| 1. |
- Aggarwal, MM, et al.
(författare)
-
Centrality dependence of charged-neutral particle fluctuations in 158A (GeVPb)-Pb-208+Pb-208 collisions
- 2003
-
Ingår i: Physical Review C (Nuclear Physics). - 0556-2813. ; 67:4
-
Tidskriftsartikel (refereegranskat)abstract
- Results on the study of localized fluctuations in the multiplicity of charged particles and photons produced in 158A GeV/c Pb+Pb collisions are presented for varying centralities. The charged versus neutral particle multiplicity correlations in common phase space regions of varying azimuthal sizes are analyzed by two different methods. Various types of mixed events are constructed to probe fluctuations arising from different sources. The measured results are compared to those from simulations and from mixed events. The comparison indicates the presence of nonstatistical fluctuations in both the charged particle and photon multiplicities in limited azimuthal regions. However, no correlated charged-neutral fluctuations, a possible signature of formation of disoriented chiral condensates, are observed. An upper limit on the production of disoriented chiral condensates is set.
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| 2. |
- Aggarwal, MM, et al.
(författare)
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Event-by-event fluctuations in particle multiplicities and transverse energy produced in 158A GeVPb plus Pb collisions
- 2002
-
Ingår i: Physical Review C (Nuclear Physics). - 0556-2813. ; 65:5
-
Tidskriftsartikel (refereegranskat)abstract
- Event-by-event fluctuations in the multiplicities of charged particles and photons, and the total transverse energy in 158A GeV Pb+Pb collisions are studied for a wide range of centralities. For narrow centrality bins the multiplicity and transverse energy distributions are found to be near perfect Gaussians. The effect of detector acceptance on the multiplicity fluctuations has been studied and demonstrated to follow statistical considerations. The centrality dependence of the charged particle multiplicity fluctuations in the measured data has been found to agree reasonably well with those obtained from a participant model. However, for photons the multiplicity fluctuations have been found to be lower compared to those obtained from a participant model. The multiplicity and transverse energy fluctuations have also been compared to those obtained from the VENUS event generator.
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| 3. |
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| 4. |
- Aggarwal, MM, et al.
(författare)
-
Transverse mass distributions of neutral pions from Pb-208-induced reactions at 158 center dot A GeV
- 2002
-
Ingår i: European Physical Journal C. Particles and Fields. - : Springer Science and Business Media LLC. - 1434-6044. ; 23:2, s. 225-236
-
Tidskriftsartikel (refereegranskat)abstract
- Results on transverse mass spectra of neutral pious measured at central rapidity are presented for impact parameter selected 158-A GeV Pb + Pb-1 and Pb + Nb collisions. The distributions cover the range 0.5 GeV/c(2) less than or equal to MT - Mo less than or equal to 4 GeV/c(2). The change of the spectral shape and the multiplicity with centrality is studied in detail. In going from p+p to semi-peripheral Pb+Pb collisions there is a nuclear enhancement increasing with transverse mass similar to the well known Cronin effect, while for very central collisions this enhancement appears to be weaker than expected.
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| 5. |
- Baev, A., et al.
(författare)
-
Geometrical information on core-excited states obtained from interference quenching of vibrational states in resonant x-ray photoemission
- 2003
-
Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 67:2
-
Tidskriftsartikel (refereegranskat)abstract
- An interference quenching of the m=1 final state vibrational line in the resonant Auger decay of N 1s-->pi(*) core-excited N-2 is observed and analyzed. The intensity ratio between the m=1 and m=0 vibrational levels of the X (2)Sigma(g)(+) final state shows a surprising nonmonotonic variation as a function of frequency detuning, going through a minimum with a complete suppression of m=1. We have developed a simple model which indicates a linear relation between the value of the detuning frequency for this minimum and the equilibrium bond distance of the core-excited state. This implies the possibility of determining the equilibrium bond distances for core-excited states to a high degree of accuracy. Simultaneously with the simple model we present a strict theory of the studied effect. This strict theory allows us to explore the accuracy of determining the bond length of the core-excited state from resonant Auger spectra. We obtain a weak influence of the core-hole lifetime on the determined bond length, whereas the number of intermediate vibrational states accounted for in the numerical simulations seems to be quite important.
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| 6. |
- De Brito, A. N., et al.
