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Phase change and co...
Phase change and combustion of iron particles in premixed CH4/O2/N2 flames
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- Xu, Shijie (författare)
- Lund University,Lunds universitet,Institutionen för energivetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Energy Sciences,Departments at LTH,Faculty of Engineering, LTH
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- Qiu, Yue (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Xu, Leilei (författare)
- Lund University,Lunds universitet,Institutionen för energivetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Energy Sciences,Departments at LTH,Faculty of Engineering, LTH
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- Huang, Jianqing (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,Shanghai Jiao Tong University,Key Lab of Education Ministry for Power Machinery and Engineering
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- Li, Shen (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Nilsson, Elna J.K. (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Aerosoler,LTH profilområden,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Aerosols,LTH Profile areas,Faculty of Engineering, LTH
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- Li, Zhongshan (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Aerosoler,LTH profilområden,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Aerosols,LTH Profile areas,Faculty of Engineering, LTH
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- Cai, Weiwei (författare)
- Shanghai Jiao Tong University
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- Aldén, Marcus (författare)
- Lund University,Lunds universitet,Förbränningsfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Combustion Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Bai, Xue Song (författare)
- Lund University,Lunds universitet,Institutionen för energivetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Energy Sciences,Departments at LTH,Faculty of Engineering, LTH
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(creator_code:org_t)
- 2024
- 2024
- Engelska.
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Ingår i: Combustion and Flame. - 0010-2180. ; 259
- Relaterad länk:
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http://dx.doi.org/10... (free)
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https://lup.lub.lu.s...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Metal powder is a promising carbon-free and recyclable energy carrier. Direct combustion of the micron-sized iron particles involves complex physical and chemical processes, such as heat transfer, surface reaction, and phase change. In this work, computational modelling of these processes is investigated and validated against experiments. A single iron particle combustion and phase change model is proposed in an Eulerian–Lagrangian framework. The new phenomenological model considers five stages, i.e., solid phase oxidation, melting of iron oxides and raw iron, liquid phase oxidation, cooling of liquid iron oxides, and solidification of super-cooled liquid iron oxides. The proposed model is first validated and then adopted in simulations of micron-sized iron particle combustion in premixed CH4/O2/N2 flames to study the effects of ambient temperature and oxygen concentration on single iron combustion. Results show that the new model is capable of replicating the melting, heterogeneous surface reaction, cooling, and solidification processes. Two-stage solidification is observed in experiments and modelled in simulations. This two-stage solidification includes a fast solidification with a significant temperature rise (∼150–200 K) and a thermal equilibrium solidification featuring a constant temperature and a slight particle radiant intensity decrease. In addition, a diffusion-controlled mechanism is identified during the melting process, in which the oxygen concentration dominates the melting time and the subsequent burning time. Furthermore, it is found that the reaction between iron and CH4/O2/N2 flame products, such as CO2 and H2O, plays a non-negligible role in the iron combustion process.
Ämnesord
- TEKNIK OCH TEKNOLOGIER -- Maskinteknik -- Energiteknik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Mechanical Engineering -- Energy Engineering (hsv//eng)
- NATURVETENSKAP -- Fysik -- Annan fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Other Physics Topics (hsv//eng)
Nyckelord
- Carbon neutral fuels
- Ignition and combustion
- Micron-sized metal particles
- Phase change
- Two-phase flow
Publikations- och innehållstyp
- art (ämneskategori)
- ref (ämneskategori)
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Till lärosätets databas
- Av författaren/redakt...
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Xu, Shijie
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Qiu, Yue
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Xu, Leilei
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Huang, Jianqing
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Li, Shen
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Nilsson, Elna J. ...
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visa fler...
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Li, Zhongshan
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Cai, Weiwei
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Aldén, Marcus
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Bai, Xue Song
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visa färre...
- Om ämnet
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- TEKNIK OCH TEKNOLOGIER
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TEKNIK OCH TEKNO ...
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och Maskinteknik
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och Energiteknik
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- NATURVETENSKAP
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NATURVETENSKAP
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och Fysik
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och Annan fysik
- Artiklar i publikationen
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Combustion and F ...
- Av lärosätet
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Lunds universitet