| 1. |
- Carney Almroth, Bethanie, et al.
(författare)
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Understanding and addressing the planetary crisis of chemicals and plastics
- 2022
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Ingår i: One Earth. - : Elsevier BV. - 2590-3330 .- 2590-3322. ; 5:10, s. 1070-1074
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Tidskriftsartikel (refereegranskat)abstract
- Planetary functions are destabilized by the releases of large quantities and numbers of anthropogenic chemicals, which go beyond planetary boundaries and threaten the safe operating space for humanity. Here, we call for urgent action to mitigate these threats and identify opportunities for intervention along the impact pathway of anthropogenic chemicals, including plastics.
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| 2. |
- de Wit, Cynthia A., 1956-, et al.
(författare)
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Influence of climate change on persistent organic pollutants and chemicals of emerging concern in the Arctic : state of knowledge and recommendations for future research
- 2022
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Ingår i: Environmental Science. - : Royal Society of Chemistry (RSC). - 2050-7887 .- 2050-7895. ; 24:10, s. 1530-1543
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Forskningsöversikt (refereegranskat)abstract
- Persistent organic pollutants (POPs) have accumulated in polar environments as a result of long-range transport from urban/industrial and agricultural source regions in the mid-latitudes. Climate change has been recognized as a factor capable of influencing POP levels and trends in the Arctic, but little empirical data have been available previously. A growing number of recent studies have now addressed the consequences of climate change for the fate of Arctic contaminants, as reviewed and assessed by the Arctic Monitoring and Assessment Programme (AMAP). For example, correlations between POP temporal trends in air or biota and climate indices, such as the North Atlantic Oscillation Index, have been found. Besides the climate indices, temperature, precipitation and sea-ice were identified as important climate parameters influencing POP levels in the Arctic environment. However, the physical changes are interlinked with complex ecological changes, including new species habitats and predator/prey relationships, resulting in a vast diversity of processes directly or indirectly affecting levels and trends of POPs. The reviews in this themed issue illustrate that the complexity of physical, chemical, and biological processes, and the rapid developments with regard to both climate change and chemical contamination, require greater interdisciplinary scientific exchange and collaboration. While some climate and biological parameters have been linked to POP levels in the Arctic, mechanisms underlying these correlations are usually not understood and need more work. Going forward there is a need for a stronger collaborative approach to understanding these processes due to high uncertainties and the incremental process of increasing knowledge of these chemicals. There is also a need to support and encourage community-based studies and the co-production of knowledge, including the utilization of Indigenous Knowledge, for interpreting trends of POPs in light of climate change.
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| 3. |
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| 4. |
- Vorkamp, Katrin, et al.
(författare)
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Influences of climate change on long-term time series of persistent organic pollutants (POPs) in Arctic and Antarctic biota
- 2022
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Ingår i: Environmental Science. - : Royal Society of Chemistry (RSC). - 2050-7887 .- 2050-7895. ; 24:10, s. 1643-1660
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Forskningsöversikt (refereegranskat)abstract
- Time series of contaminants in the Arctic are an important instrument to detect emerging issues and to monitor the effectiveness of chemicals regulation, based on the assumption of a direct reflection of changes in primary emissions. Climate change has the potential to influence these time trends, through direct physical and chemical processes and/or changes in ecosystems. This study was part of an assessment of the Arctic Monitoring and Assessment Programme (AMAP), analysing potential links between changes in climate-related physical and biological variables and time trends of persistent organic pollutants (POPs) in Arctic biota, with some additional information from the Antarctic. Several correlative relationships were identified between POP temporal trends in freshwater and marine biota and physical climate parameters such as oscillation indices, sea-ice coverage, temperature and precipitation, although the mechanisms behind these observations remain poorly understood. Biological data indicate changes in the diet and trophic level of some species, especially seabirds and polar bears, with consequences for their POP exposure. Studies from the Antarctic highlight increased POP availability after iceberg calving. Including physical and/or biological parameters in the POP time trend analysis has led to small deviations in some declining trends, but did generally not change the overall direction of the trend. In addition, regional and temporary perturbations occurred. Effects on POP time trends appear to have been more pronounced in recent years and to show time lags, suggesting that climate-related effects on the long time series might be gaining importance.
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| 5. |
- Yuan, Bo, et al.
(författare)
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Dietary Intake Contributed the Most to Chlorinated Paraffin Body Burden in a Norwegian Cohort
- 2022
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Ingår i: Environmental Science and Technology. - : American Chemical Society (ACS). - 0013-936X .- 1520-5851. ; 56:23, s. 17080-17089
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Tidskriftsartikel (refereegranskat)abstract
- Determining the major human exposure pathways is a prerequisite for the development of effective management strategies for environmental pollutants such as chlorinated paraffins (CPs). As a first step, the internal and external exposure to CPs were quantified for a well-defined human cohort. CPs in participants’ plasma and diet samples were analyzed in the present study, and previous results on paired air, dust, and hand wipe samples were used for the total exposure assessment. Both one compartment pharmacokinetic modeling and forensic fingerprinting indicate that dietary intake contributed the most to body burden of CPs in this cohort, contributing a median of 60–88% of the total daily intakes. The contribution from dust ingestion and dermal exposure was greater for the intake of long-chain CPs (LCCPs) than short-chain CPs (SCCPs), while the contribution from inhalation was greater for the intake of SCCPs than medium-chain CPs (MCCPs) and LCCPs. Significantly higher concentrations of SCCPs and MCCPs were observed in diets containing butter and eggs, respectively (p < 0.05). Additionally, other exposure sources were correlated to plasma levels of CPs, including residence construction parameters such as the construction year (p < 0.05). This human exposure to CPs is not a local case. From a global perspective, there are major knowledge gaps in biomonitoring and exposure data for CPs from regions other than China and European countries.
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| 6. |
- Yuan, Bo, et al.
(författare)
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Temporal Trends and Age-Dependent Sex Differences in Chlorinated Paraffin Accumulation in Moose
- 2022
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Ingår i: Environmental Science and Technology Letters. - : American Chemical Society (ACS). - 2328-8930. ; 9:12, s. 1044-1049
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Tidskriftsartikel (refereegranskat)abstract
- Previous studies have found relatively high chlorinated paraffin (CP) concentrations in moose (Alces alces) compared with other wildlife from Scandinavia. To explore CP accumulation behaviors in this long-lived terrestrial mammal, temporal trends of muscle concentrations of CPs were first measured in samples collected over the past 40 years from moose calves from Grimsö, Sweden. The four CP classes, i.e., very-short-chain, short-chain, medium-chain, and long-chain (LCCPs) classes, showed similar temporal trends, with increasing concentrations from 1982 to the 1990s, relatively high levels in two time periods around 1993 and 2008, and decreasing concentrations after 2012. A concentration plateau period was identified, and moose samples of both sexes and different ages from the median year (1993) of the concentration plateau period were selected for further analysis. CP levels increased exponentially with age in the male moose, while CP levels were found to exponentially decrease with age in females. LCCPs showed the slowest decreasing tendency with age in females compared with the other three classes, resulting in a general increase of the LCCP proportions with age. The sex-biased accumulation of CPs indicates additional stresses from these POP-like chemicals toward males of the largest and one of the most widespread terrestrial mammals in northern hemisphere forests.
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