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1.
  • Ampel, Linda, et al. (författare)
  • Abrupt climate change and early lake development - the Lateglacial diatom flora at Hasseldala Port, southeastern Sweden
  • 2015
  • Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 44:1, s. 94-102
  • Tidskriftsartikel (refereegranskat)abstract
    • The fossil diatom record from the Hasseldala Port palaeolake, southeastern Sweden, offers an excellent opportunity to investigate how past climatic shifts influenced catchment conditions and early lake development. The record, dating to between 13900 and 11200 cal. a BP, covers a climatically dynamic period, starting with deglaciation followed by oscillations between warmer and colder climate states. The stratigraphical changes in the fossil diatom assemblages show a trend of less open-water taxa and a successively more complex periphytic community as the lake shallows and the aquatic habitat structure develops. A diatom-based reconstruction of lake water pH indicates a natural acidification trend early in the record from 13900 to 12500 cal. a BP. From 12500 cal. a BP, coincident with the start of climate cooling, to 11300 cal. a BP this trend is disrupted and lake waters become more alkaline. A cooler and drier climate most likely resulted in reduced soil organic matter build-up as well as more frozen ground that impeded hydrological flow and decreased the input of dissolved organic matter and organic acids into the lake system. This study demonstrates the importance of the hydrological system as a link between terrestrial and aquatic ecosystems during early lake ontogeny.
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2.
  • Berntsson, Annika, et al. (författare)
  • Late Holocene high precipitation events recorded in lake sediments and catchment geomorphology, Lake Vuoksjavratje, NW Sweden
  • 2015
  • Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 44:4, s. 676-692
  • Tidskriftsartikel (refereegranskat)abstract
    • In this paper, we show the potential of combining multi-proxy analysis of lake sediments with catchment geomorphology to better understand palaeoenvironmental changes. Previous studies have suggested that alpine lakes in N Sweden may be highly sensitive to variations in catchment erosion and precipitation, and that this sensitivity may influence ecologically based reconstructions of past temperature changes. We analysed lake sediments covering the last 5100 years from the alpine Lake Vuoksjavratje in NW Sweden in order to identify different erosional regimes in the lake catchment, sediment sources and lake sedimentary processes, which ultimately affect the palaeoecological record. The measured proxies include elemental geochemistry from XRF core scanning, grain size, sediment accumulation rates, fraction of terrestrial organic carbon and geomorphological mapping, supported by previously published chironomid and total organic carbon data. From the integrated results we identified time intervals when increased intensity of precipitation altered sedimentation and lake catchment erosional processes. The most prominent event occurred c. 2900 cal. a BP and is interpreted to be the result of excessive precipitation, possibly related to the climatic shift towards cooler and wetter conditions referred to as the 2.8 ka event.
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3.
  • Björck, Svante, et al. (författare)
  • A South Atlantic island record uncovers shifts in westerlies and hydroclimate during the last glacial
  • 2019
  • Ingår i: Climate of the Past. - : Copernicus GmbH. - 1814-9324 .- 1814-9332. ; 15:6, s. 1939-1958
  • Tidskriftsartikel (refereegranskat)abstract
    • Changes in the latitudinal position and strength of the Southern Hemisphere westerlies (SHW) are thought to be tightly coupled to important climate processes, such as cross-equatorial heat fluxes, Atlantic Meridional Overturning Circulation (AMOC), the bipolar seesaw, Southern Ocean ventilation and atmospheric CO2 levels. However, many uncertainties regarding magnitude, direction, and causes and effects of past SHW shifts still exist due to lack of suitable sites and scarcity of information on SHW dynamics, especially from the last glacial. Here we present a detailed hydroclimate multiproxy record from a 36.4-18.6 kyr old lake sediment sequence on Nightingale Island (NI). It is strategically located at 37ĝF S in the central South Atlantic (SA) within the SHW belt and situated just north of the marine Subtropical Front (SF). This has enabled us to assess hydroclimate changes and their link to the regional climate development as well as to large-scale climate events in polar ice cores. The NI record exhibits a continuous impact of the SHW, recording shifts in both position and strength, and between 36 and 31 ka the westerlies show high latitudinal and strength-wise variability possibly linked to the bipolar seesaw. This was followed by 4 kyr of slightly falling temperatures, decreasing humidity and fairly southerly westerlies. After 27 ka temperatures decreased 3-4 ĝC, marking the largest hydroclimate change with drier conditions and a variable SHW position. We note that periods with more intense and southerly-positioned SHW seem to be related to periods of increased CO2 outgassing from the ocean, while changes in the cross-equatorial gradient during large northern temperature changes appear as the driving mechanism for the SHW shifts. Together with coeval shifts of the South Pacific westerlies, our results show that most of the Southern Hemisphere experienced simultaneous atmospheric circulation changes during the latter part of the last glacial. Finally we can conclude that multiproxy lake records from oceanic islands have the potential to record atmospheric variability coupled to large-scale climate shifts over vast oceanic areas..
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4.
