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Highly Diastereoselective Palladium-Catalyzed Oxidative Cascade Carbonylative Carbocyclization of Enallenols
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- Posevins, Daniels (author)
- Stockholms universitet,Institutionen för organisk kemi,Department of Organic Chemistry, Arrhenius Laboratory, Stockholm University, Stockholm, Sweden
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- Li, Man-Bo (author)
- Stockholms universitet,Institutionen för organisk kemi,Department of Organic Chemistry, Arrhenius Laboratory, Stockholm University, Stockholm, Sweden
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- Svensson Grape, Erik (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK),Department of Materials and Environmental Chemistry, Arrhenius Laboratory, Stockholm University, Stockholm, Sweden
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- (creator_code:org_t)
- 2020-01-02
- 2020
- English.
- In: Organic Letters. - : American Chemical Society (ACS). - 1523-7060 .- 1523-7052. ; 22:2, s. 417-421
- Journal article (peer-reviewed)
Abstract
Subject headings
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- A palladium-catalyzed oxidative cascade carbonylative carbocyclization of enallenols was developed. Under mild reaction conditions, a range of cis-fused [5,5] bicyclic gamma-lactones and gamma-lactams with a 1,3-diene motif were obtained in good yields with high diastereoselectivity. The obtained lactone/lactam products are viable substrates for a stereoselective Diels-Alder reaction with N-phenylmaleimide, providing polycyclic compounds with increased molecular complexity.
Subject headings
- NATURVETENSKAP -- Kemi -- Organisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Organic Chemistry (hsv//eng)
Keyword
- organisk kemi
- Organic Chemistry
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- ref (subject category)
- art (subject category)
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- Mid Sweden University
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