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1.	Addor, Nans, et al. (författare) Propagation of biases in climate models from the synoptic to the regional scale : Implications for bias adjustment 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:5, s. 2075-2089 Tidskriftsartikel (refereegranskat)abstract Bias adjustment methods usually do not account for the origins of biases in climate models and instead perform empirical adjustments. Biases in the synoptic circulation are for instance often overlooked when postprocessing regional climate model (RCM) simulations driven by general circulation models (GCMs). Yet considering atmospheric circulation helps to establish links between the synoptic and the regional scale, and thereby provides insights into the physical processes leading to RCM biases. Here we investigate how synoptic circulation biases impact regional climate simulations and influence our ability to mitigate biases in precipitation and temperature using quantile mapping. We considered 20 GCM-RCM combinations from the ENSEMBLES project and characterized the dominant atmospheric flow over the Alpine domain using circulation types. We report in particular a systematic overestimation of the frequency of westerly flow in winter. We show that it contributes to the generalized overestimation of winter precipitation over Switzerland, and this wet regional bias can be reduced by improving the simulation of synoptic circulation. We also demonstrate that statistical bias adjustment relying on quantile mapping is sensitive to circulation biases, which leads to residual errors in the postprocessed time series. Overall, decomposing GCM-RCM time series using circulation types reveals connections missed by analyses relying on monthly or seasonal values. Our results underscore the necessity to better diagnose process misrepresentation in climate models to progress with bias adjustment and impact modeling.
2.	Aires, F., et al. (författare) Microwave hyperspectral measurements for temperature and humidity atmospheric profiling from satellite: The clear-sky case 2015 Ingår i: Journal of Geophysical Research. - 0148-0227 .- 2156-2202 .- 2169-897X .- 2169-8996. ; 120:21, s. 11334-11351 Tidskriftsartikel (refereegranskat)abstract This study investigates the benefits of a satellite HYperspectral Microwave Sensor (HYMS) for the retrieval of atmospheric temperature and humidity profiles, in the context of numerical weather prediction (NWP). In the infrared, hyperspectral instruments have already improved the accuracy of NWP forecasts. Microwave instruments so far only provide observations for a limited number of carefully selected channels. An information content analysis is conducted here to assess the impact of hyperspectral microwave measurements on the retrieval of temperature and water vapor profiles under clear-sky conditions. It uses radiative transfer simulations over a large variety of atmospheric situations. It accounts for realistic observation (instrument and radiative transfer) noise and for a priori information assumptions compatible with NWP practices. The estimated retrieval performance of the HYMS instrument is compared to those of the microwave instruments to be deployed on board the future generation of European operational meteorological satellites (MetOp-SG). The results confirm the positive impact of a HYMS instrument on the atmospheric profiling capabilities compared to MetOp-SG. Temperature retrieval uncertainty, compared to a priori information, is reduced by 2 to 10%, depending on the atmospheric height, and improvement rates are much higher than what will be obtained with MetOp-SG. For humidity sounding these improvements can reach 30%, a significant benefit as compared to MetOp-SG results especially below 250 hPa. The results are not very sensitive to the instrument noise, under our assumptions. The main impact provided by the hyperspectral information originates from the higher resolution in the O2 band around 60 GHz. The results are presented over ocean at nadir, but similar conclusions are obtained for other incidence angles and over land. Key Points A hyperspectral MW instrument could improve temperature & humidity retrieval compared to MetOp-SG The main impact from HYMS comes from higher resolution in the O2 band around 60 GHz Hyperspectral information is not really sensitive to instrument noise.
3.	Akperov, Mirseid, et al. (författare) Cyclone Activity in the Arctic From an Ensemble of Regional Climate Models (Arctic CORDEX) 2018 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-8996 .- 2169-897X. ; 123:5, s. 2537-2554 Tidskriftsartikel (refereegranskat)abstract The ability of state-of-the-art regional climate models to simulate cyclone activity in the Arctic is assessed based on an ensemble of 13 simulations from 11 models from the Arctic-CORDEX initiative. Some models employ large-scale spectral nudging techniques. Cyclone characteristics simulated by the ensemble are compared with the results forced by four reanalyses (ERA-Interim, National Centers for Environmental Prediction-Climate Forecast System Reanalysis, National Aeronautics and Space Administration-Modern-Era Retrospective analysis for Research and Applications Version 2, and Japan Meteorological Agency-Japanese 55-year reanalysis) in winter and summer for 1981-2010 period. In addition, we compare cyclone statistics between ERA-Interim and the Arctic System Reanalysis reanalyses for 2000-2010. Biases in cyclone frequency, intensity, and size over the Arctic are also quantified. Variations in cyclone frequency across the models are partly attributed to the differences in cyclone frequency over land. The variations across the models are largest for small and shallow cyclones for both seasons. A connection between biases in the zonal wind at 200 hPa and cyclone characteristics is found for both seasons. Most models underestimate zonal wind speed in both seasons, which likely leads to underestimation of cyclone mean depth and deep cyclone frequency in the Arctic. In general, the regional climate models are able to represent the spatial distribution of cyclone characteristics in the Arctic but models that employ large-scale spectral nudging show a better agreement with ERA-Interim reanalysis than the rest of the models. Trends also exhibit the benefits of nudging. Models with spectral nudging are able to reproduce the cyclone trends, whereas most of the nonnudged models fail to do so. However, the cyclone characteristics and trends are sensitive to the choice of nudged variables.
4.	An, Wenling, et al. (författare) Enhanced Recent Local Moisture Recycling on the Northwestern Tibetan Plateau Deduced From Ice Core Deuterium Excess Records 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:23, s. 12541-12556 Tidskriftsartikel (refereegranskat)abstract Local moisture recycling plays an essential role in maintaining an active hydrological cycle of the Tibetan Plateau (TP). Previous studies were largely limited to the seasonal time scale due to short and sparse observations, especially for the northwestern TP. In this study, we used a two-component mixing model to estimate local moisture recycling over the past decades from the deuterium excess records of two ice cores (i.e., Chongce and Zangser Kangri) from the northwestern TP. The results show that on average almost half of the precipitation on the northwestern TP is provided by local moisture recycling. In addition, the local moisture recycling ratio has increased evidently on the northwestern TP, suggesting an enhanced hydrological cycle. This recent increase could be due to the climatic and environmental changes on the TP in the past decades. Rapid increases in temperature and precipitation have enhanced evaporation. Changes of land surface of plateau have significantly increased evapotranspiration. All of these have intensified local moisture recycling. However, the mixing model used in this study only includes a limited number of climate factors. Some of the extreme values of moisture recycling ratio could be caused by large-scale atmospheric circulation and other climatic and weather events. Moreover, the potential mechanisms for the increase in local recycling need to be further examined, since the numeric simulations from climate models did not reproduce the increased contribution of local moisture recycling in precipitation.
5.	Bibi, S., et al. (författare) Response of Groundwater Storage and Recharge in the Qaidam Basin (Tibetan Plateau) to Climate Variations From 2002 to 2016 2019 Ingår i: Journal of Geophysical Research-Atmospheres. - : American Geophysical Union (AGU). - 2169-897X .- 2169-8996. ; 124:17-17, s. 9918-9934 Tidskriftsartikel (refereegranskat)abstract Groundwater (GW) and recharge as the main drivers of the water budget are challenging to quantify due to the complexity of hydrological processes and limited observations. Understanding these processes in relation to climate is crucial for evaluating future water availability of Tibetan Plateau. By computing storage changes in Gravity Recovery and Climate Experiment terrestrial water storage and Global Land Surface Data Assimilation System land surface state variables and water balance approach, we calculated GW storage changes and recharges. In the Qaidam Basin (northern Tibetan Plateau), terrestrial water storage from the Gravity Recovery and Climate Experiment revealed a significant increasing trend of 25.5 mm/year during 2002-2012. However, an obviously turning point was found around 2012 and terrestrial water storage revealed a significant decreasing rate of 37.9 mm/year during 2013-2016. Similarly, GW (recharge) had a significant increasing trend of 21.2 (4.5) mm/year before 2012 and a decreasing rate of 32.1 (10.9) mm/year after 2012. Domain-averaged difference (P-ET) between precipitation (P) and evapotranspiration (ET) also exhibited an increasing trend of 4.4 mm/year during 2002-2012 and a decreasing rate of 9.0 mm/year during 2013-2016. Precipitation followed dissimilar pattern with an increasing rate of 5.3 mm/year during 2002-2012 while no significant trend during 2013-2016. However, ET had a consistent increasing trend over the basin during the past 15 years (0.9 mm/year before 2012 and 9.0 mm/year thereafter). This study concluded that GW amount and distribution is mainly controlled by precipitation and ET. Decrease in precipitation at high elevations and increase in ET may impact future groundwater availability in this region.
6.	Bikkina, Srinivas, et al. (författare) Carbon isotope-constrained seasonality of carbonaceous aerosol sources from an urban location (Kanpur) in the Indo-Gangetic Plain 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:9, s. 4903-4923 Tidskriftsartikel (refereegranskat)abstract The Indo-Gangetic Plain (IGP) in northern India, Pakistan, and Bangladesh is a major source of carbonaceous aerosols in South Asia. However, poorly constrained seasonality of their sources over the IGP leads to large uncertainty in climate and health effects. Here we present a first data set for year-round radiocarbon (C-14) and stable carbon (C-13)-based source apportionment of total carbon (TC) in ambient PM10 (n = 17) collected from an urban site (Kanpur: 26.5 degrees N, 80.3 degrees E) in the IGP during January 2007 to January 2008. The year-round C-14-based fraction biomass (f(bio-TC)) estimate at Kanpur averages 777% and emphasizes an impact of biomass burning emissions (BBEs). The highest f(bio-TC) (%) is observed in fall season (October-November, 856%) followed by winter (December-February, 804%) and spring (March-May, 758%), while lowest values are found in summer (June-September, 69 +/- 2%). Since biomass/coal combustion and vehicular emissions mostly contribute to carbonaceous aerosols over the IGP, we predict C-13(TC) (C-13(pred)) over Kanpur using known C-13 source signatures and the measured C-14 value of each sample. The seasonal variability of C-13(obs)-C-13(pred) versus C-14(TC) together with air mass back trajectories and Moderate Resolution Imaging Spectroradiometer fire count data reveal that carbonaceous aerosols in winter/fall are significantly influenced by atmospheric aging (downwind transport of crop residue burning/wood combustion emissions in the northern IGP), while local sources (wheat residue combustion/vehicular emissions) dominate in spring/summer. Given the large temporal and seasonal variability in sources and emission strength of TC over the IGP, C-14-based constraints are, thus, crucial for reducing their uncertainties in carbonaceous aerosol budgets in climate models.