  • Chawchai, Sakonvan, et al. (författare)
  • Testing commonly used XRF core scanning based proxies for organic rich lake sediments and peat
  • 2016
  • Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 45:1, s. 180-189
  • Tidskriftsartikel (refereegranskat)abstract
    • X-ray fluorescence (XRF) core scanning has become widely available for geological studies during the last decade. The data obtained from XRF core scanning, however, may be strongly influenced by the amount of organic matter, water content, density and porosity of the sediment matrix. In this study we discuss the usefulness of XRF core scanning to distinguish different kinds of organic-rich sediments and peat based on examples from tropical Lakes Kumphawapi and Nong Leng Sai in Thailand. We examined how sedimentary factors influence XRF core scanning analyses by comparing elemental and scattering ratios to lithological changes and quantitative LOI, TOC, biogenic silica (BSi) and grain-size values. Our comparison suggests that the (inc/coh) scattering ratio is of limited use as an indicator for variations in LOI and TOC in peaty gyttja or peat. In Lake Kumphawapi's sediments, Si/Ti ratios reflect clastic input associated with grain-size variations rather than BSi contents. The Ti-normalized ratios of Si, Zr, Sr, K and Rb are linked to mineral input and associated grain-size variations. We conclude that XRF core scanning of organic-rich tropical lake sediments and peat is useful to infer palaeoenvironmental conditions. However, XRF core scanning data does not stand-alone and needs to be underpinned by additional proxies.
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5.
  • Emmanouilidis, Alexandros, et al. (författare)
  • Middle to late Holocene palaeoenvironmental study of Gialova Lagoon, SW Peloponnese, Greece
  • 2018
  • Ingår i: Quaternary International. - : Elsevier BV. - 1040-6182 .- 1873-4553. ; 476, s. 46-62
  • Tidskriftsartikel (refereegranskat)abstract
    • The coastal areas of Eastern Mediterranean have long been the subject of research, due to their rapid geomorphological changes, but also because of their archaeological interest. Our study is focused on a shallow coastal lagoon of Peloponnese, Gialova Lagoon, which for several years has attracted the scientific interest of archaeologists, geomorphologists as well as sedimentologists. Gialova lagoon is located near the ancient city of Pylos, the kingdom of king Nestor during the Mycenaean period (1600-1100 BC). The objectives of this study are: (a) to reconstruct the middle to late Holocene depositional environments of the lagoon and (b) to correlate our data to already existing publications, in order to shed new light on the Holocene evolution of the lagoon and the associated coastal palaeoenvironmental changes. An 8m deep vibracore was drilled and a multi proxy analysis was carried out on the sediment sequence, including sedimentological (grain size analysis and moment measures, total organic carbon - TOC, total nitrogen e TN and total phosphorus - TP), high resolution geochemical (XRF-scanning) and palaeontological (micro-and macro faunal) analysis. The chronological framework is based on five C-14 datings forming the basis for an age depth model, calculated using the OxCal software. The radiocarbon dates from previous studies (6 cores, similar to 20 dates) were also taken into account. The data synthesis and interpretation provided robust and coherent indications regarding the palaeoenvironment, shoreline changes and the rate of geomorphological changes of the coastal area of Gialova Lagoon, as well as useful information about the palaeonvironmental and palaeoclimatic conditions that prevailed during the Mycenaean period. The interpretation, reveal a transition from a shallow marine environment (65005800 yr B.P.) to a brackish/lagoonal (5800-3300 yr B.P.), followed by a shift towards a freshwater/marsh environment (3300 yr B.P. to present).
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6.
  • Finné, Martin, et al. (författare)
  • Can XRF scanning of speleothems be used as a non-destructive method to identify paleoflood events in caves?
  • 2015
  • Ingår i: International Journal of Speleology. - 0392-6672 .- 1827-806X. ; 44:1, s. 17-23
  • Tidskriftsartikel (refereegranskat)abstract
    • We have developed a novel, quick and non-destructive method for tracing flood events in caves through the analysis of a stalagmite thick section with an XRF core scanner. The analyzed stalagmite has multiple horizons of fine sediments from past flood events intercalated with areas of cleaner calcite. Flood events detected from the elemental XRF core scanning data show good agreement with the position of flood horizons identified in petrographic thin sections. The geochemical composition of the individual flood layers shows that in certain cases the clay horizons had a distinct geochemical fingerprint suggesting that it may be possible to distinguish individual flood layers based on their geochemistry. This presents the possibility for using flood events as marker horizons to chronologically tie different speleothems in a cave to each other.
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7.
  • Helmens, Karin F., et al. (författare)
  • Major cooling intersecting peak Eemian Interglacial warmth in northern Europe
  • 2015
  • Ingår i: Quaternary Science Reviews. - : Elsevier BV. - 0277-3791 .- 1873-457X. ; 122, s. 293-299
  • Tidskriftsartikel (refereegranskat)abstract
    • The degree of climate instability on the continent during the warmer-than-present Eemian Interglacial (around ca. 123 kyr ago) remains unsolved. Recently published high-resolution proxy data from the North Atlantic Ocean suggest that the Eemian was punctuated by abrupt events with reductions in North Atlantic Deep Water formation accompanied by sea-surface temperature cooling. Here we present multiproxy data at an unprecedented resolution that reveals a major cooling event intersecting peak Eemian warmth on the North European continent. Two independent temperature reconstructions based on terrestrial plants and chironomids indicate a summer cooling of the order of 2-4 degrees C. The cooling event started abruptly, had a step-wise recovery, and lasted 500-1000 yr. Our results demonstrate that the common view of relatively stable interglacial climate conditions on the continent should be revised, and that perturbations in the North Atlantic oceanic circulation under warmer-than-present interglacial conditions may also lead to abrupt and dramatic changes on the adjacent continent.
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8.
