| 1. |
- Bertrand, Sebastien, et al.
(författare)
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Inorganic geochemistry of lake sediments : a review of analytical techniques and guidelines for data interpretation
- 2024
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Ingår i: Earth-Science Reviews. - : Elsevier. - 0012-8252 .- 1872-6828. ; 249
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Forskningsöversikt (refereegranskat)abstract
- Inorganic geochemistry is a powerful tool in paleolimnology. It has become one of the most commonly used techniques to analyze lake sediments, particularly due to the development and increasing availability of XRF core scanners during the last two decades. It allows for the reconstruction of the continuous processes that occur in lakes and their watersheds, and it is ideally suited to identify event deposits. How earth surface processes and limnological conditions are recorded in the inorganic geochemical composition of lake sediments is, however, relatively complex. Here, we review the main techniques used for the inorganic geochemical analysis of lake sediments and we offer guidance on sample preparation and instrument selection. We then summarize the best practices to process and interpret bulk inorganic geochemical data. In particular, we emphasize that log-ratio transformation is critical for the rigorous statistical analysis of geochemical datasets, whether they are obtained by XRF core scanning or more traditional techniques. In addition, we show that accurately interpreting inorganic geochemical data requires a sound understanding of the main components of the sediment (organic matter, biogenic silica, carbonates, lithogenic particles) and mineral assemblages. Finally, we provide a series of examples illustrating the potential and limits of inorganic geochemistry in paleolimnology. Although the examples presented in this paper focus on lake and fjord sediments, the principles presented here also apply to other sedimentary environments.
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| 2. |
- Björck, Svante, et al.
(författare)
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Nordlaguna – A unique lake basin at the foot of the Beerenberg volcano, Jan Mayen, containing partially enigmatic sediments
- 2022
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Ingår i: Quaternary Science Advances. - : Elsevier BV. - 2666-0334. ; 7
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Tidskriftsartikel (refereegranskat)abstract
- Sediments from the only permanent lake on the island of Jan Mayen (71°N, 08°30′W), Lake Nordlaguna (NL), were investigated. The lake, with an area of ∼1 km2, is situated at the foot of the world's northernmost active subaerial volcano and is separated from the sea by a 150–240 m wide beach barrier, which reaches 4–5 m above sea level. Most of the lake is deeper than 25 m, with the deepest part being 36 m. Altogether five coring sites, evenly spread out, were chosen and the sediment cores were retrieved from the lake ice with Uwitec and Nesje corers. After detailed descriptions of the very organic-poor and silt dominated sediments (of supposedly tephra-dominated origin), three sites were chosen for further analyses: macrofossils for 14C dating, tephra chemistry, C, S, grain-size, and XRF analyses. Based on 14C dates and the occurrence of the so-called Eggøya tephra (AD 1732), age models show variable bottom ages for the three sites: ∼3000, 600 and 400 cal yr BP. Due to the position of the core sites, with different sediment source areas, the elemental signals vary considerably between sites. An interesting feature of the lake is an isolated stock of Arctic char, which shows that the now land-locked lake has once been in contact with the sea. The almost total lack of organic material excluded any advanced paleo-ecologic investigations of the lake, and the study therefore focused on its marine-limnic history by different examinations of the XRF data with focus on the oldest and longest record. This development is based on elemental ratios (Br/Zn), PCA analyses of a center log ratio (clr) transformation of the original XRF data and magnetic susceptibility. It shows that the lake was isolated just before the time of the Eggøya tephra fall-out (∼220 cal yr BP), when the stock of Arctic char was most likely isolated from the sea. This was preceded by a ∼2200 yr long period of marine bay with a more or less open connection with the sea, and thus varying fresh-water impact. Between ∼2400 and 2600 cal yr BP the basin was more or less isolated, preceded by almost full marine conditions for at least the 300–400 preceding years we have data from, a period when relative sea level might have been higher.
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| 3. |
- Hällberg, Lars Petter, PhD student, 1988-
(författare)
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Paleoclimate and seasonality on Sumatra during the Late Glacial and Holocene : Insights from biomarkers and climate model simulations
- 2024
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Deep atmospheric convection in the Indo-Pacific Warm Pool (IPWP) is a key driver of the Hadley and Walker Circulations that modulate the Asian-Australian monsoons and the El Niño Southern Oscillation (ENSO). Temperature and rainfall seasonality, i.e., the amount and timing of precipitation, impacts ecosystems, carbon content in soils and peats, and human livelihoods. Yet, past climate variability in the IPWP is poorly constrained. The Maritime Continent, located in the center of the IPWP remains a “quantification desert”, with a scarcity of terrestrial paleoenvironmental reconstructions.This thesis investigates the evolution of temperature, precipitation amount and seasonality over the Late Glacial (14.7-11.7 ka BP) and the Holocene (last 11.7 ka). This is achieved by combining climate model simulations and lipid biomarker analyses of terrestrial peat archives from Sumatra. Temperature and seasonality were explored by analysis of climate model simulations for the Late Glacial and Holocene. Microbial membrane-derived glycerol dialkyl glycerol tetraethers (GDGTs) were investigated as temperature and hydro-environmental proxies. Using n-alkane distributions, the abundance of algae, aquatic and terrestrial plants was reconstructed and linked to past hydroclimate variability. The hydrogen isotopic composition (dD) of the n-alkanes was then used to disentangle seasonal and annual precipitation signals.The analysis of Sumatran GDGTs revealed that bacterial community shifts of the GDGT producers had a strong impact on reconstructed temperatures, and that H-shaped branched GDGT isomers are good tracers of such community shifts. The branched GDGT temperature reconstruction indicates gradual warming over the Holocene, consistent with models and nearby marine records.Rainfall seasonality has shifted drastically over the studied time frame, in particular during the end of the Late Glacial, and between 6-4.2 ka BP. The Late Glacial climate was characterized by a much stronger seasonality, with a cold and dry Asian winter monsoon suppressing atmospheric deep convection in the region. The resulting mean state conditions resembled the atmospheric circulation and sea surface temperature patterns during extreme El Niño events in the modern climate. The Mid-Holocene (6-4.2 ka BP) was characterized by increased seasonality, with alternating droughts and heavy rains due to strong monsoon precipitation and longer dry season.The Early Holocene was relatively dry. Wetter conditions started around 7-6 ka BP, and peaked at 4.5-3 ka BP. This is consistent with a dD reconstruction on Sulawesi, but 1.5-2 ka later than indicated by speleothem oxygen isotopic (d18O) records on Sumatra and Sulawesi. However, the speleothem records closely follow algal dD values, interpreted here as a seasonal monsoon signal, suggesting that speleothems in the region reflect monsoonal precipitation rather than an annual signal. Rapid drying was reconstructed for the Late Holocene, starting at 3 ka BP, co-occurring with the onset of strengthened ENSO variability. The Late Holocene drying caused drying out and decomposition of peat in one of the studied cores which resulted in a hiatus of 1700 years, highlighting the importance of hydroclimate for peat and carbon accumulation in tropical wetlands.In conclusion, this dissertation enhances our understanding of past climatic conditions in the Maritime Continent and contributes toward constraining the evolution of temperature, precipitation, and monsoon-driven seasonality over the Late Glacial and Holocene in a region that has a scarce coverage of paleoclimate proxy information. Additionally, the methodological aspects of this thesis advance terrestrial paleoclimatological reconstructions by constraining source shifts of GDGTs and proposing a novel approach to disentangle seasonal and annual precipitation signals from dD.
