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Inner-Shell-Ionizat...
Inner-Shell-Ionization-Induced Femtosecond Structural Dynamics of Water Molecules Imaged at an X-Ray Free-Electron Laser
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- Jahnke, T. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Guillemin, R. (author)
- Paris-Sorbonne University,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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- Inhester, L. (author)
- German Electron Synchrotron (DESY),DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.
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show more...
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- Son, S. K. (author)
- German Electron Synchrotron (DESY),Polytechnic University of Milan,DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.,Politecn Milan, Phys Dept, Milan, Italy.
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- Kastirke, G. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Ilchen, M. (author)
- European XFEL GmbH,University of Kassel,European XFEL, D-22869 Schenefeld, Germany.;Univ Kassel, Inst Phys, D-34132 Kassel, Germany.;Univ Kassel, CINSaT, D-34132 Kassel, Germany.
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- Rist, J. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Trabert, D. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Melzer, N. (author)
- Uppsala University,Paris-Sorbonne University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Anders, N. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Mazza, T. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Boll, R. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- De Fanis, A. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Music, V. (author)
- European XFEL GmbH,University of Kassel,European XFEL, D-22869 Schenefeld, Germany.;Univ Kassel, Inst Phys, D-34132 Kassel, Germany.;Univ Kassel, CINSaT, D-34132 Kassel, Germany.
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- Weber, T. (author)
- Lawrence Berkeley National Laboratory,Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA.
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- Weller, M. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Eckart, S. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Fehre, K. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Grundmann, S. (author)
- Goethe University,Albert-Ludwigs University Freiburg,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.,Univ Freiburg, Phys Inst, D-79104 Freiburg, Germany.
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- Hartung, A. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Hofmann, M. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Janke, C. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Kircher, M. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Nalin, G. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Pier, A. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Siebert, J. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Strenger, N. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Vela-Perez, I. (author)
- Goethe University,Paris-Sorbonne University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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- Baumann, T. M. (author)
- Paris-Sorbonne University,University of Hamburg,European XFEL GmbH,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.,Univ Hamburg, Inst Expt Phys, D-22761 Hamburg, Germany.,European XFEL, D-22869 Schenefeld, Germany.
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- Grychtol, P. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Montano, J. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Ovcharenko, Y. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Rennhack, N. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Rivas, D. E. (author)
- European XFEL GmbH,Goethe University,European XFEL, D-22869 Schenefeld, Germany.,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Wagner, R. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Ziolkowski, P. (author)
- European XFEL GmbH,European XFEL, D-22869 Schenefeld, Germany.
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- Schmidt, P. (author)
- European XFEL GmbH,University of Kassel,Goethe University,European XFEL, D-22869 Schenefeld, Germany.;Univ Kassel, Inst Phys, D-34132 Kassel, Germany.;Univ Kassel, CINSaT, D-34132 Kassel, Germany.,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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Marchenko, T. (author)
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- Travnikova, O. (author)
- Paris-Sorbonne University,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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- Journel, L. (author)
- Paris-Sorbonne University,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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Ismail, I. (author)
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- Kukk, E. (author)
- University of Turku,Univ Turku, Dept Phys & Astron, FI-20014 Turku, Finland.
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- Niskanen, J. (author)
- University of Turku,Univ Turku, Dept Phys & Astron, FI-20014 Turku, Finland.
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- Trinter, F. (author)
- Fritz Haber Institute of the Max Planck Society,German Electron Synchrotron (DESY),DESY, FS PETRA S, D-22607 Hamburg, Germany.;Fritz Haber Inst Max Planck Gesell, Mol Phys, D-14195 Berlin, Germany.
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- Vozzi, C. (author)
- CNR Istituto per le Tecnologie Applicate ai Beni Culturali (CNR-ITABC),CNR, IFN Ist Foton & Nanotecnol, I-20133 Milan, Italy.
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- Devetta, M. (author)
- CNR Istituto per le Tecnologie Applicate ai Beni Culturali (CNR-ITABC),CNR, IFN Ist Foton & Nanotecnol, I-20133 Milan, Italy.
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- Stagira, S. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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- Gisselbrecht, M. (author)
- Lund University,Lunds universitet,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,Lund Univ, Dept Phys, SE-22100 Lund, Sweden.
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- Jager, A. L. (author)
- Albert-Ludwigs University Freiburg,Univ Freiburg, Phys Inst, D-79104 Freiburg, Germany.
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- Li, X. (author)
- Kansas State University,Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.