  • Katrantsiotis, Christos, et al. (författare)
  • Eastern Mediterranean hydroclimate reconstruction over the last 3600 years based on sedimentary n-alkanes, their carbon and hydrogen isotope composition and XRF data from the Gialova Lagoon, SW Greece
  • 2018
  • Ingår i: Quaternary Science Reviews. - : Elsevier BV. - 0277-3791 .- 1873-457X. ; 194, s. 77-93
  • Tidskriftsartikel (refereegranskat)abstract
    • Understanding past hydroclimate variability and related drivers is essential to improve climate forecasting capabilities especially in areas with high climatic sensitivity, such as the Mediterranean. This can be achieved by using a broad spectrum of high resolution, multiple proxy records which can also allow us to assess linkages between regional hydroclimate variability and shifts in the large-scale atmospheric patterns. Here, we present a multiproxy reconstruction of the central-eastern Mediterranean hydro climate changes over the last 3600 years based on a sediment core from the Gialova Lagoon, a shallow coastal ecosystem in SW Peloponnese, Greece. Our combined dataset consists of the distribution and compound-specific carbon and hydrogen isotope (delta C-13 and 8D) composition of n-alkanes, bulk organic matter properties and X-ray fluorescence (XRF) core scanning data. This approach was complemented with a semi-quantitative analysis of plant remains in the core. The results indicate a high contribution of local aquatic vegetation to organic matter. Large delta C-13 variations in predominantly aquatic plant-derived mid-chain alkanes (C23-23) mainly reflect changes in the aquatic plant abundance and their carbon source. Our data suggest that higher delta C-13(23-25) values (up to 19 parts per thousand) largely correspond to expansion of aquatic vegetation during wet and/or cold periods causing carbon-limiting conditions in the water and assimilation of isotopically-enriched bicarbonate by the plants. The 8D records of the individual n-alkanes (C-17 to C-31) exhibit a nearly identical pattern to each other, which implies that they all reflect changes in the source water isotope composition, driven by hydroclimate variability. In addition, the 8D profiles are consistent with the XRF data with both proxies being driven by a common hydroclimate signal. We observe two major shifts from dry and/or warm periods at ca 3600-3000 cal BP and ca 17001300 cal BP to wet and/or cold episodes at ca 3000-2700 cal BP and ca 1300-900 cal BP. The period ca 700-200 cal BP is the wettest and/or coldest in our record and coeval with the Little Ice Age. The climatic fluctuation reported in this study can be explained by the relative dominance of high-latitude (e.g. North Atlantic Oscillation during winters) and the low-latitude atmospheric patterns (Intertropical convergence zone, Subtropical High and the effects of Asian monsoons during summers) which suggests an Atlantic-Mediterranean-Monsoon climate link in this area for the late Holocene.
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9.
  • Kylander, Malin E., et al. (författare)
  • Mineral dust as a driver of carbon accumulation in northern latitudes
  • 2018
  • Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322 .- 2045-2322. ; 8:1
  • Tidskriftsartikel (refereegranskat)abstract
    • Peatlands in northern latitudes sequester one third of the world's soil organic carbon. Mineral dusts can affect the primary productivity of terrestrial systems through nutrient transport but this process has not yet been documented in these peat-rich regions. Here we analysed organic and inorganic fractions of an 8900-year-old sequence from Store Mosse (the "Great Bog") in southern Sweden. Between 5420 and 4550 cal yr BP, we observe a seven-fold increase in net peat-accumulation rates corresponding to a maximum carbon-burial rate of 150 g C m(-2) yr(-1) -more than six times the global average. This high peat accumulation event occurs in parallel with a distinct change in the character of the dust deposited on the bog, which moves from being dominated by clay minerals to less weathered, phosphate and feldspar minerals. We hypothesize that this shift boosted nutrient input to the bog and stimulated ecosystem productivity. This study shows that diffuse sources and dust dynamics in northern temperate latitudes, often overlooked by the dust community in favour of arid and semi-arid regions, can be important drivers of peatland carbon accumulation and by extension, global climate, warranting further consideration in predictions of future climate variability.
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10.
  • Kylander, Malin E., et al. (författare)
  • New insights from XRF core scanning data into boreal lake ontogeny during the Eemian (Marine Isotope Stage 5e) at Sokli, northeast Finland
  • 2018
  • Ingår i: Quaternary Research. - : Cambridge University Press (CUP). - 0033-5894 .- 1096-0287. ; 89:1, s. 352-364
  • Tidskriftsartikel (refereegranskat)abstract
    • Biological proxies from the Sokli Eemian (Marine Isotope Stage 5e) paleolake sequence from northeast Finland have previously shown that, unlike many postglacial records from boreal sites, the lake becomes increasingly eutrophic over time. Here, principal components (PC) were extracted from a high resolution multi-element XRF core scanning dataset to describe minerogenic input from the wider catchment (PC1), the input of S, Fe, Mn, and Ca-rich detrital material from the surrounding Sokli Carbonatite Massif (PC2), and chemical weathering (PC3). Minerogenic inputs to the lake were elevated early in the record and during two abrupt cooling events when soils and vegetation in the catchment were poor. Chemical weathering in the catchment generally increased over time, coinciding with higher air temperatures, catchment productivity, and the presence of acidic conifer species. Abiotic edaphic processes play a key role in lake ontogeny at this site stemming from the base cation- and nutrient-rich bedrock, which supports lake alkalinity and productivity. The climate history at this site, and its integrated effects on the lake system, appear to override development processes and alters its long-term trajectory.