7.	Bikkina, Srinivas, et al. (författare) Dual carbon isotope characterization of total organic carbon in wintertime carbonaceous aerosols from northern India 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:9, s. 4797-4809 Tidskriftsartikel (refereegranskat)abstract Large-scale emissions of carbonaceous aerosols (CA) from South Asia impact both regional climate and air quality, yet their sources are not well constrained. Here we use source-diagnostic stable and radiocarbon isotopes (delta C-13 and Delta C-14) to characterize CA sources at a semiurban site (Hisar: 29.2 degrees N, 75.2 degrees E) in the NW Indo-Gangetic Plain (IGP) and a remote high-altitude location in the Himalayan foothills (Manora Peak: 29.4 degrees N, 79.5 degrees E, 1950 m above sea level) in northern India during winter. The Delta C-14 of total aerosol organic carbon (TOC) varied from -178% to -63% at Hisar and from -198% to -1% at Manora Peak. The absence of significant differences in the C-14-based fraction biomass of TOC between Hisar (0.81 +/- 0.03) and Manora Peak (0.82 +/- 0.07) reveals that biomass burning/biogenic emissions (BBEs) are the dominant sources of CA at both sites. Combining this information with d13C, other chemical tracers (K+/OC and SO42-/EC) and air mass back trajectory analyses indicate similar source regions in the IGP (e.g., Punjab and Haryana). These results highlight that CA from BBEs in the IGP are not only confined to the atmospheric boundary layer but also extend to higher elevations of the troposphere, where the synoptic-scale circulations could substantially influence their abundances both to the Himalayas and over the downwind oceanic regions such as the Indian Ocean. Given the vast emissions of CA from postharvest crop residue combustion practices in the IGP during early Northeast Monsoon, this information is important for both improved process and model understanding of climate and health effects, as well as in guiding policy decision aiming at reducing emissions.
8.	Bourgeois, Quentin, et al. (författare) Aerosol transport over the Andes from the Amazon Basin to the remote Pacific Ocean : A multiyear CALIOP assessment 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:16, s. 8411-8425 Tidskriftsartikel (refereegranskat)abstract Six years (200702012) of data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite instrument were used to investigate the vertical distribution and transport of aerosols over the tropical South American continent and the southeast Pacific Ocean. The multiyear aerosol extinction assessment indicates that aerosols, mainly biomass burning particles emitted during the dry season in the Amazon Basin, are lifted in significant amounts over the Andes. The aerosols are mainly transported in the planetary boundary layer between the surface and 2 km altitude with an aerosol extinction maximum near the surface. During the transport toward the Andes, the aerosol extinction decreases at a rate of 0.02 km(-1) per kilometer of altitude likely due to dilution and deposition processes. Aerosols reaching the top of the Andes, at altitudes typically between 4 and 5 km, are entrained into the free troposphere (FT) over the southeast Pacific Ocean. A comparison between CALIOP observations and ERA-Interim reanalysis data indicates that during their long-range transport over the tropical Pacific Ocean, these aerosols are slowly transported toward the marine boundary layer by the large-scale subsidence at a rate of 0.4 cm s(-1). The observed vertical/horizontal transport ratio is 0.700.8 m km(-1) Continental aerosols linked to transport over the Andes can be traced on average over 4000 km away from the continent indicating an aerosol residence time of 809 days in the FT over the Pacific Ocean. The FT aerosol optical depth (AOD) above the Pacific Ocean near South American coast accounts on average for 6% and 25% of the total AOD during the season of low and high biomass burning, respectively. This result shows that, during the biomass burning season, continental aerosols largely influence the AOD over the remote southeast Pacific Ocean. Overall, FT AOD decrease exponentially with the distance to continental sources at a rate of about 10% per degree of longitude over the Pacific Ocean.
9.	Brooks, Ian M., et al. (författare) The Turbulent Structure of the Arctic Summer Boundary Layer During The Arctic Summer Cloud-Ocean Study 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:18, s. 9685-9704 Tidskriftsartikel (refereegranskat)abstract The mostly ice covered Arctic Ocean is dominated by low-level liquid-or mixed-phase clouds. Turbulence within stratocumulus is primarily driven by cloud top cooling that induces convective instability. Using a suite of in situ and remote sensing instruments we characterize turbulent mixing in Arctic stratocumulus, and for the first time we estimate profiles of the gradient Richardson number at relatively high resolution in both time (10 min) and altitude (10 m). It is found that the mixing occurs both within the cloud, as expected, and by wind shear instability near the surface. About 75% of the time these two layers are separated by a stably stratified inversion at 100-200 m altitude. Exceptions are associated with low cloud bases that allow the cloud-driven turbulence to reach the surface. The results imply that turbulent coupling between the surface and the cloud is sporadic or intermittent.Plain Language Summary: The lower atmosphere over the summertime Arctic Ocean often consists of two well-mixed layers-a surface mixed layer and a cloud mixed layer-that are separated by a weak decoupling layer at about 100 to 300 m above the surface. In these cases, the cloud cannot interact directly with the surface. Large-scale forecast and climate models consistently fail to reproduce this observed structure and may thus fail to correctly reproduce the cloud properties and the amount of energy absorbed by or emitted from the surface as solar and infrared radiation. This contributes to errors in reproducing changes in sea ice concentration over time. Here we use measurements made in the central Arctic to study the processes controlling whether or not the cloud is coupled to the surface. The effect of wind at the surface is found not to be a controlling factor. The depth of the cloud mixed layer is critical, but the multiple processes influencing it cannot be separated using the data available here. However, cooling at cloud top by infrared radiation is key, as is the extension of cloud into the temperature inversion-a unique feature of Arctic clouds.
10.	Chen, Bing, et al. (författare) Reconciling modeling with observations of radiative absorption of black carbon aerosols 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:11, s. 5932-5942 Tidskriftsartikel (refereegranskat)abstract The physical treatment of internal mixing and aging of black carbon (BC) aerosols that allow for enhanced solar absorption of the BC is an important parameterization in climate models. Many climate models predict a factor of 2-3 lower aerosol absorption optical depth (AAOD) than the atmospheric columnar absorption observed from ground-based networks such as AERONET, likely because these models do not parameterize properly the BC absorption enhancement (E-MAC). Models that are configured with an internal mixing have predicted large variations of E-MAC, which are poorly constrained from ambient measurements. We determined the BC E-MAC from aerosol coatings with a two-step solvent experiment to remove both organic and inorganic coatings in ambient fine particulate matter (PM2.5). Observations in a rural North China site showed that the E-MAC varied from 1.4 to 3. The E-MAC increases simultaneously with SO42-/EC ratios, suggesting the photochemical production of sulfate coatings enhanced BC absorption. A global climate model, parameterized to account for these observational constraints, verifies that sulfates are primary drivers of the BC absorption enhancement in severely polluted area in China. This magnification of the radiative forcing of coated BC is stronger by a factor of similar to 2 than predicted by the standard parameterization (external mixing) in the climate model and is in better agreement with AERONET observations of AAOD. This result would be useful for testing the representation of solar absorption by BC-containing particles in the newer generation of climate models. Plain Language Summary Atmospheric black carbon (BC) or soot in fine particulate matter (PM2.5) is emitted from incomplete combustion of fossil fuel or biomass/biofuel. The BC is an important pollutant for both air quality and Earth's energy balance, and the BC radiative forcing maybe second only to that of CO2. The photochemical production of nonabsorbing secondary aerosols may create a coating on BC and may thereby act as a lens which may enhance the light absorption. However, this absorption enhancement is poorly constrained by ambient measurements, and thus the estimates of BC climate forcing remain highly uncertain. To this end, an aerosol filter dissolution-filtration (AFD) with two-step solvent dissolution protocol was employed to remove both organic and inorganic coatings and then investigate their effects on BC light absorption. The observations and model simulation showed that the BC warming effect likely doubled due to lens effect from secondary aerosols.
11.	Chen, Hans, 1988, et al. (författare) Interannual Arctic sea ice variability and associated winter weather patterns: A regional perspective for 1979–2014 2016 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-8996 .- 2169-897X. ; 121:24, s. 14433-14455 Tidskriftsartikel (refereegranskat)
12.	Chen, Hans W., et al. (författare) Evaluation of Regional CO2 Mole Fractions in the ECMWF CAMS Real-Time Atmospheric Analysis and NOAA CarbonTracker Near-Real-Time Reanalysis With Airborne Observations From ACT-America Field Campaigns 2019 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-8996 .- 2169-897X. ; 124:14, s. 8119-8133 Tidskriftsartikel (refereegranskat)abstract This study systematically examines the regional uncertainties and biases in carbon dioxide (CO2) mole fractions from two of the state-of-the-art global CO2 analysis products, namely, the Copernicus Atmosphere Monitoring Service (CAMS) real-time atmospheric analysis from the European Centre for Medium-Range Weather Forecasts (ECMWF) and the CarbonTracker Near-Real-Time (CT-NRT) reanalysis from the National Oceanic and Atmospheric Administration (NOAA), by evaluation against hundreds of hours of airborne in situ measurements from the summer 2016 and winter 2017 Atmospheric Carbon and Transport (ACT)-America field campaigns. Both the CAMS and CT-NRT analyses agree reasonably well with the independent ACT-America airborne CO2 measurements in the free troposphere, with root-mean-square deviations (RMSDs) between analyses and observations generally between 1 and 2 ppm but show considerably larger uncertainties in the atmospheric boundary layer where the RMSDs exceed 8 ppm in the lowermost 1 km of the troposphere in summer. There are strong variations in accuracy and bias between seasons, and across three different subregions in the United States (Mid-Atlantic, Midwest, and South), with the largest uncertainties in the Mid-Atlantic region in summer. Overall, the RMSDs of the CAMS and CT-NRT analyses against airborne data are comparable to each other and largely consistent with the differences between the two analyses. The current study provides uncertainty estimates for both analysis products over North America and suggests that these two independent estimates can be used to approximate regional CO2 analysis uncertainties. Both statistics are important in future studies in quantifying the uncertainties in regional CO2 mole fraction and flux estimates.
13.	Chiacchio, Marc, et al. (författare) Evaluation of the radiation budget with a regional climate model over Europe and inspection of dimming and brightening 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:5, s. 1951-1971 Tidskriftsartikel (refereegranskat)abstract Shortwave (SW) and longwave (LW) components of the radiation budget at the surface and top of atmosphere (TOA) are evaluated in the regional climate model RegCM version 4 driven by European Centre for Medium-Range Weather Forecasts Reanalysis over Europe. The simulated radiative components were evaluated with those from satellite-based products and reanalysis. At the surface the model overestimated the absorbed solar radiation but was compensated by a greater loss of thermal energy while both SW and LW TOA net fluxes were underestimated representing too little solar energy absorbed and too little outgoing thermal energy. Averaged biases in radiative parameters were generally within 25 Wm(-2), were dependent on differences by as much as 0.2 in cloud fraction, surface, and planetary albedo and less dependent on surface temperature associated with the surface longwave parameters, and are in line with other studies. Clear-sky fluxes showed better results when cloud cover differences had no influence. We also found a clear distinction between land versus water with smaller biases over land at the surface and over water at the TOA due to differences in cloud fraction and albedo. Finally, we inspected dimming and brightening for the period 1979-2010 with an indication for dimming early in the time series (i.e., 1979-1987) and brightening after, which agrees with surface-based observations. After 2000, however, a decrease in the brightening by more than 1 order of magnitude was evident which is in contrast to the continued brightening found in surface records and satellite-derived estimates.
