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Binder-free Three-d...
Binder-free Three-dimensional (3D) printing of Cellulose-ZIF8 (CelloZIF-8) for water treatment and carbon dioxide (CO2) adsorption
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- Abdelhamid, Hani Nasser, 1986- (författare)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK),Assiut University, Egypt; The British University in Egypt, Egypt
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- Sultan, Sahar, 1987- (författare)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK),Wallenberg Wood Science Center, Sweden
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- Mathew, Aji P., 1971- (författare)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK),Wallenberg Wood Science Center, Sweden
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(creator_code:org_t)
- 2023
- 2023
- Engelska.
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Ingår i: Chemical Engineering Journal. - 1385-8947 .- 1873-3212. ; 468
- Relaterad länk:
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https://doi.org/10.1...
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visa fler...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Metal-organic frameworks (MOFs) have advanced several applications, including energy, biomedical and envi-ronmental remediation. However, most of the reported MOF materials are in powder form limiting their ap-plications. This study reported the processing of MOF via three-dimensional (3D) printing of cellulose-MOFs (denoted as CelloMOFs). The 3D printing procedure involved a one-pot method including three steps: gel for-mation, 3D printing, and in-situ growth of MOF crystals. This procedure offered 3D printing of CelloMOF via a binder-free method with high loading of 67.5 wt%. The 3D-printed porous structures were used as adsorbents for carbon dioxide (CO2), dye, and heavy metal ions. They can be also used as catalysts for the degradation of water pollutants such as organic dyes. The materials can be separated easily without requiring extra procedures such as centrifugation or filtration. The materials offered complete (>99%) removal of organic dyes within 10 min with high selectivity toward anionic dyes e.g, methyl blue (MeB). The materials exhibited CO2 and heavy metal ions adsorption capacities of 0.63 mmol/g (27.7 mg/g) and 8-328 mg/g, respectively, with good recyclability. Our methodology will open new venues for advanced 3D printing of CelloMOF and its applications for water treatment and air purification.
Ämnesord
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Nyckelord
- 3D printing
- Cellulose-MOFs composite
- CelloMOF
- Water removal
- CO 2 adsorption
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- art (ämneskategori)
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