| 1. |
- Aiuppa, A., et al.
(författare)
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Gas measurements from the Costa Rica-Nicaragua volcanic segment suggest possible along-arc variations in volcanic gas chemistry
- 2014
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Ingår i: Earth and Planetary Science Letters. - : Elsevier BV. - 1385-013X .- 0012-821X. ; 407, s. 134-147
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Tidskriftsartikel (refereegranskat)abstract
- Obtaining accurate estimates of the CO2 output from arc volcanism requires a precise understanding of the potential along-arc variations in volcanic gas chemistry, and ultimately of the magmatic gas signature of each individual arc segment. In an attempt to more fully constrain the magmatic gas signature of the Central America Volcanic Arc (CAVA), we present here the results of a volcanic gas survey performed during March and April 2013 at five degassing volcanoes within the Costa Rica-Nicaragua volcanic segment (CNVS). Observations of the volcanic gas plume made with a multicomponent gas analyzer system (Multi-GAS) have allowed characterization of the CO2/SO2-ratio signature of the plumes at Pads (0.30 +/- 0.06, mean +/- SD), Rincon de la Vieja (27.0 +/- 15.3), and Turrialba (2.2 +/- 0.8) in Costa Rica, and at Telica (3.0 +/- 0.9) and San Cristobal (4.2 +/- 1.3) in Nicaragua (all ratios on molar basis). By scaling these plume compositions to simultaneously measured SO2 fluxes, we estimate that the CO2 outputs at CNVS volcanoes range from low (25.5 +/- 11.0 tons/day at Pods) to moderate (918 to 1270 tons/day at Turrialba). These results add a new information to the still fragmentary volcanic CO2 output data set, and allow estimating the total CO2 output from the CNVS at 2835 1364 tons/day. Our novel results, with previously available information about gas emissions in Central America, are suggestive of distinct volcanic gas CO2/S-T (= SO2 + H2S)-ratio signature for magmatic volatiles in Nicaragua (similar to 3) relative to Costa Rica (similar to 0.5-1.0). We also provide additional evidence for the earlier theory relating the CO2-richer signature of Nicaragua volcanism to increased contributions from slab-derived fluids, relative to more-MORB-like volcanism in Costa Rica. The sizeable along-arc variations in magmatic gas chemistry that the present study has suggested indicate that additional gas observations are urgently needed to more-precisely confine the volcanic CO2 from the CAVA, and from global arc volcanism.
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| 2. |
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| 3. |
- Arellano, Santiago, 1981, et al.
(författare)
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New developments on remote sensing studies of volcanic gas emissions by solar infrared spectroscopy
- 2011
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Ingår i: 11th IAVCEI-CCVG Gas Workshop, September 1 - 10, 2011, Kamchatka, Russia.
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Konferensbidrag (refereegranskat)abstract
- In this contribution, we will present some recent developments made by our group on the application of solar occultation remote sensing to the measurement of volcanic gas emissions in the infrared spectral region. These include the automation of Fourier Transform Spectrometers (FTS) and novel methods for radiation collection and spectrometric analysis.Solar FTS is a proven and versatile method for measuring volcanogenic gases. However, its relatively high cost and complexity on data collection and analysis have precluded its wider use by observatories as a permanent monitoring tool. We will present some results of a field experimentperformed at Popocatépetl volcano (Mexico) within the FIEL-VOLCAN project in April 2010, to show the feasibility of automating a solar FTS on volcanic settings to measure SO2/HCl molar ratios. The system includes a compact solar tracker for automatic radiation collection from a stationary point as well as an embedded computer for data acquisition. Data is evaluated off-line by using e.g., the Chalmers-QESOF program.Further simplifications of the transfer optics and spectroscopic analysis have been investigatedby our group and their operation principles and preliminary results will be presented.
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| 4. |
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| 5. |
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| 6. |
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| 7. |
- Bobrowski, N., et al.
(författare)
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Gas emission measurements of the active lava lake of Nyiragongo, DR Congo
- 2011
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Ingår i: Geophysical Research Abstracts, Vol. 13, EGU2011-10804, EGU General Assembly 2011, Vienna, Austria.
