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Träfflista för sökning "WFRF:(Matic Aleksandar 1968) "

Sökning: WFRF:(Matic Aleksandar 1968)

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61.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • 2,3,6,7,10,11-Hexamethoxytriphenylene (HMTP): A new organic cathode material for lithium batteries
  • 2012
  • Ingår i: Electrochemistry Communications. - 1388-2481. ; 21:1, s. 50-53
  • Tidskriftsartikel (refereegranskat)abstract
    • We propose a new organic cathode material for rechargeable lithium battery applications: 2,3,6,7,10,11-hexamethoxytriphenylene (HMTP). HMTP is composed of six methoxy functional groups substituted onto a central triphenylene moiety. The cell, incorporating 40 wt.% of organic cathode material, exhibits full specific capacity at current densities up to 3 C. The main advantage of HMTP as organic cathode material lies in a stable cell performance and negligible self discharge, even though the capacity is lower, similar to 66 mAh/g, compared to other organic cathode materials. Cells with the HMTP cathode showed >95% retention of the initial discharge capacity after 50 cycles at 1 C and self-discharge was not observed during a full month of open circuit voltage measurements. The latter is due to the fact that the nature of the HMTP radical is fundamentally different from other organic cathode materials' radicals.
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62.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • An Imidazolium based ionic liquid electrolyte for lithium batteries
  • 2010
  • Ingår i: Journal of Power Sources. - 0378-7753. ; 195:22, s. 7639-7643
  • Tidskriftsartikel (refereegranskat)abstract
    • An electrolyte for lithium batteries based on the ionic liquid 3-methy-1-propylimidazolium bis(trifluoromethysulfony)imide (PMIMTFSI) complexed with lithium bis(trifluoromethysulfony)imide (LiTFSI) at a molar ratio of 1:1 has been investigated. The electrolyte shows a high ionic conductivity (1.2 × 10−3 S cm−1) at room temperature. Over the whole investigated temperature range the ionic conductivity is more than one order of magnitude higher than for an analogue electrolyte based on N-butyl-N-methyl-pyrrolidinium bis(trifluoromethanesulfonyl)imide (Py14TFSI) complexed with LiTFSI and used here as a benchmark. Raman results indicate furthermore that the degree of lithium coordinated TFSI is slightly lower in the electrolyte based on PMIMTFSI and thus that the Li+ charge carriers should be higher than in electrolytes based on Py14TFSI. An ionic liquid gel electrolyte membrane was obtained by soaking a fibrous fully interconnected membrane, made of electrospun P(VdF-HFP), in the electrolyte. The gel electrolyte was cycled in Li/ionic liquid polymer electrolyte/Li cells over 15 days and in Li/LiFePO4 cells demonstrating good interfacial stability and highly stable discharge capacities with a retention of >96% after 50 cycles (146 mAh g−1).
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63.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Characterization of N-butyl-N-methyl-pyrrolidinium bis(trifluoromethanesulfonyl)imide-based polymer electrolytes for high safety lithium batteries
  • 2013
  • Ingår i: Journal of Power Sources. - 0378-7753. ; 224:15 Feb. 2013, s. 93-98
  • Tidskriftsartikel (refereegranskat)abstract
    • Poly(vinylidene difluoride-co-hexafluoropropylene) (PVdF-HFP) membrane was prepared by electrospinning. The membranes served as host matrices for the preparation of ionic liquid-based polymer electrolytes (ILPEs) by activation with non-volatile, highly thermally stable, and safe room temperature ionic liquid (RTIL) electrolytes; N-butyl-N-methyl-pyrrolidinium bis(trifluoromethanesulfonyl)imide (Py14TFSI) complexed with 1 M lithium bis(trifluoromethanesulfonyl)imide (LiTFSI). In this work, the first combination of electrospun PVdF-HFP fiber polymer host and pyrrolidinium-based ionic electrolyte was employed for highly stable lithium batteries. The ILPE exhibited low Li+-TFSI coordination, low crystallinity, high thermal stability, high electrochemical stability, and high ionic conductivity with a maximum of 1.1 x 10(-4) S cm(-1) at 0 degrees C. The ILPE exhibited good compatibility with a LiFePO4 electrode on storage and good charge-discharge performance in Li/ILPE/LiFePO4!
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64.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Effect of carbon coating methods on structural characteristics and electrochemical properties of carbon-coated lithium iron phosphate
  • 2014
  • Ingår i: Solid State Ionics. - 0167-2738. ; 262, s. 25-29
  • Tidskriftsartikel (refereegranskat)abstract
    • The potential of LiFePO4 as cathode material has not been fully exploited due to its intrinsic poor electronic and ionic conductivities. Attempts have been made to improve these properties of which coating of the active carbon on the particle surface is the most viable method so far. Phase-pure LiFePO4 and two LiFePO4/C composites were synthesized by mechanical activation process employing two different methods: (i) direct addition of acetylene black carbon and (ii) addition of sucrose as carbon precursor. The samples were well characterized by various techniques like elemental analysis, Brunauer-Emmett-Teller (BET) method, scanning electron microscopy (SEM), X-ray powder diffraction (XRD), and Raman spectroscopy to establish their composition, morphology, particle size and surface area. The structure of these samples is investigated as olivine structure space group Prima by X-ray powder diffraction. Transmission electron microscopy (TEM) confirms that the carbon nanocoating on the LiFePO4 particles has no visible dislocations and fractures. The electrochemical performance of LiFePO4/C is significantly affected by the nature of the carbon nanocoating, which in turn is affected by the choice of synthesis method.
