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  • Lin, Jian-Bin, et al. (author)
  • A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture
  • 2021
  • In: Science. - : American Association for the Advancement of Science. - 0036-8075 .- 1095-9203. ; 374:6574, s. 1464-1469
  • Journal article (peer-reviewed)abstract
    • Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches.  
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