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| 4. |
- Kylander, Malin E., et al.
(författare)
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It's in your glass : a history of sea level and storminess from the Laphroaig bog, Islay (southwestern Scotland)
- 2020
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Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 49:1, s. 152-167
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Tidskriftsartikel (refereegranskat)abstract
- Severe winter windstorms have become an increasingly common occurrence over recent decades in northwestern Europe. Although there exists considerable uncertainty, storminess is projected to increase in the future. On centennial to millennial time scales in particular, the mechanisms forcing storminess remain unsettled. We contribute to available palaeostorm records by reconstructing changes over the last 6670 years using a coastal peat sequence retrieved from the ombrotrophic Laphroaig bog on Islay, southwestern Scotland. We use a combination of ash content, grain size and elemental chemistry to identify periods of greater storminess, which are dated to 6605, 6290-6225, 5315-5085, 4505, 3900-3635, 3310-3130, 2920-2380, 2275-2190, 2005-1860, 1305-1090, 805-435 and 275 cal. a BP. Storm signals in the first half of the record up to similar to 3000 cal. a BP are mainly apparent in the grain-size changes. Samples from this time period also have a different elemental signature than those later in the record. We speculate that this is due to receding sea levels and the consequent establishment of a new sand source in the form of dunes, which are still present today. The most significant events and strongest winds are found during the Iron Ages Cold Epoch (2645 cal. a BP), the transition into, and in the middle of, the Roman Ages Warm Period (2235 and 1965 cal. a BP) and early in the Little Ice Age (545 cal. a BP). The Laphroaig record generally agrees with regionally relevant peat palaeostorm records from Wales and the Outer Hebrides, although the relative importance of the different storm periods is not the same. In general, stormier periods are coeval with cold periods in the region as evidenced by parallels with increased ice-rafted debris in the North Atlantic, highlighting that sea-ice conditions could impact future storminess and storm track position.
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| 5. |
- Kylander, Malin E., et al.
(författare)
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Late glacial (17,060-13,400 cal yr BP) sedimentary and paleoenvironmental evolution of the Sekhokong Range (Drakensberg), southern Africa
- 2021
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Ingår i: PLOS ONE. - : Public Library of Science (PLoS). - 1932-6203. ; 16:3
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Tidskriftsartikel (refereegranskat)abstract
- Southern Africa sits at the junction of tropical and temperate systems, leading to the formation of seasonal precipitation zones. Understanding late Quaternary paleoclimatic change in this vulnerable region is hampered by a lack of available, reliably-dated records. Here we present a sequence from a well-stratified sedimentary infill occupying a lower slope basin which covers 17,060 to 13,400 cal yr BP with the aim to reconstruct paleoclimatic variability in the high Drakensberg during the Late Glacial. We use a combination of pollen, total organic carbon and nitrogen, delta C-13, Fourier transform infrared spectroscopy attenuated total reflectance (FTIR-ATR) spectral and elemental data on contiguous samples with high temporal resolution (10 to 80 years per sample). Our data support a relatively humid environment with considerable cold season precipitation during what might have been the final stage of niche-glaciation on the adjoining southern aspects around 17,000 cal yr BP. Then, after an initial warmer and drier period starting similar to 15,600 cal yr BP, we identify a return to colder and drier conditions with more winter precipitation starting similar to 14,380 cal yr BP, which represents the first local evidence for the Antarctic Cold Reversal (ACR) in this region. On decadal to centennial timescales, the Late Glacial period was one marked by considerable climatic fluctuation and bi-directional environmental change, which has not been identified in previous studies for this region. Our study shows complex changes in both moisture and thermal conditions providing a more nuanced picture of the Late Glacial for the high Drakensburg.
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| 6. |
- Kylander, Malin E., 1977-, et al.
