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Exhaustive characterization of modified Si vacancies in 4H-SiC
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- Davidsson, Joel, 1989- (författare)
- Linköpings universitet,Teoretisk Fysik,Tekniska fakulteten
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- Babar, Rohit (författare)
- Linköpings universitet,Teoretisk Fysik,Tekniska fakulteten
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- Shafizadeh, Danial (författare)
- Linköpings universitet,Halvledarmaterial,Tekniska fakulteten
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- Ivanov, Ivan Gueorguiev, 1955- (författare)
- Linköpings universitet,Halvledarmaterial,Tekniska fakulteten
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- Ivády, Viktor, 1986- (författare)
- Linköpings universitet,Teoretisk Fysik,Tekniska fakulteten,Max Planck Inst Phys komplexer Syst, Germany
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- Armiento, Rickard, 1976- (författare)
- Linköpings universitet,Teoretisk Fysik,Tekniska fakulteten
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- Abrikosov, Igor A., Professor, 1965- (författare)
- Linköpings universitet,Teoretisk Fysik,Tekniska fakulteten
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(creator_code:org_t)
- 2022-09-05
- Engelska.
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Ingår i: Nanophotonics. - : Walter de Gruyter. - 2192-8606 .- 2192-8614. ; 11:20, s. 4565-4580
- Relaterad länk:
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https://liu.diva-por... (primary) (Raw object)
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- The negatively charged silicon vacancy (V-Si(-)) in silicon carbide is a well-studied point defect for quantum applications. At the same time, a closer inspection of ensemble photoluminescence and electron paramagnetic resonance measurements reveals an abundance of related but so far unidentified signals. In this study, we search for defects in 4H-SiC that explain the above magneto-optical signals in a defect database generated by automatic defect analysis and qualification (ADAQ) workflows. This search reveals only one class of atomic structures that exhibit silicon-vacancy-like properties in the data: a carbon anti-site (C-Si) within sub-nanometer distances from the silicon vacancy only slightly alters the latter without affecting the charge or spin state. Such a perturbation is energetically bound. We consider the formation of V-Si(-) + C-Si; up to 2 nm distance and report their zero phonon lines and zero field splitting values. In addition, we perform high-resolution photoluminescence experiments in the silicon vacancy region and find an abundance of lines. Comparing our computational and experimental results, several configurations show great agreement. Our work demonstrates the effectiveness of a database with high-throughput results in the search for defects in quantum applications.
Ämnesord
- NATURVETENSKAP -- Fysik -- Annan fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Other Physics Topics (hsv//eng)
Nyckelord
- high-throughput; photoluminescence; point defects; SiC; silicon vacancy
Publikations- och innehållstyp
- ref (ämneskategori)
- art (ämneskategori)