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11.
  • Kylander, Malin E., et al. (författare)
  • Potentials and problems of building detailed dust records using peat archives : An example from Store Mosse (the "Great Bog"), Sweden
  • 2016
  • Ingår i: Geochimica et Cosmochimica Acta. - : Elsevier BV. - 0016-7037 .- 1872-9533 .- 0046-564X. ; 190, s. 156-174
  • Tidskriftsartikel (refereegranskat)abstract
    • Mineral dust deposition is a process often overlooked in northern mid-latitudes, despite its potential effects on ecosystems. These areas are often peat-rich, providing ample material for the reconstruction of past changes in atmospheric deposition. The highly organic (up to 99% in some cases) matrix of atmospherically fed mires, however, makes studying the actual dust particles (grain size, mineralogy) challenging. Here we explore some of the potentials and problems of using geochemical data from conservative, lithogenic elements (Al, Ga, Rb, Sc, Y, Zr, Th, Ti and REE) to build detailed dust records by using an example from the 8900-yr peat sequence from Store Mosse (the "Great Bog"), which is the largest mire complex in the boreo-nemoral region of southern Sweden. The four dust events recorded at this site were elementally distinct, suggesting different dominant mineral hosts. The oldest and longest event (6385-5300 cal yr BP) sees a clear signal of clay input but with increasing contributions of mica, feldspar and middle-REE- rich phosphate minerals over time. These clays are likely transported from a long-distance source (< 100 km). While dust deposition was reduced during the second event (5300-4370 cal yr BP), this is the most distinct in terms of its source character with [Eu/Eu*] UCC revealing the input of plagioclase feldspar from a local source, possibly active during this stormier period. The third (2380- 2200 cal yr BP) and fourth (1275-1080 cal yr BP) events are much shorter in duration and the presence of clays and heavy minerals is inferred. Elemental mass accumulation rates reflect these changes in mineralogy where the relative importance of the four dust events varies by element. The broad changes in major mineral hosts, grain size, source location and approximated net dust deposition rates observed in the earlier dust events of longer duration agree well with paleoclimatic changes observed in northern Europe. The two most recent dust events are much shorter in duration, which in combination with evidence of their local and regional character, may explain why they have not been seen elsewhere. 
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12.
  • Ljung, Karl, et al. (författare)
  • The last termination in the central South Atlantic
  • 2015
  • Ingår i: Quaternary Science Reviews. - : Elsevier BV. - 0277-3791 .- 1873-457X. ; 123, s. 193-214
  • Tidskriftsartikel (refereegranskat)abstract
    • Lake sediments and peat deposits from two basins on Nightingale Island (37 degrees S), in the Tristan da Cunha archipelago, South Atlantic, have been analyzed. The studies were focused on the time period 16.2-10.0 cal ka BP, determined by 36 C-14 dates from the two sequences. A wide variety of proxies were used, including pollen and diatom analyzes, biogenic silica content, C and N analyzes, stable isotopes (C-13 and N-15), elemental concentrations and magnetic susceptibility measurements, to detect environmental changes that can be related to shifts of the circulation belts of the Southern Ocean. In addition, climate model simulations were carried out. We find that the sediments are underlain by a >2 cal ka BP long hiatus, possibly representing a dried-out lake bed. The climate simulations corroborate that the area might have been exposed to arid conditions as a consequence of the Heinrich I event in the north and a southward displacement of the ITCZ. The development on the island after 16.2 cal ka BP is determined by the position of the Subtropical Front (STF) and the Southern Hemisphere Westerlies (SHW). The period 16.2-14.75 cal ka BP was characterized by varying influence from SHW and with STF situated south of Tristan da Cunha, ending with a humidity peak and cooler conditions. The stable conditions 14.7-14.1 cal ka BP with cool and fairly arid conditions imply that STF and SHW were both north of the islands during the first part of the Antarctic Cold Reversal. The most unstable period, 14.1-12.7 cal ka BP, indicates incessant latitudinal shifts of the zonal circulation, perhaps related to climate variability in the Northern Hemisphere and bipolar seesaw mechanisms as the strength of the Atlantic Meridional Overturning Circulation (AMOC) varied. At 12.7 cal ka BP the Holocene warming began with a gradually drier and warmer climate as a result of a dampened AMOC during the Younger Dryas cooling in the north with ITCZ, STF and SHW being displaced southwards. Peak warming seems to have occurred in the earliest part of the Holocene, but this period was also characterized by humidity shifts, possibly an effect of retraction and expansion phases of SHW during AMOC variations in the north. (C) 2015 Elsevier Ltd. All rights reserved.
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13.
  • Löwemark, Ludvig, et al. (författare)
  • Practical guidelines and recent advances in the Itrax XRF core-scanning procedure
  • 2019
  • Ingår i: Quaternary International. - : Elsevier BV. - 1040-6182 .- 1873-4553. ; 514, s. 16-29
  • Tidskriftsartikel (refereegranskat)abstract
    • XRF core scanning has evolved to become a standard analytical technique for the rapid assessment of elemental, density and textural variations in a wide range of sediments and other materials, with applications ranging from palaeoceanography, paleoclimatology, geology, and environmental forensics to environmental protection. In general, scanning provides rapid, non-destructive acquisition of elemental and textural variations at sub-millimetre resolution for a wide range of materials. Numerous procedural adaptations have been developed for the growing number of applications, such as analyses of unconsolidated, water-rich sediments, powdered soil samples, or resin bags. Here, practical expertise and guidance from the Itrax community, gained over 15 years, is presented that should provide insights for new and experienced users.