(författare)
-
Evidence against atomiclike resonant auger decay in N2 doubly excited core states by high-resolution experiments
- 2001
-
Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947. ; 64:5, s. 547021-547024
-
Tidskriftsartikel (refereegranskat)abstract
- The resonant Auger decay spectra associated with doubly excited core-hole states near the N 1s threshold in the nitrogen molecule was measured. Electron-yield spectrum was obtained by setting a kinetic-energy window at 384 eV and scanning across the threshold region. At ground 410, 414, and 416 eV, photon energy, three dominant structures were observed. The increased signal-to-background ratio, intensity and resolution at third generation facilities were found to cast a different light on the dynamics of core photoionization in molecules.
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| 7. |
- Feifel, R., et al.
(författare)
-
Generalization of the duration-time concept for interpreting high-resolution resonant photoemission spectra
- 2004
-
Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 69:2, s. 022707-
-
Tidskriftsartikel (refereegranskat)abstract
- The duration-time concept, vastly successful for interpreting the frequency dependence of resonant radiative and nonradiative x-ray scattering spectra, is tested for fine-scale features that can be obtained with state of the art high-resolution spectroscopy. For that purpose resonant photoelectron (RPE) spectra of the first three outermost singly ionized valence states X (2)Sigma(g)(+), A (2)Pi(u), and B (2)Sigma(u)(+), are measured for selective excitations to different vibrational levels (up to n=13) of the N 1s-->pi(*) photoabsorption resonance in N-2 and for negative photon frequency detuning relative to the adiabatic 0-0 transition of this resonance. It is found that different parts of the RPE spectrum converge to the spectral profile of direct photoionization (fast scattering) for different detunings, and that the RPE profiles are asymmetrical as a function of frequency detuning. The observed asymmetry contradicts the picture based on the simplified notation of a common scattering duration time, but is shown to agree with the here elaborated concept of partial and mean duration times. Results of the measurements and the simulations show that the duration time of the scattering process varies for different final electronic and different final vibrational states. This owes to two physical reasons: one is the competition between the fast vertical and the slow resonant scattering channels and the other is the slowing down of the scattering process near the zeros of the real part of the scattering amplitude.
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| 8. |
- Feifel, R., et al.
(författare)
-
Interference quenching of nu('')=1 vibrational line in resonant photoemission of N-2 : A possibility to obtain geometrical information on the core-excited state
- 2002
-
Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 89:10
-
Tidskriftsartikel (refereegranskat)abstract
- An interference quenching of the nu=1 vibrational line in the resonant Auger decay of N 1s-->pi(*) core-excited N-2 is observed and analyzed. The intensity ratio between the nu=1 and nu=0 vibrational levels of the X(2)Sigma(g)(+) final state shows a surprising nonmonotonous variation as a function of frequency detuning, going through a minimum with a complete suppression of nu=1. We have developed a simple model which shows a linear relation between the value of the detuning frequency for this minimum and the equilibrium bond distance R-c(0) of the core-excited state. A new way is thus established of determining the equilibrium bond distance for the core-excited state with a precision deltaR(c)(0)<10(-3) Angstrom.
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| 9. |
- Feifel, R, et al.
(författare)
-
Observation of a continuum-continuum interference hole in ultrafast dissociating core-excited molecules
- 2000
-
Ingår i: Physical Review Letters. - : AIP Publishing. - 0031-9007 .- 1079-7114. ; 85:15, s. 3133-3136
-
Tidskriftsartikel (refereegranskat)abstract
- The femtosecond dissociation of HCl after core excitation has been studied through the resonant Auger decay. The spectra contain contributions from decay occurring at both "molecular" and "atomic" internuclear distances. We have observed a new interference mechanism in these spectra: An atomic spectral line develops into a negative spectral contribution, a "hole," when detuning the excitation energy from the maximum of the Cl 2p(-1)sigma* resonance. Resonant x-ray scattering theory quantitatively explains this behavior as due to a novel destructive continuum-Continuum interference between molecular and atomic contributions to the Auger decay.
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| 10. |
- Feifel, R., et al.
