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Counterintuitive Re...
Counterintuitive Reconstruction of the Polar O-Terminated ZnO Surface with Zinc Vacancies and Hydrogen
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- Jacobs, R. (författare)
- University of Wisconsin Madison
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- Zheng, B. (författare)
- Beijing Institute of Technology
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- Puchala, B. (författare)
- University of Michigan
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- Voyles, P. M. (författare)
- University of Wisconsin Madison
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- Yankovich, Andrew, 1983 (författare)
- Chalmers tekniska högskola,Chalmers University of Technology
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- Morgan, D. (författare)
- University of Wisconsin Madison
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(creator_code:org_t)
- 2016-10-28
- 2016
- Engelska.
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Ingår i: Journal of Physical Chemistry A. - : American Chemical Society (ACS). - 1089-5639 .- 1520-5215 .- 1948-7185. ; 7:22, s. 4483-4487
- Relaterad länk:
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http://dx.doi.org/10...
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http://arxiv.org/pdf...
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https://research.cha...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Understanding the structure of ZnO surface reconstructions and their resultant properties is crucial to the rational design of ZnO-containing devices ranging from optoelectronics to catalysts. Here, we are motivated by recent experimental work that showed a new surface reconstruction containing Zn vacancies ordered in a Zn(3 X 3) pattern in the subsurface of (0001)-O-terminated ZnO. Reconstruction with Zn vacancies on (0001)-O is surprising and counterintuitive because Zn vacancies enhance the surface dipole rather than reduce it. In this work, we show using density functional theory (DFT) that subsurface Zn vacancies can form on (0001)-O when coupled with adsorption of surface H and are in fact stable under a wide range of common conditions. We also show that these vacancies have a significant ordering tendency and that Sb-doping-created subsurface inversion domain boundaries (IDBs) enhance the driving force of Zn vacancy alignment into large domains of the Zn(3 X 3) reconstruction.
Ämnesord
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
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