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Konferensbidrag (refereegranskat)abstract
- In June 2007 and July 2010 spectroscopic measurements and chemical in-situ studies were carried out at Nyiragongovolcano located 15 km north of the city Goma, North Kivu region (DRC), both at the crater rim and within the crater itself, next to the lava lake. Nyiragongo volcano belongs to the Virunga volcanic chain and it is associated with the Western branch of the Great Rift Valley. The volcanism at Nyiragongo is caused by the rifting of the Earth’s crust where two parts of the African plates are breaking apart. Niyragongo crater contains the biggest lava lake on Earth and it is considered one of the most active volcanoes in the world.The ground-based remote sensing technique MAX-DOAS (Multi-Axis Differential Optical Absorption Spectroscopy)using scattered sunlight has been applied during both field trips at the crater rim of the volcano tomeasure sulphur dioxide, halogen oxides and nitrogen oxide. Additionally filter pack and spectroscopic in-situ carbon dioxide measurements were carried out, as well as SO2 flux measurements by a scanning DOAS instrumentfrom the NOVAC project at the flank of the volcano.Nyiragongo is the first rift volcano where halogen oxides have been observed in the plume.Observations indicate that the gas composition of Nyiragongo might change with a changing lava lake level inshort and long-term time scales. Before and during an overflow of the lava lake the molar ratios of BrO/SO2 weredecreasing in 2007 and 2010 from about 3.10-5 to about 0 (below the detection limit). Such a decreasing trendwas also observed before and during the eruption of Mt. Etna 2006 and 2008.In a larger timescale between 2007 and 2010 the molar ratios of S/Cl and CO2/SO2 generally decreased from 6.7 -16.5 to 0.7 – 2.1, from 5 -10 to 1 - 5, respectively. The lower S/Cl and CO2/SO2 could lead to the conclusion thatthe magma reservoir below Niyragongo has had no new input from a deeper source.The chemical composition as well as its temporal variability within the volcanic plume from the lava lake will be discussed, as well as its implication on the understanding of the dynamics of the plumbing system of this volcano.
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| 8. |
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| 9. |
- Conde Jacobo, Alexander Vladimir, 1979, et al.
(författare)
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A rapid deployment instrument network for temporarily monitoring volcanic SO2 emissions - a study case from Telica volcano
- 2014
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Ingår i: Geoscientific Instrumentation, Methods and Data Systems. - : Copernicus GmbH. - 2193-0856 .- 2193-0864. ; 3:2, s. 127-134
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Tidskriftsartikel (refereegranskat)abstract
- Volcanic gas emissions play a crucial role in describing geophysical processes; hence measurements of magmatic gases such as SO2 can be used as tracers prior and during volcanic crises. Different measurement techniques based on optical spectroscopy have provided valuable information when assessing volcanic crises. This paper describes the design and implementation of a network of spectroscopic instruments based on Differential Optical Absorption Spectroscopy (DOAS) for remote sensing of volcanic SO2 emissions, which is robust, portable and can be deployed in relative short time. The setup allows the processing of raw data in situ even in remote areas with limited accessibility, and delivers pre-processed data to end-users in near real time even during periods of volcanic crisis, via a satellite link. In addition, the hardware can be used to conduct short term studies of volcanic plumes in remotes areas. The network was tested at Telica, an active volcano located in western Nicaragua, producing what is so far the largest data set of continuous SO2 flux measurements at this volcano.
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| 10. |
- Conde Jacobo, Alexander Vladimir, 1979, et al.