(författare)
-
Role of stray light in the formation of high-resolution resonant photoelectron spectra : an experimental and theoretical study of N-2
- 2004
-
Ingår i: Journal of Electron Spectroscopy and Related Phenomena. - : Elsevier BV. - 0368-2048 .- 1873-2526. ; 134:1, s. 49-65
-
Tidskriftsartikel (refereegranskat)abstract
- We show that the undular stray light, diffusely scattered by the optical system of a synchrotron beamline, can play an important role in the formation of high-resolution resonant photoelectron (RPE) spectra. The influence of the stray light is mediated through the Stokes doubling effect, with the Lorentzian tail of the spectral function being replaced by a more complicated form. This effect is shown to appear in the high-resolution resonant photoelectron spectrum of the N-2 molecule in which the spectral shape of the non-Raman (NR) bands differs qualitatively for the A(2)Pi(u) and X(2)Sigma(g)(+) final states. A particularly large enhancement of the non-Raman Stokes line is observed for the A-state while the picture is inverted for the X-state where the non-Raman band is suppressed. It is shown that the resonant photoemission profile is affected by two qualitatively different detunings, the detuning of the monochromatized line relative to the photoabsorption line and the detuning of the undulator harmonic relative to the same reference line. The experimental data show that the relative intensity of the non-Raman line strongly depends on the tuning of the undulator harmonic with respect to the selected monochromator bandpass, leading to a strong decrease of the Stokes line intensity for certain undulator detunings. A clear red-shift asymmetry for the decrease in the Stokes line intensity is observed when the monochromator line is detuned towards negative photon frequencies, whereas the picture is reverted for the situation of a positively detuned monochromator line. The results show the necessity to control the stray light and to investigate both the Raman and non-Raman contributions to the spectral profiles in order to avoid misinterpretation and in order to make full use of the information available in resonant photoemission spectra of molecules.
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| 11. |
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| 12. |
- Karlsson, J, 1966-, et al.
(författare)
-
Sequencing of the Francisella tularensis strain Schu 4 genome reveals the shikimate and purine metabolic pathways, targets for the construction of a rationally attenuated auxotrophic vaccine.
- 2000
-
Ingår i: Microbial & Comparative Genomics. - : Mary Ann Liebert Inc. - 1090-6592 .- 2168-6637. ; 5:1, s. 25-39
-
Tidskriftsartikel (refereegranskat)abstract
- Francisella tularensis is the etiological agent of tularemia, a serious disease in several Northern hemisphere countries. The organism has fastidious growth requirements and is very poorly understood at the genetic and molecular levels. Given the lack of data on this organism, we undertook the sample sequencing of its genome. A random library of DNA fragments from a highly virulent strain (Schu 4) of F. tularensis was constructed and the nucleotide sequences of 13,904 cloned fragments were determined and assembled into 353 contigs. A total of 1.83 Mb of nucleotide sequence was obtained that had a G+C content of 33.2%. Genes located on plasmids pOM1 and pNFL10, which had been previously isolated from low virulence strains of F. tularensis, were absent but all of the other known F. tularensis genes were represented in the assembled data. F. tularensis Schu4 was able to grow in the absence of aromatic amino acids and orthologues of genes which could encode enzymes in the shikimate pathway in other bacteria were identified in the assembled data. Genes that could encode all of the enzymes in the purine biosynthetic and most of the en- zymes in the purine salvage pathways were also identified. This data will be used to develop defined rationally attenuated mutants of F. tularensis, which could be used as replacements for the existing genetically undefined live vaccine strain.
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| 13. |
- Kelsall, N. S., et al.
(författare)
-
Testing mean-field models near the N=Z line : gamma-ray spectroscopy of the T-z=1/2 nucleus Kr-73
- 2002
-
Ingår i: Physical Review C. Nuclear Physics. - 0556-2813 .- 1089-490X. ; 65:4
-
Tidskriftsartikel (refereegranskat)abstract
- Excited states in the N=Z+1 nucleus Kr-73 have been investigated using the Ca-40(Ar-36,2pn) and Ca-40(Ca-40,alpha2pn) reactions at 145 and 160 MeV, respectively. gamma rays were detected using the Gammasphere array and events were recorded in coincidence with charged-particle and neutron detectors. The three previously observed bands were extended to high spin, and a new unfavored positive-parity band has been observed. The alignment characteristics and decay properties of the bands are all consistent with large-deformation prolate rotation, with no clear evidence for oblate bands or shape coexistence. This is quite different from neighboring Kr-72,Kr-74, indicating a strong shape-stabilizing role for the valence neutron. The experimental results are compared to extended total Routhian surface, cranked Nilsson Strutinsky, and cranked relativistic mean-field calculations. The results suggest that the paired calculations lack some important physics. Neutron-proton correlations may be the missing ingredient. There is also evidence for an unusual band crossing in the negative-parity bands, which may indicate the presence of T=0 pairing correlations. At high spin all the models can reproduce the experimental data.
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| 14. |
- Miron, C., et al.