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14.
  • Löwhagen, Linda, 1978- (författare)
  • Developing geochemical and mineralogical proxies for the correlation of paleotsunami layers
  • 2015
  • Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • The catastrophic Indian Ocean tsunami of December 2004 raised urgent questions about the paleotsunami history in the region. Numerous studies have since been conducted to gain better understanding of the magnitude, frequency and impact of past tsunamis, especially around the coasts of the Indian Ocean.Southwest Thailand directly faces the Sunda Arc trench where the earthquake that generated the Indian Ocean tsunami took place. The lack of historical documents and of suitable geological archives makes paleotsunami research a challenge in this area however. Phra Thong Island, on the Andaman Coast of southwest Thailand, with its marshy swales has proven an exception and is one of the few suitable locations for these types of studies. Apart from the 2004 Indian Ocean tsunami layer, three to four more distinct paleotsunami layers, separated by organic rich soil horizons have been previously identified and dated using radiocarbon and Optically Stimulated Luminescence techniques. Despite these efforts, several outstanding issues have to be resolved: (1) the correlation of tsunami/paleotsunami layers over larger distances remains ambiguous, particularly older layers; (2) age attributions for several of the paleotsunami layers differ at different locations; and (3) alterations of soil and sand layers by postdepositional processes are still poorly understoodThis thesis addresses these issues and aims to develop geochemical proxies that allow characterising each tsunami/paleotsunami layer in three different swales. As shown here, X-ray fluorescence elemental geochemistry, combined with loss-on-ignition analysis and mineralogical identification, is a promising tool for identifying paleotsunami layers. The specific geochemical signature of each sand layer can then be used for correlations over larger distances. This approach has the potential to provide a means for estimating past tsunami inundation distances, and thus their magnitude. 
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15.
  • Martínez Cortizas, Antonio, et al. (författare)
  • Early atmospheric metal pollution provides evidence for Chalcolithic/Bronze Age mining and metallurgy in Southwestern Europe
  • 2016
  • Ingår i: Science of the Total Environment. - : Elsevier BV. - 0048-9697 .- 1879-1026. ; 545-546, s. 398-406
  • Tidskriftsartikel (refereegranskat)abstract
    • Although archaeological research suggests that mining/metallurgy already started in the Chalcolithic (3rd millennium BC), the earliest atmospheric metal pollution in SW Europe has thus far been dated to similar to 3500-3200 cal. yr. BP in paleo-environmental archives. A low intensity, non-extensive mining/metallurgy and the lack of appropriately located archives may be responsible for this mismatch. We have analysed the older section (>2100 cal. yr. BP) of a peat record from La Molina (Asturias, Spain), a mire located in the proximity (35-100 km) of mines which were exploited in the Chalcolithic/Bronze Age, with the aim of assessing evidence of this early mining/metallurgy. Analyses included the determination of C as a proxy for organic matter content, lithogenic elements (Si, Al, Ti) as markers of mineral matter, and trace metals (Cr, Cu, Zn, Pb) and stable Pb isotopes as tracers of atmospheric metal pollution. From similar to 8000 to similar to 4980 cal. yr. BP the Pb composition is similar to that of the underlying sediments (Pb 15 +/- 4 mu g g(-1); Pb-206/Pb-207 1.204 +/- 0.002). A sustained period of low Pb-206/Pb-207 ratios occurred from similar to 4980 to similar to 2470 cal. yr. BP, which can be divided into four phases: Chalcolithic (similar to 4980-3700 cal. yr. BP), Pb-206/Pb-207 ratios decline to 1.175 and Pb/Al ratios increase; Early Bronze Age (similar to 3700-3500 cal. yr. BP), Pb-206/Pb-207 increase to 1.192 and metal/Al ratios remain stable; Late Bronze Age (similar to 3500-2800 cal. yr. BP), Pb-206/Pb-207 decline to their lowest values (1.167) while Pb/Al and Zn/Al increase; and Early Iron Age (similar to 2800-2470 cal. yr. BP), Pb-206/Pb-207 increase to 1.186, most metal/Al ratios decrease but Zn/Al shows a peak. At the beginning of the Late Iron Age, Pb-206/Pb-207 ratios and metal enrichments show a rapid return to pre-anthropogenic values. These results provide evidence of regional/local atmospheric metal pollution triggered by the earliest phases of mining/metallurgy in the area, and reconcile paleo-environmental and archaeological records.
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16.
  • Norström, Elin, et al. (författare)
  • Late-Holocene climate and vegetation dynamics in eastern Lesotho highlands
  • 2018
  • Ingår i: The Holocene. - : SAGE Publications. - 0959-6836 .- 1477-0911. ; 28:9, s. 1483-1494
  • Tidskriftsartikel (refereegranskat)abstract
    • The eastern Lesotho highlands are of considerable hydrological importance to southern Africa as a so-called water tower' for the surrounding region. Here, we contribute proxy-data inferring climate and vegetation changes over the past 1600 years, assessing in parallel inorganic and organic chemical analyses on a sediment core from Ladybird wetland, eastern Lesotho. Several proxies were used to determine changes in local vegetation dynamics, productivity, hydrology ((13) C, (15) N, C/N, TOC) and the input and source of the detrital components (Ca/Ti, CIA). The first part of the multi-proxy record (AD 400-800) shows stable terrestrial conditions and low detrital input, followed by higher variability in almost all proxies between ca. AD 900 and 1200. The (13) C record infers a higher proportion of C-4 vegetation, tentatively associated with higher temperatures during this phase, coeval with the Medieval Climate Anomaly (MCA). After AD 1200, local conditions change gradually from purely terrestrial, towards the typical wetland environment prevailing today. A higher proportion of C-3 plants and possibly an increase in aquatic organisms within the organic matrix corresponds with decreasing detrital input, suggesting locally high available moisture in this part of Lesotho during the Little Ice Age (LIA). Although age-model constraints impedes a robust regional comparison, the inferred climate variability is discussed as a tentative response to enhanced mid-latitude cyclonic activity during LIA, and the variable MCA climate conditions as indirectly dictated by changes in solar activity.