14.	Chiacchio, Marc, et al. (författare) On the links between meteorological variables, aerosols, and tropical cyclone frequency in individual ocean basins 2017 Ingår i: Journal of Geophysical Research. - : American Geophysical Union (AGU). - 0148-0227 .- 2156-2202. ; 122:2, s. 802-822 Tidskriftsartikel (refereegranskat)abstract A generalized linear model based on Poisson regression has been used to assess the impact of environmental variables modulating tropical cyclone frequency in six main cyclone development areas: the East Pacific, West Pacific, North Atlantic, North Indian, South Indian, and South Pacific. The analysis covers the period 1980-2009 and focuses on widely used meteorological parameters including wind shear, sea surface temperature, and relative humidity from different reanalyses as well as aerosol optical depth for different compounds simulated by the Goddard Chemistry Aerosol Radiation and Transport model. Circulation indices are also included. Cyclone frequency is obtained from the International Best Track Archive for Climate Stewardship. A strong link is found between cyclone frequency and the relative sea surface temperature, Atlantic Meridional Mode, and wind shear with significant explained log likelihoods in the North Atlantic of 37%, 27%, and 28%, respectively. A significant impact of black carbon and organic aerosols on cyclone frequency is found over the North Indian Ocean, with explained log likelihoods of 27%. A weaker but still significant impact is found for observed dust aerosols in the North Atlantic with an explained log likelihood of 11%. Changes in lower stratospheric temperatures explain 28% of the log likelihood in the North Atlantic. Lower stratospheric temperatures from a subset of Coupled Model Intercomparison Project Phase 5 models properly simulate the warming and subsequent cooling of the lower stratosphere that follows a volcanic eruption but underestimates the cooling by about 0.5 degrees C.
15.	Fang, Wenzheng, et al. (författare) Dual-Isotope Constraints on Seasonally Resolved Source Fingerprinting of Black Carbon Aerosols in Sites of the Four Emission Hot Spot Regions of China 2018 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 123:20, s. 11735-11747 Tidskriftsartikel (refereegranskat)abstract Despite much recent efforts, the emission sources of black carbon (BC) aerosols. central input to understanding and predicting environmental and climate impact. remain highly uncertain. Here we present observational delta C-13/Delta C-14-based constraints on the sources of BC aerosols over the four seasons in each of the four key hot spot emission regions of China: Beijing-Tianjin-Hebei (BTH-Wuqing; where Wuqing is the sampling location), Yangtze River Delta (YRD-Haining), Pearl River Delta (PRD-Zhongshan), and Sichuan Basin (SC-Deyang). Overall, BC loadings were highest in winter, yet elevated loadings were also observed in other seasons, for example, spring at SC-Deyang and fall at PRD-Zhongshan. Annually, the dominant BC sources were coal (50 +/- 20%) for BTH-Wuqing, liquid fossil for YRD-Haining (46 +/- 8%) and PRD-Zhongshan (48 +/- 18%), whereas liquid fossil (42 +/- 17%) and biomass burning (41 +/- 14%) equally affected SC-Deyang. There is also different but distinct seasonalities in BC sources for the different sites. As an example, for BTH-Wuqing coal burning increased from summer to winter, while summer and spring BTH-Wuqing were more influenced by liquid fossil. In contrast, for YRD-Haining, the relative importance of emission sources was more constant over the year. These quantitative observational constraints on source-seasonality of BC aerosols in receptor sites located in China's four key economic zones highlight that regulatory control on BC aerosol emissions from different fuels should consider both seasonal and regional variations. Our results also suggest that models on estimates of BC-induced climate and air quality should consider variations over both regional and seasonal scales.
16.	Giamarelou, Maria, et al. (författare) Indirect evidence of the composition of nucleation mode atmospheric particles in the high Arctic 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:2, s. 965-975 Tidskriftsartikel (refereegranskat)abstract Previous long-term observations have shown that nanoparticle formation events are common in the summer-time high Arctic and linked to local photochemical activity. However, current knowledge is limited with respect to the chemical precursors of resulting nanoparticles and the compounds involved in their subsequent growth. Here we report case-study measurements during new particle formation (NPF) events of the particle size distribution (diameter>7nm) and for the first time the volatility of monodisperse particles having diameter 40nm, providing indirect information about their composition. Volatility measurements provide indirect evidence that a predominant fraction of the 12nm particle population is ammoniated sulfates in the summertime high Arctic. Our observations further suggest that the majority of the sub-40nm particle population during NPF events does not exist in the form of sulfuric acid but rather as partly or fully neutralized ammoniated sulfates.
17.	Groot Zwaaftink, C. D., et al. (författare) Substantial contribution of northern high-latitude sources to mineral dust in the Arctic 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:22, s. 13678-13697 Tidskriftsartikel (refereegranskat)abstract In the Arctic, impurities in the atmosphere and cryosphere can strongly affect the atmospheric radiation and surface energy balance. While black carbon has hence received much attention, mineral dust has been in the background. Mineral dust is not only transported into the Arctic from remote regions but also, possibly increasingly, generated in the region itself. Here we study mineral dust in the Arctic based on global transport model simulations. For this, we have developed a dust mobilization scheme in combination with the Lagrangian particle dispersion model FLEXPART. A model evaluation, based on measurements of surface concentrations and annual deposition at a number of stations and aircraft vertical profiles, shows the suitability of this model to study global dust transport. Simulations indicate that about 3% of global dust emission originates from high-latitude dust sources in the Arctic. Due to limited convection and enhanced efficiency of removal, dust emitted in these source regions is mostly deposited closer to the source than dust from for instance Asia or Africa. This leads to dominant contributions of local dust sources to total surface dust concentrations (similar to 85%) and dust deposition (similar to 90%) in the Arctic region. Dust deposition from local sources peaks in autumn, while dust deposition from remote sources occurs mainly in spring in the Arctic. With increasing altitude, remote sources become more important for dust concentrations as well as deposition. Therefore, total atmospheric dust loads in the Arctic are strongly influenced by Asian (similar to 38%) and African (similar to 32%) dust, whereas local dust contributes only 27%. Dust loads are thus largest in spring when remote dust is efficiently transported into the Arctic. Overall, our study shows that contributions of local dust sources are more important in the Arctic than previously thought, particularly with respect to surface concentrations and dust deposition.
18.	Hallquist, Åsa, et al. (författare) Characterization of Aerosol Aging Potentials at Suburban Sites in Northern and Southern China Utilizing a Potential Aerosol Mass (Go:PAM) Reactor and an Aerosol Mass Spectrometer. 2019 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 214:10, s. 5629-5649 Tidskriftsartikel (refereegranskat)
19.	Hare, B. M., et al. (författare) LOFAR Lightning Imaging : Mapping Lightning With Nanosecond Precision 2018 Ingår i: Journal of Geophysical Research - Atmospheres. - : American Geophysical Union (AGU). - 2169-897X .- 2169-8996. ; 123:5, s. 2861-2876 Tidskriftsartikel (refereegranskat)abstract Lightning mapping technology has proven instrumental in understanding lightning. In this work we present a pipeline that can use lightning observed by the LOw-Frequency ARray (LOFAR) radio telescope to construct a 3-D map of the flash. We show that LOFAR has unparalleled precision, on the order of meters, even for lightning flashes that are over 20km outside the area enclosed by LOFAR antennas (approximate to 3,200km(2)), and can potentially locate over 10,000 sources per lightning flash. We also show that LOFAR is the first lightning mapping system that is sensitive to the spatial structure of the electrical current during individual lightning leader steps.
20.	He, Lixia, et al. (författare) An Analysis of Current and Electric Field Pulses Associated With Upward Negative Lightning Flashes Initiated from the Santis Tower 2018 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 123:8, s. 4045-4059 Tidskriftsartikel (refereegranskat)abstract We present a study on the characteristics of current and electric field pulses associated with upward lightning flashes initiated from the instrumented Santis Tower in Switzerland. The electric field was measured 15km from the tower. Upward flashes always begin with the initial stage composed of the upward-leader phase and the initial-continuous-current (ICC) phase. Four types of current pulses are identified and analyzed in the paper: (1) return-stroke pulses, which occur after the extinction of the ICC and are preceded by essentially no-current time intervals; (2) mixed-mode ICC pulses, defined as fast pulses superimposed on the ICC, which have characteristics very similar to those of return strokes and are believed to be associated with the reactivation of a decayed branch or the connection of a newly created channel to the ICC-carrying channel at relatively small junction heights; (3) classical M-component pulses superimposed on the continuing current following some return strokes; and (4) M-component-type ICC pulses, presumably associated with the reactivation of a decayed branch or the connection of a newly created channel to the ICC-carrying channel at relatively large junction heights. We consider a data set consisting of 9 return-stroke pulses, 70 mixed-mode ICC pulses, 11 classical M-component pulses, and 19 M-component-type ICC pulses (a total of 109 pulses). The salient characteristics of the current and field waveforms are analyzed. A new criterion is proposed to distinguish between mixed-mode and M-component-type pulses, which is based on the current waveform features. The characteristics of M-component-type pulses during the initial stage are found to be similar to those of classical M-component pulses occurring during the continuing current after some return strokes. It is also found that about 41% of mixed-mode ICC pulses were preceded by microsecond-scale pulses occurring in electric field records some hundreds of microseconds prior to the onset of the current, very similar to microsecond-scale electric field pulses observed for M-component-type ICC pulses and which can be attributed to the junction of an in-cloud leader channel to the current-carrying channel to ground. Classical M-component pulses and M-component-type ICC pulses tend to have larger risetimes ranging from 6.3 to 430s. On the other hand, return-stroke pulses and mixed-mode ICC pulses have current risetimes ranging from 0.5 to 28s. Finally, our data suggest that the 8-s criterion for the current risetime proposed by Flache et al. is a reasonable tool to distinguish between return strokes and classical M-components. However, mixed-mode ICC pulses superimposed on the ICC can sometimes have considerably longer risetimes, up to about 28s, as observed in this study.