(författare)
-
Nuclear motion driven by the Renner-Teller effect as observed in the resonant Auger decay to the X̃2Π electronic ground state of N2O
- 2001
-
Ingår i: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 115:2, s. 864-869
-
Tidskriftsartikel (refereegranskat)abstract
- The nuclear dynamics in the Nt 1s→π* in nitrous oxide was studied using the high resolution resonant Auger spectroscopy and ab initio quantum chemical calculations. For probing the nuclear motion of the system in the core-excited state, the frequency detuning technique was used. The results showed changes in vibrational structure for the Auger decay spectra and a strong influence of nuclear motion on the electronic decay.
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| 15. |
- Salek, Pawel, et al.
(författare)
-
Dynamical suppression of atomic peaks in resonant dissociative photoemission
- 2001
-
Ingår i: Chemical Physics Letters. - 0009-2614 .- 1873-4448. ; 343:3-4, s. 332-338
-
Tidskriftsartikel (refereegranskat)abstract
- Resonant excitation to the F1s-sigma* dissociative state in hydrogen fluoride gives a photoelectron spectrum where the spectator part contains strong atomic lines but a participator part where such lines are lacking. We demonstrate that this contrasting behaviour between the two parts is due to a strong dynamical suppression of the resonant contribution, making direct main state photoionization the dominating channel even at resonant conditions.
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| 16. |
- Achtziger, N, et al.
(författare)
-
Formation of passivated layers in p-type SiC by low energy ion implantation of hydrogen
- 2000
-
Ingår i: SILICON CARBIDE AND RELATED MATERIALS - 1999 PTS, 1 & 2. ; , s. 933-936
-
Konferensbidrag (refereegranskat)abstract
- The mobility of hydrogen and its passivating effect on accepters in p-type SiC is investigated. Hydrogen (isotope H-1 or H-2 alternatively) is implanted at temperatures between 300 K and 680 K with low energy (300 eV per atom) in order to minimize implantation damage. The depth profiles of 2H and of passivated accepters correspond closely. Up to 500 K, a fully passivated layer with a well defined thickness is formed. Its depth ton the order of 1 micrometer) is investigated as a function of doping level and hydrogen fluence. At higher temperatures, the incorporation drastically increases, but the electrical passivation is partial only. Qualitative explanations are given.
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| 17. |
- Allen, D.H., et al.
(författare)
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Modeling the viscoelastic response of GMT structural components
- 2001
-
Ingår i: Composites Science And Technology. - 0266-3538 .- 1879-1050. ; 61:4, s. 503-515
-
Tidskriftsartikel (refereegranskat)abstract
- A glass-mat-reinforced thermoplastic (GMT) composite material has been fabricated from randomly oriented continuous glass fibers embedded in a polypropylene matrix. The mechanical constitution of this composite has been characterized by using a linear viscoelastic micromechanically based material model. This material model has subsequently been implemented to several finite-element computer codes for analysis of structural components fabricated from polypropylene GMT. In this paper several example problems have been studied in order to determine the applicability of this modeling approach to predicting time-dependent deformations due to creep in GMT components. These example problems have been solved by utilizing two commercially available codes: ABAQUS, and ANSYS. Furthermore, results obtained with the codes have been compared to both analytic and experimental results, with varying degrees of success. The paper details these results for each of the example problems considered herein. © 2001 Elsevier Science Ltd. All rights reserved.
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| 18. |
- Andreoiu, Corina, et al.
(författare)
-
Yrast Superdeformed Band in 59Cu
- 2000
-
Ingår i: Physical Review C (Nuclear Physics). - 0556-2813. ; 62:5, s. 513011-513015
-
Tidskriftsartikel (refereegranskat)abstract
- High-spin states in 59Cu were populated using the fusion-evaporation reactions 28Si+40Ca at a beam energy of 125 MeV and 36Ar+28Si at a beam energy of 143 MeV. The Gammasphere array in conjunction with ancillary detector systems allowed for the identification of a superdeformed rotational band in 59Cu, which was firmly linked to low-spin yrast states. Using directional correlations of oriented states, a spin-parity assignment of Iπ = 25/2+ to the band head was possible. The average quadrupole moment of the band is measured to be Qt = (2.24±0.40) e b. The characteristics of the band are compared to neighboring nuclei and predictions of different mean-field theories.
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| 19. |
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| 20. |
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| 21. |
- Baev, A, et al.
