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Search: WFRF:(Feng Meina)

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  • Pei, Cuiying, et al. (author)
  • Quasi 3D polymerization in C60 bilayers in a fullerene solvate
  • 2017
  • In: Carbon. - : Elsevier. - 0008-6223 .- 1873-3891. ; 124, s. 499-505
  • Journal article (peer-reviewed)abstract
    • The polymerization of fullerenes has been an interesting topic for almost three decades. A rich polymeric phase diagram of C60 has been drawn under a variety of pressure-temperature conditions. However, only linear or perpendicular linkages of C60 are found in the ordered phases. Here we used a unique bilayer structural solvate, C60∙1,1,2-trichloroethane (C60∙1TCAN), to generate a novel quasi-3D C60 polymer under high pressure and/or high temperature. Using Raman, IR spectroscopy and X-ray diffraction, we observe that the solvent molecules play a crucial role in confining the [2+2] cycloaddition bonds of C60s forming in the upper and lower layers alternately. The relatively long distance between the two bilayers restricts the covalent linkage extended in a single individual bilayer. Our studies not only enrich the phase diagram of polymeric C60, but also facilitate targeted design and synthesis of unique C60 polymers.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Li, Xin (1)
Sundqvist, Bertil (1)
Wang, Lin (1)
Chen, Bin (1)
Yuan, Ye (1)
Yao, Mingguang (1)
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Shen, Ming (1)
Hu, Bingwen (1)
Pei, Cuiying (1)
Feng, Meina (1)
Yang, Zhenxing (1)
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University
Umeå University (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year
2017 (1)

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