21.	He, Lixia, et al. (författare) Electromagnetic Fields Associated With the M-Component Mode of Charge Transfer 2019 Ingår i: Journal of Geophysical Research - Atmospheres. - : AMER GEOPHYSICAL UNION. - 2169-897X .- 2169-8996. ; 124:13, s. 6791-6809 Tidskriftsartikel (refereegranskat)abstract In upward flashes, charge transfer to ground largely takes place during the initial continuous current (ICC) and its superimposed pulses (ICC pulses). ICC pulses can be associated with either M-component or leader/return-stroke-like modes of charge transfer to ground. In the latter case, the downward leader/return stroke process is believed to take place in a decayed branch or a newly created channel connected to the ICC-carrying channel at relatively short distance from the tower top, resulting in the so-called mixed mode of charge transfer to ground. In this paper, we study the electromagnetic fields associated with the M-component charge transfer mode using simultaneous records of electric fields and currents associated with upward flashes initiated from the Santis Tower. The effect of the mountainous terrain on the propagation of electromagnetic fields associated with the M-component charge transfer mode (including classical M-component pulses and M-component-type pulses superimposed on the initial continuous current) is analyzed and compared with its effect on the fields associated with the return stroke (occurring after the extinction of the ICC) and mixed charge transfer modes. For the analysis, we use a 2-Dimentional Finite-Difference Time Domain method, in which the M-component is modeled by the superposition of a downward current wave and an upward current wave resulting from the reflection at the bottom of the lightning channel (Rakov et al., 1995, model) and the return stroke and mixed mode are modeled adopting the MTLE (Modified Transmission Line with Exponential Current Decay with Height) model. The finite ground conductivity and the mountainous propagation terrain between the Santis Tower and the field sensor located 15 km away at Herisau are taken into account. The effects of the mountainous path on the electromagnetic fields are examined for classical M-component and M-component-type ICC pulses. Use is made of the propagation factors defined as the ratio of the electric or magnetic field peak evaluated along the mountainous terrain to the field peak evaluated for a flat terrain. The velocity of the M-component pulse is found to have a significant effect on the risetime of the electromagnetic fields. A faster traveling wave speed results in larger peaks for the magnetic field. However, the peak of the electric field appears to be insensitive to the M-component wave speed. This can be explained by the fact that at 15 km, the electric field is still dominated by the static component, which mainly depends on the overall transferred charge. The contribution of the radiation component to the M-component fields at 100 km accounts for about 77% of the peak electric field and 81% of the peak magnetic field, considerably lower compared to the contribution of the radiation component to the return stroke fields at the same distance. The simulation results show that neither the electric nor the magnetic field propagation factors are very sensitive to the risetimes of the current pulses. However, the results indicate a high variability of the propagation factors as a function of the branch-to-channel junction point height. For junction point heights of about 1 km, the propagation factors reach a value of about 1.6 for the E-field and 1.9 for the H-field. For a junction height greater than 6 km, the E-field factor becomes slightly lower than 1. The obtained results are consistent with the findings of Li, Azadifar, Rachidi, Rubinstein, Paolone, et al. (2016, ) in which an electric field propagation factor of 1. 8 was inferred for return strokes and mixed-mode pulses, considering that junction points lower than 1 km or so would result in a mixed mode of charge transfer, in which a downward leader/return-stroke-like process is believed to take place. It is also found that the field enhancement (propagation factor) for return stroke mode is higher for larger ground conductivities. Furthermore, the enhancement effect tends to decrease with increasing current risetime, except for very short risetimes (less than 2.5 mu s or so) for which the tendency reverses. Finally, model-predicted fields associated with different charge transfer modes, namely, return stroke, mixed-mode, classical M-component, and M-component-type ICC pulse are compared with experimental observations at the Santis Tower. It is found that the vertical electric field waveforms computed considering the mountainous terrain are in very good agreement with the observed data. The adopted parameters of the models that provide the best match with the measured field waveforms were consistent with observations. The values for the current decay height constant adopted in the return stroke and mixed-mode models (1.0 km for the return stroke and 0.8 km for the mixed-mode pulse) are lower than the value of 2.0 km typically used in the literature.
22.	Höpner, Friederike, et al. (författare) Investigation of Two Optical Methods for Aerosol‐Type Classification Extended to a Northern Indian Ocean Site 2019 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 124:15, s. 8743-8763 Tidskriftsartikel (refereegranskat)abstract Methods for determining aerosol types in cases where chemical composition measurements are not available are useful for improved aerosol radiative forcing estimates. In this study, two aerosol characterization methods by Cazorla et al. (2013, https://doi.org/10.5194/acp-13-9337-2013; CA13) and Costabile et al. (2013, https://doi.org/10.5194/acp-13-2455-2013; CO13) using wavelength‐dependent particle absorption and scattering are used, to assess their applicability and examine their limitations. Long‐term ambient particle optical property and chemical composition (major inorganic ions and bulk carbon) measurements from the Maldives Climate Observatory Hanimaadhoo as well as concurrent air mass trajectories are utilized to test the classifications based on the determined absorption Ångström exponent, scattering Ångström exponent, and single scattering albedo. The resulting aerosol types from the CA13 method show a good qualitative agreement with the particle chemical composition and air mass origin. In general, the size differentiation using the scattering Ångström exponent works very well for both methods, while the composition identification depending mainly on the absorption Ångström exponent can result in aerosol misclassifications at Maldives Climate Observatory Hanimaadhoo. To broaden the applicability of the CA13 method, we suggest to include an underlying marine aerosol group in the classification scheme. The classification of the CO13 method is less clear, and its applicability is limited when it is extended to aerosols in this environment at ambient humidity.
23.	Isoz, Oscar, et al. (författare) Intercalibration of microwave temperature sounders using radio occultation measurements 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:9, s. 3758-3773 Tidskriftsartikel (refereegranskat)abstract This is a study of the usefulness of radio occultation (RO) data for intercomparing different microwave temperature (MWT) sounding instruments. The RO data used are from the Global Navigational Satellite System Receiver for Atmospheric Sounding on the Metop-A and B satellites. The MWT sounders investigated are the Advanced Microwave Sounding Unit-A instruments on the satellites NOAA 15, 16, and 18 and Metop-A. We collocate RO and MWT data and then use these collocations to study various aspects of the MWT instruments. In addition, two different versions of the MWT data are compared: standard operational data (OPR) and the NOAA Integrated Microwave Intercalibration Approach data (IMICA). The time series of monthly mean differences shows that there are robust patterns for each satellite and data version, which mostly drift only slowly over time. The intersatellite spread, measured by the standard deviation of the yearly mean values by all satellites, is between 0.1 and 0.4 K, depending on channel, with no significant differences between OPR and IMICA data. The only notable exception is Channel 8 of NOAA 16, which appears to have a time-varying offset of 0.5–1 K relative to the other instruments. At this point it is not clear whether this deviation is real or a sampling artifact, so further study is needed. Due to the large number of collocations used, it is possible to also investigate the scene brightness and scan angle dependence of the MWT bias (relative to RO). First results of such an analysis are presented and discussed. Particularly, the investigation of the scan angle dependence is novel, since this bias pattern is difficult to assess without RO data. Further work is needed on these angular dependences, before conclusions are robust enough to include in data recalibration efforts, but our overall conclusion is that RO collocations are a powerful tool for intercomparing MWT sounders.
24.	Koike, M., et al. (författare) Year-Round In Situ Measurements of Arctic Low-Level Clouds : Microphysical Properties and Their Relationships With Aerosols 2019 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 124:3, s. 1798-1822 Tidskriftsartikel (refereegranskat)abstract Two years of continuous in situ measurements of Arctic low-level clouds have been made at the Mount Zeppelin Observatory (78 degrees 56N, 11 degrees 53E), in Ny-angstrom lesund, Spitsbergen. The monthly median value of the cloud particle number concentration (N-c) showed a clear seasonal variation: Its maximum appeared in May-July (658cm(-3)), and it remained low between October and March (87cm(-3)). At temperatures warmer than 0 degrees C, a clear correlation was found between the hourly N-c values and the number concentrations of aerosols with dry diameters larger than 70nm (N-70), which are proxies for cloud condensation nuclei (CCN). When clouds were detected at temperatures colder than 0 degrees C, some of the data followed the summertime N-c to N-70 relationship, while other data showed systematically lower N-c values. The lidar-derived depolarization ratios suggested that the former (CCN-controlled) and latter (CCN-uncontrolled) data generally corresponded to clouds consisting of supercooled water droplets and those containing ice particles, respectively. The CCN-controlled data persistently appeared throughout the year at Zeppelin. The aerosol-cloud interaction index (ACI=dlnN(c)/(3dlnN(70))) for the CCN-controlled data showed high sensitivities to aerosols both in the summer (clean air) and winter-spring (Arctic haze) seasons (0.220.03 and 0.250.02, respectively). The air parcel model calculations generally reproduced these values. The threshold diameters of aerosol activation (D-act), which account for the N-c of the CCN-controlled data, were as low as 30-50nm when N-70 was less than 30cm(-3), suggesting that new particle formation can affect Arctic cloud microphysics.
25.	Li, J. J., et al. (författare) Characterization of Aerosol Aging Potentials at Suburban Sites in Northern and Southern China Utilizing a Potential Aerosol Mass (Go:PAM) Reactor and an Aerosol Mass Spectrometer 2019 Ingår i: Journal of Geophysical Research-Atmospheres. - : American Geophysical Union (AGU). - 2169-897X .- 2169-8996. ; 124:10, s. 5629-5649 Tidskriftsartikel (refereegranskat)abstract Aerosol mass spectrometry was used to characterize submicron aerosols before and after aging in a Gothenburg Potential Aerosol Mass (Go:PAM) reactor at two suburban sites in China, one in northern China at Changping (CP), Beijing, and a second in southern China at Hong Kong (HK). Organic aerosol (OA) dominated in the ambient nonrefractory particulate matter <1m (NR-PM1) for both CP (42-71%) and HK (43-61%), with a large contribution from secondary OA factors that were semivolatile oxygenated (SVOOA) and low-volatility oxygenated (LVOOA). Under constant OH exposure, OA enhancement (78-98%) dominated the NR-PM1 mass increment at both sites, while nitrate was enhanced the most among the inorganic species (7-9%). Overall, the CP site exhibited higher OA oxidation potential and more enhancement of SVOOA than LVOOA (7.5 vs. 2.7g/m(3)), but the reverse was observed in HK (0.8 vs. 2.6g/m(3)). In CP, more enhancement of the less oxygenated SVOOA suggests that aerosol aging was more sensitive to the abundant locally emitted primary OA and volatile organic compound precursors. On the contrary, the more formation of the highly oxidized LVOOA in HK indicates that aerosol aging mainly escalated the degree of oxygenation of OA as ambient aerosol was already quite aged and there was a lack of volatile organic compound precursors. The comparative measurements using the same oxidation system reveal distinct key factors and mechanisms that influence secondary aerosol formation in two suburban locations in China, providing scientific insights to assist formulation of location-specific mitigation measures of secondary pollution. Plain Language Summary Atmospheric submicron particles have significant impacts on the climate and human health. A large part of these particles are formed secondarily through successive aging of primary emissions. To study such aging processes, we used a reactor that can provide highly oxidizing conditions to simulate the oxidation of ambient aerosols at accelerated rates. An online mass spectrometer was connected after the reactor to measure changes in aerosol mass concentration and chemical composition between the ambient samples and the oxidized ones. We presented the first comparative measurements of the aging potentials of ambient aerosols in two suburban sites in northern and southern China (Changping District in Beijing, and Hong Kong). Results showed that generally aerosols at the Changping site had higher aging potentials after passing through the oxidation reactor, probably due to more local emissions of precursors, while air masses in Hong Kong were already in a higher oxidation state with lower aging potentials, mainly because of strong impacts from long-range transported pollution sources. Distinct aerosol aging pathways related to different ambient precursors were observed at the two sites. Understanding of the different characteristics of aerosol aging processes can lead to advances in air quality modeling and pollution management.