(författare)
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Storm chasing : Tracking Holocene storminess in southern Sweden using mineral proxies from inland and coastal peat bogs
- 2023
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Ingår i: Quaternary Science Reviews. - : Elsevier BV. - 0277-3791 .- 1873-457X. ; 299, s. 107854-
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Tidskriftsartikel (refereegranskat)abstract
- Severe extratropical winter storms are a recurrent feature of the European climate and cause widespread socioeconomic losses. Due to insufficient long-term data, it remains unclear whether storminess has shown a notable response to changes in external forcing over the past millennia, which impacts our ability to project future storminess in a changing climate. Reconstructing past storm variability is essential to improving our understanding of storms on these longer, missing timescales. Peat sequences from coastal ombrotrophic bogs are increasingly used for this purpose, where greater quantities of coarser grained beach sand are deposited by strong winds during storm events. Moving inland however, storm intensity decreases, as does sand availability, muting potential paleostorm signals in bogs. We circumvent these issues by taking the innovative approach of using mid-infrared (MIR) spectral data, supported by elemental information, from the inorganic fraction of Store Mosse Dune South (SMDS), a 5000-year-old sequence from a large peatland located in southern Sweden. We infer past changes in mineral composition and thereby, the grain size of the deposited material. The record is dominated by quartz, whose coarse nature was confirmed through analyses of potential local source sediments. This was supported by further mineralogical and elemental proxies of atmospheric input. Comparison of SMDS with within-bog and regionally relevant records showed that there is a difference in proxy and site response to what should be similar timing in shifts in storminess over the-100 km transect considered. We suggest the construction of regional storm stacks, built here by applying changepoint modelling to four transect sites jointly. This modelling approach has the effect of reinforcing signals in common while reducing the influence of random noise. The resulting Southern Sweden-Storm Stack dates stormier periods to 4495-4290, 3880-3790, 2885-2855, 2300-2005, 1175-1065 and 715-425 cal yr BP. By comparing with a newly constructed Western Scotland-Storm Stack and proximal dune records, we argue that regional storm stacks allow us to better compare past storminess over wider areas, gauge storm track movements and by extension, increase our understanding of the drivers of storminess on centennial to millennial timescales.
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| 7. |
- Larsson, Simon A., 1990-, et al.
(författare)
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Synchronous or Not? The Timing of the Younger Dryas and Greenland Stadial-1 Reviewed Using Tephrochronology
- 2022
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Ingår i: Quaternary. - : MDPI AG. - 2571-550X. ; 5:2
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Tidskriftsartikel (refereegranskat)abstract
- The exact spatial and temporal behaviour of rapid climate shifts during the Last Glacial– Interglacial Transition are still not entirely understood. In order to investigate these events, it is necessary to have detailed palaeoenvironmental reconstructions at geographically spread study sites combined with reliable correlations between them. Tephrochronology, i.e., using volcanic ash deposits in geological archives as a dating and correlation tool, offers opportunities to examine the timing of events across wider regional scales. This study aims to review the posited asynchrony of the Younger Dryas stadial in comparison with Greenland Stadial-1 by correlating new proxy data from southernmost Sweden to previous palaeoclimate reconstructions in Europe based on the presence of the Hässeldalen Tephra, the Vedde Ash, and the Laacher See Tephra. µ-XRF core-scanning data were projected using a recently published age–depth model based on these tephras and several radiocarbon dates, and compared to previous findings, including by adapting previous chronologies to the recently proposed earlier date of the Laacher See Tephra (13,006 ± 9 cal. a BP). Although the results to some extent support the idea of a more synchronous Younger Dryas event than previously assumed, this issue requires further high-resolution proxy studies to overcome limitations of temporal precision.
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| 8. |
- Lopez-Costas, Olalla, et al.
(författare)
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Human bones tell the story of atmospheric mercury and lead exposure at the edge of Roman World
- 2020
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Ingår i: Science of the Total Environment. - : Elsevier. - 0048-9697 .- 1879-1026. ; 710
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Tidskriftsartikel (refereegranskat)abstract
- Atmospheric metal pollution is a major health concern whose roots pre-date industrialization. This study pertains the analyses of ancient human skeletons and compares them with natural archives to trace historical environmental exposure at the edge of the Roman Empire in NW Iberia The novelty of our approach relies on the combination of mercury, lead and lead isotopes. We found over a 700-year period that rural Romans incorporated two times more mercury and lead into their bones than post-Romans inhabiting the same site, independent of sex or age. Atmospheric pollution sources contributed on average 57% (peaking at 85%) of the total lead incorporated into the bones in Roman times, which decreased to 24% after the decline of Rome. These values and accompanying changes in lead isotopic composition mirror changes in atmospheric Pb deposition recorded in local peatlands. Thus, skeletons are a time-transgressive archive reflecting contaminant exposure.
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| 9. |
- Martínez Cortizas, Antonio, et al.
(författare)
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9000 years of changes in peat organic matter composition in Store Mosse (Sweden) traced using FTIR-ATR
- 2021
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Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 50:4, s. 1161-1178
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Tidskriftsartikel (refereegranskat)abstract
- Store Mosse (the ‘Great Bog’ in Swedish) is one of the most extensive bog complexes in southern Sweden (~77 km2), where pioneering palaeoenvironmental research has been carried out since the early 20th century. This includes, for example, vegetation changes, carbon and nitrogen dynamics, peat decomposition, atmospheric metal pollution, mineral dust deposition, dendrochronology, and tephrochronology. Even though organic matter (OM) represents the bulk of the peat mass and its compositional change has the potential to provide crucial ecological information on bog responses to environmental factors, peat OM molecular composition has not been addressed in detail. Here, a 568-cm-deep peat sequence was studied at high resolution, by attenuated reflectance Fourier-transform infrared spectroscopy (FTIR-ATR) in the mid-infrared region (4000–400 cm–1). Principal components analysis was performed on selected absorbances and change-point modelling was applied to the records to determine the timing of changes. Four components accounted for peat composition: (i) depletion/accumulation of labile (i.e. carbohydrates) and recalcitrant (i.e. lignin and other aromatics, aliphatics, organic acids and some N compounds) compounds, due to peat decomposition; (ii) variations in N compounds and carbohydrates; (iii) residual variation of lignin and organic acids; and (iv) residual variation of aliphatic structures. Peat decomposition showed two main patterns: a long-term trend highly correlated to peat age (r = 0.87), and a short-term trend, which showed five main phases of increased decomposition (at ~8.4–8.1, ~7.0–5.6, ~3.5–3.1, ~2.7–2.1 and ~1.6–1.3 ka) – mostly corresponding to drier climate and its effect on bog hydrology. The high peat accumulation event (~5.6–3.9 ka), described in earlier studies, is characterized by the lowest degree of peat decomposition of the whole record. Given that FTIR-ATR is a quick, non-destructive, cost-effective technique, our results indicate that it can be applied in a systematic way (including multicore studies) to peat research and provide relevant information on the evolution of peatlands.
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| 10. |
- Martínez Cortizas, Antonio, et al.
