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Tailormade Polysacc...
Tailormade Polysaccharides with Defined Branching Patterns: Enzymatic Polymerization of Arabinoxylan Oligosaccharides
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- Senf, Deborah (author)
- Freie Universität Berlin,Max Planck Gesellschaft zur Förderung der Wissenschaften e.V. (MPG),Max Planck Society for the Advancement of Science (MPG),Max Planck Inst Colloids & Interfaces, Dept Biomol Syst, Muhlenberg 1, D-14476 Potsdam, Germany.;Free Univ Berlin, Inst Chem & Biochem, Arnimallee 22, D-14195 Berlin, Germany.
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- Ruprecht, Colin (author)
- Max Planck Gesellschaft zur Förderung der Wissenschaften e.V. (MPG),Max Planck Society for the Advancement of Science (MPG),Max Planck Inst Colloids & Interfaces, Dept Biomol Syst, Muhlenberg 1, D-14476 Potsdam, Germany.
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- Kishani, Saina (author)
- KTH,Fiber- och polymerteknologi,Wallenberg Wood Science Center
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- Matic, Aleksandar (author)
- Universität Potsdam,University of Potsdam,Max Planck Gesellschaft zur Förderung der Wissenschaften e.V. (MPG),Max Planck Society for the Advancement of Science (MPG),Max Planck Inst Colloids & Interfaces, Dept Biomol Syst, Muhlenberg 1, D-14476 Potsdam, Germany.;Univ Potsdam, Dept Chem, Karl Liebknecht Str 24-25, D-14476 Potsdam, Germany.
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- Toriz Gonzalez, Guillermo, 1968 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Chalmers Univ Technol, Dept Chem & Chem Engn, Wallenberg Wood Sci Ctr & Biopolymer Technol, S-41296 Gothenburg, Sweden.
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- Gatenholm, Paul, 1956 (author)
- Chalmers tekniska högskola,Chalmers University of Technology,Chalmers Univ Technol, Dept Chem & Chem Engn, Wallenberg Wood Sci Ctr & Biopolymer Technol, S-41296 Gothenburg, Sweden.
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- Wågberg, Lars, 1956- (author)
- KTH,Fiber- och polymerteknologi,Wallenberg Wood Science Center
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- Pfrengle, Fabian (author)
- Freie Universität Berlin,Max Planck Gesellschaft zur Förderung der Wissenschaften e.V. (MPG),Max Planck Society for the Advancement of Science (MPG),Max Planck Inst Colloids & Interfaces, Dept Biomol Syst, Muhlenberg 1, D-14476 Potsdam, Germany.;Free Univ Berlin, Inst Chem & Biochem, Arnimallee 22, D-14195 Berlin, Germany.
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Freie Universität Berlin Max Planck Gesellschaft zur Förderung der Wissenschaften eV. (MPG) (creator_code:org_t)
- 2018-08-19
- 2018
- English.
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In: Angewandte Chemie - International Edition. - : Wiley. - 1433-7851 .- 1521-3773. ; 57:37, s. 11987-11992
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https://doi.org/10.1...
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Abstract
Subject headings
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- The heterogeneous nature of non-cellulosic polysaccharides, such as arabinoxylan, makes it difficult to correlate molecular structure with macroscopic properties. To study the impact of specific structural features of the polysaccharides on crystallinity or affinity to other cell wall components, collections of polysaccharides with defined repeating units are required. Herein, a chemoenzymatic approach to artificial arabinoxylan polysaccharides with systematically altered branching patterns is described. The polysaccharides were obtained by glycosynthase-catalyzed polymerization of glycosyl fluorides derived from arabinoxylan oligosaccharides. X-ray diffraction and adsorption experiments on cellulosic surfaces revealed that the physicochemical properties of the synthetic polysaccharides strongly depend on the specific nature of their substitution patterns. The artificial polysaccharides allow structure–property relationship studies that are not accessible by other means.
Subject headings
- TEKNIK OCH TEKNOLOGIER -- Materialteknik -- Textil-, gummi- och polymermaterial (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Materials Engineering -- Textile, Rubber and Polymeric Materials (hsv//eng)
- NATURVETENSKAP -- Kemi -- Annan kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Other Chemistry Topics (hsv//eng)
- NATURVETENSKAP -- Kemi -- Organisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Organic Chemistry (hsv//eng)
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
Keyword
- synthetic methods
- enzymes
- carbohydrates
- glycosynthases
- structure elucidation
Publication and Content Type
- art (subject category)
- ref (subject category)
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- By the author/editor
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Senf, Deborah
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Ruprecht, Colin
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Kishani, Saina
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Matic, Aleksanda ...
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Toriz Gonzalez, ...
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Gatenholm, Paul, ...
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Wågberg, Lars, 1 ...
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Pfrengle, Fabian
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- About the subject
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- ENGINEERING AND TECHNOLOGY
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ENGINEERING AND ...
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and Materials Engine ...
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and Textile Rubber a ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Other Chemistry ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Organic Chemistr ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
- Articles in the publication
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Angewandte Chemi ...
- By the university
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Chalmers University of Technology
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Royal Institute of Technology