(författare)
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Picturing molecular femtosecond processes through an ultra-fast controllable X-ray shutter
- 2003
-
Ingår i: Chemical Physics. - 0301-0104 .- 1873-4421. ; 289, s. 51-56
-
Tidskriftsartikel (refereegranskat)abstract
- We show that frequency detuning in a resonant X-ray scattering experiment acts as an X-ray camera shutter by regulating the duration time of the scattering process. The camera shutter can be used to select processes at different time scales for observation. This is illustrated by a resonant Auger study of the ultra-fast dissociation of the core-excited HF molecule. We present experimental results and first principle simulations of the molecular fraction in the resonant Auger spectra of HF which is a dynamical parameter that well illustrates X-ray shutter controlled dissociation.
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| 22. |
- Björneholm, O., et al.
(författare)
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Doppler splitting of in-flight auger decay of dissociating oxygen molecules : The localization of delocalized core holes
- 2000
-
Ingår i: Physical Review Letters. - : AMERICAN PHYSICAL SOC. - 0031-9007 .- 1079-7114. ; 84:13, s. 2826-2829
-
Tidskriftsartikel (refereegranskat)abstract
- By exploiting the core-excitation-induced dissociation of O-2, we find that the Auger emission exhibits a Doppler-like energy shift. We show this to be a manifestation of localization of the core hole and propose that the problem of core-hole localization versus delocalization in core-hole spectroscopies may be resolved by considering the nature of the measurement.
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| 23. |
- Christensen, Torben, et al.
(författare)
-
Biotic controls on CO2 and CH4 exchange in wetlands - a closed environment study
- 2003
-
Ingår i: Biogeochemistry. - 0168-2563 .- 1573-515X. ; 64:3, s. 337-354
-
Tidskriftsartikel (refereegranskat)abstract
- Wetlands are significant sources of the important greenhouse gas CH4. Here we explore the use of an experimental system developed for the determination of continuous fluxes of CO2 and CH4 in closed ecosystem monoliths including the capture of (CO2)-C-14 and (CH4)-C-14 following pulse labelling with (CO2)-C-14. We show that, in the ecosystem studied, ebullition (bubble emission) may account for 18 to 50% of the total CH4 emission, representing fluxes that have been difficult to estimate accurately in the past. Furthermore, using plant removal and C-14 labelling techniques, we use the system to detail the direct influence of vascular plants on CH4 emission. This influence is observed to be dependent on the amount of vascular plants present. The results that may be produced using the presented experimental set-up have implications for an improved understanding of wetland ecosystem/atmosphere interactions, including possible feedback effects on climate change. In recent years much attention has been devoted to ascertaining and subsequently using the relationship between net ecosystem productivity and CH4 emission as a basis for extrapolation of fluxes across large areas. The experimental system presented may be used to study the complex relationship between vascular plants and CH4 emission and here we show examples of how this may vary considerably in nature between and even within ecosystems.
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| 24. |
- Christensen, Torben, et al.
(författare)
-
Factors controlling large scale variations in methane emissions from wetlands
- 2003
-
Ingår i: Geophysical Research Letters. - 0094-8276 .- 1944-8007. ; 30:7
-
Tidskriftsartikel (refereegranskat)abstract
- [1] Global wetlands are, at estimate ranging 115-237 Tg CH4/yr, the largest single atmospheric source of the greenhouse gas methane (CH4). We present a dataset on CH4 flux rates totaling 12 measurement years at sites from Greenland, Iceland, Scandinavia and Siberia. We find that temperature and microbial substrate availability (expressed as the organic acid concentration in peat water) combined explain almost 100% of the variations in mean annual CH4 emissions. The temperature sensitivity of the CH4 emissions shown suggests a feedback mechanism on climate change that could validate incorporation in further developments of global circulation models.
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| 25. |
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| 26. |
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| 27. |
- de Villiers, SHL, et al.