(författare)
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Holocene atmospheric dust deposition in NW Spain
- 2020
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Ingår i: The Holocene. - : SAGE Publications. - 0959-6836 .- 1477-0911. ; 30:4, s. 507-518
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Tidskriftsartikel (refereegranskat)abstract
- Atmospheric dust plays an important role in terrestrial and marine ecosystems, particularly those that are nutrient limited. Despite that most dust originates from arid and semi-arid regions, recent research has shown that past dust events may have been involved in boosting productivity in nutrient-poor peatlands. We investigated dust deposition in a mid-latitude, raised bog, which is surrounded by a complex geology (paragneiss/schist, granite, quartzite and granodiorite). As proxies for dust fluxes, we used accumulation rates of trace (Ti, Zr, Rb, Sr and Y) as well as major (K and Ca) lithogenic elements. The oldest, largest dust deposition event occurred between similar to 8.6 and similar to 7.4 ka BP, peaking at similar to 8.1 ka BP (most probably the 8.2 ka BP event). The event had a large impact on the evolution of the mire, which subsequently transitioned from a fen into a raised bog in similar to 1500 years. From similar to 6.7 to similar to 4.0 ka BP, fluxes were very low, coeval with mid-Holocene forest stability and maximum extent. In the late Holocene, after similar to 4.0 ka BP, dust events became more prevalent with relatively major deposition at similar to 3.2-2.5, similar to 1.4 ka BP and similar to 0.35-0.05 ka BP, and minor peaks at similar to 4.0-3.7, similar to 1.7, similar to 1.10-0.95 ka BP and similar to 0.74-0.58 ka BP. Strontium fluxes display a similar pattern between similar to 11 and similar to 6.7 ka BP but then became decoupled from the other elements from the mid Holocene onwards. This seems to be a specific signal of the granodiorite batholith, which has an Sr anomaly. The reconstructed variations in dust fluxes bear a strong climatic imprint, probably related to storminess controlled by North Atlantic Oscillation conditions. Complex interactions also arise because of increased pressure from human activities.
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| 11. |
- Martínez Cortizas, Antonio, et al.
(författare)
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Investigating the Mineral Composition of Peat by Combining FTIR-ATR and Multivariate Analysis
- 2021
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Ingår i: Minerals. - : MDPI AG. - 2075-163X. ; 11:10
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Tidskriftsartikel (refereegranskat)abstract
- The mineral content of peat has received little attention until the last few decades, when peat cores have been increasingly used to study past dust deposition. Paleodust deposition is commonly reconstructed through elemental datasets, which are used to infer deposition rates, storminess patterns, mineral composition, source identification, and fertilization effects. To date, only a few studies have directly analyzed the mineralogy (by XRD and SEM) and particle size of peat mineral matter, and the conducted studies have usually been constrained by the need to remove a large amount of organic matter, which risks altering the mineral component. One alternative is to use quick, nondestructive techniques, such as FTIR-ATR, that require little sample preparation. In this study, we analyzed by FTIR-ATR both the bulk peat and ash fractions of a sequence taken in a minerogenic mire that covered a wide inorganic matter content range (6%–57%). Aided by principal component analysis on transposed IR spectral data, we were able to identify the main minerals in bulk peat and ash, quartz, mica (likely muscovite), K feldspar (likely microcline), and plagioclase (likely anorthite), which are consistent with the local geology of the mire catchment. Changes in mineral composition during the last ca. 2800 years were coeval with previously reconstructed environmental changes using the same core. Our results suggest that FTIR-ATR has great potential to investigate peat mineral matter and the processes that drive its compositional change.
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| 12. |
- Martínez Cortizas, Antonio, et al.
(författare)
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Structural equation modeling of long-term controls on mercury and bromine accumulation in Pinheiro mire (Minas Gerais, Brazil)
- 2021
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Ingår i: Science of the Total Environment. - : Elsevier BV. - 0048-9697 .- 1879-1026. ; 757
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Tidskriftsartikel (refereegranskat)abstract
- The application of statistical modeling is still infrequent in mercury research in peat, despite the ongoing debate on the weight of the diverse factors (climate, peat decomposition, vegetation changes, etc.) that may affect mercury accumulation. One of the few exceptions is the Hg record of Pinheiro mire (souheast Brazil). Previous studies on this mire modeled mercury using principal components regression and partial least squares. These methods assume independence between factors, which is seldom the case in natural systems, thus hampering the identification of mediating effects and interactions. To overcome these limitations, in this reserach we use structural equation modeling (PLS-SEM) to model mercury and bromine peat records - bromine has been used in some investigations to normalize mercury accumuation. The mercury model explained 83% of the variance and suggested a complex control: increased peat decomposition, dust deposition and humid dimates enhanced mercury accumulation, while increased mineral fluxes resulted in a decrease in mercury accumulation. The bromine model explained 90% of the variation in concentrations: increased dust deposition and peat decomposition promoted bromine accumulation, while time (i.e. peat age) promoted bromine depletion. Thus, although mercury and bromine are both organically bound elements with relevant atmospheric cycles the weights of the factors involved in their accumulation differed significantly. Our results suggest caution when using bromine to normalize mercury accumulation. PLS-SEM results indicate a large time dependence of peat decomposition, catchment mineral fluxes, long-term climate change, and atmospheric deposition: while atmospheric dust, mineral fluxes and peat decomposition showed high to moderate climate dependency. In particular, they also point to a relevant role of autogenic processes (i.e. the build up and expansion of the mire within the catchment), which controlled local mineral fluxes; an aspect that has seldom been considered.
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| 13. |
- Norström, Elin, et al.