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17.
  • Pérez-Rodríguez, Marta, et al. (författare)
  • Industrial-era lead and mercury contamination in southern Greenland implicates North American sources
  • 2018
  • Ingår i: Science of the Total Environment. - : Elsevier BV. - 0048-9697 .- 1879-1026. ; 613, s. 919-930
  • Tidskriftsartikel (refereegranskat)abstract
    • To study the long-range transport of atmospheric pollutants from lower latitude industrial areas to the Arctic, we analysed a peat core spanning the last similar to 700 cal. yr (similar to 1300-2000 CE) from southern Greenland, an area sensitive to atmospheric pollution from North American and Eurasian sources. A previous investigation conducted in the same location recorded atmospheric lead (Pb) pollution after similar to 1845, with peak values recorded in the 1970s, and concluded that a North American source was most likely. To confirm the origin of the lead, we present new Pb isotope data from Sandhavn, together with a high-resolution record for mercury (Hg) deposition. Results demonstrate that the mercury accumulation rate has steadily increased since the beginning of the 19th century, with maximum values of 9.3 mu g m(-2) yr(-1) recorded similar to 1940. Lead isotopic ratios show two mixing lines: one which represents inputs from local and regional geogenic sources, and another that comprises regional geogenic and pollution sources. Detrending the Pb isotopic ratio record (thereby extracting the effect of the geogenic mixing) has enabled us to reconstruct a detailed chronology of metal pollution. The first sustained decrease in Pb isotope signals is recorded as beginning similar to 1740-1780 with the lowest values (indicating the highest pollution signature) dated to similar to 1960-1970. The 206Pb/207Pb ratio of excess Pb (measuring 1.222, and reflecting pollution generated Pb), when compared with the Pb isotopic composition of the Sandhavn peat record since the 19th century and the timing of Pb enrichments, clearly points to the dominance of pollution sources fromNorth America, although it did not prove possible to further differentiate the emissions sources geographically.
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18.
  • Plikk, Anna, et al. (författare)
  • Development of an Eemian (MIS 5e) Interglacial palaeolake at Sokli (N Finland) inferred using multiple proxies
  • 2016
  • Ingår i: Palaeogeography, Palaeoclimatology, Palaeoecology. - : Elsevier BV. - 0031-0182 .- 1872-616X. ; 463, s. 11-26
  • Tidskriftsartikel (refereegranskat)abstract
    • A 12 m long lacustrine record from Sokli, N Finland, was analyzed for diatoms, non-pollen palynomorphs, macrofossils, pollen and geochemistry in order to reconstruct the development of a high-latitude Eemian lake and investigate the influence of climatic and environmental changes on the lake ecosystem. Based on this multi-proxy dataset we distinguished five major lake phases in the lake's evolution. An initial minerogenic, glacio-lacustrine phase was followed by an organic-rich early Eemian lake phase characterized by anoxic bottom waters, high seasonality and rising nutrient levels. A long open water season, pronounced summer stratification and high productivity characterized the following early mid-Eemian lake phase, corresponding to the Eemian thermal maximum. During the late mid-Eemian lake phase decreasing water depths due to infilling and extensive mixing of the water column resulted in less stable summer stratification and decreased anoxia. The late-Eemian lake phase was characterized by shallow and dynamic conditions and a cooling climate. Superimposed on these general trends are two events characterized by colder and more arid conditions, that possibly match cold and arid events registered in palaeolimnological records on the European continent. In general, the multi-proxy record reflects a nutrient rich lake, where changes in mixing regime associated with climatic forcing and lake level changes asserted a major impact on the aquatic assemblages. The changes in the aquatic assemblages reflect the major patterns of climate change that took place during the Eemian in northern Europe; i.e. a rapid warming and high seasonality during the early Eemian, decreased seasonality during the mid Eemian and a cooling late Eemian with increased seasonality. The high latitude Sokli Eemian palaeolake record lengthens the latitudinal extent of Eemian terrestrial records across Europe, adding to the understanding of climatic gradients and drivers over Europe.
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19.
  • Salonen, J. Sakari, et al. (författare)
  • Abrupt high-latitude climate events and decoupled seasonal trends during the Eemian
  • 2018
  • Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723. ; 9
  • Tidskriftsartikel (refereegranskat)abstract
    • The Eemian (the Last Interglacial; ca. 129-116 thousand years ago) presents a testbed for assessing environmental responses and climate feedbacks under warmer-than-present boundary conditions. However, climate syntheses for the Eemian remain hampered by lack of data from the high-latitude land areas, masking the climate response and feedbacks in the Arctic. Here we present a high-resolution (sub-centennial) record of Eemian palaeoclimate from northern Finland, with multi-model reconstructions for July and January air temperature. In contrast with the mid-latitudes of Europe, our data show decoupled seasonal trends with falling July and rising January temperatures over the Eemian, due to orbital and oceanic forcings. This leads to an oceanic Late-Eemian climate, consistent with an earlier hypothesis of glacial inception in Europe. The interglacial is further intersected by two strong cooling and drying events. These abrupt events parallel shifts in marine proxy data, linked to disturbances in the North Atlantic oceanic circulation regime.