26.	Li, Ying, et al. (författare) Atmospheric Water Transport to the Endorheic Tibetan Plateau and Its Effect on the Hydrological Status in the Region 2019 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-897X .- 2169-8996. ; 124:23, s. 12864-12881 Tidskriftsartikel (refereegranskat)abstract ©2019. American Geophysical Union. All Rights Reserved. The endorheic Tibetan Plateau (ETP), which consists of all the endorheic basins of the Tibetan Plateau (TP), has exhibited an overall mass gain in recent decades. However, the role played by atmospheric water (AW) transport on the hydrological status over the ETP is poorly understood. In this study, the AW source to the ETP was tracked with the Water Accounting Model-2 layers (WAM-2) and AW transport to the ETP through its boundaries was quantified, with three reanalysis products (ERA-I, MERRA-2, and JRA-55) during 1979/1980–2015. It is found that total AW input to the ETP is about 13–25%, 59–71%, 10–13%, and 3–7% of mean annual totals in spring, summer, autumn, and winter, respectively. At annual scales, the AW source from land (52–54%) dominates the AW contribution to the ETP, while local recycling of AW over the ETP accounts for about 17–22% of the mean annual total AW contribution. Increased precipitation over the ETP during 1979–2015 was mostly attributed to the significantly increased AW contribution from the Indian Ocean, especially from increased AW inputs transported from the western and southern boundaries in summer. Comparisons between the AW budget and terrestrial water storage changes indicate that the AW budget change over the ETP modulated the variations of terrestrial water storage change during 2002–2014 and annual lake mass change during 1989–2015.
27.	Maldonado, Tito, et al. (författare) The role of the meridional sea surface temperature gradient in controlling the Caribbean low-level jet 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:11, s. 5903-5916 Tidskriftsartikel (refereegranskat)abstract The Caribbean low-level jet (CLLJ) is an important modulator of regional climate, especially precipitation, in the Caribbean and Central America. Previous work has inferred, due to their semiannual cycle, an association between CLLJ strength and meridional sea surface temperature (SST) gradients in the Caribbean Sea, suggesting that the SST gradients may control the intensity and vertical shear of the CLLJ. In addition, both the horizontal and vertical structure of the jet have been related to topographic effects via interaction with the mountains in Northern South America (NSA), including funneling effects and changes in the meridional geopotential gradient. Here we test these hypotheses, using an atmospheric general circulation model to perform a set of sensitivity experiments to examine the impact of both SST gradients and topography on the CLLJ. In one sensitivity experiment, we remove the meridional SST gradient over the Caribbean Sea and in the other, we flatten the mountains over NSA. Our results show that the SST gradient and topography have little or no impact on the jet intensity, vertical, and horizontal wind shears, contrary to previous works. However, our findings do not discount a possible one-way coupling between the SST and the wind over the Caribbean Sea through friction force. We also examined an alternative approach based on barotropic instability to understand the CLLJ intensity, vertical, and horizontal wind shears. Our results show that the current hypothesis about the CLLJ must be reviewed in order to fully understand the atmospheric dynamics governing the Caribbean region.
28.	Mccoy, D. T., et al. (författare) The global aerosol-cloud first indirect effect estimated using MODIS, MERRA, and AeroCom 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:3, s. 1779-1796 Tidskriftsartikel (refereegranskat)abstract Aerosol-cloud interactions (ACI) represent a significant source of forcing uncertainty in global climate models (GCMs). Estimates of radiative forcing due to ACI in Fifth Assessment Report range from -0.5 to -2.5 W m(-2). A portion of this uncertainty is related to the first indirect, or Twomey, effect whereby aerosols act as nuclei for cloud droplets to condense upon. At constant liquid water content this increases the number of cloud droplets (Nd) and thus increases the cloud albedo. In this study we use remote-sensing estimates of Nd within stratocumulus regions in combination with state-of-the-art aerosol reanalysis from Modern-Era Retrospective Analysis for Research and Applications version 2 (MERRA2) to diagnose how aerosols affect Nd. As in previous studies, Nd is related to sulfate mass through a power law relationship. The slope of the log-log relationship between Nd and SO4 in maritime stratocumulus is found to be 0.31, which is similar to the range of 0.2-0.8 from previous in situ studies and remote-sensing studies in the pristine Southern Ocean. Using preindustrial emissions models, the change in Nd between preindustrial and present day is estimated. Nd is inferred to have more than tripled in some regions. Cloud properties from Moderate Resolution Imaging Spectroradiometer (MODIS) are used to estimate the radiative forcing due to this change in Nd. The Twomey effect operating in isolation is estimated to create a radiative forcing of -0.97 +/- 0.23 W m(-2) relative to the preindustrial era.
29.	Messori, Gabriele, et al. (författare) On double Rossby wave breaking in the North Atlantic 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:21, s. 11129-11150 Tidskriftsartikel (refereegranskat)abstract We discuss the dynamical features associated with double Rossby wave breaking (DWB, concurrent cyclonic and anticyclonic breakings) over the North Atlantic, with a focus on the North Atlantic Oscillation (NAO), the midlatitude jet stream, and surface wind extremes over continental Europe. Objective automated algorithms for detecting wave breaking and determining the location, intensity, and direction of the jet are adopted. The analysis is performed on the European Centre for Medium-Range Weather Forecasts ERA-Interim reanalysis and the Max Planck Institute Earth System Model (MPI-ESM). We find that DWB events can project onto both phases of the NAO, albeit showing no strong preference for either. Wave-breaking pairs occurring in the northern North Atlantic project onto the positive NAO, while the opposite holds for pairs occurring farther south. DWB also affects the direction and intensity of the jet stream. Events in the eastern half of the basin (EWB) intensify and zonalize the jet, while events farther to the west (WWB) weaken the westerly flow over Europe. An analysis of destructive wind storms over Europe in the last three decades suggests that these are typically associated with a very intense, zonal jet-similar to the case of EWB. Indeed, EWB corresponds to an enhanced likelihood of destructive windstorms over the continent, although there is not a one-to-one correspondence. The MPI-ESMmodel does not capture this statistical relationship. On the contrary, WWB corresponds to a decreased likelihood of destructive weather.
30.	Modini, R. L., et al. (författare) Primary marine aerosol-cloud interactions off the coast of California 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:9, s. 4282-4303 Tidskriftsartikel (refereegranskat)abstract Primary marine aerosol (PMA)-cloud interactions off the coast of California were investigated using observations of marine aerosol, cloud condensation nuclei (CCN), and stratocumulus clouds during the Eastern Pacific Emitted Aerosol Cloud Experiment (E-PEACE) and the Stratocumulus Observations of Los-Angeles Emissions Derived Aerosol-Droplets (SOLEDAD) studies. Based on recently reported measurements of PMA size distributions, a constrained lognormal-mode-fitting procedure was devised to isolate PMA number size distributions from total aerosol size distributions and applied to E-PEACE measurements. During the 12 day E-PEACE cruise on the R/V Point Sur, PMA typically contributed less than 15% of total particle concentrations. PMA number concentrations averaged 12 cm(-3) during a relatively calmer period (average wind speed 12m/s(1)) lasting 8 days, and 71cm(-3) during a period of higher wind speeds (average 16m/s(1)) lasting 5 days. On average, PMA contributed less than 10% of total CCN at supersaturations up to 0.9% during the calmer period; however, during the higher wind speed period, PMA comprised 5-63% of CCN (average 16-28%) at supersaturations less than 0.3%. Sea salt was measured directly in the dried residuals of cloud droplets during the SOLEDAD study. The mass fractions of sea salt in the residuals averaged 12 to 24% during three cloud events. Comparing the marine stratocumulus clouds sampled in the two campaigns, measured peak supersaturations were 0.20.04% during E-PEACE and 0.05-0.1% during SOLEDAD. The available measurements show that cloud droplet number concentrations increased with >100 nm particles in E-PEACE but decreased in the three SOLEDAD cloud events.
31.	Moeller, Marco, et al. (författare) Adjustment of regional climate model output for modeling the climatic mass balance of all glaciers on Svalbard 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:10, s. 5411-5429 Tidskriftsartikel (refereegranskat)abstract Large-scale modeling of glacier mass balance relies often on the output from regional climate models (RCMs). However, the limited accuracy and spatial resolution of RCM output pose limitations on mass balance simulations at subregional or local scales. Moreover, RCM output is still rarely available over larger regions or for longer time periods. This study evaluates the extent to which it is possible to derive reliable region-wide glacier mass balance estimates, using coarse resolution (10 km) RCM output for model forcing. Our data cover the entire Svalbard archipelago over one decade. To calculate mass balance, we use an index-based model. Model parameters are not calibrated, but the RCM air temperature and precipitation fields are adjusted using in situ mass balance measurements as reference. We compare two different calibration methods: root mean square error minimization and regression optimization. The obtained air temperature shifts (+1.43 degrees C versus +2.22 degrees C) and precipitation scaling factors (1.23 versus 1.86) differ considerably between the two methods, which we attribute to inhomogeneities in the spatiotemporal distribution of the reference data. Our modeling suggests a mean annual climatic mass balance of -0.05 +/- 0.40 mw.e.a(-1) for Svalbard over 2000-2011 and a mean equilibrium line altitude of 452 +/- 200m above sea level. We find that the limited spatial resolution of the RCM forcing with respect to real surface topography and the usage of spatially homogeneous RCM output adjustments and mass balance model parameters are responsible for much of the modeling uncertainty. Sensitivity of the results to model parameter uncertainty is comparably small and of minor importance.