(författare)
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Chronostratigraphic palaeo-climate phasing based on southern African wetlands : From the escarpment to the eastern seaboard
- 2021
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Ingår i: South African Journal of Geology. - : Geological Society of South Africa. - 1012-0750 .- 1996-8590. ; 124:4, s. 977-994
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Tidskriftsartikel (refereegranskat)abstract
- This paper aims to identify chronostratigraphic palaeo-climatic boundaries based on proxy indications from mountain -and coastal wetlands in eastern South Africa and Lesotho. Phase boundaries were identified from timing of climate change inferred by proxies, as well as regime shifts in climate variability. Sometimes magnitude and/or frequency of change was also considered. Summarizing the common palaeo-climatic indications suggest the following chronostratigraphic climate phases: 25 to 18 ka, 18 to 15 ka, 15 to 11.5, 11.5 to 8 ka, 8 to 5.5 ka, 5.5 to 2 ka and 2 to 0 ka. The most robust boundaries were identified at 18 ka, 15 ka and 2 ka, i.e. these boundaries were supported by several proxies/sites. The other boundaries were less clearly detected from available proxies/sites and should be regarded tentative. The timing of a climate shift often coincides at coast and mountain sites. However, the climate conditions within each chronostratigraphic phase sometimes vary between coast and inland sites. The 25 to 18 ka phase was cool and dry with strong and frequent storms, followed by the ca. 18 to 15 ka period when conditions were less severe but still generally cool and dry. At ca. 15 to 11.5 ka several proxies infer warmer climate, with less winter rains. During 11.5 to 8 ka a general increase in wetness is inferred, followed by warming over the 8 to 5.5 ka phase. Between 5.5 and 2 ka a successive change towards wetter is indicated, although timing differ between sites. After 2 ka generally a more variable climate is seen, often with high magnitude shifts between dry and wet. The data resolution, i.e. the number of available wetland records, increases with time from very low during glacial times, to highest resolution during late Holocene. Geographically, sites in the mountain region are overrepresented compared to coastal sites. A comparison with coastal lake records suggests a more variable climate at coastal sites compared to mountain sites during mid-and late Holocene, although different proxy resolution and methodology cannot be ruled out as an explanation. A case study compares multiproxy records from Drakensberg (Sekhokong, Ntsikeni) and the coast (Mfabeni), discussing advantages and problems associated with proxy-comparisons within and between sites.
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| 14. |
- Piret, Loic, et al.
(författare)
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High-resolution fjord sediment record of a receding glacier with growing intermediate proglacial lake (Steffen Fjord, Chilean Patagonia)
- 2021
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Ingår i: Earth Surface Processes and Landforms. - : Wiley. - 0197-9337 .- 1096-9837. ; 46:1, s. 239-251
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Tidskriftsartikel (refereegranskat)abstract
- Proglacial lakes are effective sediment traps but their impact on the reliability of downstream sediment records to reconstruct glacier variability remains unclear. Here, we investigate the sedimentary signature of the recent recession of Steffen Glacier (Chilean Patagonia, 47 degrees S) in downstream fjord sediments, with a focus on identifying the trapping (decreased downstream sediment yield) and filtering (removal of coarse particles) effectiveness of a growing intermediate proglacial lake. Four sediment cores were collected along a 14 km longitudinal transect in Steffen Fjord and the sediment physical and chemical properties were compared with aerial imagery at high temporal resolution. The caesium-137 (Cs-137) chronology of the most distal core and sediment trap data suggest that sediment accumulation in the fjord remained relatively stable through time, despite the accelerating glacier recession and the growth of Steffen proglacial lake. This is in contrast with many studies that indicate a decrease in sediment yield during proglacial lake expansion. It implies that the increase in sediment export due to accelerating meltwater production may be balanced by the sediment trapping effect of the growing proglacial lake. The fjord sediments show a slight fining upward accompanied by a marked decrease in flood-induced grain-size peaks, most likely due to the increasing filtering and dampening effect of the expanding proglacial lake. Our findings show that the filtering effect of the proglacial lake reached a threshold in 1985, when the lake attained an area of 2.02 km(2). The additional 5 km of glacier recession during the following 32 years did not have any significant impact on downstream sedimentation. This study confirms that proglacial lakes act as sediment traps but it indicates that (1) the trapping effect can be outpaced by accelerating glacier recession and (2) the filtering effect becomes stable once the lake attains a certain critical size.
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| 15. |
- Rocha, Eva, et al.
(författare)
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Testing the applicability of dendrochemistry using X-ray fluorescence to trace environmental contamination at a glassworks site
- 2020
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Ingår i: Science of the Total Environment. - : Elsevier. - 0048-9697 .- 1879-1026. ; 720, s. 1-12
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Tidskriftsartikel (refereegranskat)abstract
- The potential of dendrochemistry as a tool for tracing anthropogenic contamination at a glassworks site in southeastern Sweden was investigated through a multidisciplinary approach combining continuous high-resolution time series of tree rings and sediment profiles. Tree cores from Scots pine (Pinus sylvestris), Norway spruce (Picea abies) and European aspen (Populus tremula) were analysed for their elemental composition using an energy dispersive X-ray fluorescence (ED-XRF) technique. Sediment cores were sampled along a transect extending from the pollution point source to unpolluted areas and analysed using core-scanning-XRF (CS-XRF). High contaminant concentrations in the soil were found for As (approximate to 2000 ppm), Pb (>5000 ppm), Ba (approximate to 1000 ppm) and Cd (approximate to 150 ppm). The concentrations decreased with depth and distance from the pollution source. The dendrochemical analyses revealed alterations in the Barium, Chlorine and Manganese profiles, allowing the identification of seven potential asynchronous releases from the glassworks. Our results suggest that differences in the response of tree species to elemental uptake together with soil chemical properties dictate the success of dendrochemistry as an environmental monitoring tool. (C) 2020 Elsevier B.V. All rights reserved.
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| 16. |
- Ryberg, Eleonor E., et al.