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20.
  • Sjöström, Jenny K., et al. (författare)
  • Procedure for Organic Matter Removal from Peat Samples for XRD Mineral Analysis
  • 2019
  • Ingår i: Wetlands (Wilmington, N.C.). - : Springer. - 0277-5212 .- 1943-6246. ; 39:3, s. 473-481
  • Tidskriftsartikel (refereegranskat)abstract
    • Ombrotrophic peatlands are recognized archives of past atmospheric mineral dust deposition. Net dust deposition rates, grain size, mineral hosts and source areas are typically inferred from down-core elemental data. Although elemental analysis can be time efficient and data rich, there are some inherent limitations. X-ray diffraction (XRD) analysis allowsdirect identification of mineral phases in environmental samples but few studies have applied this method to peat samples and a well-developed protocol for extracting the inorganic fraction of highly organic samples (>95%) is lacking. We tested and compared different levels of pre-treatment: no pre-treatment, thermal combustion (300, 350, 400, 450, 500 and 550 degrees C) and chemical oxidation (H2O2 and Na2S2O8) using a homogenised highly organic (>98%) composite peat sample. Subsequently, minerals were identified by XRD. The results show that combustion is preferred to chemical oxidation because it most efficiently removes organic matter (OM), an important pre-requisite for identifying mineral phases by XRD analysis. Thermally induced phase transitions can be anticipated when temperature is the only factor to take into consideration. Based on the data required in this studythe recommended combustion temperature is 500 degrees C which efficiently removes OM while preserving a majority of common dust minerals.
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21.
  • Sjöström, Jenny, 1978- (författare)
  • Reconstruction of Holocene atmospheric mineral dust deposition from raised peat bogs in south–central Sweden
  • 2018
  • Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • Atmospheric mineral dust plays a dynamic role in the climate system acting both as a forcing and a feedback mechanism. To date, the majority of paleodust studies have been conducted on marine sediments or polar ice cores, while terrestrial deposition has been less studied. As such, it is important to produce new terrestrial Holocene paleo–dust records and fill existing regional gaps. Ombrotrophic (atmospherically–fed) peat bogs can be used to reconstruct dust deposition through elemental chemistry analysis. Multi–elemental data sets are commonly used infer net dust deposition rates, source changes, grain size, and mineral composition. Mineralogical identification of dust particles is particularly important because it allows both provenance tracing and increased understanding in climate and ecosystem feedbacks. Establishing mineralogy from elemental data of mixed mineral matrixes can however be challenging. X–ray diffraction analysis (XRD) is a standard technique for mineral identification which ideally requires removal of organic matter (OM). Therefore, a test procedure was undertaken where common OM removal methods were evaluated on bulk peat samples was therefore undertaken. The results showed that combustion at 500°C was most efficient in removing OM, while leaving the majority of minerals intact, but not all. In this Licenciate thesis, early result of a paleodust study from Draftinge Mosse, southern Sweden, are also outlined. Here, the method development mentioned above was applied, enabling a combination of elemental data with mineralogy. Future work includes minor and trace element analysis by ICP–AES and ICP–MS, evaluation of the reproducibility of single core reconstructions, tests of some of the methodological assumptions used in previous paleodust studies, source tracing and paleodust reconstruction from a second site (Gällsered Mosse). 
  •  
22.
  • Swärd, Henrik, et al. (författare)
  • A chronology of environmental changes in the Lake Vättern basin from deglaciation to its final isolation
  • 2018
  • Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 47:2, s. 609-624
  • Tidskriftsartikel (refereegranskat)abstract
    • During and after deglaciation, Lake Vättern developed from a proglacial lake situated at the westernmost rim of the Baltic Ice Lake (BIL), into a brackish water body connecting the North Sea and the Baltic Sea, and finally into an isolated freshwater lake. Here we present geochemical and mineralogical data from a 70‐m composite sediment core recovered in southern Lake Vättern. Together with a radiocarbon age model of this core, we are able to delineate the character and timing of the different lake stages. In addition to a common mineralogical background signature seen throughout the sediment core, the proglacial sediments bear a calcite imprint representing ice‐sheet transported material from the limestone bedrock that borders the lake basin in the northeast. The proglacial fresh to brackish water transition is dated to 11 480±290 cal. a BP and is in close agreement with other regional chronologies. The brackish period lasted c. 300 years and was followed by a c. 1600 year freshwater period before the Vättern basin became isolated from the Initial Littorina Sea. Decreasing detrital input, increasing δ13C values and the appearance of diatoms in the upper 15 m of the sediment succession are interpreted as an overall increase in biological productivity. This mode of sedimentation continues until the present and is interpreted to mark the final isolation of the lake at 9530±50 cal. a BP. Consequently, the isolation of Lake Vättern was not an outcome of the Ancylus Lake regression, but rather because of ongoing continental uplift in the early Littorina period.
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23.
