| 21. |
- Dzhigaev, D, et al.
(författare)
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Three-dimensional coherent x-ray diffraction imaging of ferroelastic domains in single CsPbBr3 perovskite nanoparticles
- 2021
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:6
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Tidskriftsartikel (refereegranskat)abstract
- Metal halide perovskites attract significant interest due to their remarkable performance in optoelectronic devices. However, the gap in understanding the relationship between their nanoscale structure and properties limits their application towards novel devices. In this work, twinned ferroelastic domains in single 500 nm CsPbBr3 particles are studied with 3D Bragg coherent x-ray diffraction imaging. A preferential double-domain structure is revealed in four identical particles, with one domain oriented along the [110] and the other along the [002] direction. The particles exhibit similar scattering volume ratios of 0.12 0.026 between twin phases, suggesting the possibility of a deterministic formation process. The domains exhibit a difference in lattice tilt of 0.59 degrees, in excellent agreement with calculations of the lattice mismatch at the (112) twin boundary. These results provide important insights both for the fundamental understanding of ferroelastic nanoscale materials and for the performance improvement of perovskite-based devices. Moreover, this work paves the way towards real-time imaging of the domain dynamics in ferroic systems.
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| 22. |
- Francesco Diotallevi, Giovanni, et al.
(författare)
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Steady-state entanglement production in a quantum thermal machine with continuous feedback control
- 2024
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Ingår i: New Journal of Physics. - 1367-2630. ; 26:5
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Tidskriftsartikel (refereegranskat)abstract
- Quantum thermal machines can generate steady-state entanglement by harvesting spontaneous interactions with local environments. However, using minimal resources and control, the entanglement is typically weak. Here, we study entanglement generation in a two-qubit quantum thermal machine in the presence of a continuous feedback protocol. Each qubit is measured continuously and the outcomes are used for real-time feedback to control the local system-environment interactions. We show that there exists an ideal operation regime where the quality of entanglement is significantly improved, to the extent that it can violate standard Bell inequalities and uphold quantum teleportation. In agreement with (Khandelwal et al 2020 New J. Phys. 22 073039), we also find, for ideal operation, that the heat current across the system is proportional to the entanglement concurrence. Finally, we investigate the robustness of entanglement production when the machine operates away from the ideal conditions.
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| 23. |
- Gallardo González, I., et al.
(författare)
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Effects of the dopant concentration in laser wakefield and direct laser acceleration of electrons
- 2018
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 20:5
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Tidskriftsartikel (refereegranskat)abstract
- In this work, we experimentally study the effects of the nitrogen concentration in laser wakefield acceleration of electrons in a gas mixture of hydrogen and nitrogen. A 15 TW peak power laser pulse is focused to ionize the gas, excite a plasma wave and accelerate electrons up to 230 MeV. We find that at dopant concentrations above 2% the total divergence of the electrons is increased and the high energy electrons are emitted preferentially with an angle of ±6 mrad, leading to a forked spatio-spectral distribution associated to direct laser acceleration (DLA). However, electrons can gain more energy and have a divergence lower than 4 mrad for concentrations below 0.5% and the same laser and plasma conditions. Particle-in-cell simulations show that for dopant concentrations above 2%, the amount of trapped charge is large enough to significantly perturb the plasma wave, reducing the amplitude of the longitudinal wakefield and suppressing other trapping mechanisms. At high concentrations the number of trapped electrons overlapping with the laser fields is increased, which rises the amount of charge affected by DLA. We conclude that the dopant concentration affects the quantity of electrons that experience significant DLA and the beam loading of the plasma wave driven by the laser pulse. These two mechanisms influence the electrons final energy, and thus the dopant concentration should be considered as a factor for the optimization of the electron beam parameters.
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| 24. |
- Gower, Artur, et al.