(författare)
-
Active immunization against nicotine suppresses nicotine-induced dopamine release in the rat nucleus accumbens shell
- 2002
-
Ingår i: Respiration. - : S. Karger AG. - 0025-7931 .- 1423-0356. ; 69:3, s. 247-253
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Tidskriftsartikel (refereegranskat)abstract
- <i>Background:</i> Tobacco smoking is the largest preventable cause of morbidity and premature mortality in the world. Although its medical consequences are well documented, 20–50% of the population even in developed countries remain tobacco smokers. The drugs presently used in smoking cessation have limited efficiency and, therefore, there is a need for alternative and improved treatments. One novel approach in this regard may be provided by immunization against nicotine. <i>Objective:</i> The present study in male Wistar rats investigated if active immunization with a novel nicotine immunogen, IP18-KLH, may generate nicotine-selective antibodies and, furthermore, whether this treatment might prevent nicotine from exerting its stimulating effect on the mesolimbic, dopaminergic reward system in the brain. <i>Methods:</i> Enzyme-linked immunosorbent assay (ELISA) was used to determine the titer of nicotine antibodies in plasma after immunization with IP18-KLH in Freund’s adjuvant. Competitive ELISA was used to assess the selectivity of the antibodies. Finally, we used in vivo voltammetry to investigate whether active immunization with IP18-KLH could prevent nicotine-induced dopamine release in the shell of nucleus accumbens (NAC<sub>shell</sub>). <i>Results:</i> The present study shows that active immunization with IP18-KLH generates antibodies that are highly selective for nicotine. Furthermore, immunization with IP18-KLH prevented the nicotine-induced increase in dopamine release in the NAC<sub>shell</sub>, a biochemical correlate to the rewarding properties of nicotine. <i>Conclusions:</i> Active immunization with IP18-KLH prevents a central effect of nicotine that is considered critical for the induction of nicotine dependence. Consequently, active immunization may provide long-term protection against initiation of tobacco dependence, an effect that may prove particularly advantageous in relapse prevention.
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| 28. |
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| 29. |
- Feifel, R., et al.
(författare)
-
"Hidden" vibrations in CO : Reinvestigation of resonant Auger decay for the C 1s → π* excitation
- 2002
-
Ingår i: Physical Review A - Atomic, Molecular, and Optical Physics. - 1050-2947. ; 65:5 A, s. 527011-527018
-
Tidskriftsartikel (refereegranskat)abstract
- The higher vibrational levels of the C 1s→π* excitation in carbon monooxide (CO) were investigated by using resonant Auger electron spectroscopy. The absorption profile of the CO was recorded in the partial electron yield mode. The results showed that the vibrational states were not seen in a total yield absorption spectrum whereas they were shown to be discernable in a partial electron yield spectrum.
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| 30. |
- Feifel, R., et al.
(författare)
-
Profile of resonant photoelectron spectra versus the spectral function width and photon frequency detuning
- 2004
-
Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 70:3
-
Tidskriftsartikel (refereegranskat)abstract
- The outermost, singly ionized valence state of N-2, the X (2)Sigma(g)(+) state, is investigated in detail as a function of the photon frequency bandwidth for core excitation to the N 1s-->pi(*) resonance, where the photon frequency is tuned in between the first two vibrational levels of this bound intermediate electronic state. We find a strong, nontrivial dependence of the resulting resonant photoemission spectral profile on the monochromator function width and the frequency of its peak position. For narrow bandwidth excitation we observe a well resolved vibrational fine structure in the final electron spectrum, which for somewhat broader bandwidths gets smeared out into a continuous structure. For even broader monochromator bandwidths, it converts again into a well resolved vibrational progression. In addition, spectral features appearing below the adiabatic transition energy of the ground state of N-2(+) are observed for broadband excitation. A model taking into account the interplay of the partial scattering cross section with the spectral function is presented and applied to the X (2)Sigma(g)(+) final state of N-2(+).
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| 31. |
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| 32. |
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| 33. |
- H. Wang, R. F. Fink, M. N. Piancastelli, M. Bässler, I. Hjelte, O. Björneholm, F. Burmeister, R. Feifel, A. Giertz, C. Miron, S. L. Sorensen, K. Wiesner and S. Svensson
(författare)
-
Is there Interference in the Resonant Auger Electron Spectra of N 1s and O 1s -> 2p Core Excited NO?
- 2003
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Ingår i: Chem Phys.. ; :289, s. 31-
-
Tidskriftsartikel (refereegranskat)
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| 34. |
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| 35. |
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| 36. |
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| 37. |
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| 38. |
- Hjelte, I., et al.
(författare)
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Evidence for ultra-fast dissociation of molecular water from resonant Auger spectroscopy
- 2001
-
Ingår i: Chemical Physics Letters. - 0009-2614. ; 334:1-3, s. 151-158
-
Tidskriftsartikel (refereegranskat)abstract
- We present direct evidence for ultra-fast dissociation of molecular water in connection photo-excitation of the O1s→4a1 resonance. The core-excited H2O molecules are shown to dissociate into core-excited O*H and neutral H on a time scale comparable to the core hole lifetime, i.e. a few femtoseconds. This conclusion is based on a resonant Auger study, qualitative arguments and ab initio calculations. 'Hot bands' connected to Auger transitions from vibrationally excited OH fragments are identified, and these exhibit a dynamical behavior which qualitatively follows the change in excess energy.
