Search: WFRF:(Jankowski Piotr 1990)
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Critical Role of Fu...
Critical Role of Functional Groups Containing N, S, and O on Graphene Surface for Stable and Fast Charging Li-S Batteries
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- Sun, Jinhua, 1987 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden
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- Hwang, Jang Yeon (author)
- Chonnam National University,Department of Materials Science and Engineering, Chonnam National University, 77 Yongbong-ro, Buk-gu, Gwangju, South Korea
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- Jankowski, Piotr, 1990 (author)
- Wojskowa Akademia Techniczna im. Jarosława Dąbrowskiego w Warszawie - WAT,Military University of Technology in Warsaw,Danmarks Tekniske Universitet,Technical University of Denmark,Faculty of Chemistry, Warsaw University of Technology, Warsaw, Poland; Department of Energy Conversion and Storage, Technical University of Denmark, Kgs. Lyngby, Denmark
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- Xiao, Linhong (author)
- Umeå universitet,Kemiska institutionen,Umeå University
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- Sanchez Sanchez, Jaime, 1990 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden
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- Xia, Zhenyuan, 1983 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Istituto per la Sintesi Organica e la Fotoreattività (ISOF-CNR),Institute for organic syntheses and photoreactivity (ISOF-CNR),Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden; Institute of Organic Synthesis and Photoreactivity (ISOF), CNR, via Gobetti 101, Bologna, Italy
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- Lee, Suyeong (author)
- Chonnam National University,Department of Materials Science and Engineering, Chonnam National University, 77 Yongbong-ro, Buk-gu, Gwangju, South Korea
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- Talyzin, Aleksandr V., 1969- (author)
- Umeå universitet,Institutionen för fysik,Umeå University
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- Matic, Aleksandar, 1968 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Department of Physics, Chalmers University of Technology, Göteborg, Sweden
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- Palermo, Vincenzo, 1972 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Istituto per la Sintesi Organica e la Fotoreattività (ISOF-CNR),Institute for organic syntheses and photoreactivity (ISOF-CNR),Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden; Institute of Organic Synthesis and Photoreactivity (ISOF), CNR, via Gobetti 101, Bologna, Italy
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- Sun, Yang-Kook (author)
- Hanyang University,Department of Energy Engineering, Hanyang University, Seoul, South Korea
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- Agostini, Marco, 1987 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Department of Physics, Chalmers University of Technology, Göteborg, Sweden
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(creator_code:org_t)
- 2021-03-14
- 2021
- English.
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In: Small. - : Wiley. - 1613-6810 .- 1613-6829. ; 17:17
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Abstract
Subject headings
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- Lithium‐sulfur (Li‐S) batteries are considered one of the most promising energy storage technologies, possibly replacing the state‐of‐the‐art lithium‐ion (Li‐ion) batteries owing to their high energy density, low cost, and eco‐compatibility. However, the migration of high‐order lithium polysulfides (LiPs) to the lithium surface and the sluggish electrochemical kinetics pose challenges to their commercialization. The interactions between the cathode and LiPs can be enhanced by the doping of the carbon host with heteroatoms, however with relatively low doping content (<10%) in the bulk of the carbon, which can hardly interact with LiPs at the host surface. In this study, the grafting of versatile functional groups with designable properties (e.g., catalytic effects) directly on the surface of the carbon host is proposed to enhance interactions with LiPs. As model systems, benzene groups containing N/O and S/O atoms are vertically grafted and uniformly distributed on the surface of expanded reduced graphene oxide, fostering a stable interface between the cathode and LiPs. The combination of experiments and density functional theory calculations demonstrate improvements in chemical interactions between graphene and LiPs, with an enhancement in the electrochemical kinetics, power, and energy densities.
Subject headings
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
- MEDICIN OCH HÄLSOVETENSKAP -- Medicinsk bioteknologi -- Biomedicinsk laboratorievetenskap/teknologi (hsv//swe)
- MEDICAL AND HEALTH SCIENCES -- Medical Biotechnology -- Biomedical Laboratory Science/Technology (hsv//eng)
- MEDICIN OCH HÄLSOVETENSKAP -- Klinisk medicin -- Cancer och onkologi (hsv//swe)
- MEDICAL AND HEALTH SCIENCES -- Clinical Medicine -- Cancer and Oncology (hsv//eng)
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Keyword
- practical energy and power density
- lithium-sulfur batteries
- graphene
- surface functionalization
- electrolyte lean condition
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- art (subject category)
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Sun, Jinhua, 198 ...
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Hwang, Jang Yeon
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Jankowski, Piotr ...
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Xiao, Linhong
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Lee, Suyeong
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Chalmers University of Technology
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Umeå University