32.	Murphy, Benjamin N., et al. (författare) Organic aerosol processing in tropical deep convective clouds : Development of a new model (CRM-ORG) and implications for sources of particle number 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:19, s. 10,441-10,464 Tidskriftsartikel (refereegranskat)abstract The difficulty in assessing interactions between atmospheric particles and clouds is due in part to the chemical complexity of the particles and to the wide range of length and timescales of processes occurring simultaneously during a cloud event. The new Cloud-Resolving Model with Organics (CRM-ORG) addresses these interactions by explicitly predicting the formation, transport, uptake, and re-release of surrogate organic compounds consistent with the volatility basis set framework within a nonhydrostatic, three-dimensional cloud-resolving model. CRM-ORG incorporates photochemical production, explicit condensation/evaporation of organic and inorganic vapors, and a comprehensive set of four different mechanisms describing particle formation from organic vapors and sulfuric acid. We simulate two deep convective cloud events over the Amazon rain forest in March 1998 and compare modeled particle size distributions with airborne observations made during the time period. The model predictions agree well with the observations for Aitken mode particles in the convective outflow (10-14 km) but underpredict nucleation mode particles by a factor of 20. A strong in-cloud particle formation process from organic vapors alone is necessary to reproduce even relatively low ultrafine particle number concentrations (similar to 1500 cm(-3)). Sensitivity tests with variable initial aerosol loading and initial vertical aerosol profile demonstrate the complexity of particle redistribution and net gain or loss in the cloud. In-cloud particle number concentrations could be enhanced by as much as a factor of 3 over the base case simulation in the cloud outflow but were never reduced by more than a factor of 2 lower than the base. Additional sensitivity cases emphasize the need for constrained estimates of surface tension and affinity of organic vapors to ice surfaces. When temperature-dependent organic surface tension is introduced to the new particle formation mechanisms, the number concentration of particles decreases by 60% in the cloud outflow. These uncertainties are discussed in light of the other prominent challenges for understanding the interactions between organic aerosols and clouds. Recommendations for future theoretical, laboratory, and field work are proposed.
33.	Olenius, Tinja, et al. (författare) New particle formation from sulfuric acid and amines : Comparison of monomethylamine, dimethylamine, and trimethylamine 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:13, s. 7103-7118 Tidskriftsartikel (refereegranskat)abstract Amines are bases that originate from both anthropogenic and natural sources, and they are recognized as candidates to participate in atmospheric aerosol particle formation together with sulfuric acid. Monomethylamine, dimethylamine, and trimethylamine (MMA, DMA, and TMA, respectively) have been shown to enhance sulfuric acid-driven particle formation more efficiently than ammonia, but both theory and laboratory experiments suggest that there are differences in their enhancing potentials. However, as quantitative concentrations and thermochemical properties of different amines remain relatively uncertain, and also for computational reasons, the compounds have been treated as a single surrogate amine species in large-scale modeling studies. In this work, the differences and similarities of MMA, DMA, and TMA are studied by simulations of molecular cluster formation from sulfuric acid, water, and each of the three amines. Quantum chemistry-based cluster evaporation rate constants are applied in a cluster population dynamics model to yield cluster concentrations and formation rates at boundary layer conditions. While there are differences, for instance, in the clustering mechanisms and cluster hygroscopicity for the three amines, DMA and TMA can be approximated as a lumped species. Formation of nanometer-sized particles and its dependence on ambient conditions is roughly similar for these two: both efficiently form clusters with sulfuric acid, and cluster formation is rather insensitive to changes in temperature and relative humidity. Particle formation from sulfuric acid and MMA is weaker and significantly more sensitive to ambient conditions. Therefore, merging MMA together with DMA and TMA introduces inaccuracies in sulfuric acid-amine particle formation schemes.
34.	Olenius, Tinja, et al. (författare) New particle formation from sulfuric acid and amines : Comparison of monomethylamine, dimethylamine, and trimethylamine 2017 Ingår i: Journal of Geophysical Research-Atmospheres. - : American Geophysical Union (AGU). - 2169-897X .- 2169-8996. ; 122:13, s. 7103-7118 Tidskriftsartikel (refereegranskat)
35.	Oyabu, Ikumi, et al. (författare) Chemical compositions of solid particles present in the Greenland NEEM ice core over the last 110,000 years 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:18, s. 9789-9813 Tidskriftsartikel (refereegranskat)abstract This study reports the chemical composition of particles present along Greenland's North Greenland Eemian Ice Drilling (NEEM) ice core, back to 110,000years before present. Insoluble and soluble particles larger than 0.45 mu m were extracted from the ice core by ice sublimation, and their chemical composition was analyzed using scanning electron microscope and energy dispersive X-ray spectroscopy and micro-Raman spectroscopy. We show that the dominant insoluble components are silicates, whereas NaCl, Na2SO4, CaSO4, and CaCO3 represent major soluble salts. For the first time, particles of CaMg(CO3)(2) and Ca(NO3)(2)center dot 4H(2)O are identified in a Greenland ice core. The chemical speciation of salts varies with past climatic conditions. Whereas the fraction of Na salts (NaCl+Na2SO4) exceeds that of Ca salts (CaSO4+CaCO3) during the Holocene (0.6-11.7kyr B.P.), the two fractions are similar during the BOlling-AllerOd period (12.9-14.6kyr B.P.). During cold climate such as over the Younger Dryas (12.0-12.6kyr B.P.) and the Last Glacial Maximum (15.0-26.9kyr B.P.), the fraction of Ca salts exceeds that of Na salts, showing that the most abundant ion generally controls the salt budget in each period. High-resolution analyses reveal changing particle compositions: those in Holocene ice show seasonal changes, and those in LGM ice show a difference between cloudy bands and clear layers, which again can be largely explained by the availability of ionic components in the atmospheric aerosol body of air masses reaching Greenland.
36.	Pedersen, C. A., et al. (författare) In situ observations of black carbon in snow and the corresponding spectral surface albedo reduction 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:4, s. 1476-1489 Tidskriftsartikel (refereegranskat)abstract Black carbon (BC) particles emitted from incomplete combustion of fossil fuel and biomass and deposited on snow and ice darken the surface and reduce the surface albedo. Even small initial surface albedo reductions may have larger adjusted effects due to snow morphology changes and changes in the sublimation and snow melt rate. Most of the literature on the effect of BC on snow surface albedo is based on numerical models, and few in situ field measurements exist to confirm this reduction. Here we present an extensive set of concurrent in situ measurements of spectral surface albedo, BC concentrations in the upper 5 cm of the snowpack, snow physical parameters (grain size and depth), and incident solar flux characteristics from the Arctic. From this data set (with median BC concentrations ranging from 5 to 137 ng BC per gram of snow) we are able to separate the BC signature on the snow albedo from the natural snow variability. Our measurements show a significant correlation between BC in snow and spectral surface albedo. Based on these measurements, parameterizations are provided, relating the snow albedo, as a function of wavelength, to the equivalent BC content in the snowpack. The term equivalent BC used here is the elemental carbon concentration inferred from the thermo-optical method adjusted for the fraction of non-BC constituents absorbing sunlight in the snow. The first parameterization is a simple equation which efficiently describes the snow albedo reduction due to the equivalent BC without including details on the snow or BC microphysics. This can be used in models when a simplified description is needed. A second parameterization, including snow grain size information, shows enhanced correspondence with the measurements. The extracted parameterizations are valid for wavelength bands 400-900 nm, constrained for BC concentrations between 1 and 400 ng g(-1), and for an optically thick snowpack. The parameterizations are purely empirical, and particular focus was on the uncertainties associated with the measurements, and how these uncertainties propagate in the parameterizations. Integrated, the first parameterization (based only on the equivalent BC) gives a broadband (400-900 nm) snow albedo reduction of 0.004 due to 10 ng equivalent BC per gram of snow, while the effect is almost 5 times larger for BC concentrations 1 order of magnitude higher. The study shows that the reconstructed albedo from the second parameterization (including information on the snow grain size) corresponds better to the radiative transfer model Snow, Ice, and Aerosol Radiation albedo than the reconstructed albedo from the first parameterization (excluding grain size information).
37.	Qi, Wei, et al. (författare) Evaluations and Improvements of GLDAS2.0 and GLDAS2.1 Forcing Data's Applicability for Basin Scale Hydrological Simulations in the Tibetan Plateau 2018 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-897X .- 2169-8996. ; 123:23 Tidskriftsartikel (refereegranskat)abstract ©2018. The Authors. Hydroclimatic data are of importance to understand the water cycle and therefore for water resource assessment. Such data are of paramount importance for the Tibetan Plateau (TP), which is the source region of several large rivers in Asia. The Global Land Data Assimilation System (GLDAS) 2.0 and 2.1 provide abundant fine resolution hydroclimatic data. However, evaluations on their applicability have not been carried out for the TP. This study aims to evaluate and improve their applicability in basin-scale hydrological applications in the TP. Gauge-based data, a hydrological model including biosphere and seven state-of-the-art global precipitation products are utilized to carry out the study in four large basins in the TP. We find that GLDAS2.1 shows significant warming trends from 2001 to 2010, whereas GLDAS2.0 shows cooling trends, although only significant in the Upper Yellow River basin. The contrasting trends imply that caution should be taken when using them to analyze climate change impacts. On a monthly scale, GLDAS2.1 precipitation on average is closer to the gauge-based data than GLDAS2.0, but both of them have high uncertainty. Therefore, further quality improvements in precipitation are of importance. We also find CMORPH-BLD has better performance than other products in terms of Nash-Sutcliffe Efficiency (NSE), Relative Bias (RB), and root-mean-square error. Combining CMORPH-BLD with GLDAS2.0 forcing data generates more realistic runoff simulation than GLDAS2.1, with NSE and RB being 0.85 and 16% on average. The results provide unique insights into the studied data and are beneficial for water resource assessment in the TP.
38.	Salih, Abubakr A. M., et al. (författare) Lagrangian tracing of Sahelian Sudan moisture sources 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:14, s. 6793-6808 Tidskriftsartikel (refereegranskat)abstract The Sahelian Sudan is an arid to semiarid region that depends on the seasonal rainfall as the main source of water, but its rainfall has large interannual variability. Such dry regions usually have their main moisture sources elsewhere; thus, the rainfall variability is directly related to the moisture transport. This study seeks to identify source regions of water vapor for Sahelian Sudan during the monsoon period, from July to September. We have used the Lagrangian trajectory model FLEXPART driven by ERA-Interim reanalysis for the time period 1998 to 2008. The results show that most of the air masses that reach this region during the monsoon period have their major origins over the Arabian Peninsula, Central Africa, or are associated with the tropical easterly jet. Flow associated with Intertropical Convergence Zone contributes almost half of the total precipitated water; most of it comes from Central Africa. This suggests that moisture recycling is the major contributor, compared to Oceanic sources. The flows from the northeast (Arabian Peninsula and north Asia) and east (Horn of Africa and north Indian Ocean) contribute about one third of the precipitated water. The rest of precipitated water comes from the Mediterranean, subtropical Atlantic, and western Sahel, all with smaller contribution. Our results also indicate that different subregions of Sahelian Sudan have different moisture sources. Such result needs to be taken into account in seasonal forecasting practices.