(författare)
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Postglacial peatland vegetation succession in Store Mosse bog, south-central Sweden : An exploration of factors driving species change
- 2022
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Ingår i: Boreas. - : Wiley. - 0300-9483 .- 1502-3885. ; 51:3, s. 651-666
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Tidskriftsartikel (refereegranskat)abstract
- Boreal peatlands are facing significant changes in response to a warming climate. Sphagnum mosses are key species in these ecosystems and contribute substantially to carbon sequestration. Understanding the factors driving vegetation changes on longer time scales is therefore of high importance, yet challenging since species changes are typically affected by a range of internal and external processes acting simultaneously within the system. This study presents a high-resolution macrofossil analysis of a peat core from Store Mosse bog (south-central Sweden), dating back to nearly 10 000 cal. a BP. The aim is to identify factors driving species changes on multidecadal to millennial timescales considering internal autogenic, internal biotic and external allogenic processes. A set of independent proxy data was used as a comparison framework to estimate changes in the bog and regional effective humidity, nutrient input and cold periods. We found that Store Mosse largely follows the expected successional pathway for a boreal peatland (i.e. lake -> fen -> bog). However, the system has also been affected by other interlinked factors. Of interest, we note that external nutrient input (originating from dust deposition and climate processes) has had a negative effect on Sphagnum while favouring vascular plants, and increased fire activity (driven by allogenic and autogenic factors) typically caused post-fire, floristic wet shifts. These effects interactively caused a floristic reversal and near disappearance of a once-established Sphagnum community, during which climate acted as an indirect driver. Overall, this study highlights that the factors driving vegetation change within the peatland are multiple and complex. Consideration of the role of interlinked factors on Sphagnum is crucial for an improved understanding of the drivers of species change on short- and long-term scales.
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| 17. |
- Schillereff, Daniel N., et al.
(författare)
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Phosphorus supply affects long-term carbon accumulation in mid-latitude ombrotrophic peatlands
- 2021
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Ingår i: Communications Earth & Environment. - : Springer Science and Business Media LLC. - 2662-4435. ; 2:1
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Tidskriftsartikel (refereegranskat)abstract
- Increased long-term phosphorus accumulation reduces carbon sequestration in mid-latitude peatlands reliant on atmospheric nutrient sources, according to a synthesis of data from Central Europe, North America, Chile, Sweden and the UK. Ombrotrophic peatlands are a globally important carbon store and depend on atmospheric nutrient deposition to balance ecosystem productivity and microbial decomposition. Human activities have increased atmospheric nutrient fluxes, but the impacts of variability in phosphorus supply on carbon sequestration in ombrotrophic peatlands are unclear. Here, we synthesise phosphorus, nitrogen and carbon stoichiometric data in the surface and deeper layers of mid-latitude Sphagnum-dominated peatlands across Europe, North America and Chile. We find that long-term elevated phosphorus deposition and accumulation strongly correlate with increased organic matter decomposition and lower carbon accumulation in the catotelm. This contrasts with literature that finds short-term increases in phosphorus supply stimulates rapid carbon accumulation, suggesting phosphorus deposition imposes a threshold effect on net ecosystem productivity and carbon burial. We suggest phosphorus supply is an important, but overlooked, factor governing long-term carbon storage in ombrotrophic peatlands, raising the prospect that post-industrial phosphorus deposition may degrade this carbon sink.
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| 18. |
- Sim, Thomas G., et al.
(författare)
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Regional variability in peatland burning at mid-to high-latitudes during the Holocene
- 2023
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Ingår i: Quaternary Science Reviews. - : Elsevier. - 0277-3791 .- 1873-457X. ; 305
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Tidskriftsartikel (refereegranskat)abstract
- Northern peatlands store globally-important amounts of carbon in the form of partly decomposed plant detritus. Drying associated with climate and land-use change may lead to increased fire frequency and severity in peatlands and the rapid loss of carbon to the atmosphere. However, our understanding of the patterns and drivers of peatland burning on an appropriate decadal to millennial timescale relies heavily on individual site-based reconstructions. For the first time, we synthesise peatland macrocharcoal re-cords from across North America, Europe, and Patagonia to reveal regional variation in peatland burning during the Holocene. We used an existing database of proximal sedimentary charcoal to represent regional burning trends in the wider landscape for each region. Long-term trends in peatland burning appear to be largely climate driven, with human activities likely having an increasing influence in the late Holocene. Warmer conditions during the Holocene Thermal Maximum (similar to 9e6 cal. ka BP) were associated with greater peatland burning in North America's Atlantic coast, southern Scandinavia and the Baltics, and Patagonia. Since the Little Ice Age, peatland burning has declined across North America and in some areas of Europe. This decline is mirrored by a decrease in wider landscape burning in some, but not all sub-regions, linked to fire-suppression policies, and landscape fragmentation caused by agricultural expansion. Peatlands demonstrate lower susceptibility to burning than the wider landscape in several instances, probably because of autogenic processes that maintain high levels of near-surface wetness even during drought. Nonetheless, widespread drying and degradation of peatlands, particularly in Europe, has likely increased their vulnerability to burning in recent centuries. Consequently, peatland restoration efforts are important to mitigate the risk of peatland fire under a changing climate. Finally, we make recommendations for future research to improve our understanding of the controls on peatland fires.(c) 2023 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
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| 19. |
- Sjöström, Jenny K., et al.
(författare)
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Holocene storminess dynamics in northwestern Ireland : shifts in storm duration and frequency between the mid- and late Holocene
- 2024
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Ingår i: Quaternary Science Reviews. - : Elsevier. - 0277-3791 .- 1873-457X. ; 337
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Tidskriftsartikel (refereegranskat)abstract
- Substantial uncertainties exist regarding how future climate change will affect storminess (storm frequency and intensity) in Ireland and the United Kingdom (UK). Knowledge about spatiotemporal variations of past storminess gives us a better understanding of its mechanisms on centennial to millennial time scales, as well as the impact of external forcing on future storminess in climate models. Here, we present the oldest storm record to date from Ireland, covering the last 8000 years, reconstructed from the Roycarter Bog, a coastal blanket bog in north-western Ireland. The sequence was analysed for grain-size, chemical, mineral and organic molecular composition. The chronology was built on 11 AMS radiocarbon dates. The deposit characteristics, location and low inorganic content suggest aeolian transport of particles to the bog throughout the studied period. Cluster analysis of the grain-size frequency curves, along with the coarse to fine sand ratio, allowed the identification of eleven storm periods (cal yr BP): 6150–5500 (1); 4970–4130 (2); 4000 (3); 3490–3290 (4); 3230 (5); 2850–2590 (6); 2170–1920 (7); 1440 (8); 1225–890 (9); 620–470 (10); and 290–230 (11).During the mid-Holocene, the relative sea level was lower and the local beach sources located further away, giving a longer transport distance compared to the late Holocene. In the latter part of the mid-Holocene (6150–4130 cal yr BP), during the Holocene thermal maximum, increased storminess and wind strengths were inferred for north-western Ireland, manifested as two longer storm periods. During the late Holocene the storm frequency increased, and a greater number (9) of shorter storm periods were recorded. Comparison between our results and regional peat palaeostorm records from Scotland, north of our study site, showed an antiphase relationship between storminess in Ireland and Scotland during the latter part of the mid-Holocene, but mostly in-phase storminess over the last 3000 years. Taken together, enhanced wind strength and storminess were recorded during the warmer mid-Holocene, while an increased frequency of storm events occurred in the cooler late Holocene. Mid-Holocene storm periods occurred during locally wet periods, while most of the storm periods during late Holocene occurred during drier phases. Alternatively, the elevated mineral input during late Holocene promoted microbial activity and peat decomposition. The apparent variability in cyclicity and frequency between the mid- and late Holocene indicates that the processes governing storminess in the region shifted. This calls for further studies ahead, including climate modelling, to disentangle the complex processes governing storminess on millennial to centennial time scale.
