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Following the Cryst...
Following the Crystallization of Amorphous Ice after Ultrafast Laser Heating
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- Ladd-Parada, Marjorie, 1985- (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Amann-Winkel, Katrin (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Kim, Kyung Hwan (författare)
- Department of Chemistry, POSTECH, Pohang 37673, Republic of Korea
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- Späh, Alexander, 1989- (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden;SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, United States
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- Perakis, Fivos (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Pathak, Harshad (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Yang, Cheolhee (författare)
- Department of Chemistry, POSTECH, Pohang 37673, Republic of Korea
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- Mariedahl, Daniel (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Eklund, Tobias (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Lane, Thomas J. (författare)
- SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, United States
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- You, Seonju (författare)
- Department of Chemistry, POSTECH, Pohang 37673, Republic of Korea
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- Jeong, Sangmin (författare)
- Department of Chemistry, POSTECH, Pohang 37673, Republic of Korea
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- Weston, Matthew (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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- Lee, Jae Hyuk (författare)
- Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea
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- Eom, Intae (författare)
- Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea
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- Kim, Minseok (författare)
- Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea
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- Park, Jaeku (författare)
- Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea
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- Chun, Sae Hwan (författare)
- Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea
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- Nilsson, Anders (författare)
- Stockholms universitet,Fysikum,Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden
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(creator_code:org_t)
- 2022-03-11
- 2022
- Engelska.
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Ingår i: Journal of Physical Chemistry B. - : American Chemical Society (ACS). - 1520-6106 .- 1520-5207. ; 126:11, s. 2299-2307
- Relaterad länk:
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https://doi.org/10.1...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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https://urn.kb.se/re...
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Abstract
Ämnesord
Stäng
- Using time-resolved wide-angle X-ray scattering, we investigated the early stages (10 μs–1 ms) of crystallization of supercooled water, obtained by the ultrafast heating of high- and low-density amorphous ice (HDA and LDA) up to a temperature T = 205 K ± 10 K. We have determined that the crystallizing phase is stacking disordered ice (Isd), with a maximum cubicity of χ = 0.6, in agreement with predictions from molecular dynamics simulations at similar temperatures. However, we note that a growing small portion of hexagonal ice (Ih) was also observed, suggesting that within our timeframe, Isd starts annealing into Ih. The onset of crystallization, in both amorphous ice, occurs at a similar temperature, but the observed final crystalline fraction in the LDA sample is considerably lower than that in the HDA sample. We attribute this discrepancy to the thickness difference between the two samples.
Ämnesord
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
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Ladd-Parada, Mar ...
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Amann-Winkel, Ka ...
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Kim, Kyung Hwan
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Späh, Alexander, ...
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Perakis, Fivos
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Pathak, Harshad
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Yang, Cheolhee
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Mariedahl, Danie ...
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Eklund, Tobias
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Lane, Thomas J.
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You, Seonju
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Jeong, Sangmin
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Weston, Matthew
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Lee, Jae Hyuk
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Eom, Intae
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Kim, Minseok
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Park, Jaeku
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Chun, Sae Hwan
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Nilsson, Anders
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