Sökning: onr:"swepub:oai:research.chalmers.se:36d599c9-0924-4b62-a526-969efeb9668d" > Fluorinated Ether B...
Fältnamn | Indikatorer | Metadata |
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000 | 03184naa a2200397 4500 | |
001 | oai:research.chalmers.se:36d599c9-0924-4b62-a526-969efeb9668d | |
003 | SwePub | |
008 | 180111s2017 | |||||||||||000 ||eng| | |
024 | 7 | a https://doi.org/10.1021/acs.chemmater.7b036542 DOI |
024 | 7 | a https://research.chalmers.se/publication/2542162 URI |
040 | a (SwePub)cth | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a art2 swepub-publicationtype |
072 | 7 | a ref2 swepub-contenttype |
100 | 1 | a Drvarič Talian, Sarau Kemijski Institut,National Institute of Chemistry Slovenia,Univerza V Ljubljani,University of Ljubljana4 aut |
245 | 1 0 | a Fluorinated Ether Based Electrolyte for High-Energy Lithium-Sulfur Batteries: Li+ Solvation Role behind Reduced Polysulfide Solubility |
264 | c 2017-11-29 | |
264 | 1 | b American Chemical Society (ACS),c 2017 |
338 | a electronic2 rdacarrier | |
520 | a By employing new electrolytes, the polysulfide shuttle phenomenon, one of the main problems of lithium-sulfur (Li-S) batteries, can be significantly reduced. Here we present excellent Coulombic efficiencies as well as adequate performance of high-energy Li-S cells by the use of a fluorinated ether (TFEE) based electrolyte at low electrolyte loading. The observed altered discharge profile was investigated both by electrochemical experiments and an especially tailored COSMO-RS computational approach, while the details of the discharge mechanism were elucidated by two operando techniques: XANES and UV-vis spectroscopy. A significant decrease of polysulfide solubility compared to tetraglyme is due to different Li+ solvation mode. | |
650 | 7 | a NATURVETENSKAPx Fysikx Atom- och molekylfysik och optik0 (SwePub)103022 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Physical Sciencesx Atom and Molecular Physics and Optics0 (SwePub)103022 hsv//eng |
700 | 1 | a Jeschke, Steffen,d 1986u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)jeschke |
700 | 1 | a Vizintin, Alenu Kemijski Institut,National Institute of Chemistry Slovenia4 aut |
700 | 1 | a Pirnat, Klemenu Kemijski Institut,National Institute of Chemistry Slovenia4 aut |
700 | 1 | a Iztok, Arcˇonu Institut Jožef Stefan,Jozef Stefan Institute,University of Nova Gorica4 aut |
700 | 1 | a Aquilanti, Giulianau Elettra Sincrotrone Trieste Scpa4 aut |
700 | 1 | a Johansson, Patrik,d 1969u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)jpatrik |
700 | 1 | a Dominko, R.u Kemijski Institut,National Institute of Chemistry Slovenia,Alistore - European Research Institute,Univerza V Ljubljani,University of Ljubljana4 aut |
710 | 2 | a Kemijski Institutb Univerza V Ljubljani4 org |
773 | 0 | t Chemistry of Materialsd : American Chemical Society (ACS)g 29:23, s. 10037-10044q 29:23<10037-10044x 1520-5002x 0897-4756 |
856 | 4 | u http://publications.lib.chalmers.se/records/fulltext/254216/local_254216.pdfx primaryx freey FULLTEXT |
856 | 4 | u https://pubs.acs.org/doi/pdf/10.1021/acs.chemmater.7b03654 |
856 | 4 8 | u https://doi.org/10.1021/acs.chemmater.7b03654 |
856 | 4 8 | u https://research.chalmers.se/publication/254216 |
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