(författare)
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Effective waves for random three-dimensional particulate materials
- 2021
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:6
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Tidskriftsartikel (refereegranskat)abstract
- How do you take a reliable measurement of a material whose microstructure is random? When using wave scattering, the answer is often to take an ensemble average (average over time or space). By ensemble averaging we can calculate the average scattered wave and the effective wavenumber. To date, the literature has focused on calculating the effective wavenumber for a plate filled with particles. One clear unanswered question was how to extend this approach to a material of any geometry and for any source. For example, does the effective wavenumber depend on only the microstructure, or also on the material geometry? In this work, we demonstrate that the effective wavenumbers depend on only microstructure, though beyond the long wavelength limit there are multiple effective wavenumbers for one fixed incident frequency. We show how to calculate the average wave scattered from a random particulate material of any shape, and for broad frequency ranges. As an example, we show how to calculate the average wave scattered from a sphere filled with particles.
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| 25. |
- Gustafsson, Mats, et al.
(författare)
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Upper bounds on absorption and scattering
- 2020
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 22:7
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Tidskriftsartikel (refereegranskat)abstract
- A general framework for determining fundamental bounds in nanophotonics is introduced in this paper. The theory is based on convex optimization of dual problems constructed from operators generated by electromagnetic integral equations. The optimized variable is a contrast current defined within a prescribed region of a given material constitutive relations. Two power conservation constraints analogous to the optical theorem are utilized to tighten the bounds and to prescribe either losses or material properties. Thanks to the utilization of matrix rank-1 updates, modal decompositions, and model order reduction techniques, the optimization procedure is computationally efficient even for complicated scenarios. No dual gaps are observed. The method is well-suited to accommodate material anisotropy and inhomogeneity. To demonstrate the validity of the method, bounds on scattering, absorption, and extinction cross sections are derived first and evaluated for several canonical regions. The tightness of the bounds is verified by comparison to optimized spherical nanoparticles and shells. The next metric investigated is bi-directional scattering studied closely on a particular example of an electrically thin slab. Finally, the bounds are established for Purcell's factor and local field enhancement where a dimer is used as a practical example.
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| 26. |
- Korten, Till, et al.
(författare)
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Design of network-based biocomputation circuits for the exact cover problem
- 2021
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:8
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Tidskriftsartikel (refereegranskat)abstract
- Exact cover is a non-deterministic polynomial time (NP)-complete problem that is central to optimization challenges such as airline fleet planning and allocation of cloud computing resources. Solving exact cover requires the exploration of a solution space that increases exponentially with cardinality. Hence, it is time- and energy consuming to solve large instances of exact cover by serial computers. One approach to address these challenges is to utilize the inherent parallelism and high energy efficiency of biological systems in a network-based biocomputation (NBC) device. NBC is a parallel computing paradigm in which a given combinatorial problem is encoded into a graphical, modular network that is embedded in a nanofabricated planar device. The network is then explored in parallel using a large number of biological agents, such as molecular-motor-propelled protein filaments. The answer to the combinatorial problem can then be inferred by measuring the positions through which the agents exit the network. Here, we (i) show how exact cover can be encoded and solved in an NBC device, (ii) define a formalization that allows to prove the correctness of our approach and provides a mathematical basis for further studying NBC, and (iii) demonstrate various optimizations that significantly improve the computing performance of NBC. This work lays the ground for fabricating and scaling NBC devices to solve significantly larger combinatorial problems than have been demonstrated so far.
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| 27. |
- Maitrallain, A., et al.
(författare)
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Parametric study of high-energy ring-shaped electron beams from a laser wakefield accelerator
- 2022
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 24:1
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Tidskriftsartikel (refereegranskat)abstract
- Laser wakefield accelerators commonly produce on-axis, low-divergence, high-energy electron beams. However, a high charge, annular shaped beam can be trapped outside the bubble and accelerated to high energies. Here we present a parametric study on the production of low-energy-spread, ultra-relativistic electron ring beams in a two-stage gas cell. Ring-shaped beams with energies higher than 750 MeV are observed simultaneously with on axis, continuously injected electrons. Often multiple ring shaped beams with different energies are produced and parametric studies to control the generation and properties of these structures were conducted. Particle tracking and particle-in-cell simulations are used to determine properties of these beams and investigate how they are formed and trapped outside the bubble by the wake produced by on-axis injected electrons. These unusual femtosecond duration, high-charge, high-energy, ring electron beams may find use in beam driven plasma wakefield accelerators and radiation sources.