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| 39. |
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| 40. |
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| 41. |
- Janson, Martin S., et al.
(författare)
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Hydrogen in the wide bandgap semiconductor silicon carbide
- 2004
-
Ingår i: Physica Scripta. - 0031-8949 .- 1402-4896. ; T108, s. 99-112
-
Tidskriftsartikel (refereegranskat)abstract
- In this paper we give a review of our recent results related to the incorporation of hydrogen (H) in silicon carbide (SiC) and its interaction with acceptor doping atoms and implantation induced defects. Hydrogen is an abundant impurity in the growth of epitaxial SiC since it is present in the precursor gases and since H-2 is used as the carrier gas. High concentrations of hydrogen are indeed incorporated into highly doped p-type epi-layers and it is shown that the main source is the carrier gas. Furthermore, it is revealed that the entire substrate becomes homogeneously filled with hydrogen during growth and that this hydrogen is more thermally stable than that in the epi-layer. Incorporation of hydrogen from an H-2 ambient, at temperatures considerably lower than those used for epitaxy, is also demonstrated in p-type samples coated with a catalytic metal film. This effect is most likely the cause for the increased series resistance observed in p-type SiC Schottky sensor devices using a catalytic metal gate after annealing at 600 degrees C in a H-2 containing ambient. Hydrogen is found to passivate the acceptors Al and B by forming electrically neutral H-acceptor complexes. Unlike in Si and GaAs, the two H-acceptor complexes in SiC exhibit very different dissociation energies, suggesting that the atomic configurations of the complexes are significantly different. The migration of mobile hydrogen in the presence of externally applied, or internal built-in, electric fields further reveals that hydrogen is present as H+ in p-type SiC. Finally, the redistribution and subsequent out-diffusion of low energy implanted H-1 and H-2 is investigated. Two annealing phases for the redistribution are observed, and the activation energies for the processes are extracted.
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| 42. |
- Janson, M. S., et al.
(författare)
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Transient enhanced diffusion of implanted boron in 4H-silicon carbide
- 2000
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Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 76:11, s. 1434-1436
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Tidskriftsartikel (refereegranskat)abstract
- Experimental evidence is given for transient enhanced diffusion of boron (B) in ion-implanted silicon carbide (SiC). The implanted B is diffusing several mu m into the samples when annealed at 1600 and 1700 degrees C for 10 min, but the in-diffused tails remain unaffected when the annealing times are increased to 30 min at the same temperatures. A lower limit of the effective B diffusivity at 1600 degrees C is determined to 7x10(-12) cm(2)/s, which is 160 times larger than the equilibrium B diffusivity given in the literature.
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| 43. |
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| 44. |
- Jonsson, Rolf, et al.
(författare)
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Evaluation of SiC MESFET structures using large-signal time-domain simulations
- 2002
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Ingår i: Materials Science Forum Vols. 389-393. ; , s. 1395-1398
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Konferensbidrag (refereegranskat)abstract
- When designing transistors for microwave power applications a good understanding of their large signal behaviour in a real circuit context is essential. We have used the device simulator Medici in a novel way to simulate the large signal high frequency time domain properties of different SiC MESFET structures. The simulations show that even for transistors with good DC properties the exact design of the channel-buffer and the buffer-substrate regions is important when a good high power RF performance is required. Our simulations indicate that output power densities above 6W/mm are possible if heating problems are solved.
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| 45. |
- Kelsall, N.S., et al.
(författare)
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High-spin studies of N ~ Z nuclei in the mass 70 region
- 2003
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Ingår i: AIP Conference Proceedings. - 0094-243X .- 1551-7616. ; :656, s. 261-268
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Konferensbidrag (refereegranskat)abstract
- High-spin states have been studied in 72,73Kr using 40Ca+40Ca and 36Ar+40Ca reactions at 160, 164 and 145 MeV respectively. The properties and configurations of the bands observed are interpreted with the aid of unpaired cranked Nilsson-Strutinsky/ cranked relativistic mean-field calculations and paired total routhian surface and cranked relativistic Hartree-Bogoliubov calculations. In 73Kr the three previously known structures have been extended to a spin of ~30[h-bar] and a fourth structure, which is believed to be the signature partner to the g9/2 band, has been identified. The negative parity bands show evidence for an unusual type of band crossing. It is currently unclear whether this is a consequence of T=0 n-p pairing. At the highest spins the unpaired calculations can reproduce the observed data, suggesting that there is little evidence for pairing correlations in this spin regime. In 72Kr a new band has been identified that has the properties expected from the missing doubly aligned S-band configuration. The properties of this band can be reproduced by the unpaired CNS/ CRMF calculations, again suggesting that the structure has little pairing. However, paired calculations appear to be necessary to reproduce the properties of the previously known structure in this nucleus. The 72Kr results are also compared with projected shell model calculations. ©2003 American Institute of Physics
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| 46. |
- Kortegaard Nielsen, Hanne, et al.