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- Malakar, Y. (author)
- Kansas State University,Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.
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- Martins, M. (author)
- Paris-Sorbonne University,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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- Feifel, Raimund (author)
- University of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, SE-41296 Gothenburg, Sweden.
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Schmidt, L. P. H. (author)
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- Czasch, A. (author)
- Goethe University,Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany.
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Sansone, G. (author)
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- Rolles, D. (author)
- Kansas State University,Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.
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- Rudenko, A. (author)
- Kansas State University,Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.
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- Moshammer, R. (author)
- Max Planck Institute for Nuclear Physics,Max Planck Inst Kernphys, D-69117 Heidelberg, Germany.
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Dorner, R. (author)
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Meyer, M. (author)
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- Pfeifer, T. (author)
- Max Planck Institute for Nuclear Physics,Max Planck Inst Kernphys, D-69117 Heidelberg, Germany.
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Schoffler, M. S. (author)
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- Santra, R. (author)
- University of Hamburg,German Electron Synchrotron (DESY),DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-22607 Hamburg, Germany.
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Simon, M. (author)
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- Piancastelli, Maria Novella (author)
- Uppsala universitet,Kemisk och biomolekylär fysik,Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France.
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European XFEL GmbH European XFEL, D-22869 Schenefeld, Germany (creator_code:org_t)
- American Physical Society, 2021
- 2021
- English.
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In: Physical Review X. - : American Physical Society. - 2160-3308. ; 11:4
- Related links:
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http://dx.doi.org/10... (free)
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https://doi.org/10.1...
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https://uu.diva-port... (primary) (Raw object)
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https://gup.ub.gu.se...
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https://doi.org/10.1...
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https://lup.lub.lu.s...
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https://urn.kb.se/re...
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Abstract
Subject headings
Close
- The ultrafast structural dynamics of water following inner-shell ionization is a crucial issue in high-energy radiation chemistry. We have exposed isolated water molecules to a short x-ray pulse from a free-electron laser and detected momenta of all produced ions in coincidence. By combining experimental results and theoretical modeling, we can image dissociation dynamics of individual molecules in unprecedented detail. We reveal significant molecular structural dynamics in H2O2+, such as asymmetric deformation and bond-angle opening, leading to two-body or three-body fragmentation on a timescale of a few femtoseconds. We thus reconstruct several snapshots of structural dynamics at different time intervals, which highlight dynamical patterns that are relevant as initiating steps of subsequent radiation-damage processes.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
Keyword
- liquid water
- photofragmentation
- spectroscopy
- radiolysis
- spectrum
- surface
- origin
- ion
- Physics
Publication and Content Type
- ref (subject category)
- art (subject category)
Find in a library
To the university's database
- By the author/editor
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Jahnke, T.
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Guillemin, R.
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Inhester, L.
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Son, S. K.
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Kastirke, G.
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Ilchen, M.
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show more...
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Rist, J.
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Trabert, D.
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Melzer, N.
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Anders, N.
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Mazza, T.
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Boll, R.
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De Fanis, A.
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Music, V.
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Weber, T.
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Weller, M.
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Eckart, S.
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Fehre, K.
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Grundmann, S.
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Hartung, A.
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Hofmann, M.
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Janke, C.
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Kircher, M.
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Nalin, G.
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Pier, A.
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Siebert, J.
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Strenger, N.
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Vela-Perez, I.
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Baumann, T. M.
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Grychtol, P.
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Montano, J.
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Ovcharenko, Y.
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Rennhack, N.
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Rivas, D. E.
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Wagner, R.
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Ziolkowski, P.
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Schmidt, P.
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Marchenko, T.
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Travnikova, O.
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Journel, L.
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Ismail, I.
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Kukk, E.
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Niskanen, J.
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Trinter, F.
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Vozzi, C.
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Devetta, M.
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Stagira, S.
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Gisselbrecht, M.
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Jager, A. L.
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Li, X.
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Malakar, Y.
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Martins, M.
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Feifel, Raimund
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Schmidt, L. P. H ...
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Czasch, A.
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Sansone, G.
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Rolles, D.
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Rudenko, A.
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Moshammer, R.
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Dorner, R.
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Meyer, M.
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Pfeifer, T.
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Schoffler, M. S.
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Santra, R.
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Simon, M.
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Piancastelli, Ma ...
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Physical Chemist ...
- Articles in the publication
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Physical Review ...
- By the university
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University of Gothenburg
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Lund University
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Uppsala University
