulating NiFe2O4 spinel using ultrafast techniques up at extreme ultraviolet energies, which permit element-specific investigations. The element and time-resolved delay scans reveal a non-trivial interaction between spin excitations on the different magnetic sub-lattices of the magnetic insulator.
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| 2. |
- Malik, Rameez Saeed, 1987-, et al.
(författare)
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Ultrafast magnetization dynamics in the half-metallic Heusler alloy Co2FeAl
- 2021
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Ingår i: Physical Review B. - : American Physical Society. - 2469-9950 .- 2469-9969. ; 104:10
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Tidskriftsartikel (refereegranskat)abstract
- We report on optically induced, ultrafast magnetization dynamics in the Heusler alloy Co2FeAl, probed by time-resolved magneto-optical Kerr effect. Experimental results are compared to results from electronic structure theory and atomistic spin-dynamics simulations. Experimentally, we find that the demagnetization time (tau(M)) in films of Co2FeAl is almost independent of varying structural order, and that it is similar to that in elemental 3d ferromagnets. In contrast, the slower process of magnetization recovery, specified by tau(R), is found to occur on picosecond time scales, and is demonstrated to correlate strongly with the Gilbert damping parameter (alpha). Based on these results we argue that for Co2FeAl the remagnetization process is dominated by magnon dynamics, something which might have general applicability.
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| 3. |
- Vaskivskyi, Igor, et al.
(författare)
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Element-Specific Magnetization Dynamics in Co-Pt Alloys Induced by Strong Optical Excitation
- 2021
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Ingår i: The Journal of Physical Chemistry C. - : American Chemical Society (ACS). - 1932-7447 .- 1932-7455. ; 125:21, s. 11714-11721
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Tidskriftsartikel (refereegranskat)abstract
- Ever since its first observation, the microscopic origin of ultrafast magnetization dynamics has been actively debated. Even more questions arise when considering composite materials featuring a combination of intrinsic and proximity-induced magnetic moments. Currently, it is unknown whether the specific ultrafast dynamics of different sublattices in the popular ferromagnets consisting of 3d (Co, Fe) and 4d, 5d (Pd, Pt) transition metals are playing a crucial role in various effects, including all-optical magnetization switching. Here we investigate the element-specific dynamics of Co-Pt alloys on femtosecond and picosecond time scales using magneto-optical spectroscopy in the extended ultraviolet (EUV) region. Our results reveal that despite the proximity-induced nature of the magnetization of Pt atoms, the two sublattices in the alloy can have different responses to the optical excitation featuring distinct demagnetization rates. Additionally we show that it is important to consider the modification of magnetic anisotropy in opto-magnetic experiments as the vast majority of them are sensitive only to a single projection of the magnetic moment on the predefined axis, which may lead to experimental artifacts.
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