39.	Salih, Abubakr A. M., et al. (författare) Sources of Sahelian-Sudan moisture : Insights from a moisture-tracing atmospheric model 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:13, s. 7819-7832 Tidskriftsartikel (refereegranskat)abstract The summer rainfall across Sahelian-Sudan is one of the main sources of water for agriculture, human, and animal needs. However, the rainfall is characterized by large interannual variability, which has attracted extensive scientific efforts to understand it. This study attempts to identify the source regions that contribute to the Sahelian-Sudan moisture budget during July through September. We have used an atmospheric general circulation model with an embedded moisture-tracing module (Community Atmosphere Model version 3), forced by observed (1979-2013) sea-surface temperatures. The result suggests that about 40% of the moisture comes with the moisture flow associated with the seasonal migration of the Intertropical Convergence Zone (ITCZ) and originates from Guinea Coast, central Africa, and the Western Sahel. The Mediterranean Sea, Arabian Peninsula, and South Indian Ocean regions account for 10.2%, 8.1%, and 6.4%, respectively. Local evaporation and the rest of the globe supply the region with 20.3% and 13.2%, respectively. We also compared the result from this study to a previous analysis that used the Lagrangian model FLEXPART forced by ERA-Interim. The two approaches differ when comparing individual regions, but are in better agreement when neighboring regions of similar atmospheric flow features are grouped together. Interannual variability with the rainfall over the region is highly correlated with contributions from regions that are associated with the ITCZ movement, which is in turn linked to the Atlantic Multidecadal Oscillation. Our result is expected to provide insights for the effort on seasonal forecasting of the rainy season over Sahelian Sudan.
40.	Sanchez, K. J., et al. (författare) Meteorological and aerosol effects on marine cloud microphysical properties 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:8, s. 4142-4161 Tidskriftsartikel (refereegranskat)abstract Meteorology and microphysics affect cloud formation, cloud droplet distributions, and shortwave reflectance. The Eastern Pacific Emitted Aerosol Cloud Experiment and the Stratocumulus Observations of Los-Angeles Emissions Derived Aerosol-Droplets studies provided measurements in six case studies of cloud thermodynamic properties, initial particle number distribution and composition, and cloud drop distribution. In this study, we use simulations from a chemical and microphysical aerosol-cloud parcel (ACP) model with explicit kinetic drop activation to reproduce observed cloud droplet distributions of the case studies. Four cases had subadiabatic lapse rates, resulting in fewer activated droplets, lower liquid water content, and higher cloud base height than an adiabatic lapse rate. A weighted ensemble of simulations that reflect measured variation in updraft velocity and cloud base height was used to reproduce observed droplet distributions. Simulations show that organic hygroscopicity in internally mixed cases causes small effects on cloud reflectivity (CR) (<0.01), except for cargo ship and smoke plumes, which increased CR by 0.02 and 0.07, respectively, owing to their high organic mass fraction. Organic hygroscopicity had larger effects on droplet concentrations for cases with higher aerosol concentrations near the critical diameter (namely, polluted cases with a modal peak near 0.1 mu m). Differences in simulated droplet spectral widths (k) caused larger differences in CR than organic hygroscopicity in cases with organic mass fractions of 60% or less for the cases shown. Finally, simulations from a numerical parameterization of cloud droplet activation suitable for general circulation models compared well with the ACP model, except under high organic mass fraction.
41.	Sato, Yousuke, et al. (författare) Model Intercomparison of Atmospheric Cs-137 From the Fukushima Daiichi Nuclear Power Plant Accident : Simulations Based on Identical Input Data 2018 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 123:20, s. 11748-11765 Tidskriftsartikel (refereegranskat)abstract A model intercomparison of the atmospheric dispersion of cesium-137 (Cs-137) emitted after the Fukushima Daiichi Nuclear Power Plant accident in Japan was conducted to understand the behavior of atmospheric Cs-137 in greater detail. The same meteorological data with a fine spatiotemporal resolution and an emission inventory were applied to all models to exclude the differences among the models originating from differences in meteorological and emission data. The meteorological data were used for initial, boundary, and nudging data or offline meteorological field. Furthermore, a horizontal grid with the same resolution as that of the meteorological data was adopted for all models. This setup enabled us to focus on model variability originating from the processes included in each model, for example, physical processes. The multimodel ensemble captured 40% of the atmospheric Cs-137 events observed by measurements, and the figure of merit in space for the total deposition of Cs-137 exceeded 80. The lower score of the atmospheric Cs-137 than that of the deposition originated from the difference in timing between observed and simulated atmospheric Cs-137. Our analyses indicated that meteorological data were most critical for reproducing the atmospheric Cs-137 events. The results further revealed that differences in Cs-137 concentrations among the models originated from deposition and diffusion processes when the meteorological field was simulated reasonably well. The models with small deposition fluxes produced higher scores for atmospheric Cs-137, and those with strong diffusion succeeded in capturing the high Cs-137 concentrations observed; however, they also tended to overestimate the concentrations.
42.	Savre, Julien, et al. (författare) A theory-based parameterization for heterogeneous ice nucleation and implications for the simulation of ice processes in atmospheric models 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:10, s. 4937-4961 Tidskriftsartikel (refereegranskat)abstract A new parameterization for heterogeneous ice nucleation constrained by laboratory data and based on classical nucleation theory is introduced. Key features of the parameterization include the following: a consistent and modular modeling framework for treating condensation/immersion and deposition freezing, the possibility to consider various potential ice nucleating particle types (e.g., dust, black carbon, and bacteria), and the possibility to account for an aerosol size distribution. The ice nucleating ability of each aerosol type is described using a contact angle () probability density function (PDF). A new modeling strategy is described to allow the PDF to evolve in time so that the most efficient ice nuclei (associated with the lowest values) are progressively removed as they nucleate ice. A computationally efficient quasi Monte Carlo method is used to integrate the computed ice nucleation rates over both size and contact angle distributions. The parameterization is employed in a parcel model, forced by an ensemble of Lagrangian trajectories extracted from a three-dimensional simulation of a springtime low-level Arctic mixed-phase cloud, in order to evaluate the accuracy and convergence of the method using different settings. The same model setup is then employed to examine the importance of various parameters for the simulated ice production. Modeling the time evolution of the PDF is found to be particularly crucial; assuming a time-independent PDF significantly overestimates the ice nucleation rates. It is stressed that the capacity of black carbon (BC) to form ice in the condensation/immersion freezing mode is highly uncertain, in particular at temperatures warmer than -20 degrees C. In its current version, the parameterization most likely overestimates ice initiation by BC.
43.	Savre, Julien, et al. (författare) Large-eddy simulation of three mixed-phase cloud events during ISDAC : Conditions for persistent heterogeneous ice formation 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:15, s. 7699-7725 Tidskriftsartikel (refereegranskat)abstract A Classical-Nucleation-Theory-based parameterization for heterogenous ice nucleation, including explicit dependencies of the nucleation rates on the number concentration, size, and composition of the ambient aerosol population, is implemented in a cloud-scale, large-eddy simulation model and evaluated against Arctic mixed-phase cloud events observed during Indirect and Semi-Direct Aerosol Campaign (ISDAC). An important feature of the parameterization is that the ice nucleation efficiency of each considered aerosol type is described using a contact angle distribution which evolves with time so that the model accounts for the inhibition of ice nucleation as the most efficient ice-forming particles are nucleated and scavenged. The model gives a reasonable representation of first-order (ice water paths) and second-order (ice crystal size distributions) ice microphysical properties. The production of new ice crystals in the upper part of the cloud, essential to guarantee sustained mixed-phase conditions, is found to be controlled mostly by the competition between radiative cooling (resulting in more aerosol particles becoming efficient ice nuclei as the temperature decreases), cloud-top entrainment (entraining fresh particles into the cloud), and nucleation scavenging of the ice+forming aerosol particles. The relative contribution of each process is mostly determined by the cloud-top temperature and the entrainment rates. Accounting for the evolution of the contact angle probability density function with time seems to be essential to capture the persistence of in-cloud ice production without having to, for example, increase the free tropospheric aerosol concentration. Although limited to only three cases and despite important limitations of the parameterization (e.g., the present version only considers dust and black carbon as potential ice nuclei), the results suggest that modeling the time evolution of the ice nuclei population ability to form ice is required to accurately model Arctic mixed-phase cloud processes.
44.	Sharma, S., et al. (författare) A Factor and Trends Analysis of Multidecadal Lower Tropospheric Observations of Arctic Aerosol Composition, Black Carbon, Ozone, and Mercury at Alert, Canada 2019 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 124:24, s. 14133-14161 Tidskriftsartikel (refereegranskat)abstract Observations from 1980 to 2013 of 20 aerosol constituents, ozone and mercury at Alert, Canada (82.50 degrees N, 62.35 degrees W), were analyzed for trends and dominant factors of the Arctic haze during winter and spring. Trends reflect changing emissions in Eurasia, the main source region for surface pollution in the high Arctic. SO42-, H+, NH4,+ K+, Cu, Ni, Pb, Zn, nonsoil V, nonsoil Mn, and equivalent black carbon decreased between 23% and 80% as emissions declined rapidly in northern Eurasia during the early 1990s. NO3- increased by 20% as aerosol acidity declined. Metals were linked to emissions from smelting and fossil fuel combustion. In winter, ozone increased by 5% over 23 years, consistent with other observations and global modeling. Twelve PMF factors emerged for the dark period (November to February) and 13 for the light period (March to May). Eleven PMF factors are common to both dark and light, a twelfth factor was associated with sulfate in the dark and nitrate in the light, and the thirteenth (light period) was related to ozone and gaseous mercury depletion near Alert. IODINE and NITRATE factors, important for Arctic chemistry, changed with sunlight. In the light, 50% of all NO3- was on the NITRATE factor, while in the dark, most was associated with MODIFIED SEA SALT and equivalent black carbon. In the dark (light), 90% (28%) of iodine were found on the factor IODINE and 58% associated with SEA-SALT and MODIFIED SEA-SALT. These results help in understanding the role of atmospheric chemistry in weather and climate processes.