(författare)
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Measurements of volcanic SO2 and CO2 fluxes by combined DOAS, Multi-GAS and FTIR observations: a case study from Turrialba and Telica volcanoes
- 2014
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Ingår i: International Journal of Earth Sciences. - : Springer Science and Business Media LLC. - 1437-3262 .- 1437-3254. ; 103:8, s. 2335-2347
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Tidskriftsartikel (refereegranskat)abstract
- Over the past few decades, substantial progress has been made to overcome the technical difficulties of continuously measuring volcanic SO2 emissions. However, measurements of CO2 emissions still present many difficulties, partly due to the lack of instruments that can directly measure CO2 emissions and partly due to its strong atmospheric background. In order to overcome these difficulties, a commonly taken approach is to combine differential optical absorption spectroscopy (DOAS) by using NOVAC scan-DOAS instruments for continuous measurements of crateric SO2 emissions, and electrochemical/NDIR multi-component gas analyser system (multi-GAS) instruments for measuring CO2/SO2 ratios of excerpts of the volcanic plume. This study aims to quantify the representativeness of excerpts of CO2/SO2 ratios measured by Multi-GAS as a fraction of the whole plume composition, by comparison with simultaneously measured CO2/SO2 ratios using cross-crater Fourier transform infrared spectroscopy (FTIR). Two study cases are presented: Telica volcano (Nicaragua), with a homogenous plume, quiescent degassing from a deep source and ambient temperature, and Turrialba volcano (Costa Rica), which has a non-homogeneous plume from three main sources with different compositions and temperatures. Our comparison shows that in our "easier case" (Telica), FTIR and Multi-GAS CO2/SO2 ratios agree within a factor about 3 %. In our "complicated case" (Turrialba), Multi-GAS and FTIR yield CO2/SO2 ratios differing by approximately 13-25 % at most. These results suggest that a fair estimation of volcanic CO2 emissions can be provided by the combination of DOAS and Multi-GAS instruments for volcanoes with similar degassing conditions as Telica or Turrialba. Based on the results of this comparison, we report that by the time our measurements were made, Telica and Turrialba were emitting approximately 100 and 1,000 t day(-1) of CO2, respectively.
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| 11. |
- Conde Jacobo, Alexander Vladimir, 1979, et al.
(författare)
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SO2 degassing from Turrialba Volcano linked to seismic signatures during the period 2008-2012
- 2014
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Ingår i: International Journal of Earth Sciences. - : Springer Science and Business Media LLC. - 1437-3262 .- 1437-3254. ; 103:7, s. 1983-1998
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Tidskriftsartikel (refereegranskat)abstract
- wIn 1996, after 150 years of relative calm, Turrialba Volcano was reawakening. A visible plume and serious damage to surrounding vegetation due to acid rain are the most obvious signals. As part of the Network for Observation of Volcanic and Atmospheric Change project, four gas-monitoring stations were initially installed on the west flank of the volcano with the purpose of measuring sulphur dioxide emissions during this period of increased activity using the scanning-differential optical absorption spectroscopy technique. We present here the results of semicontinuous gas flux measurements over a period of 5 years (from 2008 to 2012), providing a novel data set that documents a relatively rapid increase in SO2 fluxes from around 350 t day(-1) to around 4,000 t day(-1) leading up to an eruptive period, followed by a gradual return to the former baseline values. Gas flux data were also compared with seismic data for selected periods of interest, providing insights into the link between degassing and seismicity. The most important result from this comparison is the identification of an inflexion point in the gas emissions followed by a clearly increasing trend in seismic activity, distinguishable 6 months prior to a phreatic eruptive event that occurred on 5 January 2010. This signal can be interpreted as a possible indicator of future eruptive events. Monitoring of SO2 thus complements seismic monitoring as a forecasting tool for eruptive events. Such monitoring is critical considering the proximity of Turrialba to the Central Valley, an area inhabited by more than 50 % of Costa Rica's population.
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| 12. |
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| 13. |
- Galle, Bo, 1952, et al.
(författare)
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Network for Observation of Volcanic and Atmospheric Change (NOVAC)-A global network for volcanic gas monitoring: Network layout and instrument description
- 2010
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Ingår i: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 115:D5, s. Art. no. D05304-
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Tidskriftsartikel (refereegranskat)abstract
- This paper presents the global project Network for Observation of Volcanic and Atmospheric Change (NOVAC), the aim of which is automatic gas emission monitoring at active volcanoes worldwide. Data from the network will be used primarily for volcanic risk assessment but also for geophysical research, studies of atmospheric change, and ground validation of satellite instruments. A novel type of instrument, the scanning miniaturized differential optical absorption spectroscopy (Mini-DOAS) instrument, is applied in the network to measure volcanic gas emissions by UV absorption spectroscopy. The instrument is set up 5-10 km downwind of the volcano under study, and typically two to four instruments are deployed at each volcano in order to cover different wind directions and to facilitate measurements of plume height and plume direction. Two different versions of the instrument have been developed. Version I was designed to be a robust and simple instrument for measurement of volcanic SO2 emissions at high time resolution with minimal power consumption. Version II was designed to allow the best possible spectroscopy and enhanced flexibility in regard to measurement geometry at the cost of larger complexity, power consumption, and price. In this paper the project is described, as well as the developed software, the hardware of the two instrument versions, measurement strategies, data communication, and archiving routines. As of April 2009 a total of 46 instruments have been installed at 18 volcanoes worldwide. As a typical example, the installation at Tungurahua volcano in Ecuador is described, together with some results from the first 21 months of operation at this volcano.
