Ab initio modelling of interfaces in nanocomposites for high voltage insulation

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Fältnamn	Indikatorer	Metadata
000		03384nam a2200325 4500
001		oai:DiVA.org:kth-225964
003		SwePub
008		180411s2018 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
020		a 9789177297437q print
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-2259642 URI
040		a (SwePub)kth
041		a engb eng
042		9 SwePub
072	7	a vet2 swepub-contenttype
072	7	a dok2 swepub-publicationtype
100	1	a Kubyshkina, Elena,d 1990-u KTH,Elektroteknisk teori och konstruktion4 aut0 (Swepub:kth)u1qn036z
245	1 0	a Ab initio modelling of interfaces in nanocomposites for high voltage insulation
264	1	b KTH Royal Institute of Technology,c 2018
300		a 67 s.
338		a electronic2 rdacarrier
500		a QC 20180413
520		a Dielectric nanocomposite materials have been experimentally proven to have properties that are beneficial in applications for efficient energy transport. However, today there are still no empirical models or rules that can predict the performance of a certain combination of materials in the nanocomposite, and there are also no definitive explanations of their dielectric behavior. A deeper understanding of the phenomena behind these materials' response to an applied electric field can open new possibilities for improvement of the insulating properties of nanocomposites.The goal of this work is to locate the key processes that are responsible for dielectric performance. The methodology of the study is based on ab initio technology, that relies solely on the knowledge of chemical and structural composition of the material. In this work, the charge-related properties of nanocomposite interfaces are studied. The primary material of the study is chosen to be polyethylene-based composite with magnesium oxide nanoparticles.The impact of the nanoparticle crystal surface termination and its silane treatment on the electronic structure of the interface between MgO and polyethylene are investigated here. Moreover, the effects of presence of carboxyl defect and water molecule near the interface are considered in this work as well.Based on the calculated electronic structure data, a model for charge dynamics is proposed. The model explains mechanisms for conductivity and space charge reduction in nanocomposites, but also predicts an increase in thermal stress and susceptibility for chemical defects. It is suggested here that the suppression mechanisms for space charge and conductivity in nanocomposites are inherently unstable and can also accelerate material aging.
650	7	a TEKNIK OCH TEKNOLOGIERx Elektroteknik och elektronik0 (SwePub)2022 hsv//swe
650	7	a ENGINEERING AND TECHNOLOGYx Electrical Engineering, Electronic Engineering, Information Engineering0 (SwePub)2022 hsv//eng
700	1	a Jonsson, B. Lars G.,c Professoru KTH,Elektroteknisk teori och konstruktion4 ths0 (Swepub:kth)u12ind03
700	1	a Unge, Mikael,c Assistant Professor (Affiliated faculty)u KTH,Polymera material,ABB Corporate Research4 ths
700	1	a Åstrand, Per-Olof,c Professoru Norwegian University of Science and Technology4 opn
710	2	a KTHb Elektroteknisk teori och konstruktion4 org
856	4	u https://kth.diva-portal.org/smash/get/diva2:1197042/FULLTEXT01.pdfx primaryx Raw objecty fulltext
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-225964

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Av författaren/redakt...: Kubyshkina, Elen ...; Jonsson, B. Lars ...; Unge, Mikael, As ...; Åstrand, Per-Olo ...

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