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65.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Electrochemical properties of a full cell of lithium iron phosphate cathode using thin amorphous silicon anode
  • 2014
  • Ingår i: Solid State Ionics. - 0167-2738. ; 268:Part B, s. 256-260
  • Tidskriftsartikel (refereegranskat)abstract
    • Carbon-coated lithium iron phosphate (LiFePO4/C) with uniform carbon coating was synthesized by a mechanical activation method. Silicon negative electrode material was obtained in the form of thin films of amorphous silicon on a Cu foil substrate by vertical deposition technique. The electrochemical performance of the full cell, LiFePO4/C-Si, was tested with 1 M LiPF6 in EC/DMC at 0.5 and 1 C-rates. The cell exhibited an initial discharge capacity of 143.9 mAh g(-1) at 0.5 C-rate at room temperature. A reasonably good cycling performance under a high current density of 1 C-rate could be obtained with the full cell.
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66.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Highly porous LiMnPO4 in combination with an ionic liquid-based polymer gel electrolyte for lithium batteries
  • 2011
  • Ingår i: Electrochemistry Communications. - 1388-2481. ; 13:10, s. 1105-1108
  • Tidskriftsartikel (refereegranskat)abstract
    • A porous well defined LiMnPO(4) cathode material is synthesized by a sol-gel method. The electrochemical performance of the cathode material is evaluated in a cell with an ionic liquid-based polymer electrolyte (0.5 M LITFSI in EMlmTFSI) and a lithium metal electrode. The results are compared to a cell with a traditional organic carbonate-based electrolyte (1 M LiPF(6) in EC/DMC). The cell with the ionic liquid-based polymer electrolyte presents an enhanced electrochemical intercalation performance of lithium ions, a high electrochemical stability window of 5 V, and an excellent cycling ability as compared with the organic based counterpart. Furthermore, the ionic liquid-based polymer gel electrolyte effectively prevents the dissolution of manganese - otherwise a common problem.
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67.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Improving the stability of an organic battery with an ionic liquid-based plymer electrolyte
  • 2012
  • Ingår i: RSC Advances. - 2046-2069. ; 2:26, s. 9795-9797
  • Tidskriftsartikel (refereegranskat)abstract
    • A gel polymer electrolyte based on the ionic liquid {N-butyl-N-methyl-pyrrolidiniumbis(trifluoromethanesulfonyl) imide (Py14TFSI) and lithium bis(trifluoromethanesulfony)imide (LiTFSI)} is shown to prevent the dissolution from an organic electrode. The composite cell shows high energy efficiency although poor cycle stability is exhibited at very high current density (10 C-rate).
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68.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Nano-fibrous polymer films for organic rechargeable batteries
  • 2013
  • Ingår i: Journal of Materials Chemistry A. - 2050-7488 .- 2050-7496. ; 1:7, s. 2426-2430
  • Tidskriftsartikel (refereegranskat)abstract
    • We propose a nano-fibrous polymer (NFP) film, fabricated by electrospinning poly(2,2,6,6-tetramethylpiperidinyloxy-4-yl methacrylate) (PTMA), as a key component in high performance organic batteries. The new strategy with a NFP film enables extraordinary rate capability and excellent cyclability, due to its special morphology. Moreover, the NFP film enhances the flexibility of the electrode at a low cost and prevents dissolution of PTMA into the electrolyte.
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69.
  • Kim, Jae-Kwang, 1978, et al. (författare)
  • Preparation and application of TEMPO-based di-radical organic electrode with ionic liquid-based polymer electrolyte
  • 2012
  • Ingår i: RSC Advances. - 2046-2069. ; 2:27, s. 10394-10399
  • Tidskriftsartikel (refereegranskat)abstract
    • In this study we report the synthesis and use of new organic materials, TEMPO di-radical [1,3-bis(4-(2,2,6,6,-tetramethyl-1-oxyl-4-piperidoxyl)butyl) imidazolium trifluorosulfonate]. Two cells were prepared with Li metal anode and the TEMPO di-radical based cathode with a microporous polymer electrolyte [1-butyl-3-methyl imidazolium bis(trifluoromethane sulfonyl) imide (BMImTFSI) in 0.5 M LiTFSI, and in 1 M LiPF6 in ethylene carbonate/dimethyl carbonate (EC/DMC)] hosted in electrospun poly(vinylidenefluoride-co-hexafluoropropylene) (PVdF-HFP) membrane. The nature of the solvent was not found to affect the basic redox reaction behavior of TEMPO. The anodic and cathodic peaks were obtained at almost the same position and with some difference in the separation of peaks. The presence of BMImTFSI significantly affects the electrochemical performance of the battery as the cell having this RTIL exhibited far better electrochemical performance with 100% utilization of the active material and reasonably good cycling performance up to 200 cycles. We believe that this composite cell will contribute to organic green rechargeable batteries, although the cell is not fully organic composite.
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70.
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Eriksson, Sten, 1958 (13)
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