  • Swärd, Henrik, et al. (författare)
  • Regional deglaciation and postglacial lake development as reflected in a 74m sedimentary record from Lake Vättern, southern Sweden
  • 2016
  • Ingår i: GFF. - : Informa UK Limited. - 1103-5897 .- 2000-0863. ; 138:2, s. 336-354
  • Tidskriftsartikel (refereegranskat)abstract
    • The withdrawal of the Late Weichselian ice sheet and rapid isostatic uplift in southern Scandinavia led to the entrainment of large volumes of melt water within the proglacial Baltic Ice Lake (BIL). The eventual western outpost of BIL, Lake Vattern, has been a focal point for studying the dynamic retreat history of the Late Weichselian ice sheet in south central Sweden. This part of the deglacial history is described from an abundance of terrestrial studies, but, to date, no complimentary long sediment cores from Lake Vattern have been available. Here, we present the results from a unique, 74m borehole in southern Lake Vattern that recovered a Late Pleistocene to Holocene sedimentary sequence. Physical and chemical analyses of the sediment and pore water, together with geophysical mapping, reveal glacial as well as postglacial imprints implying an oscillating ice sheet margin, evidence for neotectonic activity and one or more marine incursions into the lake during deglaciation. We attribute the glaciotectonic deformation of the sediments at 54m below the lake floor to an ice readvance that likely occurred at the same time or before the advance that formed the Levene moraine (approximate to 13.8-13.4cal.kaBP). After this event, potential readvances were likely restricted to a more northerly position in the basin. We identify the final drainage of the BIL, but find evidence for an earlier marine incursion into the Vattern basin (approximate to 13.0cal.kaBP), indicating water exchange between the North Atlantic and the Baltic Ice Lake during the late Allerod.
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24.
  • Wohlfarth, Barbara, et al. (författare)
  • Climate and environment in southwest Sweden 15.5-11.3 cal. ka BP
  • 2018
  • Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 47:3, s. 687-710
  • Tidskriftsartikel (refereegranskat)abstract
    • Lake sedimentary records that allow documentation of the distinct climatic and environmental shifts during the early part of the Last Termination are scarce for northern Europe. This multi-proxy study of the sediments of Attekopsmosse, southwest Sweden, therefore fills an important gap and provides detailed information regarding past hydroclimatic conditions and local environmental responses to climatic shifts. Lake infilling started c. 15.5 cal. ka BP, but low aquatic productivity, cold summer lake water temperatures, unstable catchments, and scarce herb and shrub vegetation prevailed until c. 14.7-14.5 cal. ka BP. Inflow of warmer air masses and higher July air temperatures favoured a rise in aquatic productivity and lake water summer temperatures, and the establishment of a diverse herb, shrub and dwarf shrub vegetation, which also included tree birch c. 14.5 cal. ka BP. Freshening of the moisture source region c. 13.7-13.6 cal. ka BP does not seem to have had a large impact on the ancient lake and its catchment, as lake aquatic productivity increased further and lake water summer temperatures and minimum mean July air temperatures remained around 12-14 degrees C. In contrast, further freshening of the moisture source region c. 13 cal. ka BP triggered a decrease in lake productivity, drier conditions and lower lake water summer temperatures. Macroscopic finds of tree Betula and Pinus sylvestris at 13-12.8 cal. ka BP demonstrate the presence of these trees in the lake's catchment. The transition into the Holocene (11.6-11.5 cal. ka BP) is marked by a change in chironomid assemblages and by a rise in lake water summer temperatures and aquatic productivity. These changes were followed by the re-establishment of a diverse aquatic and terrestrial vegetation, including tree birch and Pinus sylvestris at 11.4 cal. ka BP.
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25.
  • Wohlfarth, Barbara, et al. (författare)
  • Hässeldala – a key site for Last Termination events in southern Sweden
  • 2017
  • Ingår i: Boreas. - London : John Wiley & Sons. - 0300-9483 .- 1502-3885. ; 46, s. 143-161
  • Tidskriftsartikel (refereegranskat)abstract
    • The Last Termination (19 000–11 000 a BP) with its rapid and distinct climate shifts provides a perfect laboratory to study the nature and regional impact of climate variability. The sedimentary succession from the ancient lake at Hässeldala Port in southern Sweden with its distinct Lateglacial/early Holocene stratigraphy (>14.1–9.5 cal. ka BP) is one of the few chronologically well-constrained, multi-proxy sites in Europe that capture a variety of local and regional climatic and environmental signals. Here we present Hässeldala's multi-proxy records (lithology, geochemistry, pollen, diatoms, chironomids, biomarkers, hydrogen isotopes) in a refined age model and place the observed changes in lake status, catchment vegetation, summer temperatures and hydroclimate in a wider regional context. Reconstructed mean July temperatures increased between c. 14.1 and c. 13.1 cal. ka BP and subsequently declined. This latter cooling coincided with drier hydroclimatic conditions that were probably associated with a freshening of the Nordic Seas and started a few hundred years before the onset of Greenland Stadial 1 (c. 12.9 cal. ka BP). Our proxies suggest a further shift towards colder and drier conditions as late as c. 12.7 cal. ka BP, which was followed by the establishment of a stadial climate regime (c. 12.5–11.8 cal. ka BP). The onset of warmer and wetter conditions preceded the Holocene warming over Greenland by c. 200 years. Hässeldala's proxies thus highlight the complexity of environmental and hydrological responses across abrupt climate transitions in northern Europe.
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