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| 28. |
- Maroju, P. K., et al.
(författare)
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Analysis of two-color photoelectron spectroscopy for attosecond metrology at seeded free-electron lasers
- 2021
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:4
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Tidskriftsartikel (refereegranskat)abstract
- The generation of attosecond pulse trains at free-electron lasers opens new opportunities in ultrafast science, as it gives access, for the first time, to reproducible, programmable, extreme ultraviolet (XUV) waveforms with high intensity. In this work, we present a detailed analysis of the theoretical model underlying the temporal characterization of the attosecond pulse trains recently generated at the free-electron laser FERMI. In particular, the validity of the approximations used for the correlated analysis of the photoelectron spectra generated in the two-color photoionization experiments are thoroughly discussed. The ranges of validity of the assumptions, in connection with the main experimental parameters, are derived.
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| 29. |
- Miranda, M. Sanchez, et al.
(författare)
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Prospects for single-molecule electrostatic detection in molecular motor gliding motility assays
- 2021
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:6
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Tidskriftsartikel (refereegranskat)abstract
- Molecular motor gliding motility assays based on myosin/actin or kinesin/microtubules are of interest for nanotechnology applications ranging from cargo-trafficking in lab-on-a-chip devices to novel biocomputation strategies. Prototype systems are typically monitored by expensive and bulky fluorescence microscopy systems. The development of integrated, direct electric detection of single filaments would strongly benefit applications and scale-up. We present estimates for the viability of such a detector by calculating the electrostatic potential change generated at a carbon nanotube transistor by a motile actin filament or microtubule under realistic gliding assay conditions. We combine this with detection limits based on previous state-of-the-art experiments using carbon nanotube transistors to detect catalysis by a bound lysozyme molecule and melting of a bound short-strand DNA molecule. Our results show that detection should be possible for both actin and microtubules using existing low ionic strength buffers given good device design, e.g., by raising the transistor slightly above the guiding channel floor. We perform studies as a function of buffer ionic strength, height of the transistor above the guiding channel floor, presence/absence of the casein surface passivation layer for microtubule assays and the linear charge density of the actin filaments/microtubules. We show that detection of microtubules is a more likely prospect given their smaller height of travel above the surface, higher negative charge density and the casein passivation, and may possibly be achieved with the nanoscale transistor sitting directly on the guiding channel floor.
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| 30. |
- Nicolaï, L., et al.
(författare)
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Bi ultra-thin crystalline films on InAs(1 1 1)A and B substrates : A combined core-level and valence-band angle-resolved and dichroic photoemission study
- 2019
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 21:12
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Tidskriftsartikel (refereegranskat)abstract
- The growth of Bi on both the In-terminated (A) face and the As-terminated (B) face of InAs(1 1 1) has been investigated by low-energy electron diffraction, scanning tunnelling microscopy, and photoelectron spectroscopy using synchrotron radiation. The changes upon Bi deposition of the In 4d and Bi 5d5/2 photoelectron signals allow to get a comprehensive picture of the Bi/InAs(1 1 1) interface. From the early stage the Bi growth on the A face is epitaxial, contrary to that on the B face that proceeds via the formation of islands. Angle-resolved photoelectron spectra show that the electronic structure of a Bi deposit of ≈10 bi-layers on the A face is identical to that of bulk Bi, while more than ≈30 bi-layers are needed for the B face. Both bulk and surface electronic states observed are well accounted for by fully relativistic ab initio calculations performed using the one-step model of photoemission. These calculations are used to analyse the dichroic photoemission data recorded in the vicinity of the Fermi level around the Γ&bar; point of the Brillouin zone.
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