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| 14. |
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| 15. |
- Galle, Bo, 1952, et al.
(författare)
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NOVAC – Network for Observation of Volcanic and Atmospheric Change, recent developments and present status
- 2011
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Ingår i: 11th IAVCEI-CCVG Gas Workshop, September 1 - 10, 2011, Kamchatka, Russia.
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Konferensbidrag (refereegranskat)abstract
- The NOVAC project, funded by European Union, was started in October 2005 with the aim to establish a global network of stations for the quantitative measurement of volcanic gas emissions. The network is based on a novel type of instrument, the Scanning Dual-beam mini-DOAS. Primarily theinstruments will be used to provide new parameters in the toolbox of observatories for gas emission estimates, geophysical research and hazard assessment. In addition, data are exploited for other scientific purposes, e.g. global estimates of volcanic gas emissions, regional to global statistical analysis, and studies of atmospheric chemistry. In particular large scale validation of satellite measurements of volcanic gas emissions will be possible, bringing space-borne observation of volcanoes a significant step forward.The Scanning Dual-beam Mini-DOAS instrument is capable of real-time automatic, unattended measurement of the total emission fluxes of SO2 and BrO from a volcano with better then 5 minutes time resolution during daylight. The high time-resolution of the data enables correlations with othergeophysical data, e.g. seismicity, thus significantly extending the information available for real-time hazard assessment and research. By comparing high time resolution gas emission data with emissions from neighboring volcanoes on different geographical scales, or with other geophysical events (earthquakes, tidal waves) mechanisms of volcanic forcing may be revealed.The network today encompasses 58 instruments installed on 24 volcanoes, including some of the most active and strongest degassing volcanoes in the world.In addition a mobile version of the instrument has been developed intended for rapid deployment at a volcano in relation to a volcanic crisis.The project and its present status will be presented.
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| 16. |
- Geirsson, H., et al.
(författare)
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Multidisciplinary observations of the 2011 explosive eruption of Telica volcano, Nicaragua: Implications for the dynamics of low-explosivity ash eruptions
- 2014
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Ingår i: Journal of Volcanology and Geothermal Research. - : Elsevier BV. - 0377-0273. ; 271, s. 55-69
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Tidskriftsartikel (refereegranskat)abstract
- We present multidisciplinary observations of the March-June 2011 VEI 2 eruptive episode of the basalticandesite Telica volcano, Nicaragua, which allow for a comprehensive study of the eruption mechanics of low-explosivity eruptions at persistently active volcanoes. The observations are from a dense network of seismic and GPS instrumentation augmented by visual observations of the eruptive episode, geochemical and petrologic analysis of eruptive products, plume SO2 measurements, and temperature measurements of fumaroles inside and outside the active vent. The 2011 eruptive episode was Telica's most explosive since 1999 and consisted of numerous vulcanian explosions, with maximum column heights of 1.5-2 km above the crater rim, depositing a low volume of dominantly hydrothermally altered ash. Based on observed variations in seismicity, temperature, and SO2 flux, the lack of deformation of the edifice, the non-juvenile origin of and predominance of accretionary lapilli in the ash, we propose that temporary sealing of the hydrothermal system between similar to 0.5 and 2 km depth, allowed pressure to build up prior to vulcanian explosions, making this a phreatic eruptive episode.
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| 17. |
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| 18. |
- Hidalgo, Silvana, et al.
(författare)
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Correlation between SO2 fluxes and acoustic energy related to explosive activity at Tungurahua volcano (Ecuador)
- 2011
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Ingår i: 11th IAVCEI-CCVG Gas Workshop, September 1 - 10, 2011, Kamchatka, Russia.