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| 20. |
- Sjöström, Jenny K., 1978-, et al.
(författare)
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Late Holocene peat paleodust deposition in south-western Sweden : exploring geochemical properties, local mineral sources and regional aeolian activity
- 2022
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Ingår i: Chemical Geology. - : Elsevier. - 0009-2541 .- 1872-6836. ; 602
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Tidskriftsartikel (refereegranskat)abstract
- Atmospheric mineral dust not only interacts with the climate system by scattering incoming solar radiation and affecting atmospheric photochemistry, but also contributes critical nutrients to marine and terrestrial ecosystems. In a high-resolution analysis of paleodust deposition, peat development and soil dust sources, we assess the interplay between dust deposition and bog development of the Davidsmosse bog in south-western Sweden. Analyses of the 5400-year record (458 cm) included radiocarbon dating, bulk density, ash content, chemical and mineralogical composition and carbon stable isotopes, subsequently explored using principal component analysis. Fourteen dust events (DEs) were recorded (cal BP) in the peat sequence: 3580–3490; 3280; 3140; 3010–2840; 2740; 2610; 2480; 2340; 2240–2130; 1690; 1240; 960, 890–760, and 620–360. The majority of the DEs were coupled to increases in peat accumulation rates and increased nutrient content (N, P and K) suggesting that the DEs contributed with nutrients to the bog ecosystem, promoting increased accumulation. We also analyzed the chemical and mineral composition of potential mineral source deposits (separated into 6 grain-size fractions) from sites within a 4 km radius as well as aeolian dunes closer to the coast (25 km). The composition deposited on the present-day bog surface indicates that the bulk of the contemporary minerals have a local origin (<1.5 km), but the DEs may be of a more distant origin. The results also indicate that quartz and plagioclase feldspar content consistently increase with increasing grain-size, both in the source samples as well as in the peat sequence, and that the Si/Al ratio can be used to infer grain size changes in the peat. Two longer phases saw numerous DEs, between 2800 and 2130 cal BP and a stepwise increase from 960 towards 360 cal BP. The episodic character of the events, together with the inferred coarse grain size, suggest that the particles were deposited by (winter) storms. Future studies should include grain size analysis as well as a more in-depth comparison with regional paleo dust and storm records to increase knowledge on both transport processes (creep, saltation, suspension) and the climate processes driving late Holocene dust and storm events in Scandinavia.
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| 21. |
- Sjöström, Jenny K., et al.
(författare)
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Paleodust deposition and peat accumulation rates : bog size matters
- 2020
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Ingår i: Chemical Geology. - : Elsevier. - 0009-2541 .- 1872-6836. ; 554
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Tidskriftsartikel (refereegranskat)abstract
- We present a high-resolution peat paleodust and accumulation rate record spanning the last 8300 years from Draftinge Mosse (400 ha), southern Sweden (57 degrees 06'27.6 '' N 13 degrees 42'54.1 '' E). The record was analysed for peat accumulation rates (PAR), elemental concentrations, mineralogy, and plant macrofossil content. Five periods of increased mineral deposition were recorded. The first event occurred between similar to 6280 and similar to 5570 cal BP, during the fen to bog transition. This is followed by four atmospheric mineral dust events (DE) which were recorded in the ombrotrophic section of the sequence at (cal BP): similar to 2200; similar to 1385-1150; similar to 830-590, and from similar to 420 to the present. Statistical analysis and elemental ratios indicated that both the mineralogy and grain size shifted when the system transitioned from fen into bog, showing that the governing transport process shifted with the peat-land succession stages. This highlights the importance of identifying peatland succession stages within peat paleodust studies. Following all four DE, increases in PAR were observed, implying a coupling to dust deposition. Comparison of DE and PAR with a paleodust record from Store Mosse, a 20 times larger bog located ca 18 km away (Kylander et al. 2016), showed that both PAR and dust deposition are largely represented by single-core reconstructions, indicating that they are driven by a common climate forcing mechanism. However, higher PAR and dust deposition rates were observed in the more moderately sized Draftinge Mosse, suggesting that the size of the bog is important to consider in peat paleodust studies. Furthermore, the smaller bog responded more rapidly to hydrological changes, indicating that the size of the bog affects its' buffering capacity. Authigenic carbonates, observed here during episodes of rapid peat growth, coincide with changes in REE ratios, indicating that authigenic peat processes potentially cause REE fractionation.