(författare)
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Electrically active defects in silicon produced by ion channeling
- 2003
-
Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 82:22, s. 3865-3867
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Tidskriftsartikel (refereegranskat)abstract
- Low-dose implantations with 65 Si and 150 keV Ge ions into the n(+) top layer of Si n(+)p diodes have been carried out. The defects produced in deeper-lying layers were studied by deep level transient spectroscopy. Results were compared to crystal-TRIM calculations and results from 2 MeV electron irradiations. Previously, ion channeling was disregarded in studies on point defect migration at room temperature using ion implantation in surface layers. In our studies, ion channeling is dominant and it overwhelms any contribution from point defect diffusion.
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| 47. |
- Kuznetsov, A. Y., et al.
(författare)
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Self-interstitial migration during ion irradiation of boron delta-doped silicon
- 2000
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Ingår i: Materials Science in Semiconductor Processing. - 1369-8001 .- 1873-4081. ; 3:4, s. 279-283
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Tidskriftsartikel (refereegranskat)abstract
- Boron delta layers in silicon, grown by molecular beam epitaxy and characterized by the secondary ion mass spectrometry, have been employed to investigate the migration of silicon self-interstitials during irradiation with MeV protons in the 500-850 degreesC temperature range. After growth, the samples were thinned from the backside to a thickness that made them transparent for the proton energies used. As a result, the generation rate of point defects can be considered as essentially uniform throughout the samples. However: the evolution of the boron profiles is almost identical to that observed after injection of self-interstitials caused by thermal oxidation of the samples at elevated temperature. This strongly indicates that the surface acts as a reflective boundary for the migrating self-interstitials or/ and an efficient sink for mobile vacancies. Furthermore, higher value of interstitial supersaturation in the near-surface region in proton-irradiated samples is consistent with experimentally detected depth dependence for immobile fraction in boron clusters. Then, activation energy of boron mobilization, (0.9 +/- 0.4) eV, was attributed to the dissociation of boron clusters.
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| 48. |
- Lindblom, N, et al.
(författare)
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Active immunization against nicotine prevents reinstatement of nicotine-seeking behavior in rats
- 2002
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Ingår i: Respiration. - : S. Karger AG. - 0025-7931 .- 1423-0356. ; 69:3, s. 254-260
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Tidskriftsartikel (refereegranskat)abstract
- <i>Background:</i> The presently available pharmaceutical aids in smoking cessation possess a rather limited effectiveness. Therefore, we have synthesized a series of immunoconjugates that stimulate the induction of antibodies which may bind nicotine in the blood, thereby preventing it from passing the blood-brain barrier. Thus, the reinforcing action of nicotine in the brain, which is the driving force in tobacco smoking, should be abolished. <i>Objective:</i> The present study was undertaken to test this notion in a long-term relapse model in rats, measuring the reinstatement of nicotine-seeking behavior, following active immunization with IP18-KLH, one of our immunoconjugates. <i>Methods:</i> Male Wistar rats were immunized with a nicotine-KLH conjugate (nicotine immunogen) and Freund’s adjuvant after having been trained to meet the criteria of stable nicotine self-administration on a fixed ratio (FR3) schedule. The rats were subsequently extinguished from nicotine self-administration behavior and finally, as extinction was completed, they were exposed to small, priming doses of nicotine, which previously have been shown to reinstate the nicotine-seeking behavior. The antibody titers were measured by ELISA. <i>Results:</i> It was found that rats with high titers (>1:10,000) of antibodies against nicotine, in contrast to those with low/no nicotine selective antibodies, do not reinstate nicotine self-administration behavior when they are exposed to nicotine. <i>Conclusions:</i> Our findings indicate that active immunization against nicotine may effectively abolish the reinforcing action of nicotine in brain, an effect which is critical for relapse in nicotine dependence. These data suggest the potential utility of active immunization in smoking cessation programs.
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| 49. |
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| 50. |
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