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Träfflista för sökning "WFRF:(Matic Aleksandar 1968) "

Sökning: WFRF:(Matic Aleksandar 1968)

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  • Iselau, Frida, 1979, et al. (författare)
  • Competitive adsorption of amylopectin and amylose on cationic nanoparticles: a study on the aggregation mechanism
  • 2016
  • Ingår i: Soft Matter. - 1744-6848 .- 1744-683X. ; 12:14, s. 3388-3397
  • Tidskriftsartikel (refereegranskat)abstract
    • In this study we investigate the interactions between cationic nanoparticles and anionic starch, where the starch was composed of 20 wt% of amylose, a linear polymer, and 80 wt% of amylopectin, a branched polymer. The mechanism of aggregation was investigated by scattering techniques. It was found that the cationic particles formed large aggregates with the starch as a result of selective adsorption of the amylopectin. Amylose did not participate significantly in the aggregate formation even when the charge ratio of starch to particles was
  • Iselau, Frida, 1979, et al. (författare)
  • Formation and relaxation kinetics of starch-particle complexes
  • 2016
  • Ingår i: Soft Matter. - 1744-6848 .- 1744-683X. ; 12:47, s. 9509-9519
  • Tidskriftsartikel (refereegranskat)abstract
    • © The Royal Society of Chemistry.The formation and relaxation kinetics of starch-particle complexes were investigated in this study. The combination of cationic nanoparticles in suspension and anionic starch in solution gave rise to aggregate formation which was studied by dynamic light scattering, revealing the initial adsorption of the starch molecules on the particle surface. By examining the stability ratio, W, it was found that even in the most destabilized state, i.e. at charge neutralization, the starch chains had induced steric stabilization to the system. At higher particle and starch concentrations relaxation of the aggregates could be seen, as monitored by a decrease in turbidity with time. This relaxation was evaluated by fitting the data to the Kohlrausch-Williams-Watts function. It was found that irrespective of the starch to particle charge ratio the relaxation time was similar. Moreover, a molecular weight dependence on the relaxation time was found, as well as a more pronounced initial aggregated state for the higher molecular weight starch. This initial aggregate state could be due to bridging flocculation. With time, as the starch chains have relaxed into a final conformation on the particle surface, bridging will be less important and is gradually replaced by patches that will cause patchwise flocculation. After an equilibration time no molecular weight dependence on aggregation could be seen, which confirms the patchwise flocculation mechanism.
  • Izzo, M. G., et al. (författare)
  • Rayleigh scattering and disorder-induced mixing of polarizations in amorphous solids at the nanoscale: 1-octyl-3-methylimidazolium chloride glass
  • 2020
  • Ingår i: PHYSICAL REVIEW B. - 2469-9969 .- 2469-9950. ; 102:21
  • Tidskriftsartikel (refereegranskat)abstract
    • Acousticlike excitations in topologically disordered media at mesocale/nanoscale present anomalous features with respect to the Debye's theory. The so-called Rayleigh scattering manifests in a strong increase of the attenuation of the acousticlike excitations and a softening of the phase velocity with respect to its continuum limit value. Mean field models developed in the random media theory framework can successfully predict the occurrence, at the proper length scale, of Rayleigh scattering. The overall attenuation in the Rayleigh region is, however, underestimated. In the framework of random media theory we developed an analytical model, which permits a quantitative description of the acousticlike excitations in topological glasses in the whole first pseudo-Brillouin zone. The underestimation of the Rayleigh scattering is avoided and, importantly, the model allows to account also for the polarization properties of the acousticlike excitations. In a three-dimensional medium an acoustic wave is characterized by its phase velocity, intensity, and polarization. Rayleigh scattering emphasizes how the topological disorder affects the first two properties. The topological disorder is, however, expected to influence also the third one. In common with the Rayleigh scattering, hallmarks possibly related to the mixing of polarizations have been traced in different classes of amorphous solids at nanoscale. The quantitative theoretical approach developed permits to demonstrate how the mixing of polarizations generates a distinctive feature in the dynamic structure factor of amorphous solids. The modeling capability of the proposed mean field theory is tested on glassy 1-octyl-3-methylimidazolium chloride, whose spatial distribution of the elastic moduli is well assessed and can be experimentally characterized. Contrast between theoretical and experimental features for the selected glass reveals an excellent agreement. The mean field approach we present retains a certain degree of generality and can be possibly extended to different stochastic media or different wave fields.
  • Johansson, Patrik, 1969, et al. (författare)
  • The conductivity of pyrrolidinium and sulfonylimide based ionic liquids: A combined experimental and computational study
  • 2010
  • Ingår i: Journal of Power Sources. - 0378-7753. ; 195:7, s. 2074-2076
  • Tidskriftsartikel (refereegranskat)abstract
    • Ionic conductivity is a fundamental property of ionic liquids with its origin and exact nature under debate. Using a specially selected system of pyrrolidinium cations (PYR1x, x = 3,4) and sulfonylimide anions (FSI, TFSI, BETI, and IM14)-based ionic liquids we observe a simple and accurate connection between ab initio computed cation and anion volumes and measured molar ionic conductivities.
  • Karlsson, Maths, 1978, et al. (författare)
  • Alkali-ion concentration dependence of the structure of proton-conducting alkali thio-hydroxogermanates investigated with neutron diffraction
  • 2015
  • Ingår i: Solid State Ionics. - 0167-2738. ; 274, s. 40-45
  • Tidskriftsartikel (refereegranskat)abstract
    • The proton-conducting hydrated alkali thio-hydroxogermanate's MxGeSx(OH)(4) - x center dot yH(2)O (M = Na and K; x = 1 - 4,y approximate to 0.5 - 2) were investigated by means of neutron diffraction with the aim to elucidate how the structure changes as a function of alkali-ion concentration, x, type of alkali ion, M, and water content, y. For x = 1 - 3 we find that the materials are amorphous and composed of thio-hydroxogermanate anions, water molecules, and charge balancing alkali ions, whereas for x = 4 we find that the materials contain also a crystalline phase, suggesting that it is difficult to prepare purely amorphous materials for the highest alkali-ion concentration, for both the Na and K based materials. For x = 1 - 3, the structure is reflected by an intermediate-range ordering, with a characteristic length-scale ranging from approximately 6 to 9 angstrom, which is dependent on both x and M and which may be related to the separation distance between dimers of thio-hydroxogermanate anions. As x increases, the intermediate-range ordering shortens, possibly as the result of an increasing level of hydration water that may act as a dielectric medium that reduces the repulsive interaction between the negatively charged thio-hydroxogermanate anions and/or between the positively charged alkali ions. A comparison of the structural results to the reported conductivities of the same materials indicates a non-trivial relationship, which depends on both the type and concentration of alkali ions, as well as on the level of hydration water.
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