| 1. |
- Bladh, Henrik, et al.
(author)
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Experimental and theoretical comparison of spatially resolved laser-induced incandescence signals in a sooting flame
- 2005
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In: Proceedings of the European Combustion Meeting.
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Conference paper (other academic/artistic)abstract
- A detailed experimental and theoretical investigation has been made on the use of Laser-Induced Incandescence (LII) in two configurations; right-angle LII and backward LII. Both right-angle and backward LII imaging measurements were conducted in simultaneous experiments at various pulse energies. The theoretically calculated LII signals were based on a heat transfer model for soot particles exposed to laser radiation, and were compared with the experimental LII images. Both the experimental and theoretical results from this initial comparison showed similar general behaviour, for example the broadening of the spatial LII distribution and the hole-burning effect at centre for increasing laser pulse energies.
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| 2. |
- Bladh, Henrik, et al.
(author)
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Probing the smallest soot particles in low-sooting premixed flames using laser-induced incandescence
- 2015
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In: Proceedings of the Combustion Institute. - : Elsevier BV. - 1540-7489. ; 35, s. 1843-1850
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Journal article (peer-reviewed)abstract
- In this work we investigate nascent soot particles by analyzing laser-induced incandescence (LII) signals obtained in low-sooting premixed flames. The analysis covers two data sets obtained in separate experimental campaigns. The first data set was obtained in a previous work (Mouton et al., 2013) in methane/oxygen/nitrogen flames (equivalence ratio range 1.95 < Phi < 2.32) at 26.7 kPa, whereas the second was performed in atmospheric ethylene/air flames (1.77 < Phi < 2.00). Both studies show similar trends, i.e. a gradual change of the fluence curves (evolution of the LII signal as function of the laser fluence) from the well-known S-shaped curve for mature soot found at high heights above the burner (HAB) and high equivalence ratio, to a nearly linear behavior for nascent soot found at low HAB and reduced equivalence ratio. With this change comes a decrease in the LII decay time (and hence inferred particle size). Also, this decay time appears to be almost constant with HAB in flames having the lowest equivalence ratio at which the incandescence signal could be detected. In these flames, so-called nucleation flames, the stability of the particle size with HAB suggests that recently nucleated particles have undergone marginal surface growth and coagulation. Existence of such nucleation flames is of great interest for improving the theoretical description of the nucleation step. Experimental results are analyzed by using a theoretical model for LII to determine the particle size evolution throughout the flame at various experimental conditions. We highlight the size difference from nascent soot particles up to mature soot, giving insight into the particle nucleation and the surface growth processes as a function of reaction time and flame conditions. (C) 2014 The Combustion Institute. Published by Elsevier Inc. All rights reserved.
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| 3. |
- Michelsen, Hope A., et al.
(author)
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A Review of Terminology Used to Describe Soot Formation and Evolution under Combustion and Pyrolytic Conditions
- 2020
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In: ACS Nano. - : American Chemical Society (ACS). - 1936-086X .- 1936-0851. ; 14:10, s. 12470-12490
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Journal article (peer-reviewed)abstract
- This review presents a glossary and review of terminology used to describe the chemical and physical processes involved in soot formation and evolution and is intended to aid in communication within the field and across disciplines. There are large gaps in our understanding of soot formation and evolution and inconsistencies in the language used to describe the associated mechanisms. These inconsistencies lead to confusion within the field and hinder progress in addressing the gaps in our understanding. This review provides a list of definitions of terms and presents a description of their historical usage. It also addresses the inconsistencies in the use of terminology in order to dispel confusion and facilitate the advancement of our understanding of soot chemistry and particle characteristics. The intended audience includes senior and junior members of the soot, black carbon, brown carbon, and carbon black scientific communities, researchers new to the field, and scientists and engineers in associated fields with an interest in carbonaceous material production via high-temperature hydrocarbon chemistry.
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