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Multicomponent new particle formation from sulfuric acid, ammonia, and biogenic vapors

Lehtipalo, Katrianne (author)
Yan, Chao (author)
Dada, Lubna (author)
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Bianchi, Federico (author)
Xiao, Mao (author)
Wagner, Robert (author)
Stolzenburg, Dominik (author)
Ahonen, Lauri R. (author)
Amorim, Antonio (author)
Baccarini, Andrea (author)
Bauer, Paulus S. (author)
Baumgartner, Bernhard (author)
Bergen, Anton (author)
Bernhammer, Anne-Kathrin (author)
Breitenlechner, Martin (author)
Brilke, Sophia (author)
Buchholz, Angela (author)
Mazon, Stephany Buenrostro (author)
Chen, Dexian (author)
Chen, Xuemeng (author)
Dias, Antonio (author)
Dommen, Josef (author)
Draper, Danielle C. (author)
Duplissy, Jonathan (author)
Ehn, Mikael (author)
Finkenzeller, Henning (author)
Fischer, Lukas (author)
Frege, Carla (author)
Fuchs, Claudia (author)
Garmash, Olga (author)
Gordon, Hamish (author)
Hakala, Jani (author)
He, Xucheng (author)
Heikkinen, Liine (author)
Heinritzi, Martin (author)
Helm, Johanna C. (author)
Hofbauer, Victoria (author)
Hoyle, Christopher R. (author)
Jokinen, Tuija (author)
Kangasluoma, Juha (author)
Kerminen, Veli-Matti (author)
Kim, Changhyuk (author)
Kirkby, Jasper (author)
Kontkanen, Jenni (author)
Stockholms universitet,Institutionen för miljövetenskap och analytisk kemi,University of Helsinki, Finland
Kuerten, Andreas (author)
Lawler, Michael J. (author)
Mai, Huajun (author)
Mathot, Serge (author)
Mauldin, Roy L. (author)
Molteni, Ugo (author)
Nichman, Leonid (author)
Nie, Wei (author)
Nieminen, Tuomo (author)
Ojdanic, Andrea (author)
Onnela, Antti (author)
Passananti, Monica (author)
Petaja, Tuukka (author)
Piel, Felix (author)
Pospisilova, Veronika (author)
Quelever, Lauriane L. J. (author)
Rissanen, Matti P. (author)
Rose, Clemence (author)
Sarnela, Nina (author)
Schallhart, Simon (author)
Schuchmann, Simone (author)
Sengupta, Kamalika (author)
Simon, Mario (author)
Sipila, Mikko (author)
Tauber, Christian (author)
Tome, Antonio (author)
Trostl, Jasmin (author)
Vaisanen, Olli (author)
Vogel, Alexander L. (author)
Volkamer, Rainer (author)
Wagner, Andrea C. (author)
Wang, Mingyi (author)
Weitz, Lena (author)
Wimmer, Daniela (author)
Ye, Penglin (author)
Ylisirnio, Arttu (author)
Zha, Qiaozhi (author)
Carslaw, Kenneth S. (author)
Curtius, Joachim (author)
Donahue, Neil M. (author)
Flagan, Richard C. (author)
Hansel, Armin (author)
Riipinen, Ilona (author)
Stockholms universitet,Institutionen för miljövetenskap och analytisk kemi,Tampere University of Technology, Finland
Virtanen, Annele (author)
Winkler, Paul M. (author)
Baltensperger, Urs (author)
Kulmala, Markku (author)
Worsnop, Douglas R. (author)
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 (creator_code:org_t)
American Association for the Advancement of Science (AAAS), 2018
2018
English.
In: Science Advances. - : American Association for the Advancement of Science (AAAS). - 2375-2548. ; 4:12
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • A major fraction of atmospheric aerosol particles, which affect both air quality and climate, form from gaseous precursors in the atmosphere. Highly oxygenated organic molecules (HOMs), formed by oxidation of biogenic volatile organic compounds, are known to participate in particle formation and growth. However, it is not well understood how they interact with atmospheric pollutants, such as nitrogen oxides (NOx) and sulfur oxides (SOx) from fossil fuel combustion, as well as ammonia (NH3) from livestock and fertilizers. Here, we show how NOx suppresses particle formation, while HOMs, sulfuric acid, and NH3 have a synergistic enhancing effect on particle formation. We postulate a novel mechanism, involving HOMs, sulfuric acid, and ammonia, which is able to closely reproduce observations of particle formation and growth in daytime boreal forest and similar environments. The findings elucidate the complex interactions between biogenic and anthropogenic vapors in the atmospheric aerosol system.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)
NATURVETENSKAP  -- Kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences (hsv//eng)

Publication and Content Type

ref (subject category)
art (subject category)

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By the author/editor
Lehtipalo, Katri ...
Yan, Chao
Dada, Lubna
Bianchi, Federic ...
Xiao, Mao
Wagner, Robert
show more...
Stolzenburg, Dom ...
Ahonen, Lauri R.
Amorim, Antonio
Baccarini, Andre ...
Bauer, Paulus S.
Baumgartner, Ber ...
Bergen, Anton
Bernhammer, Anne ...
Breitenlechner, ...
Brilke, Sophia
Buchholz, Angela
Mazon, Stephany ...
Chen, Dexian
Chen, Xuemeng
Dias, Antonio
Dommen, Josef
Draper, Danielle ...
Duplissy, Jonath ...
Ehn, Mikael
Finkenzeller, He ...
Fischer, Lukas
Frege, Carla
Fuchs, Claudia
Garmash, Olga
Gordon, Hamish
Hakala, Jani
He, Xucheng
Heikkinen, Liine
Heinritzi, Marti ...
Helm, Johanna C.
Hofbauer, Victor ...
Hoyle, Christoph ...
Jokinen, Tuija
Kangasluoma, Juh ...
Kerminen, Veli-M ...
Kim, Changhyuk
Kirkby, Jasper
Kontkanen, Jenni
Kuerten, Andreas
Lawler, Michael ...
Mai, Huajun
Mathot, Serge
Mauldin, Roy L.
Molteni, Ugo
Nichman, Leonid
Nie, Wei
Nieminen, Tuomo
Ojdanic, Andrea
Onnela, Antti
Passananti, Moni ...
Petaja, Tuukka
Piel, Felix
Pospisilova, Ver ...
Quelever, Lauria ...
Rissanen, Matti ...
Rose, Clemence
Sarnela, Nina
Schallhart, Simo ...
Schuchmann, Simo ...
Sengupta, Kamali ...
Simon, Mario
Sipila, Mikko
Tauber, Christia ...
Tome, Antonio
Trostl, Jasmin
Vaisanen, Olli
Vogel, Alexander ...
Volkamer, Rainer
Wagner, Andrea C ...
Wang, Mingyi
Weitz, Lena
Wimmer, Daniela
Ye, Penglin
Ylisirnio, Arttu
Zha, Qiaozhi
Carslaw, Kenneth ...
Curtius, Joachim
Donahue, Neil M.
Flagan, Richard ...
Hansel, Armin
Riipinen, Ilona
Virtanen, Annele
Winkler, Paul M.
Baltensperger, U ...
Kulmala, Markku
Worsnop, Douglas ...
show less...
About the subject
NATURAL SCIENCES
NATURAL SCIENCES
and Physical Science ...
NATURAL SCIENCES
NATURAL SCIENCES
and Chemical Science ...
Articles in the publication
Science Advances
By the university
Stockholm University

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