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Konferensbidrag (refereegranskat)abstract
- Tungurahua is a steep-sided (5023 m high) andesitic stratovolcano located in the southern part of the Ecuadorian volcanic arc, with its summit crater lying just 8 km to both the touristic town of Baños and to a hydroelectric power plant that supplies 13% of the country’s total electric energy. Activity at Tungurahua resumed in September 1999 after 74 years of quiescence and since this time, the volcano has exhibited cyclic phases of activity. Typically, periods of high explosivity often characterized by strombolian to vulcanian behavior alternate with episodes of low to non explosive activity characterized by passive degassing.The monitoring network deployed at Tungurahua is comprehensive, allowing an extensive record of seismic events, acoustic energy, SO2 emissions and changes in deformation, to be recorded. In July 2006, five broad-band seismic stations with accompanying infrasound receptors were installed, allowing seismic and acoustic energy to be calculated for each discrete explosion event. As well, SO2fluxes have been recorded continuously since 2004 using two DOAS stations, before being enhanced to three sites in 2007. This complete record of both acoustic energy and SO2 fluxes subsequently allows meaningful correlations between the two parameters to be detected. Two clearly different kinds of behavior were distinguished:1.- From July 2007 to August 2008: degassing was most of the time above the normal background levels of passive degassing (1000 ton/day). During this corresponding period, explosive activity was also continuous. Total SO2 released between July 2007 and October 2008 was in the region of 328 kton, giving a daily average emission of 960 ton/day, which was associated with a cumulate meanacoustic energy of 93 kPa, which daily average is 247 Pa.2.- From August 2008 to the present: high SO2 emissions are related to explosive activity.Passive SO2 degassing which corresponds to approximately 65% of the time (during this period) reaches about 247 kton (456 ton/day) and is related to zero acoustic energy production. In contrast, explosive SO2 degassing reaches a total release of 456 kton (1,534 ton/day) and is related to a cumulate mean acoustic energy of 137 kPa, with a daily average of 508 Pa. These trends suggest that before August 2008 magma levels at Tungurahua may have been closer to the surface or that conduit geometry was more favorable for efficient degassing showing moderate explosive activity, displaying conditions reminiscent of an open-vent system. Since this time however, volcanic behavior appears to alter to a more closed or blocked conduit regime with degassing efficiency becoming appreciably reduced. During such activity, explosive behavior dominates within well defined eruptive episodes, characterized by more energetic explosions with associated pyroclastic flows and higher SO2 fluxes, such as May and December 2010 eruptive events.
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| 19. |
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| 20. |
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| 21. |
- Lübcke, Peter, et al.
(författare)
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BrO/SO2 molar ratios from scanning DOAS measurements in the NOVAC network
- 2014
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Ingår i: Solid Earth. - : Copernicus GmbH. - 1869-9510 .- 1869-9529. ; 5:1, s. 409-424
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Tidskriftsartikel (refereegranskat)abstract
- The molar ratio of BrO to SO2 is, like other halogen/sulfur ratios, a possible precursor for dynamic changes in the shallow part of a volcanic system. While the predictive significance of the BrO/SO2 ratio has not been well constrained yet, it has the major advantage that this ratio can be readily measured using the remote-sensing technique differential optical absorption spectroscopy (DOAS) in the UV. While BrO/SO2 ratios have been measured during several short-term field campaigns, this article presents an algorithm that can be used to obtain long-term time series of BrO/SO2 ratios from the scanning DOAS instruments of the Network for Observation of Volcanic and Atmospheric Change (NOVAC) or comparable networks. Parameters of the DOAS retrieval of both trace gases are given. The influence of co-adding spectra on the retrieval error and influences of radiative transfer will be investigated. Difficulties in the evaluation of spectroscopic data from monitoring instruments in volcanic environments and possible solutions are discussed. The new algorithm is demonstrated by evaluating data from the NOVAC scanning DOAS systems at Nevado del Ruiz, Colombia, encompassing almost 4 years of measurements between November 2009 and end of June 2013. This data set shows variations of the BrO/SO2 ratio several weeks prior to the eruption on 30 June 2012.
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| 22. |
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| 23. |
- Platt, U., et al.
(författare)
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Spectroscopic Observation of Volcanic Emissions – Status and Future Trends
- 2011
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Ingår i: 11th IAVCEI-CCVG Gas Workshop, September 1 - 10, 2011, Kamchatka, Russia.