45.	Sinha, P. R., et al. (författare) Evaluation of ground-based black carbon measurements by filter-based photometers at two Arctic sites 2017 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 122:6, s. 3544-3572 Tidskriftsartikel (refereegranskat)abstract Long-term measurements of the light absorption coefficient (b(abs)) obtained with a particle soot absorption photometer (PSAP), b(abs) (PSAP), have been previously reported for Barrow, Alaska, and Ny-angstrom lesund, Spitsbergen, in the Arctic. However, the effects on b(abs) of other aerosol chemical species coexisting with black carbon (BC) have not been critically evaluated. Furthermore, different mass absorption cross section (MAC) values have been used to convert b(abs) to BC mass concentration (M-BC=b(abs)/MAC). We used a continuous soot monitoring system (COSMOS), which uses a heated inlet to remove volatile aerosol compounds, to measure b(abs) (b(abs) (COSMOS)) at these sites during 2012-2015. Field measurements and laboratory experiments have suggested that b(abs) (COSMOS) is affected by about 9% on average by sea-salt aerosols. M-BC values derived by COSMOS (M-BC (COSMOS)) using a MAC value obtained by our previous studies agreed to within 9% with elemental carbon concentrations at Barrow measured over 11months. b(abs) (PSAP) was higher than b(abs) (COSMOS), by 22% at Barrow (PM1) and by 43% at Ny-angstrom lesund (PM10), presumably due to the contribution of volatile aerosol species to b(abs) (PSAP). Using b(abs) (COSMOS) as a reference, we derived M-BC (PSAP) from b(abs) (PSAP) measured since 1998. We also established the seasonal variations of M-BC at these sites. Seasonally averaged M-BC (PSAP) decreased at a rate of about 0.550.30ngm(-3)yr(-1). We also compared M-BC (COSMOS) and scaled M-BC (PSAP) values with previously reported data and evaluated the degree of inconsistency in the previous data.
46.	Smorgonskiy, Alexander, et al. (författare) A model for the evaluation of the electric field associated with the lightning-triggering rocket wire and its corona 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:20, s. 10964-10973 Tidskriftsartikel (refereegranskat)abstract In this paper, we analyze the electric field at ground level during the first stage of triggered lightning experiments, i.e., during the rocket ascent and prior to the lightning initiation. At distances of some tens of meters from the triggering wire, the electric field decreases significantly, while at distances of several hundred meters, there is only a very small decrease of the electric field. Two effects determine the level of the electric field reduction: the corona layer at ground level and the corona sheath around the triggering wire. We present an analytical solution based on the charge simulation method to study the phenomenon. The model is validated by comparing its results to those obtained by numerical simulations using the finite element method. A ground space charge layer and a corona sheath around the rocket-triggered lightning wire are included in the simulation. It is shown that, depending on the charge distribution, the change of the sign of the electric field is correctly predicted by our model. The obtained reductions of the electric field are consistent with simulations and experiments presented in the literature. Moreover, the proposed analytical solution is faster, and it allows studying the influence of several parameters simultaneously, i.e., the radius of the corona sheath and the space charge layer parameters. The described analytical model allows the estimation of the corona sheath radius if the parameters of the space charge layer are known from experiment.
47.	Vega, Carmen P., et al. (författare) First Ice Core Records of NO3- Stable Isotopes from Lomonosovfonna, Svalbard 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:1, s. 313-330 Tidskriftsartikel (refereegranskat)abstract Samples from two ice cores drilled at Lomonosovfonna, Svalbard, covering the period 1957-2009, and 1650-1995, respectively, were analyzed for NO(3)(-)concentrations, and NO3- stable isotopes (N-15 and O-18). Post-1950 N-15 has an average of (-6.91.9), which is lower than the isotopic signal known for Summit, Greenland but agrees with values observed in recent Svalbard snow and aerosol. Pre-1900 N-15 has an average of (4.21.6)parts per thousand suggesting that natural sources, enriched in the N-15 isotope, dominated before industrialization. The post-1950 O-18 average of (75.1 +/- 4.1)parts per thousand agrees with data from low and polar latitudes, suggesting similar atmospheric NOy (NOy=NO+NO2+HNO3) processing pathways. The combination of anthropogenic source N-15 and transport isotope effect was estimated as -29.1 parts per thousand for the last 60years. This value is below the usual range of NOx (NOx=NO+NO2) anthropogenic sources which is likely the result of a transport isotope effect of -32 parts per thousand. We suggest that the N-15 recorded at Lomonosovfonna is influenced mainly by fossil fuel combustion, soil emissions, and forest fires; the first and second being responsible for the marked decrease in N-15 observed in the post-1950s record with soil emissions being associated to the decreasing trend in N-15 observed up to present time, and the third being responsible for the sharp increase of N-15 around 2000.
48.	Verrot, Lucile, et al. (författare) Data-model comparison of temporal variability in long-term time series of large-scale soil moisture 2016 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 121:17, s. 10,056-10,073 Tidskriftsartikel (refereegranskat)abstract Soil moisture is at the heart of many processes connected to water cycle, climate, ecosystem and societal conditions. This paper investigates the ability of a relatively simple analytical soil-moisture model to reproduce temporal variability dynamics in long-term data series for: (i) remotely sensed large-scale water storage change in twenty-five large catchments around the world, and (ii) measured soil water content and groundwater level in individual stations within ten smaller catchments across the United States. The model-data comparison for large-scale water storage change (i) shows good model ability to reproduce the observed temporal variability around long-term average conditions in most of the large study catchments. Also the model comparison with locally measured data for soil water content and groundwater level in the smaller U.S. catchments (ii) shows good representation of relative seasonal and longer-term fluctuations and their timings and frequencies. Overall, the model results tend to underestimate rather than exaggerate the range of temporal soil moisture fluctuations and storage changes. The model synthesis of large-scale hydro-climatic data is based on fundamental catchment-scale water balance and is as such useful for identifying flux imbalance biases in the hydro-climatic data series that are used as model inputs.
49.	Xu, Guobao, et al. (författare) Tree ring O-18's indication of a shift to a wetter climate since the 1880s in the western Tianshan Mountains of northwestern China 2015 Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 120:13, s. 6409-6425 Tidskriftsartikel (refereegranskat)abstract Central Asian droughts have drastically and significantly affected agriculture and water resource management in these arid and semiarid areas. Based on tree ring O-18 from native, dominant Schrenk spruce (Picea schrenkiana Fisch. et Mey.), we developed a 300year (1710-2010) standard precipitation-evaporation index (SPEI) reconstruction from January to August for China's western Tianshan Mountains. The regression model explained 37.6% of the variation in the SPEI reconstruction during the calibration period from 1950 to 2010. Comparison with previous drought reconstructions confirmed the robustness of our reconstruction. The 20th century has been a relatively wet period during the past 300years. The SPEI showed quasi 2, 5, and 10year cycles. Several pluvials and droughts with covariability over large areas were revealed clearly in the reconstruction. The two longest pluvials (lasting for 12years), separated by 50years, appeared in the 1900s and the 1960s. The most severe drought occurred from 1739 to 1761 and from 1886 to 1911 was the wettest period since 1710. Compared to previous investigations of hydroclimatic changes in the western Tianshan Mountains, our reconstruction revealed more low-frequency variability and indicated that climate in the western Tianshan Mountains shifted from dry to wet in 1886. This regime shift was generally consistent with other moisture reconstructions for the northeastern Tibetan Plateau and northern Pakistan and may have resulted from a strengthened westerly circulation. The opposite hydrological trends in the western Tianshan Mountains and southeastern Tibetan Plateau reveal a substantial influence of strengthened westerlies and weakening of the Indian summer monsoon.
50.	Zhou, X., et al. (författare) Evaluation of WRF Simulations With Different Selections of Subgrid Orographic Drag Over the Tibetan Plateau 2017 Ingår i: Journal of Geophysical Research: Atmospheres. - 2169-897X .- 2169-8996. ; 122:18, s. 9759-9772 Tidskriftsartikel (refereegranskat)abstract ©2017. American Geophysical Union. All Rights Reserved. Weather Research and Forecasting (WRF) simulations with different selections of subgrid orographic drag over the Tibetan Plateau have been evaluated with observation and ERA-Interim reanalysis. Results show that the subgrid orographic drag schemes, especially the turbulent orographic form drag (TOFD) scheme, efficiently reduce the 10m wind speed bias and RMS error with respect to station measurements. With the combination of gravity wave, flow blocking and TOFD schemes, wind speed is simulated more realistically than with the individual schemes only. Improvements are also seen in the 2m air temperature and surface pressure. The gravity wave drag, flow blocking drag, and TOFD schemes combined have the smallest station mean bias (−2.05°C in 2m air temperature and 1.27hPa in surface pressure) and RMS error (3.59°C in 2m air temperature and 2.37hPa in surface pressure). Meanwhile, the TOFD scheme contributes more to the improvements than the gravity wave drag and flow blocking schemes. The improvements are more pronounced at low levels of the atmosphere than at high levels due to the stronger drag enhancement on the low-level flow. The reduced near-surface cold bias and high-pressure bias over the Tibetan Plateau are the result of changes in the low-level wind components associated with the geostrophic balance. The enhanced drag directly leads to weakened westerlies but also enhances the a-geostrophic flow in this case reducing (enhancing) the northerlies (southerlies), which bring more warm air across the Himalaya Mountain ranges from South Asia (bring less cold air from the north) to the interior Tibetan Plateau.

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Författare/redaktör: Ekman, Annica M. L. (6); Gustafsson, Örjan (5); Andersson, August (5); Chen, Deliang, 1961 (4); Zhang, Qiong (4); Henschel, Henning (4); visa fler...; Tjernström, Michael (3); Pausata, Francesco S ... (3); Riipinen, Ilona (3); Rachidi, Farhad (3); Tunved, Peter (3); Leaitch, W. R. (3); Rubinstein, Marcos (3); Ström, Johan (2); Wang, Z. (2); Jonsson, H (2); Cooray, Vernon, 1952 ... (2); Macdonald, A. M. (2); Sjolte, Jesper (2); Ahlm, L (2); Eriksson, Patrick, 1 ... (2); Isaksson, E (2); Russell, L. M. (2); Zhao, R. (2); Ortega, Ismael K. (2); Kurten, Theo (2); Olenius, Tinja (2); Vehkamaki, Hanna (2); Caballero, Rodrigo (2); Savre, Julien (2); Bender, Frida A.-M. (2); Messori, Gabriele (2); Bikkina, Srinivas (2); Sarin, M. M. (2); Rengarajan, R. (2); Sudheer, A. K. (2); Sheesley, R. J. (2); Zhang, Fuqing, 1969 (2); Chiacchio, Marc (2); Pavanello, Davide (2); Rakov, Vladimir A. (2); Iizuka, Yoshinori (2); Halonen, Roope (2); Pedersen, C.A. (2); Nenes, A. (2); Koike, M. (2); Noone, Kevin J. (2); Seinfeld, J. H. (2); He, Lixia (2); Azadifar, Mohammad (2); visa färre...

Lärosäte: Stockholms universitet (32); Uppsala universitet (10); Lunds universitet (9); Göteborgs universitet (8); Chalmers tekniska högskola (5); Luleå tekniska universitet (2); visa fler...; Kungliga Tekniska Högskolan (1); Linnéuniversitetet (1); IVL Svenska Miljöinstitutet (1); visa färre...

Språk: Engelska (64)

Forskningsämne (UKÄ/SCB): Naturvetenskap (60); Teknik (6)

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