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| 22. |
- Sjöström, Jenny, 1978-
(författare)
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Mid-Holocene mineral dust deposition in raised bogs in southern Sweden : Processes and links
- 2021
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- Atmospheric mineral dust is a key component of the climate system, which affects insolation, brings nutrients to marine and terrestrial ecosystems, and acts as a cloud condensation nuclei. To reconstruct past patterns in terrestrial dust deposition natural archives may be utilized, such as loess, dunes, lakes, and peat bogs. Bogs became an established dust archive in the early 2000s, and the number of studies has since increased. However, most studies use single records to represent dust deposition, meaning that we have limited understanding of regional paleodust dynamics or about the representativeness of single bog records. This thesis aims to address these uncertainties by comparing paleodust deposition between bogs located on a 65 km transect. The thesis includes a methodological development for organic matter removal from peat samples for XRD mineral analysis (Paper I) and two peat paleodust reconstruction studies (Paper II, III). The first paleodust reconstruction from Draftinge Mosse (mosse translates to bog in English), Småland, showed that four dust events (DE) were recorded during the ombrotrophic stage (Paper II). These results were compared to a previously conducted study on Store Mosse, 20 km northeast of Draftinge Mosse, which showed similar patterns in DE and peat accumulation rate (PAR), indicating that the events were at least regional in character. However, the magnitude of the DE differed, which was related to differences in the sizes of the two bogs. The second paleodust reconstruction, from (Davidsmosse) located c. 25 km from the west coast, recorded many more DE (14) compared to the more inland sites (Paper III). Two longer periods saw numerous DE, dominated by coarse particles: between 2800 and 2130 cal BP, and from 1000 towards 490 cal BP. These two periods occurred during regionally cold periods. Human activities also intensified during the latter period, possibly amplifying the DE. Most of these episodic events were not recorded at the inland sites, and the Davidsmosse record seemed to be more in line with previously constructed coastal paleostorm records. That the bog located closer to the coast recorded many more events compared to the inland sites suggests that the location of a bog will influence the aeolian events recorded. However, the DE observed at the inland sites were also recorded at Davidsmosse, indicating that the inland events might represent winds that were sustained over longer distance, or alternatively, that regionally dry conditions prevailed during these periods. The paleostorm records from south-western Sweden, including the new results from Davidsmosse presented here, suggest that storm intensities have varied during the last 3000 years, with increased storminess frequency coupled to colder episodes related to extended sea ice and a southward shift of storm tracks. When comparing DE and PAR at both sites studied here, a recurring pattern of increased accumulation rates were observed during a majority of DE, supporting the suggestion of previous studies that dust deposition may affect peat growth, and thus also peat carbon sequestration.Combining elemental data with XRD mineral analysis enabled anchoring of elemental inferences with mineral observations, allowed identification of authigenic minerals, and aided in source tracing. Despite the fact that local factors affect mineral deposition and PAR, this work has outlined some of the possible mechanisms behind these observations (e.g. distance to the coast, or bog size difference) which may be important for future peat paleodust studies to consider. For example, future studies should include grain size analysis (down-core, as well as across a bog surface); pollen analysis to further elaborate on human activities and vegetation cover; and further investigate differences in mass accumulation rates between bogs.
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| 23. |
- Strandberg, Nichola Ann, et al.
(författare)
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Landscape development at Lina myr fen, Eastern Gotland, 9000-2500 cal. yr BP
- 2020
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Ingår i: The Holocene. - : SAGE Publications. - 0959-6836 .- 1477-0911. ; 30:8, s. 1205-1219
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Tidskriftsartikel (refereegranskat)abstract
- Using diatoms, pollen, and geochemistry, we explore human habitation around Lina myr, Gotland, in relation to shore displacement. Archeological evidence has shown that Lina myr was an important area for its prehistoric human inhabitants. We investigate if and when Lina myr was connected to the sea and could therefore have been part of an inland water system useful for transport. A chronology was based on C-14 AMS dating of terrestrial macrofossils and bulk sediments with dates ranging between 9100 and 2360 cal. yr BP. The initiation of the Littorina transgression was dated to 8500 cal. yr BP. A twofold pattern for the maximum sub-phase of the Littorina Sea is suggested from 8100 to 7500 cal. yr BP and from 6500 to 6000 cal. yr BP. The onset of cultivation and grazing was indicated by the presence of Hordeum and Plantago lanceolata in the pollen record during the Late Neolithic, at about 4580 cal. yr BP. During this time sea level was relatively higher than today and the Lina myr basin was connected with the Littorina Sea, which it continued to be until isostatic uplift caused it to become isolated at about 3820 cal. yr BP. After about 3000 cal. yr BP, human-made landscape changes intensified, grasslands increased, and shrublands decreased.
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| 24. |
- Vandekerkhove, Elke, et al.
(författare)
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Signature of modern glacial lake outburst floods in fjord sediments (Baker River, southern Chile)
- 2021
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Ingår i: Sedimentology. - : Wiley. - 0037-0746 .- 1365-3091. ; 68:6, s. 2798-2819
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Tidskriftsartikel (refereegranskat)abstract
- Glacial Lake Outburst Floods (GLOFs) constitute a major hazard in glacierized regions. They are particularly pronounced in the Baker River watershed (Chilean Patagonia, 48°S), where 23 events occurred between 2008 and 2020. Although GLOF deposits have previously been studied in lake settings, how modern GLOFs are recorded in fjord sediments remains mostly unknown. To address this issue, ten sediment cores collected in the fjord immediately downstream of the Baker River (Martínez Channel) were investigated and compared to the recent GLOF history of the river. Results show that sediments accumulate at 2.0 to 3.4 cm year−1 and that GLOF deposits can be distinguished from background sediments by their finer grain size (5.98 ± 0.82 μm) and lower organic carbon content (0.31 ± 0.06%), reflecting the release and transport in suspension of high amounts of glacial rock flour during GLOFs. Although 21 GLOFs from Cachet 2 Lake occurred between 2008 and 2017, the first events left a stronger imprint in the sediment, suggesting that more sediment of glacial origin was released during those initial events, possibly due to lake-bed erosion. An older GLOF deposit was tentatively linked to the outburst of Las Lengas Lake in 1988. The sediment cores also contain fine-grained turbidites, especially in the prodelta area. These turbidites confirm recent channel activity, but most of them seem to have been triggered by processes other than GLOFs. Overall, the results of this study suggest that GLOF deposits are distinct from typical flood turbidites. They are best identified by their low grain size and total organic carbon content, and best archived on the delta slope, away from any submarine channel influence. Finally, these results highlight the potential of fjord sediment archives to establish pre-historical GLOF records and ultimately improve GLOF hazard assessments.
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