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Konferensbidrag (refereegranskat)abstract
- In recent years spectroscopic quantification of gas emissions from volcanoes made considerable progress. In particular spectroscopic approaches observing volcanic gases in the ultra-violet spectral range evolved from an art to mature techniques, which are routinely applicable in automated installations.Using spatio-temporal correlation techniques also absolute amouts of trace gas fluxes can be determined.This is e.g. demonstrated by the NOVAC network.In addition systems operating in the infra-red (IR) spectral range have also made enormous progress. Here two varieties are in use: Absorption spectroscopy using direct sunlight and Emission spectroscopy using thermal emission from the trace constituents to be studied. Although neither of the two IR varieties is yet applicable in automated routine observation these techniques have considerable potential as well. For instance thermal emission spcetroscopy would also allow observations at night.Moreover, novel techniques for remote sensing of volcanic emissions, the SO2-Camera and imaging-DOAS (I-DOAS), where the I-DOAS technique trace gas distributions using the DOAS principle, came into widespread use recently. In particular the SO2 camera allows real time observation of the 2-dimensional evolution of volcanic plumes.Here we present a brief technical description and a critical assessment of the techniques listed above and discuss the relative merits of the different approaches for quantifying volcanic emissions by giving examples of successful applications in the field. Also expected future developments and requirements for volcanic surveillance are discussed.
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| 24. |
- Rivera, Claudia, 1976, et al.
(författare)
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NO2 fluxes from Tijuana using a mobile mini-DOAS during Cal-Mex 2010
- 2013
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Ingår i: Atmospheric Environment. - : Elsevier BV. - 1873-2844 .- 1352-2310. ; 70, s. 532-539
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Tidskriftsartikel (refereegranskat)abstract
- NO2 fluxes were measured using a mobile mini-DOAS during Cal-Mex 2010 field study, between May 15 and June 30, 2010, from the urban area of Tijuana, Baja California as well as the Rosarito power plant The average calculated NO2 fluxes were 328 +/- 184 (269 +/- 201) g s(-1), and 23.4 +/- 4.9 (12.9 +/- 11.9) g s(-1) for Tijuana urban area and Rosarito power plant, respectively, using model based wind fields and onsite measurements (in parenthesis). Wind speed and wind direction data needed to estimate the fluxes were both modeled and obtained from radiosondes launched regularly during the field campaign, whereas the mixing layer height throughout the entire field campaign was measured using a ceilometer. Large variations in the NO2 fluxes from both the Tijuana urban area and Rosarito power plant were observed during Cal-Mex 2010; however, the variability was less when model based wind fields were used. Qualitative comparisons of modeled and measured plumes from the Tijuana urban area and Rosarito power plant showed good agreement.
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| 25. |
- Smets, Benoît, et al.
(författare)
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Detailed multidisciplinary monitoring reveals pre- and co-eruptive signals at Nyamulagira volcano (North Kivu, Democratic Republic of Congo)
- 2014
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Ingår i: Bulletin of Volcanology. - : Springer Science and Business Media LLC. - 0258-8900 .- 1432-0819. ; 76:787, s. 1-35
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Tidskriftsartikel (refereegranskat)abstract
- This paper presents a thorough description of Nyamulagira’s January 2010 volcanic eruption (North Kivu, Democratic Republic of Congo), based on a combination of field observation and ground-based and space-borne data. It is the first eruption in the Virunga Volcanic Province that has been described by a combination of several modern monitoring techniques. The 2010 eruption lasted 26 days and emitted ∼45.5 × 106 m3 of lava. Field observations divided the event into four eruptive stages delimited by major changes in effusive activity. These stages are consistent with those described by Pouclet (1976) for historical eruptions of Nyamulagira. Co-eruptive signals from ground deformation, seismicity, SO2 emission and thermal flux correlate with the eruptive stages. Unambiguous pre-eruptive ground deformation was observed 3 weeks before the lava outburst, coinciding with a small but clear increase in the short period seismicity and SO2 emission. The 3 weeks of precursors contrasts with the only precursory signal previously recognized in the Virunga Volcanic Province, the short-term increase of tremor and long period seismicity, which, for example, were only detected less than 2 h prior to the 2010 eruption. The present paper is the most detailed picture of a typical flank eruption of this volcano. It provides valuable tools for re-examining former—mostly qualitative—descriptions of historical Nyamulagira eruptions that occurred during the colonial period.
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