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  • Gao, Weiming, et al. (author)
  • Synthesis of a [3Fe2S] Cluster with Low Redox Potential from [2Fe2S] Hydrogenase Models : Electrochemical and Photochemical Generation of Hydrogen
  • 2011
  • In: European Journal of Inorganic Chemistry. - : Wiley. - 1434-1948 .- 1099-1948 .- 1099-0682. ; :7, s. 1100-1105
  • Journal article (peer-reviewed)abstract
    • In the attempted replacement of carbon monoxide by the bis(phosphane) dppv in a dinuclear [2Fe2S] complex, a trinuclear [3Fe2S] complex with two bis(phosphane) ligands was unexpectedly obtained. On protonation, this gave a bridged hydride complex with an unusually low potential for the reduction of protons to molecular hydrogen. The redox potential also appears sufficiently positive for direct electron transfer from an excited [Ru(bpy)(3)](2+) sensitizer.
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